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Tailoring BaCe0.7Zr0.1(Dy0.1|Yb0.1)0.2O3-δ electrolyte through strategic Cu doping for low temperature proton conducting fuel cells:Envisioned theoretically and experimentally

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Journal of Energy Chemistry 2025年第2期101卷 692-701页

作者： Zaheer Ud Din Babar Muhammad Bilal Hanif yan'an li Wan-Ting Wang Hanchen Tian Cheng-Xin li State Key Laboratory for Mechanical Behavior of Materials School of Materials Science and Engineering Xi'an Jiaotong University Department of Inorganic Chemistry Faculty of Natural Sciences Comenius University Bratislava

This study addresses the challenge of high sintering temperatures in proton-conducting fuel cells（PCFCs）with BaCeO3-doped *** demonstrate that 1 mol% copper（Cu） doping at the B-site of BaCe0.7Zr0.1(Dy0.1|Yb0.1)0.2O3-δ（BCZDYb） improves sintering behavior,enabling densification at1400℃.However,Cu doping disrupts stoichiometry,creating barium vacancies and reducing protonaccepting cations,affecting overall *** mechanism is confirmed through density functional theory（DFT） calculations and various experimental techniques,including crystal structure analysis using X-ray diffraction（XRD） and morphology and elemental analysis via field emission scanning electron microscopy（FESEM） and energy-dispersive X-ray spectroscopy（EDS）.Electrochemical measurements are performed using the electrochemical impedance spectroscopy（EIS）.The ionic conductivity of1 mol% Cu-doped BCZDYb（BCZDYb-1） is 1.49×10-2S cm-1at 650℃,which is～3.58 times higher than that of BCZDYb sintered at 1200℃.The BCZDYb-1 exhibits ～16 times higher grain boundary conductivity when sintered at 1400℃,compared to undoped *** single cell employing BCZDYb-1 as the electrolyte achieved a power density of ～606 mW cm-2at 550℃.These results indicate that a controlled amount of Cu doping can enhance densification while maintaining high ionic co nductivity,making it suitable for practical applications in PCFCs operating at lower temperatures.

关键词： BaCe0.7Zr0.1(Dy0.1|Yb0.1)0.2O3−δ (BCZDYb) Cu-doping Densification Electrical conductivity Proton conducting fuel cells (PCFCs) Sintering

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Hydraulic conductivity over a wide suction range of loess with different dry densities

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Journal of Rock Mechanics and Geotechnical Engineering 2025年第1期17卷 481-492页

作者： Xiaokun Hou Shengwen Qi yan li Fangcui liu Tonglu li Hua li State Key Laboratory of lithospheric and Environmental Coevolution Institute of Geology and GeophysicsChinese Academy of SciencesBeijing100029China University of Chinese Academy of Sciences Beijing100049China Innovation Academy for Earth Science Beijing100029China School of Civil Engineering University of A CoruñaA Coruña15071Spain Department of Geological Engineering Chang’an UniversityXi’an710054China School of Civil Engineering and Architecture Xi’an Jiaotong University of City CollegeXi’an710018China

Experimental research into the hydraulic conductivity curve (HCC) of unsaturated soil is limited due to the inherent challenge associated with labor, cost, and time. Typically, the HCC is estimated using the soil water characteristic curve (SWCC) based models and saturated hydraulic conductivity (SHC). However, the efficiency of the SWCC-based model is rarely assessed, and the influence of soil density and pore structure on HCC remains incomplete due to limited experimental data. To address this gap, this study employs an innovative filter-paper-based column method, which can measure the HCC over a wide suction range (e.g. 0−105 kPa), to capture the HCCs of both intact and compacted specimens with varying dry densities. The efficiency of two typical SWCC-based models is assessed using the measured data. Meanwhile, the mercury intrusion porosity (MIP) technique is employed to obtain the pore characteristic (i.e. pore size distribution (PSD)) and a method of predicting the HCC using the PSD data is proposed, emphasizing the dominant role of the pore structure in shaping the HCC. The results reveal that the dry density's influence on the HCC is primarily observed within the low suction range, corresponding to variations in the dominant and large pores. In the high suction range, the HCCs align along a linear trajectory when plotted in a log-log format. A notable finding is the overestimation of the HCC obtained from the SWCC-based models using the measured SHC. When the SHC is regarded as a fitting parameter, good agreement is achieved. The adjusted SHC value is typically 0-1 order of magnitude lower than the measured value, and this discrepancy diminishes as dry density increases. On the other hand, the proposed PSD-based model performs well with the measured SHC data. Caution is exercised when using the SHC to estimate the HCC for modeling water movement in partially saturated soil.

关键词： Hydraulic conductivity curve Wide suction range Dry density Pore size distribution Saturated hydraulic conductivity

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On the existence of solutions for prescribing fractional Q-curvature problem on S~n

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Acta Mathematica Sinica,English Series 2025年

作者： yan li Zhongwei TANG College of Science China University of Petroleum(Beijing) School of Mathematical Sciences Laboratory of Mathematics and Complex Systems MOEBeijing Normal University

The aim of this paper is to investigate the existence of solutions to the prescribing fractional Q-curvature problem on S~n under some reasonable assumption of the Laplacian sign at the critical point of prescribing curvature function K. Due to the lack of compactness, we choose to return to the basic elements of variational theory and study the deformation along the flow lines. The novelty of the paper is that we obtain the existence without assuming any symmetry and periodicity on K. In addition,to overcome the loss of compactness for high-order operator problem, we need more delicate estimates with the second order cases.

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Broadband low-frequency sound absorption of multifunctional composite metastructure

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Science China(Technological Sciences) 2025年第2期68卷 114-124页

作者： Yilong yanG Shanshan liU yan li Tong GAO Yongdong PAN Yong li Yabin JIN School of Aerospace Engineering and Applied Mechanics Tongji UniversityShanghai 200092China State International Joint Research Center of Aerospace Design and Additive Manufacturing Northwestern Polytechnical UniversityXi’an 710072China Institute of Acoustics School of Physics Science and EngineeringTongji UniversityShanghai 200092China Shanghai Key Laboratory of Intelligent Sensing and Detection Technology School of Mechanical and Power EngineeringEast China University of Science and TechnologyShanghai 200237China Shanghai Institute of Aircraft Mechanics and Control Shanghai 200092China

In this study,we fabricated multifunctional metastructures from carbon fiber-reinforced plastic composites using additive manufacturing *** metastructures are characterized by their lightweight,load-bearing capacity,and broadband low-frequency sound absorption *** metastructure consists of 36 unit cells,and non-local coupling mechanism was considered for designing the sound absorption *** developed an acoustic impedance theory tailored for the metastructure,facilitating an analysis of thermal and viscous dissipation *** is proven theoretically and experimentally that the proposed composite metastructure can achieve a noise reduction with an average sound absorption coefficient greater than 0.9 across frequencies in the rage of 330-1500 *** also studied the metastructure’s quasi-static and cyclic compression performance,confirming its efficient absorption capabilities after cyclic *** proposed design and additive manufacturing method for composite metastructures provides a novel pathway for creating lightweight,multifunctional structures with diverse applications,such as aerospace engineering.

关键词： composite metastructure broadband sound absorption additive manufacturing

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Hierarchical Polyimide Nonwoven Fabric with Ultralow-Reflectivity Electromagnetic Interference Shielding and High-Temperature Resistant Infrared Stealth Performance

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Nano-Micro Letters 2025年第4期17卷 111-129页

作者： Xinwei Tang Yezi Lu Shuangshuang li Mingyang Zhu Zixuan Wang yan li Zaiyin Hu Penglun Zheng Zicheng Wang Tianxi liu The Key Laboratory of Synthetic and Biological Colloids Ministry of EducationSchool of Chemical and Material EngineeringInternational Joint Research Laboratory for Nano Energy CompositesJiangnan UniversityWuxi 214122JiangsuPeople’s Republic of China Jiangsu Ferrotec Semiconductor Technology Co. Ltd.Yancheng 214000JiangsuPeople’s Republic of China Guizhou Aerospace Wujiang Electro-Mechanical Equipment Co. Ltd.No.20-5Dalian Road Aerospace Industrial ParkHuichuan DistrictZunyi City 563000GuizhouPeople’s Republic of China Civil Aircraft Fire Science and Safety Engineering Key Laboratory of Sichuan Province College of Civil Aviation Safety EngineeringCivil Aviation Flight University of ChinaGuanghan 618307SichuanPeople’s Republic of China

Designing and fabricating a compatible low-reflectivity electromagnetic interference(EMI)shielding/high-temperature resistant infrared stealth material possesses a critical significance in the field of ***,a hierarchical polyimide(PI)nonwoven fabric is fabricated by alkali treatment,in-situ growth of magnetic particles and"self-activated"electroless Ag plating ***,the hierarchical impedance matching can be constructed by systematically assembling Fe_(3)O_(4)/Ag-loaded PI nonwoven fabric(PFA)and pure Ag-coated PI nonwoven fabric(PA),endowing it with an ultralowreflectivity EMI shielding *** addition,thermal insulation of fluffy three-dimensional(3D)space structure in PFA and low infrared emissivity of PA originated from Ag plating bring an excellent infrared stealth *** importantly,the strong bonding interaction between Fe_(3)O_(4),Ag,and PI fiber improves thermal stability in EMI shielding and high-temperature resistant infrared stealth *** excellent comprehensive performance makes it promising for military tents to protect internal equipment from electromagnetic interference stemmed from adjacent equipment and/or enemy,and inhibit external infrared detection.

关键词： Polyimide Electromagnetic interference shielding Low reflectivity Infrared stealth Compatibility

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From steroidal glycoalkaloids to steroidal saponins:Biosynthesis and ecological role in the Solanum genus

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Molecular Plant 2025年第1期18卷 22-24页

作者： yan li Jie Luo School of Breeding and Multiplication(Sanya Institute of Breeding and Multiplication) Hainan UniversitySanya 572025China Yazhouwan National Laboratory Sanya 572025China

Solanaceae plants produce two major classes of valuable steroid-derived specialized metabolites:steroidal glycoalkaloids(SGAs)and steroidal saponins(STSs)(Grzech et al.,2025).SGAs are crucial in plant defense despite their anti-nutritional effects on *** also exhibit diverse biological activities,including anti-cancer,anti-microbial,anti-inflammatory,anti-viral,and anti-pyretic activities(Lucier et al.,2024).Similarly,STSs have garnered significant interest from the pharmaceutical,cosmetic,and food industries for many years due to their detergent-like properties(Grzech et al.,2025).However,the ecological roles of STSs are still unknown,and efforts to reconstitute the biosynthesis of SGAs and STSs in heterologous hosts have not been successful.A recent work,published in Science by Sarah E.O’Connor and Prashant ***’s team,unveils a cellulose synthase-like protein(GLYCOALKALOID METABOliSM15[GAME15])that is required for the biosynthesis of both SGAs and STSs and provides the first definitive evidence for STSs’role in plant defense(Boccia et al.,2024).This discovery elucidates the entire biosynthetic pathway of SGAs and STSs,opening up new opportunities for their metabolic engineering.

关键词： steroidal alkaloids saponins

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Exploring Mechanism of Electroacupuncture in Modulating Neuroinflammation Based on Intestinal Flora and Its Metabolites

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Chinese Journal of Integrative Medicine 2025年第2期31卷 183-192页

作者： YE Hai-min li Zhuo-yan ZHANG Peng KANG Zhen ZHOU De-sheng School of Integrated Chinese and Western Medicine Hunan University of Chinese MedicineChangsha(410208)China Neurology Department The Second Affiliated Hospital of Hunan University of Chinese MedicineChangsha(410005)China Acupuncture and Moxibustion Massage Rehabilitation Department The Second Affiliated Hospital of Hunan University of Chinese MedicineChangsha(410005)China Neurology Department The First Hospital of Hunan University of Chinese MedicineChangsha(410011)China

Neuroinflammatory responses play an important role in the pathogenesis of various diseases,particularly those affecting the central nervous *** of neuroinflammation is a crucial therapeutic strategy for the management of central nervous system *** intestinal microbial-gut-brain axis serves as a key regulatory pathway that modulates neuroinflammatory *** flora metabolites such as short-chain fatty acids,indoles and their derivatives,lipopolysaccharides,trimethylamine oxide,and secondary bile acids exert direct or indirect effects on *** have shown that electroacupuncture(EA)modulates the composition of the intestinal microbiota and its metabolites,while also suppressing neuroinflammation by targeting the TLR4/NF-κB,NLRP3/caspase-1,and microglial cell M2-type transformation *** review discusses the mechanisms by which EA regulates neuroinflammation via intestinal microbiota and its metabolites,providing information and a foundation for further investigation of the precise therapeutic mechanisms of EA in neurological disorders.

关键词： electroacupuncture intestinal flora metabolites of intestinal flora neuroinflammation nervous system disease review

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A smart finger patch with coupled magnetoelastic and resistive bending sensors

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Journal of Semiconductors 2025年第1期46卷 194-203页

作者： Ziyi Dai Mingrui Wang Yu Wang Zechuan Yu yan li Weidong Qin Kai Qian School of Integrated Circuits Shandong UniversityJinan 250100China Department of Mechanical Engineering University of AucklandAuckland 1010New Zealand Department of Urology Qilu Hospital of Shandong UniversityJinan 250100China Shenzhen Research Institute of Shandong University Shenzhen 518000China Department of Critical Care Medicine Qilu hospital of Shandong universityJinan 250100China

In the era of Metaverse and virtual reality(VR)/augmented reality(AR),capturing finger motion and force interactions is crucial for immersive human-machine *** study introduces a flexible electronic skin for the index finger,addressing coupled perception of both state and process in dynamic tactile *** device integrates resistive and giant magnetoelastic sensors,enabling detection of surface pressure and finger joint *** e-skin identifies three phases of finger action:bending state,dynamic normal force and tangential force(sweeping).The system comprises resistive carbon nanotubes(CNT)/polydimethylsiloxane(PDMS)films for bending sensing and magnetoelastic sensors(NdFeB particles,EcoFlex,and flexible coils)for pressure *** inward bending resistive sensor,based on self-assembled microstructures,exhibits directional specificity with a response time under 120 ms and bending sensitivity from 0°to 120°.The magnetoelastic sensors demonstrate specific responses to frequency and deformation magnitude,as well as sensitivity to surface roughness during sliding and material *** system’s capability is demonstrated through tactile-based bread type and condition recognition,achieving 92%*** intelligent patch shows broad potential in enhancing interactions across various fields,from VR/AR interfaces and medical diagnostics to smart manufacturing and industrial automation.

关键词： human machine interface flexible sensor wearable sensor giant magnetoelastic effect inward bending sensor

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High-energy-density lithium manganese iron phosphate for lithium-ion batteries:Progresses,challenges,and prospects

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Journal of Energy Chemistry 2025年第1期100卷 1-17页

作者： Bokun Zhang Xiaoyun Wang Shuai Wang yan li libo Chen Handong Jiao Zhijing Yu Jiguo Tu State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China Research Institute for Intelligent Wearable Systems The Hong Kong Polytechnic University Hong Kong 9977China Institute of Advanced Structure Technology Beijing Institute of TechnologyBeijing 100081China

The soaring demand for smart portable electronics and electric vehicles is propelling the advancements in high-energy–density lithium-ion *** manganese iron phosphate(liMn_(x)Fe_(1-x)PO_(4))has garnered significant attention as a promising positive electrode material for lithium-ion batteries due to its advantages of low cost,high safety,long cycle life,high voltage,good high-temperature performance,and high energy *** liMn_(x)Fe_(1-x)PO_(4)has made significant breakthroughs in the past few decades,there are still facing great challenges in poor electronic conductivity and li-ion diffusion,manganese dissolution affecting battery cycling performance,as well as low tap *** review systematically summarizes the reaction mechanisms,various synthesis methods,and electrochemical properties of liMn_(x)Fe_(1-x)PO_(4)to analyze reaction processes accurately and guide material ***,the main challenges currently faced are concluded,and the corresponding various modification strategies are discussed to enhance the reaction kinetics and electrochemical performance of liMn_(x)Fe_(1-x)PO_(4),including multi-scale particle regulation,heteroatom doping,surface coating,as well as microscopic morphology ***,in view of the current research challenges faced by intrinsic reaction processes,kinetics,and energy storage applications,the promising research directions are *** importantly,it is expected to provide key insights into the development of high-performance and stable liMn_(x)Fe_(1-x)PO_(4)materials,to achieve practical energy storage requirements.

关键词： lithiummanganese iron phosphate High energydensity lithium-ionbatteries Reactionmechanism Tap density

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Activation of adult endogenous neurogenesis by a hyaluronic acid collagen gel containing basic fibroblast growth factor promotes remodeling and functional recovery of the injured cerebral cortex

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Neural Regeneration Research 2025年第10期20卷 2923-2937页

作者： yan li Peng Hao Hongmei Duan Fei Hao Wen Zhao Yudan Gao Zhaoyang yang Kwok-Fai So Xiaoguang li Department of Neurobiology School of Basic Medical SciencesCapital Medical UniversityBeijingChina China Rehabilitation Science Institute China Rehabilitation Research CenterBeijing Key Laboratory of Neural Injury and RehabilitationBeijingChina Center of Neural Injury and Repair Beijing Institute for Brain DisordersBeijingChina Beijing Key Laboratory for Biomaterials and Neural Regeneration School of Engineering MedicineBeihang UniversityBeijingChina Guangdong-HongKong-Macao Institute of CNS Regeneration Ministry of Education CNS Regeneration Collaborative Joint LaboratoryJinan UniversityGuangzhouGuangdong ProvinceChina Bioland Laboratory(Guangzhou Regenerative Medicine and Health Guangdong Laboratory) GuangzhouGuangdong ProvinceChina Department of Ophthalmology and State Key Laboratory of Brain and Cognitive Sciences The University of Hong KongHong Kong Special Administration RegionChina Center for Brain Science and Brain-Inspired Intelligence Guangdong-HongKong-Macao Greater Bay AreaGuangzhouGuangdong ProvinceChina Co-innovation Center of Neuroregeneration Nantong UniversityNantongJiangsu ProvinceChina Department of Biomedical Engineering School of Biological Science and Medical EngineeringBeihang UniversityBeijingChina

The presence of endogenous neural stem/progenitor cells in the adult mammalian brain suggests that the central nervous system can be repaired and regenerated after ***,whether it is possible to stimulate neurogenesis and reconstruct cortical layers II to VI in non-neurogenic regions,such as the cortex,remains *** this study,we implanted a hyaluronic acid collagen gel loaded with basic fibroblast growth factor into the motor cortex immediately following traumatic *** findings reveal that this gel effectively stimulated the proliferation and migration of endogenous neural stem/progenitor cells,as well as their differentiation into mature and functionally integrated ***,these new neurons reconstructed the architecture of cortical layers II to VI,integrated into the existing neural circuitry,and ultimately led to improved brain *** findings offer novel insight into potential clinical treatments for traumatic cerebral cortex injuries.

关键词： adult endogenous neurogenesis basic fibroblast growth factor-hyaluronic acid collagen gel cortical remodeling functional recovery migration motor cortex injury neural circuits neural stem cells newborn neurons proliferation

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