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Fabrication of Novel Scaffolds Containing Collagen-I/Polylactic Acid/Nanohydroxyapatite via Co-electrospinning Methods

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Chemical Research in Chinese Universities 2010年第4期26卷 662-666页

作者： ZANG Jun-ting QI Xin li shu-qiang li Dong-song GONG Yu-bao YANG Chen XU Feng liU Jian-guo Department of Bone and Joint Surgery First Hospital of Jilin University Changchun 130021 P R. China

A novel scaffold containing collagen-I/polylactic acid（PLA）/nanohydroxyapatite（nHA） was prepared via co-electrospinning method. Different target substrates were used to improve the collection efficiency of this scaffold. The properties of the novel scaffold were compared with those of conventionally prepared ones. Compared to con- ventional method, the modified method was more efficient in producing the scaffold. Moreover, the porosity, thickness, and morphology of the novel scaffold were better than those of scaffolds prepared by conventional methods. The properties of collagen-I, collagen-I/PLA and collagen-I/PLA/nHA scaffolds were also compared. Diameters of the electrospun fibers ranged from 180 to 405 nm, and roughness was present on the surface of the fibers due to the deposition of crystals of nHA along the long axis of the fibers. The fibers of the collagen-I/PLA/nHA scaffold and the fibers of natural bone tissue had similar structure.

关键词： Electrospinning Collagen-I PLA Nanohydroxyapatite

QTL analysis of the developmental changes in cell wall components and forage digestibility in maize(Zea mays L.)

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Journal of Integrative Agriculture 2022年第12期21卷 3501-3513页

作者： li Kun YANG Xue liU Xiao-gang HU Xiao-jiao WU Yu-jin WANG Qi MA Fei-qian li shu-qiang WANG Hong-wu liU Zhi-fang HUANG Chang-ling Institute of Crop Sciences Chinese Academy of Agricultural SciencesBeijing 100081P.R.China National Engineering Laboratory for Crop Molecular Breeding Beijing 10081P.R.China

Cell wall architecture plays a key role in stalk strength and forage ***,cellulose,and hemicellulose are the three main components of plant cell walls,and they can impact stalk quality by affecting the structure and strength of the cell *** explore cell wall development during secondary cell wall lignification in maize stalks,conventional and conditional genetic mapping were used to identify the dynamic quantitative trait loci(QTLs)of the cell wall components and digestibility traits during five growth stages after *** detergent lignin(ADL),cellulose(CEL),acid detergent fiber(ADF),neutral detergent fiber(NDF),and in vitro dry matter digestibility(IVDMD)were evaluated in a maize recombinant inbred line(RIL)***,CEL,ADF,and NDF gradually increased from 10 to 40 days after silking(DAS),and then they *** initially decreased until 40 DAS,and then it increased *** QTLs were identified for the five traits,and each accounted for 3.48–24.04%of the phenotypic *** QTL hotspots were found,and they were localized in the 1.08,2.04,2.07,7.03,8.05,and 9.03 bins of the maize *** the interval of the pleiotropic QTL identified in bin 1.08 of the maize genome,six genes associated with cell wall component biosynthesis were identified as potential candidate genes for stalk strength as well as cell wall-related *** addition,26 conditional QTLs were detected in the five stages for all of the investigated ***-two of the 26 conditional QTLs were found at 30 DAS conditioned using the values of 20 DAS,and at 50 DAS conditioned using the values of 40 *** results indicated that cell wall-related traits are regulated by many genes,which are specifically expressed at different stages after *** improvements in both forage digestibility and lodging resistance could be achieved by pyramiding multiple beneficial QTL alleles identified in this study.

关键词： quantitative trait loci maize(Zea mays L.) cell wall components forage quality

Improving Multi-task GNNs for Molecular Property Prediction via Missing Label Imputation

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Machine Intelligence Research 2025年第1期22卷 131-144页

作者： Fenyu Hu Dingshuo Chen qiang liu shu Wu University of Chinese Academy of Sciences Beijing100190China Center for Research on Intelligent Perception and Computing State Key Laboratory of Multimodal Artificial Intelligence SystemsInstitute of AutomationChinese Academy of SciencesBeijing100190China

The prediction of molecular properties is a fundamental task in the field of drug ***,graph neural networks(GNNs)have been gaining prominence in this *** a molecule tends to have multiple correlated properties,there is a great need to develop the multi-task learning ability of ***,limited by expensive and time-consuming human annotations,collecting complete labels for each task is *** a result,most existing benchmarks involve many missing labels in training data,and the performance of GNNs is impaired due to the lack of sufficient supervision *** overcome this obstacle,we propose to improve multi-task molecular property prediction by missing label ***,a bipartite graph is first introduced to model the molecule-task co-occurrence ***,the imputation of missing labels is transformed into predicting missing edges on this bipartite *** predict the missing edges,a graph neural network is devised,which can learn the complex molecule-task co-occurrence *** that,we select reliable pseudo labels according to the uncertainty of the prediction *** with enough and reliable supervision information,our approach achieves state-of-the-art performance on a variety of real-world datasets.

关键词： Graph classification imbalance learning prediction bias mixture of experts multiview representations

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巨蟹蛛一种畸形雄性触肢器记述(英文)

动物分类学报 2002年第1期27卷 183-185页

作者： Peter Jaeger li shu qiang Institut fuer Zoologie Johannes Gutenberg Universitaet Institute of Zoology Chinese Academy of Sciences Saarstrasse2255099 MainzGermanyZhongguancun-LuBeijing100080China

During examination of spider material in the Institute of Zoology, Chinese Academy of sciences (IZCAS), one male specimen came to our attention, which showed a unique anomaly in its palp. The morphology of this specim... 详细信息

关键词：巨蟹蛛雄性触肢器形态畸形标本

Emerging progress:photochemical transformation of nitroso compounds

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Science China Chemistry 2025年第1期68卷 118-133页

作者： Ze-Le Chen qiang-qiang li Armido Studer Jun Xuan Anhui Province Key Laboratory of Chemistry for Inorganic/Organic Hybrid Functionalized Materials School of Chemistry&Chemical EngineeringAnhui UniversityHefei 230601China Organisch-Chemisches Institut Universitat MünsterMunster 48149Germany

Nitroso compounds have emerged as highly valuable reaction partners or reagents in organic synthesis due to their rich *** versatile profile of these compounds allows them to function as electrophiles,nucleophiles,diradicals,and radical acceptors in diverse *** recent years,notable progress has been made in harnessing photochemical reactions with nitroso compounds to prepare N,O-containing structures using mild and eco-friendly *** nitroso compounds like nitrosoarenes,acyloxy nitroso compounds,N-nitrosoamines and nitrites have received significant attention for their ability to introduce NO moieties into complex molecules that are otherwise difficult to *** this review,we provide an overview of the recent advancements in the visible light-induced conversion of nitroso compounds,with particular emphasis on their role as bifunctional reagents and acceptors of radicals,carbenes and nitrenes.

关键词： nitroso compounds photochemistry radical reaction carbene transformation nitrosoarenes

B2-CuZr reinforced amorphous alloy matrix composites:A review

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China Foundry 2025年第1期22卷 1-11页

作者： Wei Guo Run-hua Huang Zhen Zhang Mi Zhao Jin-cheng Wang Yan-qiang Qiao shu-lin Lü shu-sen Wu State Key Lab of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Solidification Processing Northwestern Polytechnical UniversityXi’an 710072China School of Aerospace Engineering Huazhong University of Science and TechnologyWuhan 430074China Research Institute of Huazhong University of Science and Technology in Shenzhen Shenzhen 518057GuangdongChina

B2-CuZr phase reinforced amorphous alloy matrix composites has become one of the research hotspots in the field of materials science due to the“transformation-induced plasticity”phenomenon,which makes the composites show better macroscopic plastic deformability and obvious work-hardening behavior compared to the conventional amorphous alloy matrix composites reinforced with ductile ***,the in-situ metastable B2-CuZr phase tends to undergo eutectoid decomposition during solidification,and the volume fraction,size,and distribution of B2-CuZr phase are difficult to control,which limits the development and application of these *** date,much efforts have been made to solve the above problems through composition optimization,casting parameter tailoring,and post-processing *** this study,a review was given based on relevant studies,focusing on the predictive approach,reinforcing mechanism,and microstructure tailoring methods of B2-CuZr phase reinforced amorphous alloy matrix *** research focus and future prospects were also given for the future development of the present composite system.

关键词： amorphous alloy matrix composite B2-CuZr phase plasticity microstructure tailoring

Ti^(3+)/Ti^(4+)and Co^(2+)/Co^(3+)redox couples in Ce-doped Co-Ce/TiO2 for enhancing photothermocatalytic toluene oxidation

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Journal of Environmental Sciences 2025年第3期149卷 164-176页

作者： Guanghui li Xiaolan li Xinhui Hao qiang li Meng Zhang Hongpeng Jia Xiamen Key Laboratory of Materials for Gaseous Pollutant Control Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China Key Laboratory of Urban Pollutant Conversion Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China CAS Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China University of Chinese Academy of Sciences Beijing 100049China

Cerium and cobalt loaded Co-Ce/TiO_(2)catalyst prepared by impregnation method was investigated for photothermal catalytic toluene *** on catalyst characterizations(XPS,EPR and H2-TPR),redox cycle between Co and TiO_(2)(Co^(2+)+Ti^(4+)↔Co^(3+)+Ti^(3+))results in the formation of Co^(3+),Ti^(3+)and oxygen vacancies,which play important roles in toluene catalytic oxidation *** introduction of Ce brings in the dual redox cycles(Co^(2+)+Ti^(4+)↔Co^(3+)+Ti^(3+),Co^(2+)+Ce4+↔Co^(3+)+Ce3+),further promoting the elevation of reaction sites *** full spectrum irradiation with light intensity of 580mW/cm^(2),Co-Ce/TiO_(2)catalyst achieved 96%of toluene conversion and 73%of CO_(2)yield,obviously higher than Co/P25 and Co/TiO_(2).Co-Ce/TiO_(2)efficiently maintains 10-hour stability test under water vapor conditions and exhibits better photothermal catalytic performance than counterparts under different wavelengths *** catalytic reaction displays improved activities compared with thermal catalysis,which is attributed to the promotional effect of light including photocatalysis and light activation of reactive oxygen species.

关键词： Photothermal catalysis Redox cycle Oxygen vacancy VOCs Titanium dioxide

Abiotic aerobic oxidation pathways of stibnite revealed by oxygen and sulfur isotope systematics of sulfate

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Journal of Environmental Sciences 2025年第1期147卷 83-92页

作者： Ningjie He shu li Xiaoqian li Yaning Tang Jiaxue Yang Jianwei Zhou School of Environment Studies China University of GeosciencesWuhan 430074China Key Laboratory of Mine Ecological Effects and Systematic Restoration Ministry of Natural ResourcesBeijing 100081China State Environmental Protection Key Laboratory of Source Apportionment and Control of Aquatic Pollution Ministry of Ecology and EnvironmentWuhan 430074China Institute of Geological Survey China University of GeosciencesWuhan 430074China

The environmental threat posed by stibnite is an important geoenvironmental issue of current *** better understand stibnite oxidation pathways,aerobic abiotic batch experiments were conducted in aqueous solution with varyingδ^(18)O_(H_(2)O) value at initial neutral pH for different lengths of time(15-300 days).The sulfate oxygen and sulfur isotope compositions as well as concentrations of sulfur and antimony species were *** sulfur isotope fractionation factor(△^(34)S_(SO4-stibnite))values decreased from 0.8‰to-2.1‰during the first 90 days,and increased to 2.6‰at the 180 days,indicating the dominated intermediate sulfur species such as S_(2)O_(3)^(2-),S0,and H_(2)S(g)involved in Sb2S3 oxidation *** incorporation of O into sulfate derived from O_(2)(~100%)indicated that the dissociated O_(2)was only directly adsorbed on the stibnite-S sites in the initial stage(0-90 days).The proportion of O incorporation into sulfate from water(27%-52%)increased in the late stage(90-300 days),which suggested the oxidation mechanism changed to hydroxyl attack on stibnite-S sites promoted by nearby adsorbed O_(2)on stibnite-Sb *** exchange of oxygen between sulfite and water may also contributed to the increase of water derived O into SO42-.The new insight of stibnite oxidation pathway contributes to the understanding of sulfide oxidation mechanism and helps to interpret field data.

关键词： Sulfide oxidation δ^(34)S_(SO4) δ^(18)O_(SO4) Oxygen source of sulfate

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一种玉米苗期冠层叶片营养诊断动态光谱指数

光谱学与光谱分析 2014年第6期34卷 1605-1609页

作者：李树强李民赞孙红河南科技大学车辆与动力工程学院河南洛阳471003 中国农业大学现代精细农业系统集成研究教育部重点实验室北京100083

为了有效的解决玉米苗期冠层叶片营养状态车载动态诊断过程中,土壤干扰信息无法剔除的问题,本文提出了一种动态测量用光谱指数MPRI,根据MPRI的构成和特点、论述了利用MPRI辨识土壤与冠层光谱信息的机理,构建了基于MPRI的玉米苗期冠层叶... 详细信息

为了有效的解决玉米苗期冠层叶片营养状态车载动态诊断过程中,土壤干扰信息无法剔除的问题,本文提出了一种动态测量用光谱指数MPRI,根据MPRI的构成和特点、论述了利用MPRI辨识土壤与冠层光谱信息的机理,构建了基于MPRI的玉米苗期冠层叶片叶绿素含量的预测模型,通过车载式作物长势检测系统平台,运用模型对玉米苗期冠层叶片营养状态进行动态诊断与评估,取得良好的效果。研究表明:在车载动态条件下测量玉米苗期冠层叶片营养状态时,土壤的MPRI呈正值而玉米冠层的MPRI呈负值,因此使用光谱指数MPRI能够有效识别土壤背景与冠层叶片光谱信息。设定固定的阈值,能够较为准确和便捷的去除土壤背景光谱信息。基于MPRI构建的冠层叶片叶绿素含量的动态测量预测模型,能够准确的表征冠层叶片的叶绿素含量,模型决定系数R2达0.72,动态测量中对植株冠层的识别率达80%。与其他常用的指数相比,在车载动态测量环境下,光谱指数MPRI具有土壤背景信息识别速度快、正确率高,模型预测精度良好等特点,为玉米苗期冠层营养状态的诊断提供了新的途径。

关键词：动态光谱指数土壤背景光谱作物长势车载系统