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Rational modulation of fluorophosphate cathode by anionic groups to reduce the polarization behavior for fast-charging sodium-ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 509-521页

作者： Xinyuan Wang Fan Zhang Xingyu Zhou Qian Wang Changyu liu Yangyang liu Hui Wang Xiaojie liu Key Laboratory of Synthetic and Natural Functional Molecule of the Ministry of Education College of Chemistry & Materials Science Northwest University

Na3V2（PO4）2O2F （VP） is recognized as a promising cathode material for sodium-ion batteries due to its stable structural framework and high specific *** functional theory （DFT） and finite element simulations show that incorporating SO42-into VP decreases its band gap,lowers the migration energy barrier,and ensures a uniform Na+concentration gradient and stress distribution during charge and discharge ***,the average Na+diffusion coefficient of Na3V2（PO4）1.95（SO4）0.05O2F（VPS-1） is roughly double that of VP,leading to enhanced rate capability (80 C,75.5 mAh g-1) and cycling stability (111.0 mAh g-1capacity after 1000 cycles at 10 C current density) for ***-1 exhibits outstanding fast-charging capabilities,achieving an 80%state of charge in just 8.1 *** assembled VPS-1//SbSn/NPC full cell demonstrated stable cycling over 200 cycles at a high 5 C current,maintaining an average coulombic efficiency of 95.35%.

关键词： Anionic group modulation Polarization behavior Fast-charging Sodium-ion battery Fluorophosphate Cathode

Post-tunable salt gel electrolytes toward flexible supercapacitor switches

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Journal of Energy Chemistry 2025年第1期100卷 114-124页

作者： Hui Wang Shuang Chen Xuming liu Qin Zhang Xin liu Polymeric and Soft Materials Laboratory School of Chemistry and Life Science and Advanced Institute of Materials Science Changchun University of Technology Polymeric and Soft Materials Laboratory School of Chemical Engineering and Advanced Institute of Materials Science Changchun University of Technology

Convertible hydrogel supercapacitors have emerged as promising energy storage devices in switches,diodes, and transistors. However, inherent weaknesses in ionic conductivity, mechanical properties,and water retention of hydrogel electrolytes seriously hinder their development. Inspired by the hardness conversion of sea cucumber skin, a conductivity and mechanics dual-tunable salt gel electrolyte is successfully designed. The salt gel presents a reversible switching of conductors-insulators and a mechanical regulation between softness and hardness via the dissolution-crystallization transition of sodium acetate trihydrate（SAT）. Meanwhile, the salt gels spontaneously grow a layer of “armor” through saturated phase-change salt crystals effectively reducing water evaporation of hydrogel ***, this phase-change soft-rigid conversion strategy will expand the capabilities of gel-based flexible supercapacitors(area capacitance: 258.6 mF cm-2), and the capacitance retention rate could still reach 86.9% after 3000 cycles at high temperatures. Moreover, the salt gel supercapacitor is potentially used in over-heat alarm systems. It is anticipated that the strategy of conductivity and mechanics of dual-tunable salt gel would provide a new perspective on the development of energy storage devices,wearable electronics, and flexible robots.

关键词： Capacitance

射频处理对红枣中短波红外干燥动力学及品质特性的影响

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食品科学 2020年第7期41卷 117-123页

作者：王坤华李佳美彭飞刘昱迪马琦李梅徐怀德西北农林科技大学食品科学与工程学院陕西杨凌712100

为缩短红枣干燥时间、提高红枣干燥品质,将射频技术(radio frequency,RF)应用于红枣干燥前处理,运用中短波红外干燥技术在不同干燥温度(50、60、70℃)下干燥红枣,研究RF处理红枣的干燥动力学及品质特性,并选取8个常用的薄层干燥数学模型... 详细信息

为缩短红枣干燥时间、提高红枣干燥品质,将射频技术(radio frequency,RF)应用于红枣干燥前处理,运用中短波红外干燥技术在不同干燥温度(50、60、70℃)下干燥红枣,研究RF处理红枣的干燥动力学及品质特性,并选取8个常用的薄层干燥数学模型,采用非线性回归的方式对实验结果进行拟合,得出最适于RF处理后红枣中短波红外干燥的数学干燥模型。结果表明:RF处理组红枣的干燥时间较未处理组红枣缩短了21.2%~29.3%,水分有效扩散系数提高了16.7%~49.6%,干燥活化能降低了13.13%;比较各数学模型的决定系数、均方根误差和卡方值,发现Weibull distribution模型拟合效果最好,可用于描述、预测RF处理后红枣的中短波红外干燥过程;经RF处理后干燥的红枣较未处理红枣色差值降低了19.3%~31.4%,总酚含量提高了14.9%~19.1%,环磷酸腺苷含量提高了27.5%~31.9%。与未处理红枣相比,RF处理红枣的干燥效率高,干燥后产品质量好,表明RF处理是一种优良的红枣干燥前处理方法。

关键词：红枣射频处理中短波红外干燥干燥动力学品质数学模型

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β平面上斜压波热力结构特性的实验研究

力学学报 2001年第2期33卷 205-214页

作者：林上金仲孝恭成新喜魏岗周凯刘宇迪解放军理工大学南京211101

首次用转环实验模拟方法研究了β效应对斜压波热力结构的影响：发现β效应有抑制流动的水平混合和垂直混合的作用，使流动趋于正压；β平面上急流随高度降低而减弱，在急流的内外两侧各有一个无量纲温度值分布的突跃区，它们的空间结构... 详细信息

首次用转环实验模拟方法研究了β效应对斜压波热力结构的影响：发现β效应有抑制流动的水平混合和垂直混合的作用，使流动趋于正压；β平面上急流随高度降低而减弱，在急流的内外两侧各有一个无量纲温度值分布的突跃区，它们的空间结构与大气环流中的极锋锋区和北极锋锋区的结构相似．

关键词：转环实验斜压波热力结构 β效应突跃区大气环流

Economic effect of China's carbon neutrality target under shared socioeconomic pathways

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Science China Earth Sciences 2025年第1期68卷 142-157页

作者： Zemiao liu Xianjin HUANG Xinxian QI School of Geography and Ocean Science Nanjing University Key Laboratory of Carbon Neutrality and Territory Optimization Ministry of Natural Resources Frontiers Science Center for Critical Earth Material Cycling Nanjing University

Economic feasibility is crucial for achieving the carbon neutrality target. However, current integrated assessments often underestimate the economic impacts of mitigation policies due to the lack of consideration of their economic benefits. This study integrates a warming-labour productivity model with a typical integrated assessment model using shared socioeconomic pathways. It simulates China's economic development and carbon emission levels under both baseline and carbon-neutral policy scenarios, evaluating the economic costs and benefits of emission reduction policies aimed at achieving carbon neutrality. These findings reveal the following:(1) The economic costs of emission reduction policies are projected to peak between 2050 and 2060, ranging from 0.41% to 9.37% of total GDP in the baseline scenario, primarily due to increased energy prices and R&D investments. These costs are expected to decline rapidly after 2070.(2) China's carbon-neutral policies will mitigate global warming, with the economic benefits of mitigation projected to reach 5.65% to 17.24% of China's total GDP by 2100.(3) Lowcarbon scenarios SSP1 and SSP4 could significantly reduce initial economic costs and advance the onset of net economic gains to 2060. This integrated assessment confirms that China's carbon neutrality target offers substantial net economic benefits in the long term. To minimize initial economic costs, efforts should focus on enhancing consumption-side transitions, upgrading lowcarbon technologies, and adopting new energy sources.

关键词： Climate change China Carbon neutrality Economic effects Policy

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温度、水稻生育期和白背飞虱若虫龄期对南方水稻黑条矮缩病毒介体获毒率的影响

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植物保护 2016年第1期42卷 129-133页

作者：刘丹凤李沛弓少龙安兴奎刘玉娣侯茂林植物病虫害生物学国家重点实验室中国农业科学院植物保护研究所北京100193

南方水稻黑条矮缩病毒(Southern rice black-streaked dwarf virus,SRBSDV)是由白背飞虱(Sogatella furcifera)传播的一种新病毒。为明确白背飞虱获毒的影响因子及南方水稻黑条矮缩病的流行规律,本文采用三因素试验,研究温度(22、27和32... 详细信息

南方水稻黑条矮缩病毒(Southern rice black-streaked dwarf virus,SRBSDV)是由白背飞虱(Sogatella furcifera)传播的一种新病毒。为明确白背飞虱获毒的影响因子及南方水稻黑条矮缩病的流行规律,本文采用三因素试验,研究温度(22、27和32℃)、水稻生育期(三叶期、分蘖期和孕穗期)和白背飞虱若虫龄期(3龄和5龄)对白背飞虱获毒效率的影响。结果表明,白背飞虱在27℃和32℃下的获毒率显著高于22℃下的获毒率;在不同生育期水稻上,白背飞虱在分蘖期水稻上的获毒率高于三叶期和孕穗期;白背飞虱若虫龄期也显著影响获毒率,3龄若虫获毒率高于5龄若虫;但这些因素的交互作用对白背飞虱的获毒率无显著影响。

关键词：白背飞虱 SRBSDV 水稻病毒传播温度介体昆虫

Oxidation Resistance of Form-stable Hightemperature Phase Change Thermal Energy Storage Materials Doped by Impregnated Graphite

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Journal of Wuhan University of Technology(Materials Science) 2025年第1期40卷 1-12页

作者： LI Baorang DAI Jianhuan ZHANG Wei liu Xiangchen YANG liu School of Energy Power and Mechanical Engineering North China Electric Power UniversityBeijing 102206China School of Ener-gy and Environment Southeast UniversityNanjing 210096China

We adopted the solution impregnation route with aluminum dihydrogen phosphate solution as liquid medium for effective surface modification on graphite *** mass ratio of graphite to Al(H_(2)PO_(4))_(3) changed from 0.5:1 to 4:1,and the impregnation time changed from 1 to 7 *** typical composite phase change thermal storage materials doped with the as-treated graphite were fabricated using form-stable *** investigate the oxidation and anti-oxidation behavior of the impregnated graphite at high temperatures,the samples were put into a muffle furnace for a cyclic heat *** on SEM,EDS,DSC techniques,analyses on the impregnated technique suggested an optimized processing conditions of a 3 h impregnation time with the ratio of graphite:Al(H_(2)PO_(4))_(3) as 1:3 for graphite impregnation *** investigations on high-temperature phase change heat storage materials doped by the treated graphite suggested excellent oxidation resistance and thermal cycling performance.

关键词： phase change materials graphite impregnation method oxidation,sintering thermal analysis

Engineering nanoparticle structure at synergistic Ru-Na interface for integrated CO2 capture and hydrogenation

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Journal of Energy Chemistry 2025年第1期100卷 779-791页

作者： Hanzi liu Ling Cen Xinlin Xie Lei liu Zhao Sun Zhiqiang Sun Hunan Engineering Research Center of Clean and Low-Carbon Energy Technology School of Energy Science and Engineering Central South University

The development of dual functional material for cyclic CO2capture and hydrogenation is of great significance for converting diluted CO2into valuable fuels,but suffers from kinetic limitation and deactivation of adsorbent and ***,we engineered a series of RuNa/γ-Al2O3materials,varying the size of ruthenium from single atoms to clusters/*** coordination environment and structure sensitivity of ruthenium were quantitatively investigated at atomic *** findings reveal that the reduced Ru nanoparticles,approximately 7.1 nm in diameter with a Ru-Ru coordination number of 5.9,exhibit high methane formation activity and selectivity at 340°*** Ru-Na interfacial sites facilitate CO2migration through a deoxygenation pathway,involving carbonate dissociation,carbonyl formation,and ***-situ experiments and theoretical calculations show that stable carbonyl intermediates on metallic Ru nanoparticles facilitate heterolytic C–O scission and C–H bonding,significantly lowering the energy barrier for activating stored CO2.

关键词： Carbon capture and utilization

基于电网电压补偿的多电平变频器控制方法研究

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现代电子技术 2005年第5期28卷 19-21页

作者：武贵林刘雨棣韦力西安科技大学陕西西安710054 西安航空技术高等专科学校陕西西安710077

提出了一种基于电网电压补偿的多电平变频器控制方法 ,从主回路拓扑结构出发 ,以低压变频器规则采样法为基本理论 ,详细介绍了适合于多电平变频器控制的理论分析和算法推导过程。并给出了适合数字信号处理的采样原理和采样时序。直接根... 详细信息

提出了一种基于电网电压补偿的多电平变频器控制方法 ,从主回路拓扑结构出发 ,以低压变频器规则采样法为基本理论 ,详细介绍了适合于多电平变频器控制的理论分析和算法推导过程。并给出了适合数字信号处理的采样原理和采样时序。直接根据电网电压的变化 ,实时调节输出电压 ,能获得与闭环系统相媲美的理想机械特性和运行效果。该方法不仅具有计算步骤简单、输出 SPWM对称性好、精度高和控制方便的特点 ,而且适用于任何电平数目及拓扑结构。试验结果表明 ,和其他多电平控制方法相比 ,使用效果好 ,有很高的利用价值。

关键词：电网电压补偿多电平变频器采样 SPWM