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Alcohol solvent effect on the self-assembly behaviors of lignin oligomers

Green Energy & Environment 2024年第4期9卷 597-603页

作者： Ya Ma Zhicheng Jiang Yafei luo Xingjie Guo Xudong liu Yiping luo Bi Shi College of Biomass Science and Engineering Sichuan UniversityChengdu610065China National Engineering Research Center of Clean Technology in Leather Industry Sichuan UniversityChengdu610065China College of Pharmacy(International Academy of Targeted Therapeutics and Innovation) Chongqing University of Arts and SciencesChongqing402160China State Key Laboratory of Utilization of Woody Oil Resource Hunan Academy of ForestryChangsha410004China CAS Key Laboratory of Environmental and Applied Microbiology Environmental Microbiology Key Laboratory of Sichuan ProvinceChengdu Institute of BiologyChinese Academy of SciencesChengdu610041China

The interactions between lignin oligomers and solvents determine the behaviors of lignin oligomers self-assembling into uniform lignin nanoparticles(LNPs).Herein,several alcohol solvents,which readily interact with the lignin oligomers,were adopted to study their effects during solvent shifting process for LNPs’*** lignin oligomers with widely distributed molecular weight and abundant guaiacyl units were extracted from wood waste(mainly consists of pine wood),exerting outstanding self-assembly *** and spherical LNPs were generated in H_(2)O-n-propanol cosolvent,whereas irregular LNPs were obtained in H_(2)O-methanol *** unsatisfactory self-assembly performance of the lignin oligomers in H_(2)O-methanol cosolvent could be attributed to two *** one hand,for the initial dissolution state,the distinguishing Hansen solubility parameter and polarity between methanol solvent and lignin oligomers resulted in the poor dispersion of the lignin *** the other hand,strong hydrogen bonds between methanol solvent and lignin oligomers during solvent shifting process,hindered the interactions among the lignin oligomers for self-assembly.

关键词： Lignin oligomers Alcohol solvent Self-assembly LNPs Solvent effects

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Effects of seepage pressure on the mechanical behaviors and microstructure of sandstone

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第6期16卷 2033-2051页

作者： Xuewei liu Juxiang Chen Bin liu Sai Wang Quansheng liu Jin luo State Key Laboratory of Geomechanics and Geotechnical Engineering Institute of Rock and Soil MechanicsChinese Academy of SciencesWuhan430071China Faculty of Engineering China University of GeosciencesWuhan430074China Key Laboratory of Safety for Geotechnical and Structural Engineering of Hubei Province School of Civil EngineeringWuhan UniversityWuhan430072China

Surrounding rocks of underground engineering are subjected to long-term seepage pressure,which can deteriorate the mechanical properties and cause serious *** order to understand the impact of seepage pressure on the mechanical property of sandstone,uniaxial compression tests,P-wave velocity measurements,and nuclear magnetic resonance(NMR)tests were conducted on saturated sandstone samples with varied seepage pressures(i.e.0 MPa,3 MPa,4 MPa,5 MPa,6 MPa,7 MPa).The results demonstrate that the mechanical parameters(uniaxial compressive strength,peak strain,elastic modulus,and brittleness index),total energy,elastic strain energy,as well as elastic strain energy ratio,decrease with increasing seepage pressure,while the dissipation energy and dissipation energy ratio ***,as seepage pressure increases,the micro-pores gradually transform into meso-pores and *** increases the cumulative porosity of sandstone and decreases P-wave *** numerical results indicate that as seepage pressure rises,the number of tensile cracks increases progressively,the angle range of microcracks is basically from 50-120to 80-100,and as a result,the failure mode transforms to the tensile-shear mixed failure ***,the effects of seepage pressure on mechanical properties were *** results show that decrease in the effective stress and cohesion under the action of seepage pressure could lead to deterioration of strength behaviors of sandstone.

关键词： Rock mechanics Mechanical property Seepage pressure Numerical simulation Microcracks

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A High-Performance MoS_(2)-Based Visible-Near-Infrared Photodetector from Gateless Photogating Effect Induced by Nickel Nanoparticles

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Research 2024年第2期6卷 171-179页

作者： Ran Duan Weihong Qi Panke Li Kewei Tang Guoliang ru Weimin liu State Key Laboratory of Solidification Processing Center of Advanced Lubrication and Seal MaterialsNorthwestern Polytechnical UniversityXi'an 710072China Shandong Laboratory of Yantai Advanced Materials and Green Manufacturing Yantai 265503China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

Recent advancements in two-dimensional materials have shown huge potential for optoelectronic *** is challenging to achieve highly effective and sensitive broadband photodetection based on MoS_(2)*** engineering,such as introducing vacancies,can narrow the bandgap and boost the separation of photogenerated carriers by defect states but leads to a slow response ***,we propose a nickel nanoparticle-induced gateless photogating effect with a unique energy band structure to enable the application of defect engineering and achieve high optoelectronic *** device based on Ni nanoparticle-decorated MoS_(2)with S vacancies exhibited high responsivities of 106.21 and 1.38 A W^(-1)and detectivities of 1.9×10^(12)and 8.9×10^(9)Jones under 532 and 980 nm illumination(visible to near infrared),respectively,with highly accelerated response *** strategy provides new insight into optimizing defect engineering to design high-performance optoelectronic devices capable of broadband photodetection.

关键词： defect Infrared illumination

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Hole mobility enhancement in monolayer WSe2 p-type transistors through molecular doping

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Science China(Information Sciences) 2024年第6期67卷 207-213页

作者： Shiyuan liu Xiong XIONG Xin WANG Xinhang SHI ru HUANG Yanqing WU School of Integrated Circuits and Beijing Advanced Innovation Center for Integrated Circuits Peking University Wuhan National High Magnetic Field Center and School of Integrated Circuits Huazhong University of Science and Technology

Two-dimensional （2D） transition metal dichalcogenide （TMDC） semiconductor materials exhibit extraordinary electrical properties,holding promise for the realization of next-generation complementary metal-oxide-semiconductor （CMOS） devices at ultimate ***,constrained by effective device doping strategies,the hole mobility and device performance of tungsten diselenide （WSe2） p-type transistors,especially monolayer chemical vapor deposition （CVD）-grown WSe2,have not met *** this paper,an effective performance enhancement of monolayer WSe2p-type transistor was achieved through a molecular doping *** monolayer WSe2directly on SiO2back-gated substrates and leveraging energy band alignment design,4-nitrobenzenediazonium tetrafluoroborate （4-NBD） molecular dopant with a concentration of 10 m M was utilized to modulate the Fermi level position of monolayer WSe2for hole *** devices demonstrated a more than 98%increase in hole mobility,reaching up to 97 cm2·V-1·s-1while maintaining the current on/off ratio of *** p-type WSe2transistors with 1μm channel length exhibit a high drive current surpassing 176μA·μm-1,exceeding previous CVD-WSe2devices with similar channel *** straightforward and effective approach to improving the electrical performance of WSe2transistors paves the way for advanced logic technologies based on transition metal dichalcogenide semiconductors.

关键词： CVD-grown WSe2 molecular doping 4-NBD p-type transistors hole mobility

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Modulating charge separation and transfer for high-performance photoelectrodes via built-in electric field

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International Journal of Minerals,Metallurgy and Materials 2024年第5期31卷 1126-1146页

作者： Houyan Cheng Peng liu Yuntao Cui ru Ya Yuxiang Hu Jinshu Wang Key Laboratory of Advanced Functional Materials of Education Ministry of China Faculty of Engineering and ManufacturingBeijing University of TechnologyBeijing 100124China Key Laboratory of Cryogenic Science and Technology and Beijing Key Lab of Cryo-Biomedical Engineering Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190China Inner Mongolia Academy of Science and Technology Hohhot 010020China

Constructing a built-in electric field has emerged as a key strategy for enhancing charge separation and transfer,thereby improving photoelectrochemical ***,considerable efforts have been devoted to this *** review systematically summarizes the impact of built-in electric fields on enhancing charge separation and transfer mechanisms,focusing on the modulation of built-in electric fields in terms of depth and ***,mechanisms and tuning strategies for built-in electric fields are ***,the state-of-the-art works regarding built-in electric fields for modulating charge separation and transfer are summarized and categorized according to surface and interface ***,current strategies for constructing bulk built-in electric fields in photoelectrodes are explored,and insights into future developments for enhancing charge separation and transfer in high-performance photoelectrochemical applications are provided.

关键词： photoelectrochemical water splitting bulk built-in electric field cation intercalation charge separation and transfer

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Potential use of large language models for mitigating students’problematic social media use:ChatGPT as an example

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World Journal of Psychiatry 2024年第3期14卷 334-341页

作者： Xin-Qiao liu Zi-ru Zhang School of Education Tianjin UniversityTianjin 300350China

The problematic use of social media has numerous negative impacts on individuals'daily lives,interpersonal relationships,physical and mental health,and ***,there are few methods and tools to alleviate problematic social media,and their potential is yet to be fully *** large language models(LLMs)are becoming increasingly popular for providing information and assistance to people and are being applied in many aspects of *** mitigating problematic social media use,LLMs such as ChatGPT can play a positive role by serving as conversational partners and outlets for users,providing personalized information and resources,monitoring and intervening in problematic social media use,and *** this process,we should recognize both the enormous potential and endless possibilities of LLMs such as ChatGPT,leveraging their advantages to better address problematic social media use,while also acknowledging the limitations and potential pitfalls of ChatGPT technology,such as errors,limitations in issue resolution,privacy and security concerns,and potential *** we leverage the advantages of LLMs to address issues in social media usage,we must adopt a cautious and ethical approach,being vigilant of the potential adverse effects that LLMs may have in addressing problematic social media use to better harness technology to serve individuals and society.

关键词： Problematic use of social media Social media Large language models ChatGPT Chatbots

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Plant-derived nanovesicles as an emerging platform for cancer therapy

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Acta Pharmaceutica Sinica B 2024年第1期14卷 133-154页

作者： Hanzhe liu Guo-Feng luo Zhengjun Shang The State Key Laboratory Breeding Base of Basic Science of Stomatology(Hubei-MOST)&Key Laboratory of Oral Biomedicine Ministry of Education School and Hospital of StomatologyWuhan UniversityWuhan 430079China

Plant-derived nanovesicles(PDNVs)derived from natural green products have emerged as an attractive nanoplatform in biomedical *** are usually characterized by unique structural and biological functions,such as the bioactive lipids/proteins/nucleic acids as therapeutics and targeting groups,immune-modulation,and long-term *** the rapid development of nanotechnology,materials,and synthetic chemistry,PDNVs can be engineered with multiple functions for efficient drug delivery and specific killing of diseased cells,which represent an innovative biomaterial with high biocompatibility for fighting against *** this review,we provide an overview of the state-of-theart studies concerning the development of PDNVs for cancer *** original sources,methods for obtaining PDNVs,composition and structure are introduced *** an emphasis on the featured application,the inherent anticancer properties of PDNVs as well as the strategies in constructing multifunctional PDNVs-based nanomaterials will be discussed in ***,some scientific issues and technical challenges of PDNVs as promising options in improving anticancer therapy will be discussed,which are expected to promote the further development of PDNVs in clinical translation.

关键词： Naturally occurring nanovesicles Plant Nanotechnology Drug delivery Cancer therapy

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Rockburst proneness considering energy characteristics and sample shape effects

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第7期16卷 2441-2465页

作者： Song luo Fengqiang Gong Kang Peng Zhixiang liu School of Resources and Safety Engineering Central South UniversityChangsha410083China School of Civil Engineering Southeast UniversityNanjing211189China

Accurate prediction of rockburst proneness is one of challenges for assessing the rockburst risk and selecting effective control *** study aims to assess rockburst proneness by considering the energy characteristics and qualitative information during rock *** representative rock types in cylindrical and cuboidal sample shapes were tested under uniaxial compression conditions and the failure progress was detected by a high-speed *** far-field ejection mass ratio(FEMR)was determined considering the qualitative failure information of the rock *** peak-strength energy impact index and the residual elastic energy index were used to quantitatively evaluate the rockburst proneness of both cylindrical and cuboidal ***,the performance of these two indices was analyzed by comparing their estimates with the *** results show that the accuracy of the residual elastic energy index is significantly higher than that of the peak-strength energy impact *** residual elastic energy index and the FEMR are in good agreement for both cylindrical and cuboidal rock *** is because these two indices can essentially reflect the common energy release mechanism characterized by the mass,ejection velocity,and ejection distance of rock *** suggests that both the FEMR and the residual elastic energy index can be used to accurately measure the rockburst proneness of cylindrical and cuboidal samples based on uniaxial compression test.

关键词： Rockburst proneness Sample shape Strain energy Energy release Far-field ejection mass ratio(FEMR)

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Optimal Stochastic Scheduling Strategy of Multi-vector Energy Complex Integrated with Full-blown Power-to-biomethane Model

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Journal of Modern Power Systems and Clean Energy 2024年第3期12卷 863-873页

作者： Guanwei Zeng Chengxi liu Minfang Liao Yongjian luo Xuzhu Dong Hubei Engineering and Technology Research Center for AC/DC Intelligent Distribution Network WuhanChina the School of Electrical Engineering and Automation Wuhan UniversityWuhanChina

We propose an optimal stochastic scheduling strategy for a multi-vector energy complex(MEC),considering a fullblown model of the power-to-biomethane(Pt M)*** conventional optimization that uses a simple efficiency coefficient to coarsely model energy conversion between electricity and biomethane,a detailed Pt M model is introduced to emphasize the reactor kinetics and chemical equilibria of *** model crystallizes the interactions between the Pt M process and MEC flexibility,allowing to adjust the operating condition of the methanation reactor for optimal MEC operation in stochastic *** optimization and flowsheet design of the Pt M process increase the average selectivity of methane(i.e.,ratio between net biomethane production and hydrogen consumption)up to 83.7%in the proposed synthesis *** results can provide information and predictions to operators about the optimal operating conditions of a Pt M unit while improving the MEC flexibility.

关键词： Multi-vector energy complex optimal stochastic scheduling power-to-biomethane unit process synthesis natural gas

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3D robust anisotropic diffusion filtering algorithm for sparse view neutron computed tomography 3D image reconstruction

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Nuclear Science and Techniques 2024年第3期35卷 13-29页

作者： Yang liu Teng-Fei Zhu Zhi luo Xiao-Ping Ouyang School of Nuclear Science and Engineering North China Electric Power UniversityBeijing 102206China State Key Laboratory of Nuclear Resources and Environment East China University of TechnologyNanchang 330013China State Key Laboratory of Intense Pulsed Radiation Simulation and Effect Xi’an 710024China

The most critical part of a neutron computed tomography(NCT) system is the image processing algorithm,which directly affects the quality and speed of the reconstructed *** types of noise in the system can degrade the quality of the reconstructed ***,to improve the quality of the reconstructed images of NCT systems,efficient image processing algorithms must be *** anisotropic diffusion filtering(ADF) algorithm can not only effectively suppress the noise in the projection data,but also preserve the image edge structure information by reducing the diffusion at the image ***,we propose the application of the ADF algorithm for NCT image *** compare the performance of different algorithms in NCT systems,we reconstructed images using the ordered subset simultaneous algebraic reconstruction technique(OS-SART) algorithm with different regular terms as image processing *** the iterative reconstruction,we selected two image processing algorithms,the Total Variation and split Bregman solved total variation algorithms,for comparison with the performance of the ADF ***,the filtered back-projection algorithm was used for comparison with an iterative *** reconstructing the projection data of the numerical and clock models,we compared and analyzed the effects of each algorithm applied in the NCT *** on the reconstruction results,OS-SART-ADF outperformed the other algorithms in terms of denoising,preserving the edge structure,and suppressing *** example,when the 3D Shepp–Logan was reconstructed at 25 views,the root mean square error of OS-SART-ADF was the smallest among the four iterative algorithms,at only *** universal quality index,mean structural similarity,and correlation coefficient of the reconstructed image were the largest among all algorithms,with values of 0.9877,0.9878,and 0.9887,respectively.

关键词： NCT OS-SART Sparse-view Anisotropic diffusion filtering

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