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Timing effect of high temperature exposure on the plasticity of internode and plant architecture in maize

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Journal of Integrative Agriculture 2024年第2期23卷 551-565页

作者： binbin li Xianmin Chen Tao Deng Xue Zhao Fang li bingchao Zhang Xin Wang Si shen Shunli Zhou College of Agronomy and Biotechnology China Agricultural UniversityBeijing 100193China China Tobacco Hunan Industrial Corporation Changsha 410019China Innovation Center of Agricultural Technology for Lowland Plain of Hebei Wuqiao 061802China

The occurrence of high temperature(HT)in crop production is becoming more frequent and unpredictable with global warming,severely threatening food *** state of an organ’s growth and development is largely determined by the temperature conditions it is exposed to over *** is the main cereal crop,and its stem growth and plant architecture are closely related to lodging resistance,and especially sensitive to ***,systematic research on the timing effect of HT on the sequentially developing internode and stem is currently *** identify the timing effect of HT on the morphology and plasticity of the stem in maize,two hybrids(Zhengdan 958(ZD958),Xianyu 335(XY335))characterized by distinct morphological traits in the stem were exposed to a 7-day HT treatment from the V6 to V17 stages(Vn presents the vegetative stage with n leaves fully expanded)in *** results demonstrated that exposure to HT during V6-V12 accelerated the rapid elongation of *** instance,HT occurring at V7 and V12 specifically promoted the lengths and weights of the 3rd-5th and 9th-11th internodes,***,HT slowed the growth of internodes adjacent to the promoted ***,compared with control,the plant height was significantly increased soon after HT treatment,but the promotion effect became narrower at the subsequent flowering stage,demonstrating a self-adjusting mechanism in the maize plant in response to ***,HT altered the plant architectures,including a rising of the ear position and increase in the ear position ***335 exhibited greater sensitivity in stem development than ZD958 under HT *** findings improve our systematic understanding of the plasticity of internode and plant architecture in response to the timing of HT exposure.

关键词： maize high temperature internode growth plasticity plant architecture

Salt-assisted vapor-liquid-solid growth of high-quality ultrathin nickel oxide flakes for artificial synapses in image recognition applications

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Nano Research 2024年第5期17卷 4622-4630页

作者： Hui Zhang Zongjie shen Alei li lin Wang Qinan Wang Yunfei li Yunlei Zhong Juntong Zhu Yong Zhang Mengjiao Han Dan Tian Chun Zhao lixing Kang Qingwen li School of Physical Science and Technology Shanghai Tech UniversityShanghai 201210China Division of Advanced Materials Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China College of Energy Soochow Institute for Energy and Materials Innovationsand Key Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu ProvinceSoochow UniversitySuzhou 215123China Songshan Lake Materials Laboratory Dongguan 523808China School of Advanced Technology Xi’an Jiaotong-Liverpool UniversitySuzhou 215123China College of Materials Science and Engineering Co-Innovation Center of Efficient Processing and Utilization of Forest ResourcesNanjing Forestry UniversityNanjing 210037China

Transition metal oxides have attracted intense interest owing to their abundant physical and chemical *** controlled preparation of large-area,high-quality two-dimensional crystals is essential for revealing their inherent properties and realizing high-performance ***,fabricating two-dimensional(2D)transition metal oxides using a general approach still presents substantial ***,we successfully achieve highly crystalline nickel oxide(NiO)flakes with a thickness as thin as 3.3 nm through the salt-assisted vapor-liquid-solid(VLS)growth method,which demonstrated exceptional stability under ambient *** explore the great potential of the NiO crystal in this work,an artificial synapse based on the NiO-flake resistive switching(RS)layer is ***-term and long-term synaptic behaviors are obtained with external *** artificial synaptic performance provides the foundation of the neuromorphic application,including handwriting number recognition based on artificial neuron network(ANN)and the virtually unsupervised learning capability based on generative adversarial network(GAN).This pioneering work not only paves new paths for the synthesis of 2D oxides in the future but also demonstrates the substantial potential of oxides in the field of neuromorphic computing.

关键词： nickel oxide(NiO)flakes vapor-liquid-solid(VLS)growth memristor synapse generative adversarial network(GAN)

A Calculation Method of Double Strength Reduction for Layered Slope Based on the Reduction of Water Content Intensity

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工程与科学中的计算机建模(英文) 2024年第1期138卷 221-243页

作者： Feng shen Yang Zhao bingyi li Kai Wu School of Civil Engineering Suzhou University of Science and TechnologySuzhou215011China R&D Department Suzhou Jcon Greenbuild Fabricated Co.Ltd.Suzhou215004China

The calculation of the factor of safety(FOS)is an important means of slope *** paper proposed an improved double strength reductionmethod(DRM)to analyze the safety of layered *** physical properties of different soil layers of the slopes are different,so the single coefficient strength reduction method(SRM)is not enough to reflect the actual critical state of the *** that the water content of the soil in the natural state is the main factor for the strength of the soil,the attenuation law of shear strength of clayey soil changing with water content is *** paper also establishes the functional relationship between different reduction ***,a USDFLD subroutine is programmed using the secondary development function of finite element *** the relationship between field variables and calculation time realizes double strength reduction applicable to the layered ***,by comparing the calculation results of different examples,it is proved that the stress and displacement distribution of the critical slope state obtained by the improved method is more realistic,and the calculated safety factor is more *** newly proposedmethod considers the difference of intensity attenuation between different soil layers under natural conditions and avoids the disadvantage of the strength reduction method with uniform parameters,which provides a new idea and method for stability analysis of layered and complex slopes.

关键词： Double strength reduction slopes stability water content factor of safety numerical methods

Modulation on electrostatic potential to build a firm bridge at NiO_(x)/perovskite interface for efficient and stable perovskite solar cells

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Journal of Energy Chemistry 2024年第9期96卷 249-258页

作者： Xiangbao Yuan Xufeng ling Hongyu Wang Chengxia shen Ru li Yehao Deng Shijian Chen Chongqing Key Laboratory of Interface Physics in Energy Conversion College of PhysicsChongqing UniversityChongqing 401331China Key Laboratory of Optoelectronic Technology&Systems(Ministry of Education) College of Optoelectronic EngineeringChongqing UniversityChongqing 400044China Center of Modern Physics Institute for Smart City of Chongqing University in LiyangLiyang 213300JiangsuChina

The NiO_(x)/perovskite interface in NiO_(x)-based inverted perovskite solar cells(PSCs)is one of the main issues that restrict device performance and long-term stability,as the unwanted interfacial defects and undesirable redox reactions cause severe interfacial non-radiative recombination and open-circuit voltage(Voc)***,a series of self-assembled molecules(SAMs)are employed to bind,bridge,and stabilize the NiO_(x)/perovskite interface by regulating the electrostatic *** on systematically theoretical and experimental studies,4-pyrazolecarboxylic acid(4-PCA)is proven as an efficient molecule to simultaneously passivate the NiO_(x)and perovskite surface traps,release the interfacial tensile stress as well as quench the detrimental interface redox reactions,thus effectively suppressing the interfacial non-radiative recombination and enhancing the quality of perovskite ***,the PSCs with 4-PCA treatment exhibited an eminently increased Voc,leading to a significant increase in power conversion efficiency from 21.28%to 23.77%.Furthermore,the unencapsulated devices maintain 92.6%and 81.3%of their initial PCEs after storing in air with a relative humidity of 20%–30%for 1000 h and heating at 65℃for 500 h in a N_(2)-filled glovebox,respectively.

关键词： Perovskite solar cells Nickel oxide Interface defects passivation Redox reaction Nonradiative recombination

Visible-light-induced organocatalyzed C（sp2）–H bond functionalization of 1,3-azoles with trifluoroacetylsilanes

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Science China Chemistry 2024年第11期67卷 3662-3668页

作者： Zhengyu li Zeguo Zhang Zhihan Zhang Gang Zhou Yizhi Zhang Shanshan liu Xiao shen The Institute for Advanced Studies Engineering Research Center of Organosilicon Compounds & Materials Ministry of EducationWuhan University College of Chemistry Central China Normal University

Previous carbene insertion to C–H bonds of 1,3-azoles relied on metal carbene species. Herein, we report a metal-free C（sp2）–H bond functionalization of 1,3-azoles with trifluoroacetylsilanes. The reaction features mild conditions, broad substrate scope and wide functional group tolerance. The mechanistic study supports that the success of the reaction is probably attributed to the dual roles of trifluoroacetylsilanes under the photocatalyzed conditions: generating carbenes which undergo cyclopropanation and generating biradicals which promote ring-opening aromatization of the in situ generated fused cyclopropanes.

关键词： C(sp2)–H bond functionalization carbenes biradicals cyclopropanation brook rearrangement

Resolving controversies surrounding carbon sinks from carbonate weathering

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Science China Earth Sciences 2024年第9期67卷 2705-2717页

作者： Xiaoyong BAI Sirui ZHANG Pete SMITH Chaojun li lian XIONG Chaochao DU Yingying XUE Zilin li Mingkang LONG Minghui li Xiaoyun ZHANG Shu YANG Qing LUO Xiaoqian shen State Key Laboratory of Environmental Geochemistry Institute of GeochemistryChinese Academy of SciencesGuiyang 550081China University of Chinese Academy of Sciences Beijing 100049China Institute of Biological and Environmental Sciences University of AberdeenAberdeen AB243UUUK College of Resources and Environmental Engineering Guizhou UniversityGuiyang 550025China School of Geography and Environmental Sciences Guizhou Normal UniversityGuiyang 550025China CAS Center for Excellence in Quaternary Science and Global Change Xi’an 710061China

The importance of carbonate weathering carbon sinks(CCSs)is almost equal to that of vegetation photosynthesis in the global carbon ***,CCSs have become controversial in formulating carbon neutral policies to deal with global climate problems in various countries,since the carbonate dissolution is *** order to address these controversies,we reviewed recent advances in understanding CCSs and examined the outstanding controversies surrounding *** have analyzed the five controversies,revealing the existence of CCSs,quantifying their magnitude,clarifying their spatiotemporal pattern,and documenting how they have increased and how they evolved under the background of global *** addressing these five controversies,we help to bring clarity to the role of CCSs in the carbon cycle of global terrestrial ecosystems.

关键词： Carbon sink Carbonate weathering Carbon cycle Climate change Anthropogenic driver

Ring-Opening Copolymerization of Biorenewable -Caprolactone with trans-Hexahydro-(4,5)-benzofuranone toward Closed-Loop Recyclable Copolyesters and Their Application as Pressure- Sensitive Adhesives

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Chinese Journal of Chemistry 2024年第17期42卷 2035-2042页

作者： Haining Niu liying Wang Zihan Zhang Yalei liu Yong shen Zhibo li State Key Laboratory Base of Eco-Chemical Engineering College of Chemical EngineeringQingdao University of Science and TechnologyQingdaoShandong266042China Key Laboratory of Biobased Polymer Materials Shandong Provincial Education DepartmentQingdao University of Science and TechnologyQingdaoShandong266042China

Copolymerization as an efficient strategy can provide an opportunity to create new closed-loop recyclable polymeric materials with tailored properties that are generally inaccessible to the individual *** this contribution,the bulk ring-opening copolymerization of bio-renewable-caprolactone and trans-hexahydro-(4,5)-benzofuranone was achieved to produce closed-loop recyclable copolyesters by using an organobase/urea binary catalyst at room *** obtained copolyesters exhibited composition-dependent thermal ***,the obtained copolyesters were able to depolymerize back to recover the corresponding monomers under mild conditions.

关键词： Recyclable polymers Ring-opening polymerization Copolymerization Pressure-sensitive adhesives Aliphatic polyesters

Extraction of Eugenol from Essential Oils by In Situ Formation of Deep Eutectic Solvents:A Green Recyclable Process

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Journal of Analysis and Testing 2024年第1期8卷 63-73页

作者： lingqi shen Xiangzi Jin Zhihui Zhang Yuexing Yi Jingyu Zhang Zuguang li College of Chemical Engineering Zhejiang University of TechnologyHangzhou 310014China Department of Chemistry Yanbian UniversityYanji 133002China Transfar Zhilian Co. Ltd.Hangzhou 311215China

Eugenol is extensively utilized in chemical *** actual production,it is mainly separated from clove essential oils(EOs)through acid-base *** this work,a simple,rapid and effective extraction process was developed for the extraction of eugenol from EOs samples by directly forming deep eutectic solvents(DESs)without using acid-base *** proposed process is designed to dissolve EOs in n-hexane and eugenol was highly selective extracted into DESs with tetrabutylammonium chloride(TBAC).Hydrogen bonds in DESs can be broken by addition of water,resulting in a separation of the two phases,thus obtaining a hydrophobic yellowish eugenol in the upper *** quaternary ammonium salt in the lower aqueous solution can be reused after *** most determining influence factors such as the structure of quaternary ammonium salt,the mole ratio of quaternary ammonium salt to eugenol and the amount of n-hexane were *** forming conditions of DESs were studied by Box-Behnken design(BBD).Experiment was carried out under the optimal conditions and good experimental result was demonstrated by the developed process,a high extraction recovery of 92.51% and the purity was about 98.50%,which verifies the excellent performance for the proposed process.

关键词： Eugenol Deep eutectic solvent Essential oils Tetrabutylammonium chloride

A multifunctional flexible sensor based on PI-MXene/SrTiO_(3) hybrid aerogel for tactile perception

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The Innovation 2024年第3期5卷 44-54页

作者： Shihao Deng Yue li shengzhao li shen Yuan Hao Zhu Ju Bai Jingyi Xu Lu Peng Tie li Ting Zhang Nano Science and Technology Institute University of Science and Technology of China(USTC)Suzhou 215123China i-lab Nano-X Vacuum Interconnected WorkstationKey Laboratory of Multifunctional Nanomaterials and Smart SystemsSuzhou Institute of Nano-Tech and Nano-Bionics(SINANO)Chinese Academy of Sciences(CAS)Suzhou 215123China School of Nano-Tech and Nano-Bionics University of Science and Technology of China(USTC)Hefei 230026China Jiangxi Institute of Nanotechnology 278 Luozhu RoadXiaolan Economic and Technological Development ZoneNanchang 330200China

The inadequacy of tactile perception systems in humanoid robotic manipulators limits the breadth of available robotic ***,we designed a multifunctional flexible tactile sensor for robotic fingers that provides capabilities similar to those of human skin sensing *** sensor utilizes a novel PI-MXene/SrTiO_(3) hybrid aerogel developed as a sensing unit with the additional abilities of electromagnetic transmission and thermal insulation to adapt to certain complex ***,polyimide(PI)provides a high-strength skeleton,MXene realizes a pressure-sensing function,and MXene/SrTiO_(3) achieves both thermoelectric and infrared radiation response ***,via the pressure response mechanism and unsteady-state heat transfer,these aerogel-derived flexible sensors realize multimodal sensing and recognition capabilities with minimal *** can differentiate among 13 types of hardness and four types of material from objects with accuracies of 94%and 85%,respectively,using a decision tree *** addition,based on the infrared radiation-sensing function,a sensory array was assembled,and different shapes of objects were successfully *** findings demonstrate that this PI-MXene/SrTiO_(3) aerogel provides a new concept for expanding the multifunctionality of flexible sensors such that the manipulator can more closely reach the tactile level of the human *** advancement reduces the difficulty of integrating humanoid robots and provides a new breadth of application scenarios for their possibility.

关键词： utilize integrating insulation