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Hydrophobic long-chain two-dimensional perovskite scintillators for underwater X-ray imaging

Rare Metals 2024年第1期43卷 175-185页

作者： Jin-Xiao Zheng Zi-An Zhou Tiao Feng Hui li Cheng-hua Sun NüWang Yang Tian yong Zhao Shu-Yun Zhou Key Laboratory of Photochemical Conversion and Optoelectronic Materials Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China Laboratory of Bioinspired Smart Interfacial Science and Technology of the Ministry of Education Beijing Key Laboratory of Bioinspired Energy Materials and DevicesSchool of ChemistryBeijing Advanced Innovation Center for Biomedical EngineeringBeihang UniversityBeijing 100191China Department of Engineering Physics Tsinghua University and Key Laboratory of Particle and Radiation Imaging Ministry of EducationTsinghua UniversityBeijing 100084China e-mail:yangt@***

The underwater X-ray imaging technology development is significant to subaqueous target reconnaissance/detection/identification, subfluvial archaeology,submerged resource exploration, etc. As the core of X-ray imaging detection, the scintillator has been plagued by inherent moisture absorption and decomposition, and strict requirements for seamless packaging and ***, we designed a manganese-doped two-dimensional(2D) perovskite scintillator modified by hydrophobic longchain organic amine through the combination of component and doping engineering. The modified perovskites show high water repellency that can be used as an underwater X-ray scintillator. X-ray images of aquatic organisms or other objects with a high spatial resolution of10 lp·mm^(-1) at a big view field(32 mm × 32 mm) were obtained by scintillation screen. This hydrophobic perovskite scintillator based on molecular design is of great promise in underwater X-ray nondestructive testing technology development.

关键词： Two-dimensional perovskite Hydrophobic Scintillators Underwater X-ray imaging Underwater nondestructive testing technology

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Carbon dots-derived three-dimensional-ordered macroporous host with high penetrability and catalytic activity for LSBs under lean electrolyte

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Rare Metals 2024年第6期43卷 2560-2573页

作者： Jiao-Zi Duan hua-Yu Pei Quan Yang Xue li Xin Ba Xue yong Jun-ling Guo Si-Yu Lu Green Catalysis Center College of ChemistryZhengzhou UniversityZhengzhou 450001China Country State Center for International Cooperation On Designer Low-Carbon&Environmental Materials School of Materials Science and EngineeringZhengzhou UniversityZhengzhou 450001China Hubei Institute of Quality Supervision Inspection Wuhan 430061China Department of Chemistry University of SheffieldSheffeld S37HFUK

The practical energy density of lithium-sulfur batteries(LSBs)is seriously limited by the high electrolyte-to-sulfur ratios(E/S).The E/S can be reduced by employing hosts with easy-to-infiltrate structure that ensures the uniform distribution of a lean electrolyte and high catalytic activity that can suppress"shuttle effect"via accelerating the slow conversion of soluble poly sulfides to insoluble *** the easy-to-infiltrate structures,the three-dimensional-ordered macroporous(3DOM)structure is easier to scale preparation and more suitable for the existing industrial ***,it is difficult to obtain the 3DOM with(1)high penetrability due to the high viscosity of frequently-used organic polymer precursors and(2)high catalytic activity due to the low confinement effect,meaning that uniformly dispersed small-sized catalytic materials are difficult to load on ***,using carbon dots(CDs)with both organic and inorganic properties as a precursor and aggregation limiting agent,a 3DOM host with high penetrability and homodispersed Ni particles of small sizes(Ni-CDs-3DOM)was *** this host:(1)CDs precursor with suitable viscosity can improve the penetrability.(2)CDs can effectively inhibit the agglomeration of Ni particles.(3)Uniformly dispersed small-size Ni particles offer high-efficiency catalytic activity toward sulfur ***,the Ni-CDs-3DOM/sulfur cathode exhibits high sulfur utilization and stable cycling performance even under high sulfur loading(5.5 mg·cm^(-2))and low E/S(6.5μl·mg^(-1)).This work indicates the usefulness of CDs in constructing hosts for LSBs with high energy density.

关键词： lithium-sulfur batteries Carbon dots Catalytic action Easy-to-infiltrate structure Lean electrolyte

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东平湖表层沉积物重金属环境容量评价及趋势预测

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物探与化探 2024年第4期48卷 1146-1156页

作者：于林松胡蕾王东平刘辉陈子万李华勇邓焕广安阳师范学院资源环境与旅游学院河南安阳455000 山东省地质勘查工程技术研究中心山东济南250013 山东省物化探勘查院山东济南250013 云南省地质调查院云南昆明650216 聊城大学地理与环境学院山东聊城252000

湖泊沉积物环境容量是评价湖泊系统环境承载力的重要指标,可有效反映湖泊系统的稳定性和可持续发展能力。以黄河流域下游东平湖为研究对象,对表层沉积物中的As、Cd、Cr、Co、Cu、Hg、Mn、Ni、Pb、Tl和Zn共11种重金属元素进行采样和测定... 详细信息

湖泊沉积物环境容量是评价湖泊系统环境承载力的重要指标,可有效反映湖泊系统的稳定性和可持续发展能力。以黄河流域下游东平湖为研究对象,对表层沉积物中的As、Cd、Cr、Co、Cu、Hg、Mn、Ni、Pb、Tl和Zn共11种重金属元素进行采样和测定,采用统计分析和GIS技术对重金属含量及环境承载力空间分布进行讨论,并对重金属百年尺度环境容量变化趋势进行预测。结果表明:①研究区沉积物中As最大值超过土壤污染风险筛选值(允许限值),其余元素均低于允许限值。②重金属单项环境容量指数(P i)均值排序为:Hg>Pb>Cr>Ni>Zn>Cd>Cu>Co>Mn>Tl>As,其中As存在过载水平和警戒水平点位,Mn和Tl存在警戒水平点位;经计算,研究区综合容量指数(PI)介于中容量至高容量水平,而以“单项环境容量指数劣等水平”衡量的综合容量等级显示,研究区中容量至过载水平均有分布。③重金属静态年容量限值和动态年容量排序分别为:Mn>Zn>Cr>Ni>Cu>Pb>As>Co>Tl>Cd>Hg和Mn>Zn>Cr>Ni>Pb>Cu>Co>As>Hg>Cd>Tl;静态年容量限值和动态年容量分别在5~40年和5~15年年限内呈现由陡倾转缓的降低趋势,之后趋于平缓稳定;不同年限平均动态年容量均大于静态年容量限值,表现出对环境的容纳承载能力较好。本研究揭示了东平湖环境容量现状及未来变化趋势,可为湖泊环境质量评价和生态保护修复提供科学依据。

关键词：表层沉积物重金属环境容量趋势预测东平湖

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On the bounds of frequency-selective channel capacity with doubly correlated geometrical MIMO channel model

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The Journal of China Universities of Posts and Telecommunications 2010年第2期17卷 8-13页

作者： li yong-hua , Lü Tie-jun, WU Xiao-fei, ZHANG lin Key Laboratory of Universal Wireless Communications, Ministry of Education, Beijing University of Posts and Telecommunications, Beijing 100876, China Key Laboratory of Universal Wireless Communications Ministry of Education Beijing University of Posts and Telecommunications Beijing 100876 China

The multi-input multi-output （MIMO） technology plays an important role in link transmissions. This article considers the general case for the ergodic capacity in doubly correlated frequency-selective MIMO channel. In the study, the geometrical MIMO channel model is presented. Based on the formula of MIMO ergodic capacity, the capacity limits are studied with arbitrary finite number of antennas in the frequency-selective MIMO channel. It first derives the exact expressions for the upper bound and lower bound in doubly correlated MIMO channel. The results for the single-ended correlation and independent identically distributed （i.i.d.） MIMO channel are also obtained as special cases. Then the simple expressions of the capacity bounds are attained at high SNR. Finally, results are provided by Monte Carlo simulations to verify the tightness of the derived bounds.

关键词： MIMO correlation capacity bounds

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Alarm Log Data Augmentation Algorithm Based on a GAN Model and Apriori

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Journal of Computer Science & Technology 2024年第4期39卷 951-966页

作者： Yang Yang Yu-Ting li yong-hua Huo Zhi-Peng Gao Lan-Lan Rui State Key Laboratory of Network and Switching Technology Beijing University of Posts and TelecommunicationsBeijing 100876China The 54th Research Institute of China Electronics Technology Group Corporation Shijiazhuang 050081China

The complexity of alarm detection and diagnosis tasks often results in a lack of alarm log *** to the strong rule associations inherent in alarm log data,existing data augmentation algorithms cannot obtain good results for alarm log *** address this problem,this paper introduces a new algorithm for augmenting alarm log data,termed APRGAN,which combines a generative adversarial network(GAN)with the Apriori *** generates alarm log data under the guidance of rules mined by the rule ***,we propose a new dynamic updating mechanism to alleviate the mode collapse problem of the *** addition to updating the real reference dataset used to train the discriminator in the GAN,we dynamically update the parameters and the rule set of the Apriori algorithm according to the data generated in each *** extensive experimentation on two public datasets,it is demonstrated that APRGAN surpasses other data augmentation algorithms in the domain with respect to alarm log data augmentation,as evidenced by its superior performance on metrics such as BLEU,ROUGE,and METEOR.

关键词： data augmentation alarm log data Apriori generative adversarial network(GAN)

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Development of a Decision Aid for Family Surrogate Decision Makers of Critically Ill Patients Requiring Renal Replacement Therapy in ICU:A User-Centered Design for Rapid Prototyping

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Chinese Medical Sciences Journal 2024年第2期39卷 91-101页

作者： Miao Zheng yong-Hui Zhang Ying Cao Chang-lin Yin li-hua Wang Department of Outpatient First Affiliated Hospital of Army Medical UniversityChongqing 400038China Department of Critical Care Medicine First Affiliated Hospital of Army Medical UniversityChongqing 400038China Administration Office First Affiliated Hospital of Army Medical UniversityChongqing 400038China

Objectives Renal replacement therapy(RRT)is increasingly adopted for critically ill patients diagnosed with acute kidney injury,but the optimal time for initiation remains unclear and prognosis is uncertain,leading to medical complexity,ethical conflicts,and decision dilemmas in intensive care unit(ICU)*** study aimed to develop a decision aid(DA)for the family surrogate of critically ill patients to support their engagement in shared decision-making process with *** Development of DA employed a systematic process with user-centered design(UCD)principle,which included:(i)competitive analysis:searched,screened,and assessed the existing DAs to gather insights for design strategies,developmental techniques,and functionalities;(ii)user needs assessment:interviewed family surrogates in our hospital to explore target user group's decision-making experience and identify their unmet needs;(iii)evidence syntheses:integrate latest clinical evidence and pertinent information to inform the content development of *** The competitive analysis included 16 relevant DAs,from which we derived valuable insights using existing *** decision needs were explored among a cohort of 15 family surrogates,revealing four thematic issues in decision-making,including stuck into dilemmas,sense of uncertainty,limited capacity,and delayed decision confirmation.A total of 27 articles were included for evidence *** decision making knowledge on disease and treatment,as delineated in the literature sourced from decision support system or clinical guidelines,were formatted as the foundational knowledge ***-one items of evidence were extracted and integrated into the content panels of benefits and risks of RRT,possible outcomes,and reasons to *** DA was drafted into a web-based phototype using the elements of *** platform could guide users in their preparation of decision-making through a sequential four-step process:identifying

关键词： decision aids renal replacement therapy intensive care units shared decision-making user-centered design surrogate

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Strong Solutions of an Incompressible Phase-field Model with Variable Density

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Acta Mathematicae Applicatae Sinica 2024年

作者： Ying-hua li yong WANG Han-bin CAI School of Mathematical Sciences South China Normal University

We study the initial-boundary value problem of an incompressible Navier-Stokes-Cahn-Hilliard system with variable density. We prove the existence and uniqueness of the local strong solution in two or three dimensions. Moreover, we establish a two-dimensional blow-up criterion in terms of the temporal integral of the square of maximum norm of velocity.

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Concentration breaking on two optimization problems

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Science China Mathematics 2024年第7期67卷 1555-1570页

作者： yong huang Qinfeng li Qiuqi li School of Mathematics Hunan UniversityChangsha410082China

In the present paper, we study the boundary concentration-breaking phenomena on two thermal insulation problems considered on lipschitz domains, based on Serrin's overdetermined result, the perturbation argument, and a comparison of Laplacian eigenvalues with different boundary conditions. Since neither of the functionals in the two problems is C^(1), another key ingredient is to obtain the global H?lder regularity of minimizers of both problems on lipschitz domains. Also, the exact dependence on the domain of breaking thresholds is given in the first problem, and the breaking values are obtained in the second problem on ball domains, which are related to 2π in dimension 2.

关键词： spectral inequalities symmetry breaking Laplacian eigenvalue

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Bioinspired Double-stranded Yarn with Alternating Hydrophobic/Hydrophilic Patterns for High-efficiency Fog Collection

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Chinese Journal of Polymer Science 2024年第7期42卷 968-975,I0008页

作者： Lan-Lan Hou Meng-Na Qiu Ya-Qiong Wang Tong-hua Bai Zhi-Min Cui Jing-Chong liu Ying-Qun Qi Nü Wang yong li yong Zhao Beijing Institute of Graphic Communication Beijing102600China Key Laboratory of Bioinspired Smart Interfacial Science and Technology of Ministry of Education Beijing Key Laboratory of Bioinspired Energy Materials and DevicesSchool of ChemistryBeijing Advanced Innovation Center for Biomedical EngineeringBeihang UniversityBeijing100191China Key Laboratory of Cryogenics Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing100190China Beijing Key Laboratory for Bioengineering and Sensing TechnologyDaxing Research InstituteSchool of Chemistry and Biological EngineeringUniversity of Science and Technology BeijingBeijing100083China

Efforts to develop innovative water harvesting strategies offer powerful solutions to alleviate the water crisis,especially in remote and arid *** by the hydrophobic/hydrophilic pattern of desert beetles and water self-propulsion property of spider silks,a double-strand hydrophobic PVDF-HFP/hydrophilic PAN nanofibers yarn is proposed by electrospinning and twisting *** double-strand cooperation approach allows for water deposition on hydrophobic PVDF-HFP segment and transport under the asymmetric capillary driving force of hydrophilic PAN segment,thus speeded up the aggregation and growth of *** effects of the composition and the diameter ratio of the two primary yarns were studied and optimized for boosting fog collection *** double-strand anisotropic yarn not only provide an effective method for water harvesting,but also hold the potential to inspire innovative design concepts for fog collection materials in challenging environments.

关键词： Fog collection Wettability Electrospinning Nanofibers Spider silk

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Improving anammox activity and reactor start-up speed by using CO_(2)/NaHCO_(3) buffer

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Journal of Environmental Sciences 2024年第5期139卷 60-71页

作者： Shaoan Cheng huahua li Xinyuan He hua Chen Longxin li State Key Laboratory of Clean Energy Utilization College of Energy EngineeringZhejiang UniversityHangzhou 310027China

Anammox bacteria grow slowly and can be affected by large pH *** suitable buffers could make the start-up of anammox reactors easy and *** this study,the effects of three kinds of buffers on the nitrogen removal and growth characteristics of anammox sludge were *** with CO_(2)/NaHCO_(3)buffer solution(CCBS)performed the best in nitrogen removal,while 4-(2-hydroxyerhyl)piperazine-1-ethanesulfonic acid(HEPES)and phosphate buffer solution(PBS)inhibited the anammox *** with 50 mmol/L CCBS could start up in 20 days,showing the specific anammox activity and anammox activity of 1.01±0.10 gN/(gVSS·day)and 0.83±0.06 kgN/(m^(3)·day),*** Kuenenia was the dominant anammox bacteria,with a relative abundance of 71.8%.Notably,anammox reactors could also start quickly by using 50 mmol/L CCBS under nonstrict anaerobic *** findings are meaningful for the quick start-up of engineered anammox reactors and prompt enrichment of anammox bacteria.

关键词： Anammox bacteria Buffer solution CO_(2)/NaHCO_(3) Physiological characteristics Microbial community shift

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