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Comparison of dark energy models:A perspective from the latest observational data

中国科学：物理学、力学、天文学英文版 2010年第9期53卷 1631-1645页

作者： li miao1,2,li xiaodong2,3 & zhang xin1,4.1kavli institute for theoretical physics china,{4.,Beijing 100190,china 2Key Laboratory of Frontiers in theoretical physics,institute of theoretical physics,{4.,Beijing 100190,china 3Interdisciplinary Center for theoretical Study,University of Science and Technology of china,Hefei 230026,china 4.epartment of physics,College of sciences,Northeastern University,Shenyang 110004.china kavli institute for theoretical physics {4. Chinese Academy of Sciences Beijing China Key Laboratory of Frontiers in theoretical physics Institute of Theoretical Physics Chinese Academy of Sciences Beijing China Interdisciplinary Center for theoretical Study University of Science and Technology of China Hefei China Department of physics College of Sciences Northeastern University Shenyang China

We compare some popular dark energy models under the assumption of a flat universe by using the latest observational data including the type Ia supernovae Constitution compilation,the baryon acoustic oscillation measurement from the Sloan Digital Sky Survey,the cosmic microwave background measurement given by the seven-year Wilkinson Microwave Anisotropy Probe observations and the determination of H0 from the Hubble Space *** comparison statistics such as the Bayesian and Akaike information criteria are applied to assess the worth of the *** statistics favor models that give a good fit with fewer *** on this analysis,we find that the simplest cosmological constant model that has only one free parameter is still preferred by the current *** other dynamical dark energy models,we find that some of them,such as the αdark energy,constant w,generalized Chaplygin gas,Chevalliear-Polarski-linder parametrization,and holographic dark energy models,can provide good fits to the current data,and three of them,namely,the Ricci dark energy,agegraphic dark energy,and Dvali-Gabadadze-Porrati models,are clearly disfavored by the data.

关键词： dark energy models observational constraints model comparison information criteria

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Heteroatom tuning in agarose derived carbon aerogel for enhanced potassium ion multiple energy storage

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Carbon Energy 2024年第3期6卷 239-254页

作者： Kaijun Xie xin liu Haolin li Long Fang Kai Xia Dongjiang Yang Yihui Zou {4. zhang State Key Laboratory of Bio-fibers and Eco-textiles Shandong Collaborative Innovation Center of Marine Biobased Fibers and Ecological TextilesInstitute of Marine Biobased MaterialsCollege of Chemistry and Chemical EngineeringCollege of Environmental Science and EngineeringQingdao UniversityQingdaoChina

The incorporation of heteroatoms into carbon aerogels(CAs)can lead to structural distortions and changes in active sites due to their smaller size and electronegativity compared to pure ***,the evolution of the electronic structure from single-atom doping to heteroatom codoping in CAs has not yet been thoroughly investigated,and the impact of codoping on potassium ion(K+)storage and diffusion pathways as electrode material remains *** this study,experimental and theoretical simulations were conducted to demonstrate that heteroatom codoping,composed of multiple heteroatoms(O/N/B)with different properties,has the potential to improve the electrical properties and stability of CAs compared to single-atom *** states near the Fermi level have revealed that doping with O/N/B generates a greater number of active centers on adjacent carbon atoms than doping with O and O/N *** a result of synergy with enhanced wetting ability(contact angle of 9.26°)derived from amino groups and hierarchical porous structure,ON-CA has the most optimized adsorption capacity(−1.62 eV)and diffusion barrier(0.12 eV)of K^(+).The optimal pathway of K^(+)in ON-CA is along the carbon ring with N or O *** K^(+)storage material for supercapacitors and ion batteries,it shows an outstanding specific capacity and capacitance,electrochemical stability,and rate ***,the assembled symmetrical K^(+)supercapacitor demonstrates an energy density of 51.8 Wh kg^(−1),an ultrahigh power density of 4.3Wkg^(−1),and outstanding cycling stability(maintaining 83.3%after 10,000 cycles in 1M KPF6 organic electrolyte).This research provides valuable insights into the design of highperformance potassium ion storage materials.

关键词： agarose carbon aerogels O/N/B codoping potassium-ion battery potassium-ion supercapacitor

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Single-atom-mediated electron islands boost photocatalytic CO_(2)chemical fixation

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Science china Chemistry 2024年第7期67卷 2292-2299页

作者： Shu Shang Lei li xin He Hui Wang lirong Zheng Wei Shao xiaodong {4. Yi Xie Hefei National Research Center for Physical sciences at the Microscale University of Science and Technology of ChinaHefei 230026China institute of Energy Hefei Comprehensive National Science CenterHefei 230031China Beijing Synchrotron Radiation Facility Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China School of Chemistry and Chemical Engineering Hefei Normal UniversityHefei 230031China

Photocatalytic cycloadditions of CO_(2)with epoxides are emerging as a significant platform for the green synthesis of valuable carbonates,where efficient catalytic systems with spatially separated charge carriers are ***,a single p-block metal atom is proposed to be a candidate for photogenerated electron localization on a metal oxide *** taking the Bi single-atom supported on ZnO nanosheet(Bi1/ZnO)as an example,we show that the Bi atom plays the role of an electron island in the sea of delocalized holes within ***,the as-formed electron island could readily promote the rate-determining ring-opening process of cycloaddition *** from the unique spatially separated electrons and holes,the Bi1/ZnO achieves a high yield of cyclic carbonates with almost 100%*** study provides a pioneering strategy for enhancing the performances of photocatalytic CO_(2)chemical fixation.

关键词： electron islands CO_(2)photofixation photogenerated charge carriers

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Fabrication of MXene-Bi_(2)WO_(6)heterojunction by Bi_(2)Ti_(2)O_(7)hinge for extraordinary LED-light-driven photocatalytic performance

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Nano Research 2024年第6期17卷 4729-4736页

作者： Zhiwen li liangliang Xu Zaheer Ud Din Babar Ali Raza Yifei {4. xinrui Gu Yu-xin miao Zhen Zhao Gao li institute of Catalysis for Energy and Environment College of Chemistry and Chemical EngineeringShenyang Normal UniversityShenyang 110034China State Key Laboratory of Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China Scuola Superiore Meridionale(SSM) University of Naples Federico IILargo S.Marcellino1080138Italy Department of Chemical and Biomolecular Engineering Korea Advanced Institute of Science and Technology(KAIST)Daejeon 34141Republic of Korea University of chinese academy of sciences Beijing 100049China

Heterojunction composites with intimate interfaces can shorten the diffusion distance,which leads to a shorter path for photogenerated carriers,thereby increasing photocatalytic ***,we report the fabrication of Ti_(3)C_(2)-Bi_(2)WO_(6)(TC-BW)heterojunctions hinged by Bi_(2)Ti_(2)O_(7)joints via an in situ hydrothermal reaction of Ti_(3)C_(2)in the presence of Na_(2)WO_(4.and Bi(NO_(3))_(3).The TC-BW was characterized using X-ray diffraction(XRD),scanning transmission electron microscopy(STEM),and Raman ***-BW showed superior photocatalytic activity(productivity over 15TC-WB reaches up to 5.0 mmolreacted BA·gcat.^(−1)·h^(−1))in the oxidation of benzyl alcohol using light-emitting diode(LED)light,arising from the surface defects and intimate heterojunction interface between the Ti_(3)C_(2)MXene and Bi_(2)WO_(6)***-BW heterojunctions provide an enhanced separation efficiency of photogenerated charges,which in turn yields superior photocatalytic ***,it is well substantiated by density functional theory(DFT)*** summary,this study elucidates the preparation of heterojunction composites with intimate interfaces for highly efficient photooxidation.

关键词： MXene-Bi_(2)WO_(6) heterojunction LED-light-driven photocatalysis Bi_(2)Ti_(2)O_(7) photooxidation

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A quantum-enhanced magnetometer using a single high-spin nucleus in silicon

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chinese physics B 2024年第9期33卷 110-115页

作者： Tao xin Ke zhang Jun li Shenzhen institute for Quantum Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Guangdong Provincial Key Laboratory of Quantum Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Physikalisch-Technische Bundesanstalt Bundesallee 10038116 BraunschweigGermany institute of Quantum Precision Measurement State Key Laboratory of Radio Frequency Heterogeneous IntegrationShenzhen UniversityShenzhen 518060China College of physics and Optoelectronic Engineering Shenzhen UniversityShenzhen 518060China

Quantum enhanced metrology has the potential to go beyond the standard quantum limit and eventually to the ultimate Heisenberg *** particular,quantum probes prepared in nonclassical coherent states have recently been recognized as a useful resource for ***,there has been considerable interest in constructing magnetic quantum sensors that combine high resolution and high ***,we explore a nanoscale magnetometer with quantum-enhanced sensitivity,based on 123Sb(I=7/2)nuclear spin doped in silicon,that takes advantage of techniques of spin-squeezing and coherent *** the optimal squeezed initial state,the magnetic field sensitivity may be expected to approach 6 aT·Hz^(−1/2)·cm^(−3/2) and 603 nT·Hz^(−1/2) at the single-spin *** magnetic sensor may provide a novel sensitive and high-resolution route to microscopic mapping of magnetic fields as well as other applications.

关键词： quantum magnetometer silicon quantum qubit nuclear electrical resonance

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MXenes/CNTs-based hybrids:Fabrications,mechanisms,and modification strategies for energy and environmental applications

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Nano Research 2024年第5期17卷 3429-3454页

作者： Jizhou Jiang Fangyi li Lei Ding Chengxun zhang Arramel xin li School of Environmental Ecology and Biological Engineering School of Chemistry and Environmental EngineeringKey Laboratory of Green Chemical Engineering Process of Ministry of EducationEngineering Research Center of Phosphorus Resources Development and Utilization of Ministry of EducationNovel Catalytic Materials of Hubei Engineering Research CenterWuhan Institute of TechnologyWuhan 430205China Nano Center Indonesia Jl.PUSPIPTEK Tangerang SelatanBanten 15314Indonesia institute of Biomass Engineering Key Laboratory of Energy Plants Resource and UtilizationMinistry of Agriculture and Rural AffairsSouth China Agricultural UniversityGuangzhou 510642China

Emerging two-dimensional(2D)layered metal carbide and nitride materials,commonly termed MXenes,are increasingly recognized for their applications across diverse fields such as energy,environment,and *** the past few years,MXenes/carbon nanotubes(CNTs)-based hybrids have attracted extensive attention as an important catalyst in energy and environmental fields,due to their superior multifunctions and mechanical *** review aims to address the fabrication strategies,the identification of the enhancement mechanisms,and recent progress regarding the design and modification of MXenes/CNTs-based hybrids.A myriad of fabrication techniques have been systematically summarized,including mechanical mixing,spray drying,three-dimensional(3D)printing,self-assembly/in-situ growth,freeze drying,templating,hydrothermal methods,chemical vapor deposition(CVD),and ***,the identification of the enhancement mechanisms was thoroughly discussed from the two dimensions of theoretical simulations and in-situ ***,the recent advancements in profound applications of MXenes/CNTs-based hybrids have also been carefully revealed,including energy storage devices,sensors,water purification systems,and microwave *** also underscore anticipated challenges related to their fabrication,structure,underlying mechanisms,modification approaches,and emergent ***,this review offers insights into prospective directions and the future trajectory for these promising *** is expected that this review can inspire new ideas or provide new research methods for future studies.

关键词： MXenes/carbon nanotubes(CNTs)-based hybrids fabrication applications modification strategies

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Progress in the preparation and physical properties of two-dimensional Cr-based chalcogenide materials and heterojunctions

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Frontiers of physics 2024年第2期19卷 105-130页

作者： Xiulian Fan Ruifeng xin li li Bo {4. Cheng li Xilong Zhou Huanzhi Chen Hongyan {4. Fangping OuYang Yu Zhou School of physics and Electronics Hunan Key Laboratory of Nanophotonics and DevicesCentral South UniversityChangsha 410083China Jincheng Research institute of Opto-mechatronics Industry Jincheng 048000China Shanxi Key Laboratory of Advanced Semiconductor Optoelectronic Devices and Integrated Systems Jincheng 048000China School of Physical Science and Technology Xinjiang UniversityUrumqi 830046China State Key Laboratory of Powder Metallurgy Central South UniversityChangsha 410083China

Two-dimensional transition metal dichalcogenides(TMDs)exhibit promising application prospects in the domains of electronic devices,optoelectronic devices and spintronic devices due to their distinctive energy band structures and spin−orbit coupling ***-based chalcogenides with narrow or even zero bandgap,covering from semiconductors to metallic materials,have considerable potential for wide-band photodetection and two-dimensional ***,the preparation of 2D CrX_(n)(X=S,Se,Te)nanosheets primarily relies on chemical vapor deposition(CVD)and molecule beam epitaxy(MBE),which enable the production of high-quality large-area *** review article focuses on recent progress of 2D Cr-based chalcogenides,including unique crystal structure of the CrX_(n)system,phase-controlled synthesis,and heterojunction ***,a detailed introduction of room-temperature ferromagnetism and electrical/optoelectronic properties of 2D CrXn is ***,this paper summarizes the challenges associated with utilizing 2D Cr-based chalcogenides in preparation strategies,optoelectronics devices,and spintronic devices while providing further insights.

关键词： physical properties two-dimensional materials Cr-based chalcogenide controlled synthesis heterojunction eletronic and optoelectronic devices

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Predominant types of regional cold waves in North china and their historical changes

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Atmospheric and Oceanic Science Letters 2024年第4期17卷 46-51页

作者： xinyi Cheng Yiyi zhang Jiandong li xin Hao Center for Climate System Prediction Research/Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters/Key Laboratory of Meteorological Disaster Ministry of EducationNanjing University of Information Science&TechnologyNanjingChina Nansen-Zhu International Research Centre Institute of Atmospheric PhysicsChinese Academy of SciencesBeijingChina Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science&TechnologyNanjingChina

寒潮事件对东亚地区的社会经济,生态系统和人体健康影响巨大.根据1980-2019年间10月至次年3月的每日寒潮记录和K-means聚类,本文识别出了中国两种不同类型的区域性寒潮(T1和T2). T1区域性寒潮主要影响东北地区,T2区域性寒潮则主要影响... 详细信息

寒潮事件对东亚地区的社会经济,生态系统和人体健康影响巨大.根据1980-2019年间10月至次年3月的每日寒潮记录和K-means聚类,本文识别出了中国两种不同类型的区域性寒潮(T1和T2). T1区域性寒潮主要影响东北地区,T2区域性寒潮则主要影响华北和东部地区.与T1区域性寒潮相比, T2区域性寒潮强度更强,持续时间更长,影响范围更广. 1980–2019年期间, T1区域性寒潮的频率显著增加,而T2区域性寒潮的频率则没有趋势变化. T1和T2区域性寒潮事件均与西伯利亚高压增强有关,然而与它们相关的对流层中层波列明显不同.在T1区域性寒潮事件发生期间,西伯利亚-蒙古上空出现负-正模态的500-hPa位势高度异常波列,削弱了东亚大槽,导致西伯利亚冷空气东移.T1区域寒潮频次增加趋势可能与全球变暖引起的500-hPa位势高度的线性趋势变化有关.与T2区域寒潮事件相关的波列则在乌拉尔山脉,蒙古和华北地区形成了脊-槽-脊环流异常,导致冷空气向东南方向入侵.本文得出结论,由于两类区域寒潮影响不同,西伯利亚高压增强和对流层中层波列模态在我国区域性寒潮事件的预报中应综合考虑.

关键词：寒潮 K-means聚类西伯利亚高压波列

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Operando measurement of lattice deformation profiles of synchrotron radiation monochromator

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Nuclear Science and Techniques 2024年第7期35卷 8-19页

作者： Yue zhang Zhong-liang li Shang-Yu Si lian Xue Hong-{4. Luo Xiao-Wei zhang Jun Hu Shanghai Synchrotron Radiation Facility Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai201204China ShanghaiTech University Shanghai201210China University of the chinese academy of sciences Beijing100049China Beijing Synchrotron Radiation Facility Institute of High Energy PhysicsChinese Academy of ScienceBeijing100049China

This study presents a new method for characterizing the thermal lattice deformation of a monochromator with high precision under service conditions and first reports the operando measurements of nanoscale thermal lattice deformation on a double-crystal monochromator at different incident *** nanoscale thermal lattice deformation of the monochromator first crystal was obtained by analyzing the intensity of the distorted DuMond *** diagrams of the 333 diffraction index,sensitive to lattice deformation,were obtained directly using a 2D detector and an analyzer crystal orthogonal to the *** increasing incident power and power density,the maximum height of the lattice deformation increased from 3.2 to 18.5 nm,and the deformation coefficient of the maximum height increased from 1.1 to 3.2 nm/*** maximum relative standard deviation was 4.2%,and the maximum standard deviation was 0.1 *** on the measured thermal deformations,the flux saturation phenomenon and critical point for the linear operation of the monochromator were predicted with increasing incident *** study provides a simple solution to the problem of the lower precision of synchrotron radiation monochromator characterizations compared to simulations.

关键词： Synchrotron radiation Monochromator Lattice deformation X-ray dynamic diffraction

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An intrinsically self-healing and anti-freezing molecular chains induced polyacrylamide-based hydrogel electrolytes for zinc manganese dioxide batteries

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Journal of Energy Chemistry 2024年第2期89卷 565-578,I0013页

作者： Haiyang liao Wenzhao Zhong Chen li Jieling Han Xiao Sun xinhui Xia Ting li Abolhassan Noori Mir F.Mousavi xin liu Yongqi zhang institute of Fundamental and Frontier sciences University of Electronic Science and Technology of ChinaChengdu 611731SichuanChina School of Mechanical Engineering Hunan University of TechnologyZhuzhou 412007HunanChina School of Materials Science and Engineering Zhejiang University of TechnologyHangzhou 310014ZhejiangChina Department of Chemistry Faculty of Basic SciencesTarbiat Modares UniversityTehran 14117-13116Iran State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile UniversityWuhan 430200HubeiChina

The anti-freezing strategy of hydrogels and their self-healing structure are often contradictory,it is vital to break through the molecular structure to design and construct hydrogels with intrinsic anti-freezing/self-healing for meeting the rapid development of flexible and wearable devices in diverse service ***,we design a new hydrogel electrolyte(AF/SH-Hydrogel)with intrinsic anti-freezing/self-healing capabilities by introducing ethylene glycol molecules,dynamic chemical bonding(disulfide bond),and supramolecular interaction(multi-hydrogen bond)into the polyacrylamide molecular *** to the exceptional freeze resistance(84.capacity retention at-20℃)and intrinsic self-healing capabilities(95%capacity retention after 5 cutting/self-healing cycles),the obtained AF/SH-Hydrogel makes the zinc||manganese dioxide cell an economically feasible battery for the state-of-the-art *** Zn||AF/SH-Hydrogel||MnO_(2)device offers a near-theoretical specific capacity of 285 m A h g^(-1)at 0.1 A g^(-1)(Coulombic efficiency≈100%),as well as good self-healing capability and mechanical flexibility in an ice *** work provides insight that can be utilized to develop multifunctional hydrogel electrolytes for application in next generation of self-healable and freeze-resistance smart aqueous energy storage devices.

关键词： Flexible aqueous battery Hydrogel electrolyte Anti-freezing Self-healing Dual-dynamic reversible bond

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