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Ultrathin organic solvent nanofiltration membrane with polydopamine-HKUST-1 interlayer for organic solvent separation

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Journal of Environmental Sciences 2024年第7期141卷 182-193页

作者： Haike li Xindong li Guozai Ouyang lijinhong Huang lang li Wenhao li Wanfu Huang Duokun li Ganzhou Key Laboratory of Basin Pollution Simulation and Control Jiangxi University of Science and TechnologyGanzhou 341000China Innovation Center for Water Quality Security Technology at Ganjiang River Basin Jiangxi University of Science and TechnologyGanzhou 341000China School of Architecture and Design Jiangxi University of Science and TechnologyGanzhou 341000China WA School of Mines:Minerals Energy and Chemical EngineeringCurtin UniversityWA 6845Australia School of Materials Science and Engineering Tiangong UniversityTianjin 300387China

Polydopamine(PDA)and metal-organic skeleton HKUST-1 were co-deposited on the base membrane of hexamethylenediamine(HDA)-crosslinked polyetherimide(PEI)ultrafiltration membrane as the interlayer,and high-throughput organic solvent nanofiltration membrane(OSN)was prepared by interfacial polymerization and solvent activation *** polyamide(PA)layer surface roughness from 28.4 nm in PA/PEI to 78.3 nm in PA/PDA-HKUST-10.6/PEI membrane,reduced the thickness of the separation layer from 79 to 14 nm,and significantly improved the hydrophilic,thermal and mechanical *** flux of the PA/PDA-HKUST-10.6/PEI membrane in a 0.1 g/L Congo Red(CR)ethanol solution at 0.6 MPa test pressure reached 21.8 L/(m^(2)·hr)and the rejection of CR was 92.8%.Solvent adsorption test,N,N-dimethylformamide(DMF)immersion experiment,and long-term operation test in ethanol showed that the membranes had high solvent *** solvent flux test demonstrated that,under the test pressure of 0.6 MPa,the flux of different solvents ranked as follows:methanol(56.9 L/(m^(2)·hr))>DMF(39.6 L/(m^(2)·hr))>ethanol(31.2 L/(m^(2)·hr))>IPA(4.5 L/(m^(2)·hr))>N-hexane(1.9 L/(m^(2)·hr)).The ability of the membranes to retain dyes in IPA/water dyes solution was also *** flux of the membrane was 30.4 L/(m^(2)·hr)and the rejection of CR was 91.6%when the IPA concentration reached 50%.This OSN membrane-making strategy is economical,environment-friendly and efficient,and has a great application prospect in organic solvent separation systems.

关键词： Interfacial polymerization Organic solvent nanofiltration Interlayer Metal-organic frameworks Polydopamine

Efficient and selective recovery of Gd(Ⅲ)via polyethyleneimine modification of lanthanum-based metal-organic frameworks

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Journal of Rare Earths 2024年第1期42卷 210-219,I0007页

作者： Wenhao li lijinhong Huang Bin Xiao Xiaoguang Duan Haike li lang li Wanfu Huang Ganzhou Key Laboratory of Basin Pollution Simulation and Control Jiangxi University of Science and TechnologyGanzhou341000China Innovation Center for Water Quality Security Technology at Ganjiang River Basin Jiangxi University of Science and TechnologyGanzhou341000China Faculty of Science and Engineering WA School of Mines:MineralsEnergy and Chemical EngineeringCurtin UniversityWAAustralia School of Architecture and Design Jiangxi University of Science and TechnologyGanzhou341000China School of Resources and Architectural Engineering Gannan University of Science and TechnologyGanzhou341000China School of Chemical Engineering and Advanced Materials The University of AdelaideAdelaideSA5005Australia School of Resource and Environmental Engineering Jiangxi University of Science and TechnologyGanzhou341000China

With the development of the economy and the increasing demand for environmental protection,the efficient and selective recovery of Gd(Ⅲ)from actual wastewater is of critical *** this work,lanthanum-based metal-organic framework(LaBDC)materials were prepared by a hydrothermal method,and then polyethyleneimine(PEI)and LaBDC were combined by an impregnation method to form a novel LaBDC@xPEI *** prepared materials were characterized using Fourier transfo rm infrared spectroscopy(FTIR),X-ray diffraction(XRD),scanning electron microscopy(SEM),energy dispersive X-ray spectroscopy(EDX),B runauer-Emmett-Teller(BET),thermogravimetric analysis(TGA)and X-ray photoelectron spectroscopy(XPS).Experiments show that LaBDC@50%PEI has the highest adsorption capacity(181.77 mg/g)among lanthanum-based MOFs with different PEI loadings at pH=5.5,which is about 5.1 times that of bare *** adsorption isotherm analysis shows that LaBDC@50%PEI follows the langmuir *** addition,the adsorption kinetics of LaBDC@50%PEI follows a pseudo-second-order kinetic model,indicating that the adsorption process is chemical *** is worth noting that LaBDC@50%PEI maintains good adsorption performance and stability after three recycling tests,and exhibits excellent selectivity in cation interference ***,the LaBDC@50%PEI composites possess good stability and hold great promises in rapid recovery of Gd(Ⅲ)from practical aqueous environments.

关键词： Wet-impregnation method Polyethylene imine Metaleorganic frameworks Lanthanum Recovery of Gd(Ⅲ) Rare earths

SFGA-CPA: A Novel Screening Correlation Power Analysis Framework Based on Genetic Algorithm

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Computers, Materials & Continua 2024年第6期79卷 4641-4657页

作者： Jiahui liu lang li Di li Yu Ou College of Computer Science and Technology Hengyang Normal UniversityHengyang421002China Hunan Provincial Key Laboratory of Intelligent Information Processing and Application Hengyang Normal UniversityHengyang421002China

Correlation power analysis(CPA)combined with genetic algorithms(GA)now achieves greater attack efficiency and can recover all subkeys ***,two issues in GA-based CPA still need to be addressed:key degeneration and slow evolution within *** challenges significantly hinder key recovery *** paper proposes a screening correlation power analysis framework combined with a genetic algorithm,named SFGA-CPA,to address these ***-CPA introduces three operations designed to exploit CPA characteris-tics:propagative operation,constrained crossover,and constrained ***,the propagative operation accelerates population evolution by maximizing the number of correct bytes in each ***,the constrained crossover and mutation operations effectively address key degeneration by preventing the compromise of correct ***,an intelligent search method is proposed to identify optimal parameters,further improving attack *** were conducted on both simulated environments and real power traces collected from the SAKURA-G *** the case of simulation,SFGA-CPA reduces the number of traces by 27.3%and 60%compared to CPA based on multiple screening methods(MS-CPA)and CPA based on simple GA method(SGA-CPA)when the success rate reaches 90%.Moreover,real experimental results on the SAKURA-G platform demonstrate that our approach outperforms other methods.

关键词： Side-channel analysis correlation power analysis genetic algorithm crossover mutation

Yuzaoea gen. nov., a new biraphid diatom(Bacillariophyceae)genus and its phylogenetic significance

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Acta Oceanologica Sinica 2024年第2期43卷 130-136页

作者： Honghan liu Chenhong li lang li Xuesong li lin Sun Junrong liang Jun Zhang Yahui Gao Changping Chen Key Laboratory of Ministry of Education for Coastal and Wetland Ecosystems and School of life Sciences Xiamen UniversityXiamen 361102China State Key Laboratory of Marine Environmental Science Xiamen UniversityXiamen 361102China Guangxi Key Laboratory of Marine Environmental Science Guangxi Academy of Marine SciencesGuangxi Academy of SciencesNanning 530007China Beibu Gulf Marine Industry Research Institute Fangchenggang 538000China

The flexed frustules in pennate diatoms are usually associated with monoraphid diatoms. Interestingly, we found a biraphid diatom species with flexed frustules in an offshore intertidal beach environment on Weizhou Island,Beihai City, Guangxi Zhuang Autonomous Region, China. Therefore, based on morphological characteristics, we described a new genus of diatoms Yuzaoea sinensis gen. et sp. nov. CH li, HH liu, YH Gao & CP Chen. The frustule of this genus is characterized by heterogeneous frustule with one concave valve and one convex valve,complete raphe on both valves, straight and moderately eccentric raphe, uniseriate striae and girdle bands with a single row of areolae. The most identifying feature of this genus was the flexed frustule, which is rare in biraphid diatoms and common in monoraphid diatoms. We compared the morphometric characteristics of genus Yuzaoea with genus Rhoikoneis and several genera within the family Rhoicospheniaceae, including Rhoicosphenia,Campylopyxis, and Cuneolus. Phylogenetic analyses based on SSU rRNA and rbc L showed that the genus Yuzaoea was the sister group to the clade of Rhoicosphenia with a high support value(bootstrap values = 100%), and the clade “Yuzaoea+Rhoicosphenia” was sister to the clade of monoraphid diatoms, in which the genera Achnanthidium, Planothidium and some Cocconeis with high support values(bootstrap = 100%).Morphologically, the genus Yuzaoea shares many morphological features with monoraphid diatoms like genera Achnanthidium and Planothidium and the members within the Rhoicospheniaceae. Therefore, based on a combined morphological studies and phylogenetic results we suggested that this branch may represented the evolution of one kind monoraphid diatoms, from biraphid diatoms(e.g. genus Yuzaoea), to incompleted biraphid diatoms(e.g. genera Rhoicosphenia, Campylopyxis), to monoraphid diatoms(e.g. genera Achnanthidium and Planothidium).

关键词： biraphid diatom marine new genus Rhoicospheniaceae taxonomy Yuzaoea

Deformation,structure and potential hazard of a landslide based on InSAR in Banbar county,Xizang(Tibet)

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China Geology 2024年第2期7卷 203-221页

作者： Guan-hua Zhao Heng-xing Lan Hui-yong Yin lang-ping li Alexander Strom Wei-feng Sun Chao-yang Tian College of Earth Science and Engineering Shandong University of Science and TechnologyQingdao 266590China State Key Laboratory of Resources and Environmental Information System Institute of Geographic Sciences and Natural Resources ResearchChinese Academy of SciencesBeijing 100101China School of Geological Engineering and Geomatics Chang’an UniversityXi’an 710054China Key Laboratory of Ecological Geology and Disaster Prevention Ministry of Natural ResourcesXi’an 710054China University of Chinese Academy of Sciences Beijing 100049China JSC“Hydroproject Institute” Moscow 125993Russia

The Tibetan Plateau is characterized by complex geological conditions and a relatively fragile ecological *** recent years,there has been continuous development and increased human activity in the Tibetan Plateau region,leading to a rising risk of *** landslide in Banbar County,Xizang(Tibet),have been perturbed by ongoing disturbances from human engineering activities,making it susceptible to instability and displaying distinct *** this study,small baseline subset synthetic aperture radar interferometry(SBAS-InSAR)technology is used to obtain the line of Sight(LOS)deformation velocity field in the study area,and then the slope-orientation deformation field of the landslide is obtained according to the spatial geometric relationship between the satellite’s LOS direction and the ***,the landslide thickness is inverted by applying the mass conservation *** results show that the movement area of the landslide is about 6.57×10^(4)m^(2),and the landslide volume is about 1.45×10^(6)m^(3).The maximum estimated thickness and average thickness of the landslide are 39 m and 22 m,*** thickness estimation results align with the findings from on-site investigation,indicating the applicability of this method to large-scale earth *** deformation rate of the landslide exhibits a notable correlation with temperature variations,with rainfall playing a supportive role in the deformation process and displaying a certain *** activities exert the most substantial influence on the spatial heterogeneity of landslide deformation,leading to the direct impact of several prominent deformation areas due to human ***,utilizing the long short-term memory(LSTM)model to predict landslide displacement,and the forecast results demonstrate the effectiveness of the LSTM model in predicting landslides that are in a continuous development and movement *** landslide is still active,and based

关键词： Landslide InSAR Human activity Deformation Structure LSTM model Engineering construction Thickness Neural network Machine learning Prediction and prevention Tibetan Plateau Geological hazards survey engineering

Effect of speed humps on instantaneous traffic emissions in a microscopic model with limited deceleration capacity

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Chinese Physics B 2024年第6期33卷 413-420页

作者：胡宇晨李启朗刘军王君霞汪秉宏 School of Mathematics and Physics Anhui Jianzhu UniversityHefei 230601China School of Civil Engineering and Transportation Northeast Forestry UniversityHarbin 150040China Department of Modern Physics University of Science and Technology of ChinaHefei 230026China

As a common transportation facility, speed humps can control the speed of vehicles on special road sections to reduce traffic risks. At the same time, they also cause instantaneous traffic emissions. Based on the classic instantaneous traffic emission model and the limited deceleration capacity microscopic traffic flow model with slow-to-start rules, this paper has investigated the impact of speed humps on traffic flow and the instantaneous emissions of vehicle pollutants in a single lane situation. The numerical simulation results have shown that speed humps have significant effects on traffic flow and traffic emissions. In a free-flow region, the increase of speed humps leads to the continuous rise of CO_(2), NO_(X) and PM emissions. Within some density ranges, one finds that these pollutant emissions can evolve into some higher values under some random seeds. Under other random seeds, they can evolve into some lower values. In a wide moving jam region, the emission values of these pollutants sometimes appear as continuous or intermittent phenomenon. Compared to the refined Na Sch model, the present model has lower instantaneous emissions such as CO_(2), NO_(X) and PM and higher volatile organic components(VOC) emissions. Compared to the limited deceleration capacity model without slow-to-start rules, the present model also has lower instantaneous emissions such as CO_(2), NO_(X) and PM and higher VOC emissions in a wide moving jam region. These results can also be confirmed or explained by the statistical values of vehicle velocity and acceleration.

关键词： traffic emissions speed humps slow-to-start rules deceleration capacity

面向星地激光通信的大气湍流预报研究进展(特邀)

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红外与激光工程 2024年第3期53卷 19-31页

作者：郭盈池李浪李晨高春清付时尧北京理工大学光电学院北京100081 光电成像技术与系统教育部重点实验室北京100081 信息光子技术工信部重点实验室北京100081

激光通信系统在大气环境下应用的性能受到严重制约,当激光在大气湍流中传输时,其波面会发生畸变。在激光通信系统中,对大气湍流相关参数进行预报可以提前对星地数据传输链路进行调度,避免建立无效的通信任务。此外,大气湍流预报在天文... 详细信息

激光通信系统在大气环境下应用的性能受到严重制约,当激光在大气湍流中传输时,其波面会发生畸变。在激光通信系统中,对大气湍流相关参数进行预报可以提前对星地数据传输链路进行调度,避免建立无效的通信任务。此外,大气湍流预报在天文选址、光学遥感等领域也有重要价值。随着国内外相关工作的长期积累以及算力、观测设备等硬件的能力提升,当前科研人员已经提出了一些大气湍流预报方案。文中主要综述了国内外学者在大气湍流预报方面的研究进展,首先详细介绍了目前应用比较广泛的中尺度数值预报技术,列举了使用中尺度数值预报方法对国内外典型区域的大气湍流进行预报的相关工作;然后介绍了深度学习方法在大气湍流预报中的应用情况,对其优势与局限性进行了讨论;最后介绍了一种面向星地激光通信的大气相干长度短时预报方法。

关键词：大气湍流湍流预报 Cn2廓线大气相干长度

基于机器视觉与光谱融合的柑橘品质无损检测分级系统设计与试验

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江苏大学学报（自然科学版） 2024年第1期45卷 38-45页

作者：文韬代兴勇李浪刘豪中南林业科技大学机电工程学院湖南长沙410004

针对柑橘果径、着色率和内部糖度3项关键品质指标,基于双锥滚子式果杯传输线设计了一套柑橘综合品质无损检测分级系统,该系统主要包括喂料部分、机器视觉检测模块、近红外光谱检测模块和分级执行部分.机器视觉检测模块采用单相机拍摄不... 详细信息

针对柑橘果径、着色率和内部糖度3项关键品质指标,基于双锥滚子式果杯传输线设计了一套柑橘综合品质无损检测分级系统,该系统主要包括喂料部分、机器视觉检测模块、近红外光谱检测模块和分级执行部分.机器视觉检测模块采用单相机拍摄不断翻滚的柑橘视频来获取大量不同姿态的柑橘图像,并进行轮廓提取,以单个柑橘所有帧图像的最小外接圆直径的平均值计算果径,以每一帧图像得到的其二维黄色占比的平均值作为全表面着色率.在近红外光谱检测模块中设计了透射式光路,采集柑橘透射率光谱,并按在线检测时柑橘出现的两种高频姿态建立了混合姿态糖度检测模型,对比不同预处理方法下的建模结果,选取应用效果较优的多元散射校正(MSC)后建立的偏最小二乘法(PLS)模型.在线试验结果表明:果径检测的最大绝对误差为-1.42 mm,着色率检测的最大绝对误差为0.048,糖度检测结果的相关系数为0.817,均方根误差为0.658%.内外品质的联合检测分级按判别树决策方法确定了3种品质的联合分级方式,在分选速度为5个/s时,综合分级的平均准确率可达到91.16%,该检测分级系统整体结构简单,对于类球形水果具有较强的适用性,在产业化应用上有很大的潜力.

关键词：柑橘无损检测机器视觉近红外光谱分级

土石坝黏土心墙压实度影响因素的灰关联熵分析

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人民珠江 2024年第S01期45卷 170-174页

作者：向鹏李浪中水珠江规划勘测设计有限公司广东广州510610

黏土心墙是土石坝中常用的防渗体,其填筑标准以压实度作为设计控制指标之一。影响压实度的因素较多,主要包括含水率、碾压机械、碾压厚度、碾压遍数、碾压速度等,本次主要考查含水率、碾压厚度及碾压遍数等指标。通过碾压试验测定不同... 详细信息

黏土心墙是土石坝中常用的防渗体,其填筑标准以压实度作为设计控制指标之一。影响压实度的因素较多,主要包括含水率、碾压机械、碾压厚度、碾压遍数、碾压速度等,本次主要考查含水率、碾压厚度及碾压遍数等指标。通过碾压试验测定不同条件下的压实度,应用灰关联熵分析方法,探讨了不同因素对黏土心墙压实度的影响程度。结果表明:含水率的灰熵关联度最大,其次是碾压厚度,再次是碾压遍数。因此,含水率是压实度的最优控制因素,黏土心墙填筑过程中应该优先考虑并严格控制其偏差值。

关键词：黏土心墙灰关联熵压实度影响因素