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semicrystalline Unfused Polymer Donors with Backbone Halogenation toward Cost-Effective Organic solar Cells

Chinese Journal of Chemistry 2024年第7期42卷 752-759页

作者： Yuxin Kong shijie Ju Hongmei Qin Min Hun Jee simeng Xia Jiaqi ren Chao Gao Jianyu Yuan Wenyan su Han Young Woo Yuxiang li school of Materials science and Engineering Xi'an University of Science and TechnologyXianShaanxi 710054China Department of Chemistry Korea UniversitySeoul 02841Republic of Korea Xi'an Key laboratory of liquid Crystal and Organic Photovoltaic Materials State Key Laboratory of Fluorine&Nitrogen ChemicalsXi'an Modern Chemistry Research InstituteXi'anShaanxi 710065China Jiangsu Key laboratory for Carbon-Based functional Materials&Devices Institute of Functional Nano&Soft Materials(FUNSOM)Soochow University199 Ren'ai RoadSuzhouJiangsu 215123China

Developing novel unfused building blocks with simple synthesis and low cost is essential to advance and enrich cost-effective poly-mer donors;however,it remains a challenge due to the lack of efficient molecular ***,a class of low-cost and fully unfused polymer donors with precisely regulated backbone planarity via halogenation was designed and synthesized,namely PDTBTBz-2H,PDTBTBz-2f,and *** polymer donors possess a four-step synthesis route with over 80%yield from cheap raw chemicals comparable to existing low-cost polymer donors,such as *** from the planar backbone via in-corporating the f…s non-covalent interactions,PDTBTBz-2f exhibits more robust J-type aggregation in solution and a long-ranged molecular stacking in film relative to PDTBTBz-2H and ***,the systematical study of PDTBTBz-based organic so-lar cells(OsCs)reveals the close relationship between optimized molecular self-assembly and charge separation/transport regarding backbone halogenation when paired with the non-fullerene acceptor(Y6-BO-4f).As a result,the photovoltaic devices based on semicrystalline PDTBTBz-2f achieved a promising power conversion efficiency(PCE)of 12.37%.Our work highlighted the influence of backbone halogenation on the molecular self-assembly properties and a potential unfused backbone motif for further developing cost-effective OsCs.

关键词： low-cost Polymer donors Backbone halogenation Molecular self-assembly Organic solar cells

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Effects of the level and source of dietary physically effective fiber on feed intake, nutrient utilization, heat energy, ruminal fermentation,and milk production by Alpine goats

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Animal Nutrition 2024年第2期17卷 312-324页

作者： Raquel V.lourencon Amlan K.Patra luana P.s.Ribeiro Ryszard Puchala Wei Wang Terry A.Gipson Arthur l.Goetsch American Institute for Goat Research Langston University

Thirty-two primiparous and 31 multiparous Alpine goats were used to determine influences of diets varying in level and source of forage on performance in early to mid-lactation for 16 wk. Diets consisted of 40%, 50%, 60%, and 70% forage(designated as 40f, 50f, 60f, and 70f, respectively) with 60f and 70f containing coarsely ground grass hay(primarily orchardgrass) and 40f and 50f containing cottonseed hulls, alfalfa pellets, and coarsely ground wheat hay. Diets contained 15.9% to 16.3% crude protein and37.8%, 42.1%, 53.5%, and 55.4% neutral detergent fiber(NDf) with 10.0%, 15.8%, 50.1%, and 55.5% particle retention on a 19-mm sieve, and 26.1%, 29.6%, 38.3%, and 40.0% physically effective NDf(pe NDf) for 40f,50f, 60f, and 70f, respectively. Dry matter intake(2.71, 2.75, 1.96, and 1.95 kg/d) and milk yield(2.82,2.71, 2.23, and 2.10 kg/d for 40f, 50f, 60f, and 70f, respectively) were lower(P for the two diets highest in forage. Digestion of organic matter was similar among diets(P > 0.05), but digestibility of NDf was greater(P for 60f and 70f(57.5%, 58.4%, 68.9%, and 72.2% for 40f, 50f, 60f, and 70f,respectively). Diet affected(P lk fat(3.16%, 3.37%, 2.93%, and 2.97%) and protein concentrations(2.62%, 2.69%, 2.58%, and 2.52% for 40f, 50f, 60f, and 70f, respectively). Milk energy yield was greater(P for the two diets lowest in forage(7.51, 7.45, 5.68, and 5.34 MJ/d), although yield relative to dry matter intake was not affected(P > 0.05) by diet and was lower(P for primiparous vs. multiparous goats(2.71 and 3.09 MJ/kg). Ruminal p H and acetate proportion were greater for 60f and 70f than for the other diets and the proportion of butyrate was lower for the two diets highest in fiber. The mean lengths of time spent ruminating, eating, standing, and lying were not affected(P > 0.05) by diet or parity, but many interactions involving diet, period, hour, and parity were significant(P lusion, lactational performance o

关键词： Physically effective fiber Alpine goat lactation Ruminal fermentation feeding behavior

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Application of ^(18)f-fluorodeoxyglucose positron emission tomography/computed tomography imaging in recurrent anastomotic tumors after surgery in digestive tract tumors

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World Journal of Gastrointestinal surgery 2024年第8期16卷 2474-2483页

作者： Deng-feng Ge Hao ren Zi-Chen Yang shou-Xiang Zhao Zhen-Ting Cheng Da-Da Wu Bin Zhang Department of Cardiothoracic surgery Nanjing University of Chinese MedicineNanjing 210023Jiangsu ProvinceChina Department of Gastrointestinal surgery Shanghai Sixth People’s HospitalShanghai 250063China

BACKGROUND This study was to investigate the application value of whole-body dynamic ^(18)f-fluorodeoxyglucose(fDG)positron emission tomography/computed tomogra-phy(PET/CT)imaging in recurrent anastomotic tumors of digestive tract after gastric and esophageal cancer *** patients with gastric and esophageal cancer have a high risk of tumor recurrence,and traditional imaging methods have certain limitations in early detection of recurrent ***-body dynamic ^(18)f-fDG PET/CT imaging,due to its high sensitivity and specifi-city,can provide comprehensive information on tumor metabolic activity,which is expected to improve the early diagnosis rate of postoperative recurrent tumors,and provide an important reference for clinical treatment *** A retrospective analysis was performed on 53 patients with upper digestive tract tumors after operation and systemic dynamic ^(18)f-fDG PET/CT imaging indi-cating abnormal fDG uptake by anastomosis,including 29 cases of gastric cancer and 24 cases of esophageal *** to the follow-up results of gas-troscopy and other imaging examinations before and after PET/CT examination,the patients were divided into an anastomotic recurrence group and anastomotic inflammation *** multi-parameter analysis software was used to obtain the metabolic rate(MRfDG),volume of distribution maximum(DVmax)of anastomotic lesions,and MRmean and DVmean of normal liver *** lesion/background ratio(lBR)was calculated by dividing the MRfDG and DVmax of the anastomotic lesion by the MRmean and DVmean of the normal liver tissue,respectively,to obtain lBR-MRfDG and *** independent sample t test was used for statistical analysis,and a receiver operating characteristic curve was used to analyze the differential diagnostic efficacy of each parameter for anastomotic recurrence and *** The dynamic ^(18)f-fDG PET/CT imaging parameters MRfDG,DVmax,lBR-MRfDG,and lBR-DVmax of post

关键词： Gastric cancer Esophageal cancer Anastomosis Dynamic positron emission tomography Differential diagnosis Metabolic rate

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spatial analysis of Dengue through the reproduction numbers relating to socioeconomic features:Case studies on two Brazilian urban centers

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Infectious Disease Modelling 2024年第1期9卷 142-157页

作者： Ana T.C.silva Rejane C.Dorn lívia R.Tomás leonardo B.l.santos lacita M.skalinski suani T.R.Pinho Departamento de física Universidade Estadual de Feira de SantanaAv.Transnordestinas/n.Novo HorizonteFeira de Santana44036-900BABrazil Instituto de física Universidade Federal da BahiaRua Barão de Jeremoabo s/nCampus Universitário de OndinaSalvador40170-115BABrazil Centro Nacional de Monitoramento e Alertas de Desastres Naturais(CEMADEN) Estrada Dr.Altino Bondensan500São Josédos Campos12247-016SPBrazil Universidade Estadual de santa Cruz Campus Soane Nazaréde AndradeRodovia Jorge AmadoKm 16SalobrinhoIlhéus45662-900BABrazil Instituto de saúde Coletiva Universidade Federal da BahiaR.Basílio da Gamas/n-CanelaSalvador40110-140BABrazil Instituto Nacional de Ciência e Tecnologia-sistemas Complexos Virtual InstitutionBrazil

The study of the propagation of infectious diseases in urban centers finds a close connection with their population's social characteristics and *** work performs a spatial analysis of dengue cases in urban centers based on the basic reproduction numbers,R0,and incidence by planning areas(PAs),as well as their correlations with the Human Development Index(HDI)and the number of *** analyzed dengue epidemics in 2002 at two Brazilian urban centers,Belo Horizonte(BH)and Rio de Janeiro(RJ),using PAs as spatial *** results reveal heterogeneous spatial scenarios for both cities,with very weak correlations between R0 and both the number of trips and the HDI;in BH,the values of R0 show a less spatial heterogeneous pattern than in *** BH,there are moderate correlations between incidence and both the number of trips and the HDI;meanwhile,they weakly correlate for ***,the absence of strong correlations between the considered measures indicates that the transmission process should be treated considering the city as a whole.

关键词： Dengue Mathematical mode lBasic reproduction number Urban mobility Urban indices

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Multi-timescale Modeling and Dynamic stability Analysis for sustainable Microgrids:state-of-the-art and Perspectives

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Protection and Control of Modern Power systems 2024年第3期9卷 1-35页

作者： Mingyue Zhang Yang Han Yuxiang liu Amr s.Zalhaf Ensheng Zhao Karar Mahmoud Mohamed M.f.Darwish frede Blaabjerg the school of Mechanical and Electrical Engineering University of Electronic Science and Technology of ChinaChengdu 611731China IEEE 不详 the University of Electronic science and Technology of China(UEsTC) ChengduChina Aswan University the school of Electrical Engineering Aalto UniversityFinland the Department of Electrical Engineering Faculty of Engineering at ShoubraBenha University the Department of EEA School of Electrical EngineeringAalto University

The increasing trend for integrating renewable energy sources into the grid to achieve a cleaner energy system is one of the main reasons for the development of sustainable microgrid(MG)*** typical power-electronized power systems,MGs make extensive use of power electronics converters,which are highly controllable and flexible but lead to a profound impact on the dynamic performance of the whole *** with traditional large-capacity power systems,MGs are less resistant to perturbations,and various dynamic variables are coupled with each other on multiple timescales,resulting in a more complex system instability *** meet the technical and economic challenges,such as active and reactive power-sharing,voltage,and frequency deviations,and imbalances between power supply and demand,the concept of hierarchical control has been introduced into MGs,allowing systems to control and manage the high capacity of renewable energy sources and ***,as the capacity and scale of the MG system increase,along with a multi-timescale control loop design,the multi-timescale interactions in the system may become more significant,posing a serious threat to its safe and stable *** investigate the multi-timescale behaviors and instability mechanisms under dynamic inter-actions for AC MGs,existing coordinated control strategies are discussed,and the dynamic stability of the system is defined and classified in this ***,the modeling and assessment methods for the stability analysis of multi-timescale systems are also ***,an outlook and discussion of future research directions for AC MGs are also presented.

关键词： sustainable microgrid hierarchical control modeling model simplification multi-timescale dynamic stability analysis timescale decomposition.

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AutoRhythmAI: A Hybrid Machine and Deep learning Approach for Automated Diagnosis of Arrhythmias

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Computers, Materials & Continua 2024年第2期78卷 2137-2158页

作者： s.Jayanthi s.Prasanna Devi Department of Computer science and Engineering SRM Institute of Science and Technology-Vadapalani CampusChennaiTamil NaduIndia

In healthcare,the persistent challenge of arrhythmias,a leading cause of global mortality,has sparked extensive research into the automation of detection using machine learning(Ml)***,traditional Ml and AutoMl approaches have revealed their limitations,notably regarding feature generalization and automation *** glaring research gap has motivated the development of AutoRhythmAI,an innovative solution that integrates both machine and deep learning to revolutionize the diagnosis of *** approach encompasses two distinct pipelines tailored for binary-class and multi-class arrhythmia detection,effectively bridging the gap between data preprocessing and model *** validate our system,we have rigorously tested AutoRhythmAI using a multimodal dataset,surpassing the accuracy achieved using a single dataset and underscoring the robustness of our *** the first pipeline,we employ signal filtering and Ml algorithms for preprocessing,followed by data balancing and split for *** second pipeline is dedicated to feature extraction and classification,utilizing deep learning ***,we introduce the‘RRI-convoluted trans-former model’as a novel addition for binary-class *** ensemble-based approach then amalgamates all models,considering their respective weights,resulting in an optimal model *** our study,the VGGRes Model achieved impressive results in multi-class arrhythmia detection,with an accuracy of 97.39%and firm performance in precision(82.13%),recall(31.91%),and f1-score(82.61%).In the binary-class task,the proposed model achieved an outstanding accuracy of 96.60%.These results highlight the effectiveness of our approach in improving arrhythmia detection,with notably high accuracy and well-balanced performance metrics.

关键词： Automated machine learning neural networks deep learning arrhythmias

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The effects of local variations in conditions on carbon storage and release in the continental mantle

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National science Review 2024年第6期11卷 22-36页

作者： stephen f.foley Chunfei Chen Dorrit E.Jacob school of Natural sciences Macquarie University Research school of Earth sciences Australian National University state Key laboratory of Geological Processes and Mineral Resources School of Earth Sciences China University of Geosciences

Recent advances indicate that the amount of carbon released by gradual degassing from the mantle needs to be revised upwards, whereas the carbon supplied by plumes may have been overestimated in the *** in rock types and oxidation state may be very local and exert strong influences on carbon storage and release mechanisms. Deep subduction may be prevented by diapirism in thick sedimentary packages,whereas carbonates in thinner sequences may be subducted. Carbonates stored in the mantle transition zone will melt when they heat up, recognized by coupled stable isotope systems(e.g. Mg, Zn, Ca). There is no single ‘mantle oxygen fugacity’, particularly in the thermal boundary layer(TBl) and lowermost lithosphere, where very local mixtures of rock types coexist. Carbonate-rich melts from either subduction or melting of the uppermost asthenosphere trap carbon by redox freezing or as carbonate-rich dykes in this zone. Deeply derived, reduced melts may form further diamond reservoirs, recognized as polycrystalline diamonds associated with websteritic silicate minerals. Carbon is released by either edge-driven convection,which tears sections of the TBl and lower lithosphere down so that they melt by a mixture of heating and oxidation, or by lateral advection of solids beneath rifts. Both mechanisms operate at steps in lithosphere thickness and result in carbonate-rich melts, explaining the spatial association of craton edges and carbonate-rich magmatism. High-pressure experiments on individual rock types, and increasingly on reactions between rocks and melts, are fine-tuning our understanding of processes and turning up unexpected results that are not seen in studies of single rocks. future research should concentrate on elucidating local variations and integrating these with the interpretation of geophysical signals. Global concepts such as average sediment compositions and a uniform mantle oxidation state are not appropriate for small-scale processes; an increa

关键词： lithospheric mantle carbonate melts deep carbon cycle craton destruction continental rifts

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Machine learning algorithm partially reconfigured on fPGA for an image edge detection system

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Journal of Electronic science and Technology 2024年第2期22卷 48-68页

作者： Gracieth Cavalcanti Batista Johnny Oberg Osamu saotome Haroldo f.de Campos Velho Elcio Hideiti shiguemori Ingemar soderquist Division of Electronic and Embedded systems KTH Royal Institute of TechnologyStockholm 16440Sweden Electronic Engineering Division Aeronautics Institute of TechnologySao Josédos Campos SP 12228-900Brazil laboratory of Applied Computing and Mathematics National Institute for Space ResearchSao Josédos Campos SP 12227-900Brazil Department of C4IsR Institute of Advanced StudiesSao Josédos Campos SP 12228-001Brazil saab AB Linkoping 58188Sweden

Unmanned aerial vehicles(UAVs)have been widely used in military,medical,wireless communications,aerial surveillance,*** key topic involving UAVs is pose estimation in autonomous navigation.A standard procedure for this process is to combine inertial navigation system sensor information with the global navigation satellite system(GNss)***,some factors can interfere with the GNss signal,such as ionospheric scintillation,jamming,or *** alternative method to avoid using the GNss signal is to apply an image processing approach by matching UAV images with georeferenced *** a high effort is required for image edge *** a support vector regression(sVR)model is proposed to reduce this computational load and processing *** dynamic partial reconfiguration(DPR)of part of the sVR datapath is implemented to accelerate the process,reduce the area,and analyze its granularity by increasing the grain size of the reconfigurable *** show that the implementation in hardware is 68 times faster than that in *** architecture with DPR also facilitates the low power consumption of 4 mW,leading to a reduction of 57%than that without *** is also the lowest power consumption in current machine learning hardware ***,the circuitry area is 41 times *** with Gaussian kernel shows a success rate of 99.18%and minimum square error of 0.0146 for testing with the planning *** system is useful for adaptive applications where the user/designer can modify/reconfigure the hardware layout during its application,thus contributing to lower power consumption,smaller hardware area,and shorter execution time.

关键词： Dynamic partial reconfiguration(DPR) field programmable gate array(fPGA)implementation Image edge detection support vector regression(sVR) Unmanned aerial vehicle(UAV) pose estimation

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Understanding the neighborhoods’in-between spaces on spatial perception,social interaction,and security

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frontiers of Architectural Research 2024年第1期13卷 21-36页

作者： lizeth félix Mariel Organista Autonomous University of Baja California Ensenada 22860Mexico

This study reflects on the impact that the neighborhoods’in-between spaces have on:spatial perception,social interaction,and *** sites,characterized by their abandonment and deterioration,can also be seen as crucial spaces of opportunity for cities,in the architectural,urban and landscape *** paper aims to analyze the sociospatial relationships in the neighborhoods’in-between spaces and examine the impact of inbetween space configuration on urban *** investigation draws on a survey of perception to residents about the requirements for a suitable social interaction in these *** study was developed in a neighborhood in the city periphery,characterized by their social dynamics and location in a nature conservation *** findings indicate that the appropriation process,activities,and collective practices are dependent on the spatial legibility,in this case when this increases,gives rise to improve the habitability and the rehabilitation of the in-between ***,the lack of design on in-between spaces substantially affects the use of these spaces and the social interaction among residents.

关键词： In-between spaces socio-spatial relationships Habitability Neighborhoods security

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CD4^(+)T cells produce IfN-I to license cDC1s for induction of cytotoxic T-cell activity in human tumors

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Cellular & Molecular Immunology 2024年第4期21卷 374-392页

作者： Xin lei Daniël C.de Groot Marij J.P.Welters Tom de Wit Ellen schrama Hans van Eenennaam saskia J.santegoets Timo Oosenbrug Annemarthe van der Veen Joris l.Vos Charlotte l.Zuur Noel f.C.C.de Miranda Heinz Jacobs sjoerd H.van der Burg Jannie Borst Yanling Xiao Department of Immunology Leiden University Medical CenterLeidenThe Netherlands Oncode Institute Leiden University Medical CenterLeidenThe Netherlands Department of Tumor Biology and Immunology The Netherlands Cancer InstituteAmsterdamThe Netherlands Department of Medical Oncology Oncode InstituteLeiden University Medical CenterLeidenThe Netherlands IMMIOs B.V. OssThe Netherlands Division of Medical Oncology The Netherlands Cancer InstituteAmsterdamThe Netherlands Department of Otorhinolaryngology leiden University Medical Center LeidenThe Netherlands Department of Pathology Leiden University Medical CenterLeidenThe Netherlands

CD4^(+)T cells can"help"or"license" conventional type 1 dendritic cells(cDC1s)to induce CD8^(+)cytotoxic T lymphocyte(CTl)anticancer responses,as proven in mouse *** recently identified cDC1s with a transcriptomic imprint of CD4^(+)T-cell help,specifically in T-cell-infiltrated human cancers,and these cells were associated with a good prognosis and response to PD-1-targeting ***,we delineate the mechanism of cDC1 licensing by CD4^(+)T cells in *** CD4^(+)T cells produce IfNβvia the sTING pathway,which promotes MHC-I antigen(cross-)presentation by cDC1s and thereby improves their ability to induce CTl anticancer *** cooperation with CD40 ligand(l),IfNβalso optimizes the costimulatory and other functions of cDC1s required for CTl response ***-I-producing CD4^(+)T cells are present in diverse T-cell-infiltrated cancers and likely deliver“help”signals to CTls locally,according to their transcriptomic profile and colocalization with“helped/licensed”cDCs and tumor-reactive CD8^(+)T *** agreement with this scenario,the presence of IfN-I-producing CD4^(+)T cells in the TME is associated with overall survival and the response to PD-1 checkpoint blockade in cancer patients.

关键词： CD4^(+)T-cell help cDC1 licensing IfN-I signaling CD40 costimulation (cross-)presentation CTl priming Tumor control

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