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The In-Flight Realtime Trigger and Localization Software of GECAM

Research in Astronomy and Astrophysics 2024年第10期24卷 11-24页

作者： xiao-Yun Zhao Shao-lin xiong xiang-Yang Wen xin-Qiao li Ce Cai Shuo xiao Qi Luo Wen-xi Peng Dong-Ya Guo Zheng-Hua An Ke Gong Jin-Yuan liao Yan-Qiu Zhang Yue Huang Lu li xing Wen Fei Zhang Jing Duan Chen-Wei wang Dong-li Shi Peng Zhang Qi-Bin Yi Chao-Yang li Yan-Bing Xu xiao-Hua liang Ya-Qing liu Da-li Zhang xi-Lei Sun Fan Zhang Gang Chen Huan-Yu wang Sheng Yang xiao-Jing liu Min Gao Mao-Shun li Jin-Zhou wang xing Zhou Yi Zhao wang-Chen Xue Chao Zheng Jia-Cong liu xing-Bo Han Jin-ling Qi Jia Huang Ke-Ke Zhang Can Chen xiong-Tao Yang Dong-Jie Hou Yu-Sa wang Rui Qiao xiang Ma xiao-Bo li Ping wang xin-Ying Song li-Ming Song Shi-Jie Zheng Bing li Hong-Mei Zhang Yue Zhu Wei Chen Jian-Jian He Zhen Zhang Jin Hou Hong-jun wang Yan-Chao Hao xiang-Yu wang Zong-Yuan Yang Zhi-Long Wen Zhi Chang Yuan-Yuan Du Rui Gao xiao-Fei Lan Yan-Guo li Gang li Xu-Fang li Fang-jun Lu Hong Lu Bin Meng Feng Shi Hui wang Hui-Zhen wang Yu-Peng Xu Jia-Wei Yang Xue-Juan Yang Shuang-Nan Zhang Chao-Yue Zhang Cheng-Mo Zhang Zhi-Cheng Tang Cheng Cheng Key Laboratory of Particle Astrophysics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China university of Chinese Academy of Sciences Chinese Academy of SciencesBeijing 100049China School of Information Science and Technology Southwest Jiaotong UniversityChengdu 611756China Key Laboratory of Stellar and Interstellar Physics and Department of Physics Xiangtan UniversityXiangtan 411105China Physics and Space Science College China West Normal UniversityNanchong 637002China Department of Astronomy Beijing Normal UniversityBeijing 100875China Innovation Academy for Microsatellites of CAS Shanghai 201203China Changchun university of Science and Technology Changchun 130022China Chinese Academy of Sciences South America Center for Astronomy National Astronomical ObservatoriesCASBeijing 100101China

Realtime trigger and localization of bursts are the key functions of GECAM,an all-sky gamma-ray monitor launched on 2020 December *** developed a multifunctional trigger and localization software operating in the CPU of the GECAM Electronic *** onboard software has the following features:high trigger efficiency for real celestial bursts with a suppression of false triggers caused by charged particle bursts and background fluctuation,dedicated localization algorithm optimized for both short and long bursts,and low time latency of the trigger information which is downlinked through the Global Short Message Communication service of the global BeiDou navigation *** paper provides a detailed description of the design and development of the trigger and localization software system for *** covers the general design,workflow,the main functions,and the algorithms used in the *** paper also includes on-ground trigger tests using simulated gamma-ray bursts generated by a dedicated X-ray tube,as well as an overview of the performance for real celestial bursts during its in-orbit operation.

关键词： telescopes instrumentation:detectors methods:observational

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Proteomic analysis of mitochondria reveals a metabolic switch from fatty acid oxidation to glycolysis in the failing heart

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Science china(life Sciences) 2009年第11期52卷 1003-1010页

作者： wang jun1,2, BAI ling1,2, li Jing3, SUN ChaoFeng1,2, ZHAO Jin1, CUI ChangCong1,2, HAN Ke1,2, liU Yu1,2, ZHUO xiaoZhen1,2, wang TingZhong1,2, liU Ping1,2, FAN Fenling1,2, GUAN YouFei3 & MA AiQun1,2 1 Department of Cardiology, First affiliated hospital of medical college of xi’an Jiaotong university, xi’an 710061, china 2 Ion Channel Disease Laboratory, Key Laboratory of Environment and Genes Related to Diseases of Education Ministry, xi’an 710061, china 3 Department of Physiology and Pathophysiology Key Laboratory of Molecular Cardiovascular Sciences of the Ministry of Education, Peking university Health Science Center, Beijing 100083, china 1. Department of Cardiology First affiliated hospital of medical college of Xi’an Jiaotong University Xi’an 710061 China 2. Ion Channel Disease Laboratory Key Laboratory of Environment and Genes Related to Diseases of Education Ministry Xi’an 710061 China 3. Department of Physiology and Pathophysiology Key Laboratory of Molecular Cardiovascular Sciences of the Ministry of Education Peking University Health Science Center Beijing 100083 China

This work characterizes the mitochondrial proteomic profile in the failing heart and elucidates the molecular basis of mitochondria in heart failure. Heart failure was induced in rats by myocardial infarction, and mitochondria were isolated from hearts by differential centrifugation. Using two-dimensional gel electrophoresis and matrix-assisted laser desorption/ionization-time of flight mass spectrometry, a system biology approach was employed to investigate differences in mitochondrial proteins between normal and failing hearts. Mass spectrometry identified 27 proteins differentially expressed that involved in energy metabolism. Among those, the up-regulated proteins included tricarboxylic acid cycle enzymes and pyruvate dehydrogenase complex subunits while the down-regulated proteins were involved in fatty acid oxidation and the OXPHOS complex. These results suggest a substantial metabolic switch from free fatty acid oxidation to glycolysis in heart failure and provide molecular evidence for alterations in the structural and functional parameters of mitochondria that may contribute to cardiac dysfunction during ischemic injury.

关键词： mitochondria heart failure proteome two-dimensional electrophoresis energy metabolism

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Radical innovation breakthroughs of biodegradation of plastics by insects:history,present and future perspectives

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Frontiers of Environmental Science & Engineering 2024年第6期18卷 127-165页

作者： Shan-Shan Yang Wei-Min Wu Federica Bertocchini Mark Eric Benbow Suja P.Devipriya Hyung Joon Cha Bo-Yu Peng Meng-Qi Ding Lei He Mei-xi li Chen-Hao Cui Shao-Nan Shi Han-jun Sun Ji-Wei Pang Defu He Yalei Zhang jun Yang Deyi Hou De-Feng xing Nan-Qi Ren Jie Ding Craig S.Criddle State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China Department of Civil and Environmental Engineering William&Cloy Codiga Resource Recovery CenterStanford UniversityStanfordCA 94305USA Plasticentropy rue Thiers 28Reims 51100France Department of Entomology and Department of Osteopathic Medical Specialties Michigan State UniversityEast LansingMI 48824USA School of Environmental Studies Cochin University of Science and TechnologyKochi 682022India Department of Chemical Engineering Pohang University of Science and TechnologyPohang 37673Republic of Korea School of Environmental Science and Engineering Tongji UniversityShanghai 200092China china Energy Conservation and Environmental Protection Group CECEP Talroad Technology Co.Ltd.Beijing 100096China School of Ecological and Environmental Sciences East China Normal UniversityShanghai 200241China Research institute for Frontier Science Beihang UniversityBeijing 100191China School of Environment Tsinghua UniversityBeijing 100084China

Insects damaging and penetrating plastic packaged materials has been reported since the *** innovation breakthroughs of plastic biodegradation have been initiated since the discovery of biodegradation of plastics by Tenebrio molitor larvae in 2015 followed by Galleria mellonella in *** we review updated studies on the insect-mediated biodegradation of *** biodegradation by insect larvae,mainly by some species of darkling beetles(Tenebrionidae)and pyralid moths(Pyralidae)is currently a highly active and potentially transformative area of *** the past eight years,publications have increased explosively,including discoveries of the ability of different insect species to biodegrade plastics,biodegradation performance,and the contribution of host and microbiomes,impacts of polymer types and their physic-chemical properties,and responsible enzymes secreted by the host and gut *** date,almost all major plastics including polyethylene(PE),polypropylene(PP),polyvinyl chloride(PVC),polyethylene terephthalate(PET),polyurethane(PUR),and polystyrene(PS)can be biodegraded by *** and ten other insect species representing the Tenebrionidae and Pyralidae *** biodegradation processes are symbiotic reactions or performed by synergistic efforts of both host and gut-microbes to rapidly depolymerize and biodegrade plastics with hourly *** digestive ezymens and bioreagents screted by the insects play an essential role in plasatic biodegradation in certain species of Tenebrionidae and Pyralidae *** research on the insect itself,gut microbiomes,transcriptomes,proteomes and metabolomes has evaluated the mechanisms of plastic biodegradation in *** conclude this review by discussing future research perspectives on insect-mediated biodegradation of plastics.

关键词： Plastics Biodegradation Insects Gut microbiomes Enzymes

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Tough Hydrogen Bonding Crosslinked Poly (3-fluorothiophene) Network via Electrosynthesis for High-performance Electrochromic Supercapacitors

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Chinese Journal of Polymer Science 2024年第11期 1749-1757页

作者： Chun-Hui Du Yu-Hua Xu Hui li Zhi-xin Wu Han-jun Yang xi-Mei liu Bao-Yang Lu Guang-Ming Nie Ge Zhang Jiangxi Key Lab of Flexible Electronics Flexible Electronics Innovation InstituteJiangxi Science & Technology Normal University Key Laboratory of Optic-Electric Sensing and Analytical Chemistry for life Science MOEState Key Laboratory Base of Eco-chemical EngineeringCollege of Chemistry and Molecular EngineeringQingdao University of Science and Technology

As a type of bi-functional device,electrochromic supercapacitors （EC-SCs） have attracted extensive attention in diverse applications such as flexible ***,despite recent encouraging progress,rational design and development of high-performance EC-SC materials with desirable stability remain challenging for practical ***,we propose a fluorination strategy to develop high-performance EC-SC materials with tough hydrogen bonding cross-linked intermolecular polymer network by one-step electrosynthesis of *** electrosynthesized free-standing poly（3-fluorothiophene）(PFT) films simultaneously achieve high electrochromic performance （optical contrast 42%at 560 nm with reversible color changes between purple and blue）,and good capacitance property (290 F·g-1,1 A·g-1),as well as outstanding cyclic stability （2%reduction after 20000 cycles）.We further demonstrate the fabrication of PFT-based flexible electrochromic supercapacitor devices （FESDs）,and the resultant devices can be used to visually monitor the energy storage state in real-time and maintain outstanding stability under mechanical distortion like *** a tough fluorination hydrogen bonding cross-linking strategy may provide a new design concept for high-performance EC-SC materials and reliable FESDs toward practical applications.

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Simulation study on cuttings transport of the backreaming operation for long horizontal section wells

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Petroleum Science 2024年第2期21卷 1149-1170页

作者： Yu-Fei Chen Hui Zhang Wen-xin Wu jun li Yong Ouyang Zong-Yu Lu De-xin Ma Yong-Chuan Wu jun-Bo liu Ke-Rou liu Zhuo-xin Dong china university of Petroleum(Beijing) Beijing102249China Beijing normal university at Zhuhai Experimental and Practical Education Innovation CenterZhuhai519087GuangdongChina Oil&Gas Technology Research institute of Petrochina Changqing Oilfield Company Xi'an710016ShaanxiChina Petrochina xinjiang Oilfield Company Karamay834002XinjiangChina china Oilfield Services Ltd. Tianjin300459China

The backreaming operation plays a significant role in safe drilling for horizontal wellbores, while it may cause severe stuck pipe accidents. To lower the risk of the stuck pipe in backreaming operations, the mechanism of cuttings transport needs to be carefully investigated. In this research, a transient cuttings transport with multiple flow patterns model is developed to predict the evolution of cuttings transported in the annulus while backreaming. The established model can provide predictions of the distribution of cuttings bed along the wellbore considering the bulldozer effect caused by large-size drilling tools(LSDTs). The sensitivity analyses of the size of LSDTs, and backreaming operating parameters are conducted in Section 4. And a new theory is proposed to explain the mechanism of cuttings transport in the backreaming operation, in which both the bit and LSDTs have the “cleaning effect” and “plugging effect”.The results demonstrate that the cuttings bed in annuli is in a state of dynamic equilibrium, but the overall trend and the distribution pattern are obvious. First, larger diameters and longer drilling tools could lead to a higher risk of the stuck pipe. Second, we find that it is not the case that the higher flow rate is always better for hole cleaning, so three flow-rate intervals are discussed separately under the given conditions. When the “dangerous flow rate”(litates borehole cleaning. If the flow rate is large enough to be in the “high flow rate” interval(>35 L/s in Case 4),the higher the flow rate, the better the cleaning effect of cuttings beds. Third, an interval of tripping velocity called “dangerous velocity” is proposed, in which the cuttings bed accumulation near the LSDTs is more serious than

关键词： Backreaming Stuck pipe Hole cleaning Transient solid transport Multiple flow patterns

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NνDEx-100 conceptual design report

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Nuclear Science and Techniques 2024年第1期35卷 18-33页

作者： xi-Guang Cao Yan-Long Chang Kai Chen Emilio Ciuffoli li-Min Duan Dong-liang Fang Chao-Song Gao Surja K.Ghorui Peng-Chong Hu Qiang Hu Si-Yuan Huang Ze-Yu Huang Lei Lang Yu-Lan li Zhi-Jie li Tian-Yu liang jun liu Chen-Gui Lu Fa-Tai Mai Yuan Mei Hao Qiu xiang-Ming Sun xiao-xing Tang Hu-lin wang Qian-Ming wang Le xiao Mu-Yun xiao Jian-Yu xin Nu Xu Peng Yang Yi-Chen Yang Zhen Yang Zong-Yang Yu Dong-liang Zhang jun-Wei Zhang Cheng-xin Zhao Dou Zhu NνDEx-100 collaboration Shanghai Advanced Research institute Chinese Academy of SciencesShanghai 201210China Lanzhou university Lanzhou 730000China Central china normal university Wuhan 430079China institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China Shanghai institute of Applied Physics Chinese Academy of SciencesShanghai 201800China Lawrence Berkeley National Laboratory BerkeleyCA 94720USA North china university of Water Resources and Electric Power Zhengzhou 450045China 不详

Observing nuclear neutrinoless double beta (0vββ) decay would be a revolutionary result in particle *** such a decay would prove that the neutrinos are their own antiparticles,help to study the absolute mass of neutrinos,explore the origin of their mass,and may explain the matter-antimatter asymmetry in our universe by lepton number *** propose developing a time projection chamber (TPC) using high-pressure ^(82)SeF_(6) gas and Topmetal silicon sensors for readout in the china Jinping Underground Laboratory (CJPL) to search for neutrinoless double beta decay of82Se,called the NvDEx *** being located at CJPL with the world’s thickest rock shielding,NvDEx combines the advantages of the high Qββ(2.996 MeV) of82Se and the TPC’s ability to distinguish signal and background events using their different topological *** makes NvDEx unique,with great potential for low-background and high-sensitivity 0 vββ***-100,a NvDEx experiment phase with 100 kg of SeF_(6)gas,is being built,with plans to complete installation at CJPL by *** report introduces 0 vββ physics,the NvDEx concept and its advantages,and the schematic design of NvDEx-100,its subsystems,and background and sensitivity estimation.

关键词： Neutrinoless double beta decay Time projection chamber ^(82)SeF_(6) china Jinping Underground Laboratory

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Searching for^(76)Ge neutrinoless double beta decay with the CDEX-1B experiment

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Chinese Physics C 2024年第10期48卷 11-22页

作者： Bing-Tao Zhang jun-Zheng wang li-Tao Yang Qian Yue Ke-jun Kang Yuan-Jing li Hai-Peng An C.Greeshma Jian-Ping Chang Yun-Huan Chen Jian-Ping Cheng Wen-Han Dai Zhi Deng Chang-Hao Fang xin-Ping Geng Hui Gong Qiu-Ju Guo Xu-Yuan Guo li He Sheng-Ming He Jin-Wei Hu Han-xiong Huang Tu-Chen Huang Hai-Tao Jia xi Jiang S.Karmakar Hao-Bin li Jian-Min li Jin li Qian-Yun li Ren-Ming-Jie li Xue-Qian li Yu-Lan li Yi-Fan liang Bin liao Fong-Kay lin Shin-Ted lin Jia-Xuan liu Shu-Kui liu Yan-Dong liu Yu liu Yuan-Yuan liu Zhong-Zhi liu Hao Ma Yu-Cai Mao Qi-Yuan Nie Jin-Hua Ning Hui Pan Ning-Chun Qi Jie Ren xi-Chao Ruan Ze She Manoj Kumar Singh Tian-xi Sun Chang-Jian Tang Wei-You Tang Yang Tian Guang-Fu wang li wang Qing wang Yu-Feng wang Yun-xiang wang Henry-Tsz-King Wong Shi-Yong Wu Yu-Cheng Wu Hao-Yang xing Rui Xu Yin Xu Tao Xue Yu-Lu Yan Nan Yi Chun-Xu Yu Hai-jun Yu Jian-Feng Yue Ming Zeng Zhi Zeng Feng-Shou Zhang Lei Zhang Zhen-Hua Zhang Zhen-Yu Zhang Kang-Kang Zhao Ming-Gang Zhao Ji-Fang Zhou Zu-Ying Zhou Jing-jun Zhou Key Laboratory of Particle and Radiation Imaging(Ministry of Education)and Department of Engineering Physics Tsinghua UniversityBeijing 100084 Department of Physics Tsinghua UniversityBeijing 100084 institute of Physics Academia SinicaTaipei 11529 NUCTECH Company Beijing 100084 YaLong River Hydropower Development Company Chengdu 610051 College of Nuclear Science and Technology Beijing Normal UniversityBeijing 100875 College of Physics Sichuan UniversityChengdu 610065 School of Physics Peking UniversityBeijing 100871 Department of Nuclear Physics China Institute of Atomic EnergyBeijing 102413 Sino-French institute of Nuclear and Technology Sun Yat-sen UniversityZhuhai 519082 School of Physics Nankai UniversityTianjin 300071 Department of Physics Banaras Hindu UniversityVaranasi 221005 Department of Physics Beijing Normal UniversityBeijing 100875

We operated a p-type point contact high purity germanium(PPCGe)detector(CDEX-1B,1.008 kg)in the china Jinping Underground Laboratory(CJPL)for 500.3 days to search for neutrinoless double beta(0νββ)decay of^(76)Ge.A total of 504.3 kg⋅day effective exposure data was *** anti-coincidence and the multi/single-site event(MSE/SSE)discrimination methods were used to suppress the background in the energy region of interest(ROI,1989–2089 keV for this work)with a factor of 23.A background level of 0.33 counts/(keV⋅kg⋅yr)was *** lower limit on the half life of^(76)Ge 0νββdecay was constrained as T_(1/2)^(0ν)>1.0×10^(23)yr(90%C.L.),corresponding to the upper limits on the effective Majorana neutrino mass:2–7.5 eV.

关键词： neutrinoless double beta decay CDEX point-contact germanium detector ^(76)Ge

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Roadmap for rechargeable batteries:present and beyond

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Science china Chemistry 2024年第1期67卷 13-42页

作者： Sen xin Xu Zhang lin wang Haijun Yu xin Chang Yu-Ming Zhao Qinghai Meng Pan Xu Chen-Zi Zhao Jiahang Chen Huichao Lu xirui Kong Jiulin wang Kai Chen Gang Huang xinbo Zhang Yu Su Yao xiao Shu-Lei Chou Shilin Zhang Zaiping Guo Aobing Du Guanglei Cui Gaojing Yang Qing Zhao liubing Dong Dong Zhou Feiyu Kang Hu Hong Chunyi Zhi Zhizhang Yuan xianfeng li Yifei Mo Yizhou Zhu Dongfang Yu xincheng Lei Jianxiong Zhao Jiayi wang Dong Su Yu-Guo Guo Qiang Zhang jun Chen li-jun Wan CAS Key Laboratory of Molecular Nanostructure and Nanotechnology CAS Research/Education Center for Excellence in Molecular SciencesBeijing National Laboratory for Molecular Sciences(BNLMS)Institute of ChemistryChinese Academy of Sciences(CAS)Beijing 100190China university of Chinese Academy of Sciences.Beijing 100049 China institute of Advanced Battery Materials and Devices Faculty of Materials and ManufacturingBeijing University of TechnologyBeijing 100124China Key Laboratory of Advanced Functional Materials Ministry of EducationBeijing University of TechnologyBeijing 100124China Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical EngineeringTsinghua UniversityBeijing 100084China State Key Laboratory of Chemistry and Utilization of Carbon-Based Energy Resources College of ChemistryXinjiang UniversityUrumqi 830046China Department of Chemical Engineering Shanghai Jiao Tong UniversityShanghai 200240China State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChangchun 130022China institute for Carbon Neutralization College of Chemistry and Materials EngineeringWenzhou UniversityWenzhou 325035China School of Chemical Engineering and Advanced Materials The University of AdelaideAdelaide 5000Australia Qingdao Industrial Energy Storage Research institute Qingdao Institute of Bioenergy and Bioprocess TechnologyChinese Academy of SciencesQingdao 266101China Frontiers Science Center for New Organic Matter Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education)College of ChemistryNankai UniversityTianjin 300071China College of Chemistry and Materials Science Jinan UniversityGuangzhou 511443China Tsinghua Shenzhen International Graduate School Tsinghua UniversityShenzhen 518055China Department of Materials Science and Engineering City University of Hong KongHong Kong 999077China Division of Energy Storage Dalian National Laboratory for Clean Energy(DNL)Dalian Institute of Chem

Rechargeable batteries currently hold the largest share of the electrochemical energy storage market,and they play a major role in the sustainable energy transition and industrial decarbonization to respond to global climate *** to the increased popularity of consumer electronics and electric vehicles,lithium-ion batteries have quickly become the most successful rechargeable batteries in the past three decades,yet growing demands in diversified application scenarios call for new types of rechargeable *** efforts are made to developing the next-generation post-li-ion rechargeable batteries,which include,but are not limited to solid-state batteries,lithium–sulfur batteries,sodium-/potassium-ion batteries,organic batteries,magnesium-/zinc-ion batteries,aqueous batteries and flow *** the great achievements,challenges persist in precise understandings about the electrochemical reaction and charge transfer process,and optimal design of key materials and interfaces in a *** roadmap tends to provide an overview about the current research progress,key challenges and future prospects of various types of rechargeable *** computational methods for materials development,and characterization techniques will also be discussed as they play an important role in battery research.

关键词： energy storage rechargeable batteries battery materials electrochemistry

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典型旅游城市土壤重金属特定源生态风险评价及优先控制源分析

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环境科学 2024年第8期45卷 4837-4846页

作者：李军高占栋台喜生焦亮臧飞兰州城市学院城市环境学院兰州730070 西北师范大学甘肃省绿洲资源环境与可持续发展重点实验室兰州730070 兰州大学草地农业科技学院兰州730020

为了解西北旅游城市土壤重金属的污染现状、分布特征及污染来源,选择敦煌市主城区土壤为研究对象,采集并分析了表层土壤重金属As、Cd、Cr、Cu、Hg、Ni、Pb和Zn的含量特征.采用地累积指数法和改进内梅罗污染指数法量化土壤重金属污染水平... 详细信息

为了解西北旅游城市土壤重金属的污染现状、分布特征及污染来源,选择敦煌市主城区土壤为研究对象,采集并分析了表层土壤重金属As、Cd、Cr、Cu、Hg、Ni、Pb和Zn的含量特征.采用地累积指数法和改进内梅罗污染指数法量化土壤重金属污染水平,利用聚类分析和正定矩阵因子分解(PMF)模型定量解析重金属污染来源,并应用PMF模型和综合生态风险指数相结合的方法解析各污染源对生态风险的贡献率.结果表明,除As和Ni之外,Cd、Cr、Cu、Hg、Pb和Zn含量的均值均高于甘肃省土壤元素背景值,但所有元素的含量均低于《土壤环境质量建设用地土壤污染风险管控标准(试行)》(GB 36600-2018)中建设用地的风险筛选值,其中Cd、Pb和Hg的富集较为严重,超标率均高于90%.地累积指数评价结果显示,研究区土壤以Hg污染为主,也存在不同程度的Cd、Cr、Cu、Pb和Zn污染.改进内梅罗污染指数结果表明,土壤的综合污染程度为无污染至中度污染,总体上为轻度污染.PMF模型源解析表明,研究区土壤重金属受自然源、工业降尘源、工业源、交通源和综合源的影响,贡献率依次为29.28%、25.86%、20.13%、16.5%和8.23%.特定源-综合生态风险评价模型分析表明,工业降尘源为优先控制污染源,Hg为生态风险优先控制污染元素.

关键词：城市土壤地累积指数污染评价生态风险溯源解析

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黄河流域农田土壤重金属污染特征及其优先控制源分析

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环境科学 2024年第3期45卷 1724-1738页

作者：李军李旭李开明焦亮台喜生臧飞曹素珍兰州城市学院城市环境学院兰州730070 西北师范大学甘肃省绿洲资源环境与可持续发展重点实验室兰州730070 兰州大学草地农业科技学院兰州730020

农田土壤环境质量评价与污染溯源解析是保障国家粮食安全和农业可持续发展的基础,也是扎实推进国家净土保卫战的重要前提.基于2000~2023年黄河流域农田土壤重金属(As、 Cd、 Cr、 Cu、 Hg、 Ni、 Pb和Zn)含量数据,采用地累积指数法对重... 详细信息

农田土壤环境质量评价与污染溯源解析是保障国家粮食安全和农业可持续发展的基础,也是扎实推进国家净土保卫战的重要前提.基于2000~2023年黄河流域农田土壤重金属(As、 Cd、 Cr、 Cu、 Hg、 Ni、 Pb和Zn)含量数据,采用地累积指数法对重金属污染特征进行评价,利用正定矩阵因子分解(PMF)模型定量解析重金属的来源贡献,并通过运用蒙特卡洛(Monte Carlo)模拟和人体健康风险评价模型相耦合的方法评价重金属污染的潜在健康风险,实现优先污染源和污染元素的确定.结果表明:(1)研究区农田土壤所有重金属的含量均值均低于《土壤环境质量农用地土壤污染风险管控标准》(GB 15618-2018)(pH>7.5)的筛选值,但分别有21.69%、 5.56%和1.23%的样点Cd、 As和Zn含量超出其筛选值,Cd超标率最高.(2)Hg和Cd为偏中度污染,Cu和Pb为轻度污染,其余元素均为无污染.(3)农田土壤重金属主要来源为交通-工业源、自然-农业源、工业-自然源和农业-工业源,贡献率分别为37.04%、 26.69%、 21.72%和14.55%.(4)农田土壤重金属对成人与儿童存在致癌健康风险,但不具有非致癌风险;As和Cd为人体健康风险优先控制元素,工业-自然源和农业-工业源为研究区优先控制源.

关键词：黄河流域 Monte Carlo模拟正定矩阵因子分解(PMF)模型源解析健康风险评价

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