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Decorating crystalline YFe_(2-x)Al_(x) on the Mg_(60)la_(10)Ni_(20)Cu_(10) amorphous alloy as “hydrogen pump” to realize fast de/hydrogenation

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Journal of Materials Science & Technology 2024年第6期173卷 72-79页

作者： l.J.huang h.Wang l.Z.Ouyang M.Zhu h.J.lin School of Materials Science and Engineering Key Laboratory of Advanced Energy Storage Materials of Guangdong ProvinceSouth China University of TechnologyGuangzhou 510641China Institute of Advanced Wear&Corrosion Resistance and Functional Materials Jinan UniversityGuangzhou 510632China

Mg-based amorphous alloys are one of the potential.h.drogen storage materials but suffer from sluggish dehydrogenation/hydrogenation(de/hydrogenation)*** this work,as a new strategy,a hydrogen pump is built on the surface of amorphous alloys to solve this *** milling crystalline YFe_(2-x)Al_(x) hydrogen storage alloy with Mg_(60)la_(10)Ni_(20)Cu_(10) amorphous alloy,fine crystalline particles were seeded on amorphous alloy powder to form a“strawberry”*** to the TEM observation,a metallurgical bonding boundary formed between the Mg-based amorphous matrix and the Y-Fe-Al crystalline *** microstructure and de/hydrogenation kinetics investigation,the“hydrogen pump”effect of the seeded crystalline alloy was confirmed,which makes it much easier for the hydrogen to dissociate on and diffuse through the surface of the Mg-based amorphous *** such effect,the h absorption rate of Mg_(60)la_(10)Ni_(20)Cu_(10) amorphous alloy became almost eight times faster and it absorbs ~2.8 wt.% in 1 h at 130℃ under 4.5 MPa-h_(2).Further,fast hydrogenation can even achieve at 70℃ and the low-temperature dehydrogenation kinetics of the amorphous hydride can be also greatly *** present work proves that surface modification is of great importance for obtaining Mg-based amorphous alloy with ideal.h.drogen storage performance.

关键词： hydrogen storage Mg-based amorphous alloy hydrogen pump Composite structure

Spalling characteristics of high-temperature treated granitic rock at different strain rates

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第4期16卷 1280-1288页

作者： l.F.Fan Q.h.Yang X.l.Du The Key laboratory of Urban Security and Disaster Engineering of Ministry of Education Beijing University of TechnologyBeijing100124China

The dynamic spalling characteristics of rock are important for stability analysis in rock *** paper presented an experimental investigation on the dynamic spalling characteristics of granite with different temperatures and strain rates.A series of dynamic spalling tests with different impact velocities were conducted on thermally treated granite at different *** dynamic spalling strengths of granite with different temperatures and strain rates were determined.A model was proposed to correlate the dynamic spalling strength of granite,high temperature and strain *** results show that the spalling strength of granite decreases with increasing ***,the spalling strength of granite with a higher strain rate is larger than that with a lower strain *** proposed model can describe the relationship among dynamic spalling strength of granite,high temperature and strain rate.

关键词： Dynamic spalling characteristics high temperature Strain rate Dynamic loading Granite

Effect of cold-working on corrosion induced damage in lug joints

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Defence Technology（防务技术） 2024年第6期36卷 175-182页

作者： Ramanath M.N Chikmath l. Murthy h. Department of Aerospace Engineering Indian Institute of Technology-MadrasChennai 600036India Department of Aeronautical Engineering KLS Gogte Institute of TechnologyBelagavi 590008India

lug joints are preferred joineries for transferring heavy loads to parent components in aerospace *** experience corrosion due to environmental conditions,improper surface finishes and rubbing displacement between the pin and *** causes damage of different sizes and shapes near the *** degradation due to corrosion-induced damage is modelled as a through-pit at one of the identified critical locations through stress *** effect of this pit on fatigue crack initiation life is ***-hole is pre-stressed by cold-working and the benefits of inducing plastic wake on the intended performance of the lug joint during the damages due to corrosion are brought out and compared with non-cold-worked *** analysis is performed on this lug joint with *** results obtained highlight the benefits of cold-working and the methodology can be extended to damage growth and analyse the effect of surface treatments for better structural integrity of components of aerospace vehicles.

关键词： lug joint Corrosion Crack initiation Cold-working Structural integrity

Effect of radiative loss mechanisms on FIR thermometric parameters of Nd^(3+)-doped lithium tellurite glasses

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Journal of Rare Earths 2024年第7期42卷 1250-1257,I0002页

作者： C.Y.Morassuti A.P.l Silva l.A.O.Nunes S.M.lima l.h.C.Andrade Optical and Photothermal Spectroscopy Group(GEOF) Center for Studies in Natural Resources(CERNA)State University of Mato Grosso do Sul(UEMS)C.P.351DouradosMSBrazil Renato Archer Information Technology Center Dom Pedro I Highway(SP-65)Km 1436-Chácaras Campos dos AmaraisCampinasSPBrazil Institute of Physics of São Carlos University of São PauloSão CarlosSPBrazil

Nd^(3+)-doped tellurite glasses are promising materials for thermometers based on the fluorescence intensity ratio(FIR)***,at high Nd^(3+)concentrations,energy transfer(ET)processes such as optical reabsorption and cross-relaxation can affect the Nd^(3+)emission,which has been little explored in the ***,the present work investigated the use of Nd^(3+)-doped tellurite glass(samples doped with Nd^(3+)at 0.2 mol%,0.5 mol%,2.0 mol%,and 4.0 mol%)in fluorescence thermometers,in the temperature range from 299 to 371 *** results indicate a strong dependence of the FIR parameters on the Nd^(3+)concentration,due to changes in the emission band profiles caused by optical reabsorption of the Nd^(3+)emissions and cross-relaxation processes.A decrease of the relative sensitivity of the ratio^(4)F_(5/2)→^(4)I_(9/2)/^(4)F_(3/2)→^(4)I_(9/2)is observed for samples doped with higher amounts of Nd^(3+).The maximum relative sensitivity at 299 K is 3.00%/K,which is the highest value among the reported Nd^(3+)ions.

关键词： Nd^(3+)-doped tellurite glass Fluorescence intensity ratio Optical thermometry Judd-Ofelt Rare earths

On an isotropic porous solid cylinder:the analytical solution and sensitivity analysis of the pressure

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Applied Mathematics and Mechanics(English Edition) 2024年第9期45卷 1499-1522页

作者： h.ASGhARI l.MIllER R.PENTA J.MERODIO Departamento de Matematica Aplicada a las TIC ETS de Ingenieria de Sistemas InformaticosUniversidad Politecnica de MadridMadrid 28031Spain School of Mathematics and Statistics University of GlasgowGlasgow G128QQU.K.

Within this work,we perform a sensitivity analysis to determine the influence of the material input parameters on the pressure in an isotropic porous solid *** provide a step-by-step guide to obtain the analytical solution for a porous isotropic elastic cylinder in terms of the pressure,stresses,and elastic *** obtain the solution by performing a laplace transform on the governing equations,which are those of Biot's poroelasticity in cylindrical polar *** enforce radial boundary conditions and obtain the solution in the laplace transformed domain before reverting back to the time *** sensitivity analysis is then carried out,considering only the derived pressure *** analysis finds that the time t,Biot's modulus M,and Poisson's ratio ν have the highest influence on the pressure whereas the initial value of pressure P_(0) plays a very little role.

关键词： sensitivity analysis laplace transform cylindrical polar coordinate Biot's modulus cylinder

Uncovering the hierarchical clusters in the heat-affected zone of an electron beam weldedα/βtitanium alloy joint

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Journal of Materials Science & Technology 2024年第7期174卷 120-132页

作者： C.Xu X.h.Shao h.J.Yang M.lv h.Q.liu X.l.Ma Shenyang National laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China School of Materials Science and Engineering University of Science and Technology of ChinaShenyang 110016China Suzhou laboratory Suzhou 215028China Department of Mechanical Engineering Kyushu UniversityFukuoka 819-0395Japan Bay Area Center for Electron Microscopy Songshan Lake Materials LaboratoryDongguan 523808China

Using high-resolution transmission Kikuchi diffraction(TKD)and transmission electron microscopy(TEM),we examined the hierarchical clusters that form in situ in the heat-affected zone(hAZ),which are com-monly referred to as“ghost”structures,of bimodal titanium alloy Ti-5Al-2Sn-2Zr-4Mo-4Cr(wt%,TC17).The ghost structures are enriched with Al elements but poor in Mo and Cr compared to the surroundingβ*** results show that the ghost structure in middle-hAZ mainly consists ofα_(l)laths with a high-angle grain boundary,which exhibits the classic Burgers orientation relationship(BOR)with the host matrix,while it encircles theα_(P)grains in *** the ghost structure is evidenced to form via in-complete martensitic *** results further confirm that the ghost structure is composed ofαl and tinyβ_(l)laths with BOR,with the former being enriched with Al and poor with Cr and Mo,while the latter is the ***,twoα_(l)variant clusters with a check-mark morphology are fre-quently observed viewed along[0001]_(αl)//[110]_(βl)directions,which are dominated by the crystallographic and geometrical relationships betweenαandβ*** on the microstructural characterization,it is hypothesized that the ghost structure is transformed from the initialα_(P)phase,due to the coupling ef-fect of high thermal stress(which induces the formation of a large number of dislocations)and element diffusion caused by sudden temperature increase and plunge cooling in the hAZ during the welding pro-cess.

关键词： TC17 titanium alloy Electron beam welding(EBW) The ghost structure Transmission Kikuchi diffraction(TKD) Transmission electron microscopy(TEM)

In situ TEM investigation of electron irradiation and aging-induced high-density nanoprecipitates in an Mg-10Gd-3Y-1Zn-0.5Zr alloy

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Journal of Magnesium and Alloys 2024年第5期12卷 1841-1853页

作者： M.lv h.l.Ge Q.Q.Jin X.h.Shao Y.T.Zhou B.Zhang X.l.Ma Shenyang National laboratory for Materials Science Institute of Metal ResearchChinese Academy of Sciences72 Wenhua RoadShenyang 110016China School of Materials Science and Engineering University of Science and Technology of ChinaShenyang 110016China Materials Science and Engineering Research Center Guangxi University of Science and TechnologyLiuzhou 545006China

In-situ electron irradiation and aging are applied to introduce high-density precipitates in an Mg-10Gd-3Y-1Zn-0.5Zr(GWZ1031K,wt.%)alloy to improve the *** results show that the hardness of the Mg alloy after irradiation for 10 h and aging for 9 h at 250℃ is 1.64 GPa,which is approximately 64% higher than that of the samples before being *** is mainly attributed to γ'precipitates on the basal plane after irradiation and the high-density nanoscale β'precipitates on the prismatic plane after aging,which should be closely related to the irradiation-induced homogenous *** latter plays a key role in precipitation *** result paves a way to improve the mechanical properties of metallic materials by tailoring the precipitation through irradiation and aging.

关键词： Mg alloy Electron beam irradiation hardening Precipitates In-situ TEM

Dual Additives for Stabilizing li Deposition and SEI Formation in Anode-Free li-Metal Batteries

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Energy & Environmental Materials 2024年第3期7卷 84-92页

作者： Baolin Wu Chunguang Chen Dmitri l.Danilov Zhiqiang Chen Ming Jiang Rüdiger-A.Eichel Peter h.l.Notten Forschungszentrum Jülich(IEK-9) D-52425Jülich Germany RWTh Aachen University D-52074Aachen Germany lNM Institute of MechanicsChinese Academy of SciencesBeijing 100190China School of Engineering Sciences University of Chinese Academy of SciencesBeijing 100049China Eindhoven University of Technology P.O.Box 5135600 MBEindhoven The Netherlands School of Electronics and Information Institute of Carbon Neutrality and New EnergyHangzhou Dianzi UniversityHangzhou 310018China University of Technology Sydney BroadwaySydney NSW 2007Australia

Anode-free li-metal batteries are of significant interest to energy storage industries due to their intrinsically high ***,the accumulative li dendrites and dead li continuously consume active li during *** results in a short lifetime and low Coulombic efficiency of anode-free li-metal *** effective electrolyte additives can improve the li deposition homogeneity and solid electrolyte interphase(SEI)stability for anode-free li-metal ***,we reveal that introducing dual additives,composed of liAsF6 and fluoroethylene carbonate,into a low-cost commercial carbonate electrolyte will boost the cycle life and average Coulombic efficiency of NMC‖Cu anode-free li-metal *** NMC‖Cu anode-free li-metal batteries with the dual additives exhibit a capacity retention of about 75%after 50 cycles,much higher than those with bare electrolytes(35%).The average Coulombic efficiency of the NMC‖Cu anode-free li-metal batteries with additives can maintain 98.3%over 100 *** contrast,the average Coulombic efficiency without additives rapidly decline to 97%after only 50 *** situ Raman measurements reveal that the prepared dual additives facilitate denser and smoother li morphology during li *** dual additives significantly suppress the li dendrite growth,enabling stable SEI formation on anode and cathode *** results provide a broad view of developing low-cost and high-effective functional electrolytes for high-energy and long-life anode-free li-metal batteries.

关键词： anode-free lithium metal battery dual additives in situ Raman li growth SEI formation

Evidence for particle acceleration approaching PeV energies in the W51 complex

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Science Bulletin 2024年第18期69卷 2833-2841页

作者： lhAASO Collaboration Zhen Cao F.Aharonian Axikegu Y.X.Bai Y.W.Bao D.Bastieri X.J.Bi Y.J.Bi W.Bian A.V.Bukevich Q.Cao W.Y.Cao Zhe Cao J.Chang J.F.Chang A.M.Chen E.S.Chen h.X.Chen liang Chen lin Chen long Chen M.J.Chen M.l.Chen Q.h.Chen S.Chen S.h.Chen S.Z.Chen T.l.Chen Y.Chen N.Cheng Y.D.Cheng M.Y.Cui S.W.Cui X.h.Cui Y.D.Cui B.Z.Dai h.l.Dai Z.G.Dai Danzengluobu X.Q.Dong K.K.Duan J.h.Fan Y.Z.Fan J.Fang J.h.Fang K.Fang C.F.Feng h.Feng l.Feng S.h.Feng X.T.Feng Y.Feng Y.l.Feng S.Gabici B.Gao C.D.Gao Q.Gao W.Gao W.K.Gao M.M.Ge l.S.Geng G.Giacinti G.h.Gong Q.B.Gou M.h.Gu F.l.Guo X.l.Guo Y.Q.Guo Y.Y.Guo Y.A.han M.hasan h.h.he h.N.he J.Y.he Y.he Y.K.hor B.W.hou C.hou X.hou h.B.hu Q.hu S.C.hu D.h.huang T.Q.huang W.J.huang X.T.huang X.Y.huang Y.huang X.l.Ji h.Y.Jia K.Jia K.Jiang X.W.Jiang Z.J.Jiang M.Jin M.M.Kang I.Karpikov D.Kuleshov K.Kurinov B.B.li C.M.li Cheng li Cong li D.li F.li h.B.li h.C.li Jian li Jie li K.li S.D.li W.l.li W.l.li X.R.li Xin li Y.Z.li Zhe li Zhuo li E.W.liang Y.F.liang S.J.lin B.liu C.liu D.liu D.B.liu h.liu h.D.liu J.liu J.l.liu M.Y.liu R.Y.liu S.M.liu W.liu Y.liu Y.N.liu Q.luo Y.luo h.K.lv B.Q.Ma l.l.Ma X.h.Ma J.R.Mao Z.Min W.Mitthumsiri h.J.Mu Y.C.Nan A.Neronov l.J.Ou P.Pattarakijwanich Z.Y.Pei J.C.Qi M.Y.Qi B.Q.Qiao J.J.Qin A.Raza D.Ruffolo A.Sáiz M.Saeed D.Semikoz l.Shao O.Shchegolev X.D.Sheng F.W.Shu h.C.Song Yu.V.Stenkin V.Stepanov Y.Su D.X.Sun Q.N.Sun X.N.Sun Z.B.Sun J.Takata P.h.T.Tam Q.W.Tang R.Tang Z.B.Tang W.W.Tian C.Wang C.B.Wang G.W.Wang h.G.Wang h.h.Wang J.C.Wang Kai Wang Kai Wang l.P.Wang l.Y.Wang P.h.Wang R.Wang W.Wang X.G.Wang X.Y.Wang Y.Wang Y.D.Wang Y.J.Wang Z.h.Wang Z.X.Wang Zhen Wang Zheng Wang D.M.Wei J.J.Wei Y.J.Wei T.Wen C.Y.Wu h.R.Wu Q.W.Wu S.Wu X.F.Wu Y.S.Wu S.Q.Xi J.Xia G.M.Xiang D.X.Xiao G.Xiao Y.l.Xin Y.Xing D.R.Xiong Z.Xiong D.l.Xu R.F.Xu R.X.Xu W.l.Xu l.Xue D.h.Yan J.Z.Yan T.Yan C.W.Yang C.Y.Yang F.Yang F.F.Yang l.l.Yang M.J.Yang R.Z.Yang W.X.Yang Y.h.Yao Z.G.Yao l.Q.Yin N.Yin X.h.You Z.Y.You Y.h.Yu Q.Yuan h.Yue h.D.Zeng T.X.Zeng W.Zeng M.Zha B.B.Zhang F.Zhang h.Zhang 不详 Key laboratory of Particle Astrophysics&Experimental Physics Division&Computing Center Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China University of Chinese Academy of Sciences Beijing 100049China TIANFU Cosmic Ray Research Center ChengduChina Dublin Institute for Advanced Studies 31 Fitzwilliam Place2 DublinIreland Max-Planck-Institut for Nuclear Physics P.O.Box 103980Heidelberg 69029Germany School of Physical Science and Technology&School of Information Science and Technology Southwest Jiaotong UniversityChengdu 610031China School of Astronomy and Space Science Nanjing UniversityNanjing 210023China Center for Astrophysics Guangzhou UniversityGuangzhou 510006China Tsung-Dao lee Institute&School of Physics and Astronomy Shanghai Jiao Tong UniversityShanghai 200240China Institute for Nuclear Research of Russian Academy of Sciences Moscow 117312Russia hebei Normal University Shijiazhuang 050024China University of Science and Technology of China Hefei 230026China State Key laboratory of Particle Detection and Electronics China Key laboratory of Dark Matter and Space Astronomy&Key laboratory of Radio Astronomy Purple Mountain ObservatoryChinese Academy of SciencesNanjing 210023China Research Center for Astronomical Computing Zhejiang LaboratoryHangzhou 311121China Key laboratory for Research in Galaxies and Cosmology Shanghai Astronomical ObservatoryChinese Academy of SciencesShanghai 200030China School of Physics and Astronomy Yunnan UniversityKunming 650091China Key laboratory of Cosmic Rays(Tibet University) Ministry of EducationLhasa 850000China National Astronomical Observatories Chinese Academy of SciencesBeijing 100101China School of Physics and Astronomy(Zhuhai)&School of Physics(Guangzhou)&Sino-French Institute of Nuclear Engineering and Technology(Zhuhai) Sun Yat-sen UniversityZhuhai 519000&Guangzhou 510275GuangdongChina Institute of Frontier and Interdisciplinary Science Shandong UniversityQingdao 266237China APC UniversitéParis Cité

Theγ-ray emission from the W51 complex is widely acknowledged to be attributed to the interaction between the cosmic rays(CRs)accelerated by the shock of supernova remnant(SNR)W51C and the dense molecular clouds in the adjacent star-forming region,***,the maximum acceleration capability of W51C for CRs remains *** on observations conducted with the large high Altitude Air Shower Observatory(lhAASO),we report a significant detection ofγrays emanating from the W51 complex,with energies from 2 to 200 *** lhAASO measurements,for the first time,extend theγ-ray emission from the W51 complex beyond 100 TeV and reveal a significant spectrum bending at tens of *** combining the"π^(0)-decay bump"featured data from Fermi-lAT,the broadbandγ-ray spectrum of the W51 region can be well-characterized by a simple pp-collision *** observed spectral bending feature suggests an exponential cutoff at~400 TeV or a power-law break at~200 TeV in the CR proton spectrum,most likely providing the first evidence of SNRs serving as CR accelerators approaching the PeV ***,two young star clusters within W51B could also be theoretically viable to produce the most energeticγrays observed by *** findings strongly support the presence of extreme CR accelerators within the W51 complex and provide new insights into the origin of Galactic CRs.

关键词： UhE c-ray Cosmic rays SNR W51C Star clusters