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Impacts of Comorbidity and Mental Shock on Organic Micropollutants in Surface Water During and After the First Wave of COVID-19 Pandemic in Wuhan (2.1.–2021), china

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Engineering 2024年第6期37卷 40-48页

作者： jian Zhao Jin Kang Xiaofeng Cao rui Bian Gang liu Shengchao Hu Xinghua Wu Chong Li Dianchang Wang Weixiao Qi Cunrui Huang huijuan liu jiuhui qu center for Water and ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China Hubei Provincial research Institute of environmental Science Wuhan 430072China key laboratory of Drinking Water Science and Technology Research Centre for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Sanitary Engineering Department of Water ManagementFaculty of Civil Engineering and GeosciencesDelft University of TechnologyDelft 2600 GAThe Netherlands china Three Gorges Corporation Wuhan 430010China Vanke School of Public Health Tsinghua UniversityBeijing 100084China

The first pandemic wave of coronavirus disease 2.1.(COVID-19)induced a considerable increase in several antivirals and antibiotics in surface *** common symptoms of COVID-19 are viral and bacterial infections,while comorbidities(e.g.,hypertension and diabetes)and mental shock(e.g.,insomnia and anxiety)are ***,little is known about the long-term impacts of comorbidities and mental shock on organic micropollutants(OMPs)in surface ***,we monitored 114 OMPs in surface water and wastewater treatment plants(WWTPs)in Wuhan,china,between 2.1. and *** pandemic-induced OMP pollution in surface water was confirmed by significant increases in 26 OMP *** increases in four antihypertensives and one diabetic drug suggest that the treatment of comorbidities may induce OMP ***,cotinine(a metabolite of nicotine)increased 155 times to 187 ngL1,which might be associated with increased ***,the increases in zolpidem and sulpiride might be the result of worsened insomnia and ***,it is reasonable to note that mental-health protecting drugs/behavior also contributed to OMP *** the observed OMPs,telmisartan,lopinavir,and ritonavir were associated with significantly higher ecological risks because of their limited WWTP-removal rate and high *** study provides new insights into the effects of comorbidities and mental shock on OMPs in surface water during a pandemic and highlights the need to monitor the fate of related pharmaceuticals in the aquatic environment and to improve their removal efficiencies in WWTPs。

关键词： Coronavirus disease 2.1. Comorbidities Mental shock Micropollutant Surface water

Efficient Metal Recovery from Industrial Wastewater:Potential Oscillation and Turbulence Mode for Electrochemical System

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Engineering 2024年第7期38卷 184-193页

作者： Li Chen Gong Zhang huijuan liu Shiyu Miao Qingbai Chen Huachun Lan jiuhui qu center for Water and ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China

Efficient metal recovery from industrial wastewater facilitates addressing of the environmental hazards and resource requirements of heavy *** conventional electrodeposition recovery method is hampered by the limitations of interfacial ion transport in charge-transfer reactions,creating challenges for simultaneous rapid and high-quality metal ***,we proposed integrating a transient electric field(TE)and swirling flow(SF)to synchronously enhance bulk mass transfer and promote interfacial ion *** investigated the effects of the operation mode,transient frequency,and flow rate on metal recovery,enabling determination of the optimal operating conditions for rapid and efficient sequential recovery of Cu in TE&SF *** conditions included low and high electric levels of 0 and 4 V,a 50%duty cycle,1 kHz frequency,and 400 L·h^(-1)flow *** kinetic coefficients of TE&SF electrodeposition were 3.5-4.3 and 1.37-1.97 times that of single TE and SF electrodeposition,*** the deposition process under TE and SF conditions confirmed the efficient concurrence of interfacial ion transport and charge transfer under TE and SF synergy,which achieved rapid and highquality metal ***,the combined deposition strategy is considered an effective technique for reducing metal pollution and promoting resource recycling.

关键词： Ion transport Reaction kinetics Transient electric field Swirling flow

Characterization and adsorption behavior of a novel triolein-embedded activated carbon composite adsorbent

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chinese Science Bulletin 2005年第23期50卷 2788-2790页

作者： ru jia liu huijuan qu jiuhui WANG Aimin dai ruihua state key laboratory of environmental aquatic chemistry Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing 100085 China Graduate School of chinese academy of sciences Beijing 100039China

A novel triolein-embedded activated carbon composite adsorbent was developed. Experiments were car-ried out in areas such as the preparation method, the char-acterization of physicochemical properties, and the adsorp-tion behavior of the composite adsorbent in removing diel-drin from aqueous solution. Results suggested that the novel composite adsorbent was composed of the supporting acti-vated carbon and the surrounding triolein-embedded cellu-lose acetate membrane. The adsorbent was stable in water, for no triolein leakage was detected after soaking the ad-sorbent for five weeks. The adsorbent had good adsorption capability to dieldrin, which was indicated by a residual di-eldrin concentration of 0.204 μg·L?1. The removal efficiency of the composite adsorbent was higher than the traditional activated carbon adsorbent.

关键词：饮用水处理活性碳吸附剂三油精持久性有机污染物吸附行为

Removal of pharmaceutical in a biogenic/chemical manganese oxide system driven by manganese-oxidizing bacteria with humic acids as sole carbon source

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Journal of environmental sciences 2023年第4期126卷 734-741页

作者： Tingming Ye huijuan liu Weixiao Qi jiuhui qu key laboratory of Drinking Water Science and Technology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China center for Water and ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China University of chinese academy of sciences Beijing 100049China

Bioaugmented sand filtration has attracted considerable attention because it can effectively remove contaminants in drinking water without additional chemical reagent *** this study,a synthesized chemical manganese dioxide (MnO_(2)) -coated quartz sand(MnQS) and biogenic manganese oxide (BioMnOx) composite system was proposed to simultaneously remove typical pharmaceutical contaminants and Mn_(2)+.We demonstrated a manganese-oxidizing bacterium,Pseudomonas ***-1,could oxidize Mn_(2)+to generate BioMnOxusing humic acids (HA) as sole carbon *** coaction of MnQS,QJX-1,and the generated BioMnOxin simultaneously removing caffeine and Mn_(2)+in the presence of HA was *** found a synergistic effect between *** and BioMnOxtogether significantly increased the caffeine removal efficiency from 32.8%(MnQS alone) and 21.5%(BioMnOxalone) to 61.2%.Meanwhile,Mn_(2)+leaked from MnQS was rapidly oxidized by QJX-1 to regenerate reactive BioMnOx,which was beneficial for continuous contaminant removal and system *** degradation intermediates of caffeine oxidized by MnQS and BioMnOxwere detected by LC-QTOF-MS analysis,which implied that caffeine was oxidized by a different ***,this work promotes the potential application of bioaugmented sand filtration in pharmaceutical removal in the presence of natural organic matter in drinking water.

关键词： Bioaugmentation MnO_(2)-coated quartz sand Manganese-oxidizing bacteria Humic acid Caffeine

Phototransformation of nitrobenzene in the Songhua River:Kinetics and photoproduct analysis

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Journal of environmental sciences 2008年第7期20卷 787-795页

作者： WANG, Aimin HU, Chun qu, jiuhui YANG, Min liu, huijuan ru, jia QI, Rong SUN, Jingfang state key laboratory of environmental aquatic chemistry Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing 100085 China

Nitrobenzene (NB) pollution of the Songhua River caused by an explosion at a petrochemical plant in Jilin City,Jilin Province, china,attracted public concern over the fate of NB in the *** one of the efforts to predict the fate of residual NB in the river,the kinetics and mechanism of phototransformation of NB in natural water from four sections of the Songhua River were *** was found that photodegradation of NB in water proceeded via pseudo-first-order reaction kinetics under simulated sol...

关键词： nitrobenzene phototransformation mechanism the Songhua River nitrate by-products

Dieldrin and endrin removal from water by trioleinembedded adsorbent

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chinese Science Bulletin 2005年第23期50卷 2696-2700页

作者： HUO Jinxian liu huijuan qu jiuhui ru jia liu Haining LI Guoting tate key laboratory of environmental aquatic chemistry Research Center for Eco-environmental Science Chinese Academy of SciencesBeijing 100085 China

A novel triolein-embedded adsorbent for re-moval of persistent organic pollutants (POPs) from water was developed. In this paper, taking dieldrin and endrin as the target pollutants, different factors (temperature, ion strength, pH, and concentration of humic acid) that affect the adsorption rate were investigated. Adsorption isotherms of these two pollutants fitted to Freundlich model well identi-fied the partition mechanism between the adsorbent and water. However, the equilibrium constant of dieldrin was larger than that of endrin due to larger octanol-water coeffi-cient of dieldrin. Adsorption rate of dieldrin increased with the increase of temperature, the decrease of ion strength, pH and concentration of humic acid, whereas adsorption rate of endrin decreased with the increase of temperature and pH. Humic acid firstly increased, and then decreased the adsorp-tion rate of endrin. Ion strength hardly affected the adsorp-tion rate of endrin.

关键词：含氯杀虫剂狄氏剂异狄氏剂三油精吸附剂醇-水系数持久性有机污染物污水处理

Enhanced phosphate removal using zirconium hydroxide encapsulated in quaternized cellulose

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Journal of environmental sciences 2020年第3期32卷 102-112页

作者： Shuoxun Dong Qinghua Ji Yili Wang huijuan liu jiuhui qu center for Water and ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China College of environmental Science and Engineering Beijing Key Lab for Source Control Technology of Water PollutionBeijing Forestry UniversityBeijing 100083China

Zirconium-based materials are efficient adsorbent for aqueous phosphate ***,current zirconium-based materials still show unsatisfied performance on adsorption capacity and ***,we demonstrate a zirconium hydroxide encapsulated in quaternized cellulose(QC-Zr) for the selective phosphate *** hydroxide nanoparticles were simultaneously generated in situ with the QC framework and firmly anchored in the three-dimensional(3D) cross-linked cellulose *** maximum P adsorption capacity of QC-Zr was 83.6 mg P/***,the QC-Zr shows high P adsorption performance in a wide pH range,generally due to the electrostatic effects of quaternized *** enhanced adsorption of P was also achieved in the presence of competing anions(including Cl^-,NO3^-,SO4^2-,SO4^4-) and humic acid(HA) even at a molar ratio up to 20 *** column adsorption capacity of QC-Zr reached 4000 bed volumes(BV) at EBCT=0.5 min as the P concentration decreased from 2.5 to 0.5 mg/*** study revealed that both-N^+(CH3)3 groups and zirconium hydroxide were involved in phosphate adsorption via electrostatic interactions between -N^+(CH3)3 and phosphate,and the formation of zirconium hydrogen phosphate(Zr(HPO4)x).The 31 P nuclear magnetic resonance(NMR) study implied that P surface-precipitated and inner-sphere complexed with zirconium hydroxide at a ratio of 3:1.

关键词： Adsorption Phosphate removal Zirconium hydroxide aerogel quaternized cellulose

Removal of tetracycline from water by Fe-Mn binary oxide

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Journal of environmental sciences 2012年第2期24卷 242-247页

作者： huijuan liu Yang Yang Jin Kang Maohong Fan jiuhui qu state key laboratory of environmental aquatic chemistry Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing 100085 China Graduate University Of chinese academy of sciences BeOing 100039 China Hubei Provincial research Institute of environmental Science Wuhan 430072 China School of Energy Resources ＆ Department of Chemical ＆ Petroleum Engineering University of V~oming Laramie WY 82071 USA

Significant concerns have been raised over the presence of antibiotics including tetracyclines in aquatic environments.A series of FeMn binary oxide with different Fe：Mn molar ratios was synthesized by a simultaneous oxidation and coprecipitation process for TC *** showed that Fe-Mn binary oxide had higher removal efficiency than that of hydrous iron oxide and hydrous manganese oxide,and that the oxide with a Fe：Mn molar ratio of 5：1 was the best in removal than other molar *** tetracycline removal was highly pH *** removal of tetracycline decreased with the increase of initial concentration,but the absolute removal quantity was more at high *** presence of cations and anions such as Ca2＋,Mg2＋,CO32-and SO42-had no significant effect on the tetracycline removal in our experimental conditions,while SiO32-and PO43-had hindered the adsorption of *** mechanism investigation found that tetracycline removal was mainly achieved by the replacement of surface hydroxyl groups by the tetracycline species and formation of surface complexes at the water/oxide *** primary study suggests that Fe-Mn binary oxide with a proper Fe：Mn molar ratio will be a very promising material for the removal of tetracycline from aqueous solutions.

关键词： Fe-Mn binary oxide tetracycline abatement and removal water treatment

Utilization of aluminum hydroxide waste generated in fluoride adsorption and coagulation processes for adsorptive removal of cadmium ion

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Frontiers of environmental Science & Engineering 2016年第3期10卷 467-476页

作者： jiawei JU ruiping liu Zan HE huijuan liu Xiwang ZHANG jiuhui qu state key laboratory of environmental aquatic chemistry Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing 100085 China University of chinese academy of sciences Beijing 100039 China Department of Chemical Engineering Monash University Clayton VIC 3800 Australia

Although Al-based coagulation and adsorption processes have been proved highly efficient for fluoride （F） removal, the two processes both generate large amount of AI（OH）3 solid waste containing F （Al（OH）3-F）. This study aimed to investigate the feasibility of utilizing AI（OH）3-F generated in AI（OH）3 adsorption （Al（OH）3-Fads） and coagulation （Al（OH）3-Fcoag） for the adsorption of cadmium ion （Cd（II））. The adsorption capacity of AI（OH）3- Fads and Al（OH）a-Fcoag for Cd（II） was similar as that of pristine aluminum hydroxide （AI（OH）3）, being of 24.39 and 19.90 mg·g^-1, respectively. The adsorption of Cd（II） onto AI（OH）a-Fads and AI（OH）a-Fcoag was identified to be dominated by ion-exchange with sodium ion （Na^＋） or hydrogen ion （H^＋）, surface microprecitation, and electrostatic attraction. The maximum concentration of the leached fluoride from Al（OH）a-Fads and Al（OH）3-Feoag is below the chinese Class-I Industrial Wastewater Discharge Standard for fluoride （〈 10mg·L^-1）. This study demonstrates that the AI（OH）3 solid wastes generated in fluoride removal process could be potentially utilized as a adsorbent for Cd（II） removal.

关键词： Al(OH)3 fluoride cadmium adsorption reclamation sequential extraction