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Knowledge-guided machine learning reveals pivotal drivers for gasto-particle conversion of atmospheric nitrate

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Environmental Science and Ecotechnology 2024年第3期19卷 100-108页

作者： Bo Xu Haofei Yu Zongbo Shi Jinxing liu Yuting Wei Zhongcheng Zhang Yanqi Huangfu Han Xu yue li linlin Zhang Yinchang Feng Guoliang Shi State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control Tianjin Key Laboratory of Urban Transport Emission ResearchCollege of Environmental Science and EngineeringNankai UniversityTianjin300350China CMA-NKU Cooperative Laboratory for Atmospheric Environment-Health Research(CLAER) College of Environmental Science and EngineeringNankai UniversityTianjin300350China Department of Civil Environmentaland Construction EngineeringUniversity of Central FloridaOrlandoFLUSA School of Geography Earth and Environment Sciences University of BirminghamBirminghamB152TTUK State Key Laboratory of Precision Measuring Technology and Instruments Tianjin Key Laboratory of air Pollutants Monitoring TechnologySchool of Precision Instrument and Opto-electronics EngineeringTianjin UniversityTianjin300072China Gigantic Technology(Tianjin)Co. LtdTianjin300072China College of Computer Science Nankai UniversityTianjin300350China China National Environmental Monitoring Centre Beijing100012China

Particulate nitrate,a key component of fine particles,forms through the intricate gas-to-particle conversion *** process is regulated by the gas-to-particle conversion coefficient of nitrate(ε(NO_(3)^(-))).The mechanism betweenε(NO_(3)^(-))and its drivers is highly complex and nonlinear,and can be characterized by machine learning ***,conventional machine learning often yields results that lack clear physical meaning and may even contradict established physical/chemical mechanisms due to the influence of ambient *** urgently needs an alternative approach that possesses transparent physical interpretations and provides deeper insights into the impact ofε(NO_(3)^(-)).Here we introduce a supervised machine learning approachdthe multilevel nested random forest guided by theory *** approach robustly identifies NH4 t,SO_(4)^(2-),and temperature as pivotal drivers forε(NO_(3)^(-)).Notably,substantial disparities exist between the outcomes of traditional random forest analysis and the anticipated actual ***,our approach underscores the significance of NH4 t during both daytime(30%)and nighttime(40%)periods,while appropriately downplaying the influence of some less relevant drivers in comparison to conventional random forest *** research underscores the transformative potential of integrating domain knowledge with machine learning in atmospheric studies.

关键词： Machine learning Data driven Theoretical approach Domain knowledge Guide

Jianpi-Huatan-Huoxue-Anshen formula ameliorates gastrointestinal inflammation and microecological imbalance in chemotherapytreated mice transplanted with H22 hepatocellular carcinoma

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World Journal of Gastrointestinal Oncology 2024年第10期16卷 4209-4231页

作者： Ya-Nan Wang Xiang-Yang Zhai Zheng Wang Chun-ling Gao Sui-Cai Mi Wen-li Tang Xue-Min Fu Huai-Bang li li-Feng yue Peng-Fei li Sheng-Yan Xi Department of TCM Xiang’an HospitalSchool of MedicineXiamen UniversityXiamen 361102Fujian ProvinceChina Faculty of Chinese Medicine and State Key Laboratory of Quality Research in Chinese Medicine Macao University of Science and TechnologyMacao 999078China Department of Radiotherapy Chenggong Hospital of Xiamen UniversityPLA 73rd Army HospitalXiamen 361003Fujian ProvinceChina Department of Oncology Xiamen Hospital of Traditional Chinese MedicineXiamen 361015Fujian ProvinceChina Dongzhimen Hospital Beijing University of Chinese MedicineBeijing 100700China

BACKGROUND Jianpi-Huatan-Huoxue-Anshen formula[Tzu-Chi cancer-antagonizing&lifeprotecting II decoction(TCCL)]is a Chinese medical formula that has been clinically shown to reduce the gastrointestinal side effects of chemotherapy in cancer patients and improve their quality of ***,its effect and mechanism on the intestinal microecology after chemotherapy are not yet *** To discover the potential mechanisms of TCCL on gastrointestinal inflammation and microecological imbalance in chemotherapy-treated mice transplanted with hepatocellular carcinoma(HCC).METHODS Ninety-six mice were inoculated subcutaneously with HCC *** week later,the mice received a large dose of 5-fluorouracil by intraperitoneal injection to establish a HCC chemotherapy ***-six mice were randomly selected before administration,and feces,ileal tissue,and ileal contents were collected from each *** remaining mice were randomized into normal saline,continuous chemotherapy,Yangzheng Xiaoji capsulestreated,and three TCCL-treated *** treatment,feces,tumors,liver,spleen,thymus,stomach,jejunum,ileum,and colon tissues,and ileal contents were *** changes,serum levels of IL-1β,IL-6,IL-8,IL-10,IL-22,TNF-α,and TGF-β,intestinal SIgA,and protein and mRNA expression of ZO-1,NF-κB,Occludin,MUC-2,Claudin-1,and IκB-αin colon tissues were *** effect of TCCL on the abundance and diversity of intestinal flora was analyzed using 16S rDNA *** TCCL treatment improved thymus and spleen weight,thymus and spleen indexes,and body weight,decreased tumor volumes and tumor tissue cell density,and alleviated injury to gastric,ileal,and colonic mucosal *** proteins and genes associated with inflammation,IL-10,TGF-β,SIgA,ZO-1,MUC-2,and Occludin were upregulated,whereas NF-κB,IL-1β,IL-6,TNF-α,IL-22,IL-8,and IκB-αwere ***,TCCL increased the proportions of fecal Actinobacteria,AF12,Adlercreutzia,Clostridium,Coriobac

关键词： Chinese medicine Chemotherapy H22 hepatocellular carcinoma Intestinal barrier function Intestinal microecological balance

Trauma in The Lonely Soldier

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Journal of literature and Art Studies 2024年第8期14卷 689-692页

作者： li De-kun MA Xiao-lei li Xin-yue Undergraduate School National University of Defense TechnologyChangsha 410072China

Benedict is an award-winning novelist and non-fiction writer specializing in social *** non-fiction book The Lonely Soldier reflects the impact of war on violence against *** soldiers are always the victims of violence,before,during,and after serving in the Iraq *** thesis aims to explore their trauma and illuminate the book’s meaning.

关键词： Helen Benedict The Lonely Soldier female soldiers victims of violence meaning of writing

Dimensional regulation in gigantic molybdenum blue wheels featuring{(W)Mo_(5)}motifs for enhanced proton conductivity

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Nano Research 2024年第9期17卷 8261-8268页

作者： Yu-Lun Wu Jing Du Hai-Ying Zhang Ming-Jun Hou Qiao-yue li Wei-Chao Chen Kui-Zhan Shao Bo Zhu Chao Qin Xin-Long Wang Zhong-Min Su Key Laboratory of Polyoxometalate and Reticular Material Chemistry of Ministry of Education Department of ChemistryNortheast Normal UniversityChangchun 130024China Hebei Key Laboratory of Organic Functional Molecules National Demonstration Center for Experimental Chemistry EducationTesting and Analysis CenterCollege of Chemistry and Materials ScienceHebei Normal UniversityShijiazhuang 050024China State Key Laboratory of Supramolecular Structure and Materials Institute of Theoretical ChemistryCollege of ChemistryJilin UniversityChangchun 130021China

Dimensional regulation in polyoxometalates is an effective strategy during the design and synthesis of polyoxometalates-based high proton conductors,but it is not available to ***,the precise regulation of dimensionality has been realized in an unprecedented gigantic molybdenum blue wheel family featuring pentagonal{(W)Mo5}motifs through optimizing the molar ratio of Mo/W,including[Gd_(2)Mo_(124)W_(14)O_(422)(H_(2)O)62]38-(0D-{Mo_(124)W_(14)},1),[Mo_(126)W_(14)O441(H_(2)O)51]^(70-)(1D-{Mo_(126)W_(14)}n,2),and[Mo_(124)W_(14)O_(430)(H_(2)O)50]60-(2D-{Mo_(124)W_(14)}n,3).Such important{(W)Mo5}structural motif brings new reactivity into gigantic Mo blue *** are different numbers and sites of{Mo2}defects in each wheel-shaped monomer in 1-3,which leads to the monomers of 2 and 3 to form 1D and 2D architectures via Mo-O-Mo covalent bonds driven by{Mo2}-mediated H_(2)O ligands substitution process,respectively,thus achieving the controllable dimensional *** expected,the proton conductivity of 3 is 10 times higher than that of 1 and 1.7 times higher than that of *** continuous proton hopping sites in 2D network are responsible for the enhanced proton conductivity with lower activation *** study highlights that this dimensional regulation approach remains great potential in preparing polyoxometalates-based high proton conductive materials.

关键词： polyoxometalate molybdenum blue wheels Mo/W mixed-addenda polyoxometalates dimensional regulation proton conduction

Direct measurement of the break-out ^(19)F(p,γ)^(20)Ne reaction in the China Jinping underground laboratory(CJPL)

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Nuclear Science and Techniques 2024年第8期35卷 142-152页

作者： Yin‑Ji Chen Hao Zhang li‑Yong Zhang Jian‑Jun He Richard James deBoer Michael Wiescher Alexander Heger David Kahl Jun Su Daniel Odell Xin‑yue li Jian‑Guo Wang Long Zhang Fu‑Qiang Cao Zhi‑Cheng Zhang Xin‑Zhi Jiang Luo‑Huan Wang Zi‑Ming li Lu‑Yang Song liang‑Ting Sun Qi Wu Jia‑Qing li Bao‑Qun Cui li‑Hua Chen Rui‑Gang Ma Er‑Tao li Gang lian Yao‑De Sheng Zhi‑Hong li Bing Guo Wei‑Ping liu Key Laboratory of Beam Technology of the Ministry of Education College of Nuclear Science and TechnologyBeijing Normal UniversityBeijing 100875China Department of Physics and Astronomy The Joint Institute for Nuclear AstrophysicsUniversity of Notre DameNotre DameIN 46556USA School of Physics and Astronomy Monash UniversityClaytonVIC 3800Australia Facility for Rare Isotope Beams Michigan State UniversityEast LansingMI 48824USA Institute of Nuclear and Particle Physics and Department of Physics and Astronomy Ohio UniversityAthensOH 45701USA Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China China Institute of Atomic Energy Beijing 102413China College of Physics and Optoelectronic Engineering Shenzhen UniversityShenzhen 518060China School of Nuclear Science and Technology University of Chinese Academy of SciencesBeijing 100049China College of Science Southern University of Science and TechnologyShenzhen 518055China Institute of Radiation Technology Beijing Academy of Science and TechnologyBeijing 100875China Key Laboratory of Nuclear Physics and Ion‑Beam Application(MOE) Institute of Modern PhysicsFudan UniversityShanghai 200433China School of Mathematics and Physics Handan UniversityHandan 056005China

Calcium production and the stellar evolution of first-generation stars remain fascinating mysteries in *** one possible nucleosynthesis scenario,break-out from the hot carbon–nitrogen–oxygen(HCNO)cycle was thought to be the source of the calcium observed in these oldest ***,according to the stellar modeling,a nearly tenfold increase in the thermonuclear rate ratio of the break-out ^(19)F(p,γ)^(20) Ne reaction with respect to the competing ^(19)F(p,α)^(16) O back-processing reaction is required to reproduce the observed calcium *** performed a direct measurement of this break-out reaction at the China Jinping underground *** measurement was performed down to the low-energy limit of E_(c.m.)=186 keV in the center-of-mass *** key resonance was observed at 225.2 keV for the first *** a temperature of approximately 0.1 GK,this new resonance enhanced the thermonuclear ^(19)F(p,γ)^(20) Ne rate by up to a factor of≈7.4,compared with the previously recommended NACRE *** is of particular interest to the study of the evolution of the first stars and implies a stronger breakdown in their“warm”CNO cycle through the ^(19)F(p,γ)^(20) Ne reaction than previously *** break-out resulted in the production of the calcium observed in the oldest stars,enhancing our understanding of the evolution of the first stars.

关键词： Nuclear astrophysics First stars Abundance of calcium Reaction cross section Reaction rate China Jinping underground laboratory(CJPL) JUNA

Design and Topology-Related Physical Properties of Crystalline Conductive Metal-Organic Framework Materials

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Synergistic effects of three traditional herbs green tea,mulberry leaf and corn silk on glucose uptake level of L6 myoblasts and the hypoglycemic mechanism

第4届分子科学博士后学术年会

作者： Wansheng liu yue li Yutao Cui Daoben Zhu Institute of Chemistry Chinese Academy of Sciences

Due to the difficulty in forming conductive pathways in traditional MOF materials formed by carboxylic acid ligands, most of the reported crystalline traditional conductive MOF materials exhibit poor conductivity. This limits the application of traditional conductive MOF materials in electrochemically related fields. There is a scarcity of research on the electrical transport properties based on traditional MOF materials, and there is a lack of systematic studies.

关键词： Design and Topology-Related Physical Properties of Crystalline Conductive Metal-Organic Framework Materials Framework

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Traditional Medicine Research 2024年第7期9卷 1-12页

作者： Jing-Na Zhou Ming-yue li Ting-Ting Zhang Jing-Yang Lu Min Zhang Peng-Wei Zhuang Hai-Xia Chen Tianjin Key Laboratory for Modern Drug Delivery&High-Efficiency School of Pharmaceutical Science and TechnologyTianjin UniversityTianjin 300072China. School of Food Science and Bioengineering Tianjin Agricultural UniversityTianjin 300384China. State Key Laboratory of Nutrition and Safety Tianjin University of Science&TechnologyTianjin 300457China. Haihe Laboratory of Modern Chinese Medicine Chinese Materia Medica CollegeTianjin University of Traditional Chinese MedicineTianjin 301617China.

Background:Green tea,mulberry leaf and corn silk are traditional herbs used in the prevention and treatment of diabetes in China for a long time,but their synergistic hypoglycemic effects and mechanisms remain ***:The effective components of green tea,mulberry leaf and corn silk were extracted and *** design of experiments was used to study the influences of different combinations on the cell viability and glucose uptake level of L6 myoblasts,so as to determine the optimal synergistic hypoglycemic *** possible hypoglycemic mechanism of the optimal synergistic combination was explored by cytotoxicity assay,glucose uptake assay,and western ***:Three polyphenol enrichment fractions of the herbs,30%ethanol elution fraction of green tea(GT),50%ethanol elution fraction of mulberry leaf(ML)and 60%ethanol elution fraction of corn silk(CS)were *** antioxidant activities of GT-30%,ML-50%and CS-60%were superior to those of crude extracts,and showed strong potential inα-amylase andα-glucosidase inhibition *** optimal synergistic combination of crude extracts G7(crude extract of green tea:crude extract of mulberry leaf:crude extract of corn silk=1:5:3),polyphenol enrichment fractions R3(GT-30%:ML-50%:CS-60%=1:7:1)and monomers X2(epigallocatechin gallate:morusin:formononetin=3:1:2)were selected,respectively.G7,R3,and X2 showed promoting effects on the cell viability and glucose uptake of L6 myoblasts within the detected concentration *** addition,G7,R3,and X2 could increase the expression levels of p-PI3K/PI3K and p-Akt/Akt in L6 myoblasts,and promote the translocation of Glut4,but G7 and R3 showed more significant ***:The synergistic hypoglycemic effects of green tea,mulberry leaf and corn silk had the characteristics of multiple-components and multiple-targets with p-PI3K/PI3K,p-Akt/Akt and the translocation of Glut4 signal pathways *** three traditional herbs might have the potential

关键词： green tea mulberry leaf corn silk synergistic effect type 2 diabetes mellitus mechanism

Conjugated Cyclo[n]Thiophenes Macrocycles with unexpected dual-emissive luminogen

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Conjugated Cyclo[n]Thiophenes Macrocycles with unexpected du...

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作者： yue li Wansheng liu Yutao Cui Daoben zhu Institute of Chemistry Chinese Academy of Sciences

Cyclo[n]Thiophenes [CnTs] represent a distinctive class of macrocyclic molecules, exhibiting structural aesthetics and diverse properties such as fluorescence and donor-acceptor. In this work, two oligothiophene architectures, namely（4T-2hexyl）-DPBP and（4T-2hexyl-2Me）-DPBP, were synthesized using a Pd-catalyzed Suzuki coupling approach with the support of 5,5'-di（1H-pyrrol-1-yl）-2,2'-bipyridine（DPBP）. Notably, while both（4T-2hexyl）-DPBP and（4T-2hexyl-2Me）-DPBP exhibited only weak emission from 500-850 nm in a pure dichlorometane（DCM）, they produced a pronounced yellow light upon the addition of ethyl acetate（EA） to the DCM solution. Fluorescence emission spectra indicate that a weak emission fades out in the range of 400 to 500 nm. The luminescent behavior of（4T-2hexyl）-DPBP and（4T-2hexyl-2Me）-DPBP show the unique characteristics of both ACQ effect and AIE effect. We have identified the simultaneous presence of AIE and ACQ in the CnTs system, which facilitates the design of more fluorescence-tunable molecular structures for use in fluorescence imaging, bioassays, and other applications.

关键词： CnTs AIE ACQ

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极端天气对风电场局地风环境的影响

华中科技大学学报（自然科学版） 2024年第7期52卷 106-112页

作者：郜志腾张军李岳李晔上海交通大学船舶海洋与建筑工程学院上海201100 成都流体动力创新中心四川成都610072

以东南沿海某风电场24台兆瓦级风电机组为例,基于中尺度数值模式并结合风电场参数化模型,对台风天气下该风电场局地风速、风向、风功率密度、湍动能等特征量的时序演变特征和空间分布特性进行分析.结果表明:数值模拟结果与观测结果平均... 详细信息

以东南沿海某风电场24台兆瓦级风电机组为例,基于中尺度数值模式并结合风电场参数化模型,对台风天气下该风电场局地风速、风向、风功率密度、湍动能等特征量的时序演变特征和空间分布特性进行分析.结果表明:数值模拟结果与观测结果平均误差在1 m/s以内;未受台风影响时风电场在轮毂高度处速度亏损最大,垂向上尾流影响范围在3倍轮毂高度左右;受台风影响时,风电场尾流受台风强迫作用而呈现尾流偏转效应,尾流最大偏转角可达33°;风电场尾流会增加附近区域的湍动能水平,在水平方向上影响区域持续至下游4~8倍风场直径,在垂向上影响范围可达3.5倍轮毂高度处.风电场下游较远处湍动能分布受下垫面、风电场尾流和极端风况的耦合调制作用,进而呈现典型的大尺度旋涡绕流结构.

关键词：极端天气大气环境风电场风资源中尺度模式