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Recent Advances in Catalytic Carbonylation Reactions in Alternative Reaction Media

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Chinese Journal of Chemistry 2024年第4期42卷 406-429页

作者： Csaba Árvai lászló T.Mika department of Chemical and Environmental Process Engineering Faculty of Chemical Technology and BiotechnologyBudapest University of Technology and EconomicsMűegyetem rkp.3H-1111 BudapestHungary

Since the discovery of the hydroformylation(oxo-synthesis or Roelen reaction)and the Reppe-reaction,the transition metal-catalyzed carbonylation reactions,providing versatile,facile,and even atom-economic methods for the selective incorporation of C=O functionality to various skeletons,have gained tremendous importance in synthetic organic chemistry from laboratories to industrial *** carbonylation of carbon-carbon multiple bonds,aromatic halides,triflates,etc.,in the presence of various nucleophiles has led the way to produce aldehydes,carboxylic acids,esters,amides,etc.,in the fine chemical ***,these protocols usually proceed in conventional,fossil-based,and usually toxic reaction ***,several attempts have been directed to developing efficient carbonylation methods in alternative,less harmful,non-fossil-based and even in renewable reaction *** this review,we overview the recent applications of alternative solvents such as water,biomass-based alcohols,γ-valerolactone(GVl),2-methyltetrahydrofuran(2-MeTHF),ionic liquids(Ils),deep eutectic solvents(dES),alkyl levulinates,limonene,α-pinene,and dimethyl carbonate as well as fluorous media to improve efficiency,safety and environmentally benign nature of carbonylation protocols.

关键词： Carbonylation Catalysis Solvents Green chemistry Carbon monoxide Transition metals Homogeneous catalysis Palladium

Impacts of nuclear energy,greener energy,and economic progress on the load capacity factor:What we learn from the leading nuclear power economies?

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Geoscience Frontiers 2024年第3期15卷 322-335页

作者： Wei Teng Md.Monirul Islam lászlóVasa Shujaat Abbas Umer Shahzad School of Business Qilu Institute of TechnologyJinan 250200ShandongChina Graduate School of Economics and Management(GSEM) Ural Federal University(UrFU)YekaterinburgRussia Bangladesh Institute of Governance and Management(BIGM) University of DhakaBangladesh Széchenyi Istvàn University Faculty of EconomicsHungary School of Economics Széchenyi Istvàn UniversityGyorHungary department of Trade and Finance Faculty of Economics and ManagementCzech University of Life Sciences PragueCzech Republic Adnan Kassar School of Business Lebanese American UniversityBeirutLebanon

The worldwide tremor of environmental degradation commonly represents the escalation of emissions levels and ecological footprints that harm the planet’s *** is because of using gigantic non-renewable energy resources,urbanization stream and massive economic activities in the major industrialized *** this situation,we investigate the influence of disaggregated energy measures,e.g.,renewable,and nuclear energy,income growth and urbanization on the load capacity factor(biocapacity divided by the ecological footprint)of major nuclear power countries,such as France,the USA,Canada,China,and Russia during *** this end,we utilize the CS-ARdl procedure because of the endogeneity,common correlation,non-stationarity in data and heterogeneity in panel *** contribute to considering the supply side dynamic of environmental degradation parameter,the load capacity,from the perspective of the top nuclear power nations that deviates our analysis from the prevailing scholarly ***,our findings confirm a significantly positive impact of renewable and nuclear energy on the load capacity factor in improving environmental ***,economic growth and urbanization negatively affect the load capacity dynamics in spurring environmental *** findings are robust across an alternative estimation technique,namely the dumitrescu and Hurlin(dH)causation ***,we recommend formulating pragmatic policies to deter the detrimental effects of income and urbanization by properly utilizing sustainable energy resources to conserve the natural environment.

关键词： Renewable energy Economic growth Urbanization load capacity Environmental degradation Top nuclear power countries

linking gold prices,fossil fuel costs and energy consumption to assess progress towards sustainable development goals in newly industrialized countries

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Geoscience Frontiers 2024年第3期15卷 447-457页

作者： Muhammad Farhan Bashir Muhammad Adnan Bashir Syed Ali Raza Yuriy Bilan lászlóVasa College of Management Shenzhen UniversityShenzhen518060GuangdongPR China Huangpu Institute Guangdong University of Foreign StudiesGuangzhouGuangdongChina department of Business Administration IQRA University Karachi-75300Pakistan Adnan Kassar School of Business Lebanese American UniversityBeirutLebanon Faculty of Management Rzeszow University of Technologyal.Powstanców Warszawy 1235-959 RzeszówPoland Faculty of Economics Széchenyi Istvàn UniversityHungary

The continuous rise in global environmental challenges has led to urgency toward establishing a secure framework to achieve sustainable development *** study establishes a novel theoretical framework to analyze the role of energy prices,energy consumption,gold prices and economic growth on environmental degradation in newly industrialized *** realize sustainable development goals and foster environmental defence,this study utilizes CS-ARdl as the main econometric approach to investigate the asymmetric association between environmental degradation and relevant *** also use AMG,CS-dl,driscoll-Kray and FGlS to enhance the robustness of our *** econometric approach reveals that energy resource prices and renewable energy consumption reduce environmental degradation,while gold prices and fossil energy consumption elevate environmental *** also confirm the existence of the EKC *** findings of our extensive analysis paved the way for a welldesigned environmental policy for NIC economies should focus on renewable energy consumption,green investments,and structural changes.

关键词： Gold prices Fossil fuel costs Renewable Energy Consumption Environmental degradation Newly industrialized countries COP27

Feasibility of achieving net-zero energy performance in high-rise buildings using solar energy

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Energy and Built Environment 2024年第6期5卷 946-956页

作者： Mehrdad Shirinbakhsh l.d.danny Harvey University of Toronto 100St.George StreetTorontoONM5S 3G3Canada

As part of a broad strategy to reach net-zero greenhouse gas emissions and limit global warming,many countries are requiring all new buildings to have net-zero energy *** requires that on-site energy use not exceed on-site generation of renewable energy(taken here to be solar energy),or equivalently,that the building Energy Use Intensity(EUI,kWh/m^(2)a)not exceed the supply of on-site solar energy(electricity and heat)per m^(2)of floor area per *** this basis,we find that achieving net-zero energy performance in an archetype 40-story square building in 16 different cities of North America requires EUI of 17–24 kWh/m^(2)a using PV panels,and 19–28 kWh/m^(2)a using PVT *** building orientation to a non-square floor shape can improve maximum permitted EUI by up to 50%in PV and 60%in PVT ***,the best-performing residential and commercial buildings have EUIs of 50–75 kWh/m^(2)*** if building heights are limited to 5–10 floors does the available solar energy,and thus the permitted EUI,reach 50–75 kWh/m^(2)***,we recommend that policymakers not require high-rise buildings to be net-zero energy,unless they are prepared to limit building heights to 5–10 floors.

关键词： High-rise net-zero energy buildings Building geometry Building height Solar NZEB

Oligodendroctyes:the forgotten players of diabetes pathophysiology

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Neural Regeneration Research 2024年第11期19卷 2349-2350页

作者： Juan Antonio lópez-Villodres Beatriz García-díaz departamento Fisiología Humana Histología HumanaAnatomía Patológica y Educación Física y DeportivaFacultad de MedicinaUniversidad de MálagaMálagaSpain UGC Neurociencia.Instituto de Investigación Biomédica de Málaga y Plataforma en Nanomedicina(IBIMA Plataforma Bionand) MálagaSpain

Oligodendrocytes(Ols),glial cells that provide myelin sheaths to axons in the central nervous system(CNS),have a dual ***,this myelin fatty cover around the axons protects the nerves and is crucial for the saltatory propagation of action *** and not less important,Ols provide trophic support to neurons and ***,Ol metabolism is important for Ol well-being and the proper accomplishment of their functions,and Ol metabolism energetics directly affect the energy metabolism of neighboring neurons.

关键词： metabolism nerves myelin

Sex differences in Alzheimer's disease:an urgent research venue to follow

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Neural Regeneration Research 2024年第12期19卷 2569-2570页

作者： Raquel Jiménez-Herrera Ana Contreras Juan d.Navarro-lópez lydia Jiménez-díaz Neurophysiology&Behavior lab University of Castilla-La ManchaSchool of Medicine of Ciudad RealCiudad RealSpain

due to increasing life expectancy,the amount of people with dementia worldwide is expected to experience a substantial rise,with estimates indicating a growth from 55 million in 2019 to a staggering 139 million by the... 详细信息

关键词： Alzheimer predominant estimates

Silk-based nerve guidance conduits with macroscopic holes modulate the vascularization of regenerating rat sciatic nerve

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Neural Regeneration Research 2025年第6期20卷 1789-1800页

作者： Carina Hromada Patrick Heimel Markus Kerbl lászlóGál Sylvia Nürnberger Barbara Schaedl James Ferguson Nicole Swiadek Xavier Monforte Johannes C.Heinzel Antal Nógrádi Andreas H.Teuschl-Woller david Hercher department life Science Engineering University of Applied Sciences Technikum WienViennaAustria Austrian Cluster for Tissue Regeneration ViennaAustria ludwig Boltzmann Institute for Traumatology The Research Center in Cooperation with AUVAViennaAustria University Clinic of dentistry Medical University of ViennaViennaAustria department of Plastic Reconstructive and Aesthetic SurgeryLandesklinikum Wiener Neustadt2700 Wiener NeustadtAustria department of Anatomy Histology and EmbryologyAlbert Szent-Györgyi Medical SchoolUniversity of SzegedSzegedHungary Medical University of Vienna Department of Orthopedics and Trauma SurgeryDevision of Trauma SurgeryViennaAustria department of Hand- PlasticReconstructive and Burn SurgeryBG Unfallklinik TuebingenUniversity of TuebingenTuebingenGermany

Peripheral nerve injuries induce a severe motor and sensory deficit. Since the availability of autologous nerve transplants for nerve repair is very limited, alternative treatment strategies are sought, including the use of tubular nerve guidance conduits(tNGCs). However, the use of tNGCs results in poor functional recovery and central necrosis of the regenerating tissue, which limits their application to short nerve lesion defects(typically shorter than 3 cm). Given the importance of vascularization in nerve regeneration, we hypothesized that enabling the growth of blood vessels from the surrounding tissue into the regenerating nerve within the tNGC would help eliminate necrotic processes and lead to improved regeneration. In this study, we reported the application of macroscopic holes into the tubular walls of silk-based tNGCs and compared the various features of these improved silk^(+) tNGCs with the tubes without holes(silk^(–) tNGCs) and autologous nerve transplants in an 8-mm sciatic nerve defect in rats. Using a combination of micro-computed tomography and histological analyses, we were able to prove that the use of silk^(+) tNGCs induced the growth of blood vessels from the adjacent tissue to the intraluminal neovascular formation. A significantly higher number of blood vessels in the silk^(+) group was found compared with autologous nerve transplants and silk^(–), accompanied by improved axon regeneration at the distal coaptation point compared with the silk^(–) tNGCs at 7 weeks postoperatively. In the 15-mm(critical size) sciatic nerve defect model, we again observed a distinct ingrowth of blood vessels through the tubular walls of silk^(+) tNGCs, but without improved functional recovery at 12 weeks postoperatively. Our data proves that macroporous tNGCs increase the vascular supply of regenerating nerves and facilitate improved axonal regeneration in a short-defect model but not in a critical-size defect model. This study suggests that further optimizatio

关键词： axon regeneration blood vessel functional recovery macroporous nerve lesion peripheral nerve repair sciatic nerve silk-based nerve guidance conduit vascularization

Pathogenesis and clinical features of severe hepatitis E virus infection

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World Journal of Virology 2024年第2期13卷 19-33页

作者： lászló Orosz Károly Péter Sárvári Áron dernovics András Rosztóczy Klára Megyeri department of Medical Microbiology University of SzegedSzeged 6720Csongrád-CsanádHungary department of Internal Medicine Division of GastroenterologyUniversity of SzegedSzeged 6725Csongrád-CsanádHungary

The hepatitis E virus(HEV),a member of the Hepeviridae family,is a small,non-enveloped icosahedral virus divided into eight distinct genotypes(HEV-1 to HEV-8).Only genotypes 1 to 4 are known to cause diseases in *** 1 and 2 commonly spread via fecal-oral transmission,often through the consum-ption of contaminated *** 3 and 4 are known to infect pigs,deer,and wild boars,often transferring to humans through inadequately cooked *** hepatitis caused by HEV in healthy individuals is mostly asymptomatic or associated with minor symptoms,such as ***,in immunosup-pressed individuals,the disease can progress to chronic hepatitis and even escalate to *** pregnant women,an HEV infection can cause fulminant liver failure,with a potential mortality rate of 25%.Mortality rates also rise amongst cirrhotic patients when they contract an acute HEV infection,which can even trigger acute-on-chronic liver failure if layered onto pre-existing chronic liver *** the prevalence of HEV infection continues to rise worldwide,highlighting the particular risks associated with severe HEV infection is of major medical *** text offers a brief summary of the characteristics of hepatitis developed by patient groups at an elevated risk of severe HEV infection.

关键词： Hepatitis E virus Cirrhosis Acute-on-chronic liver failure Pregnancy Immune dysfunction Open reading frames 1-4

Competitive interactions and coexistence of sympatric flagship carnivores in Asia

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Integrative Zoology 2024年第2期19卷 183-199页

作者： Zhilin lI Jiayu lU Xiaoyi SHI li’an dUO James l.d.SMITH Tianming WANG Tianjin Key laboratory of Conservation and Utilization of Animal diversity College of Life SciencesTianjin Normal UniversityTianjinChina department of Fisheries Wildlife and Conservation BiologyUniversity of MinnesotaSt.PaulMinnesotaUSA Ministry of Education Key laboratory for Biodiversity Science and Engineering College of Life SciencesBeijing Normal UniversityBeijingChina National Forestry and Grassland Administration Key laboratory for Conservation Ecology of Northeast Tiger and leopard BeijingChina

Understanding the competition and coexistence of flagship carnivores is key to creating strategies for their conservation in the face of global carnivore *** studies exploring the dynamics and competition between tigers(Panthera tigris)and leopards(***)span decades,there is a lack of understanding regarding the factors that influence their coexistence mechanisms on a broad scale,as well as the drivers determining their exploitative and interference *** gathered a comprehensive list of research papers among which 36 papers explored the interspecific interactions between tigers and leopards and tested the influence of biotic and abiotic factors on the coexistence mechanisms along three dimensions using multiple response variables regression models;we also tested the influence of ecological drivers determining the exploitative or interference competition between tigers and *** and ungulate density were the most important predictors in regulating the coexistence *** and leopards exhibited more positive relations/higher overlaps as elevation increased in the spatial *** addition,they showed a higher dietary overlap in the prey-rich *** determined that interference competition between tigers and leopards was less frequently observed in habitats with dense tree cover and homogeneous vegetation ***,studies with multiple metrics would promote the detection of interference *** study provides new insight into the competitive interactions and coexistence mechanisms of tigers and leopards on a broad ***-makers and managers should pay more attention to the factors of elevation,prey abundance,and habitat structures for the conservation of tigers and leopards.

关键词： carnivores coexistence mechanisms competitive interactions exploitative competition interference competition