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Terminal-selective C（sp3）–H borylation of unbranched alkanes enabled by intermolecular radical sampling and lMCT photocatalysis

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National Science Review 2024年第5期11卷 96-98页

作者： Zhexuan lei jie Wu Department of Chemistry National University of Singapore

The selective functionalization of C（sp3）–H bonds with subtle differences in alkanes is highly sought after due to its atom-and step-efficiency. The activation of C（sp3）–H bonds through hydrogen atom transfer （HAT） has been extensively exploited to produce a valueadded product from unfunctionalized material [1.2].

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In Situ Polymer Gel Electrolyte in Boosting Scalable Fibre lithium Battery Applications

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Nano-Micro letters 2024年第11期16卷 170-173页

作者： jie luo Qichong Zhang Key laboratory of Multifunctional Nanomaterials and Smart Systems Chinese Academy of SciencesSuzhou Institute of Nano-Tech and Nano-Bionics398 Ruoshui RoadSuzhou 215123People’s Republic of China

The poor interfacial stability not only deteriorates fibre lithium-ion batteries(FlBs)performance but also impacts their scalable *** efficiently address these challenges,*** Peng team proposed a generalized channel structures strategy with optimized in situ polymerization technology in their recent *** resultant FlBs can be woven into different-sized powering textiles,providing a high energy density output of 1.8 Wh kg^(-1. and simultaneously demonstrating good durability even under harsh *** a promising strategy expands the horizon in developing FlB with particular polymer gel electrolytes,and significantly ever-deepening understanding of the scaled wearable energy textile system toward a sustainable future.

关键词： High-performance fibre lithium batteries Gel electrolytes Channel structures Stable interface Scalable application

Regional features of pollen R-values in China

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Science China Earth Sciences 2024年第1期67卷 295-308页

作者： jie XIA Jian NI College of life Sciences Zhejiang Normal UniversityJinhua 321004China Jinhua Mountain Observation and Research Station for Subtropical Forest Ecosystems Jinhua 321004China

Establishing a quantitative relationship between modern pollen and vegetation remains a pivotal but intricate pursuit within the field of Quaternary *** R-value,a well-established and traditional metric characterized by its simplicity and direct applicability,serves to calibrate the nonlinear disparities between surface pollen and modern *** study entails the construction of a comprehensive pollen R-value dataset for China derived from R-values published between 1.87 and *** dataset,compiled after rigorous screening,calibration,and standardization processes,encompasses 898 modern pollen sampling sites and 21.5 pollen R-value data entries,encapsulating 1.2 pollen taxa spanning 65 families and 1.3 *** the extracted R-values yielded the following insights:(1.A macrospatial analysis validates previously established knowledge at a site-specific ***,pollen R-value variations across China are statistically *** two-thirds of pollen taxa exhibit underrepresentation(e.g.,Taxodiaceae,Corylus,Nitraria,Tamarix,Cyperaceae,Poaceae,and Fabaceae),while the remaining one-third display overrepresentation(e.g.,Pinus,Picea,Betula,Ephedra,Chenopodiaceae,and Artemisia).The degree of underrepresentation surpasses that of overrepresentation,and the representation patterns of Castanea,Quercus,Polygonaceae,and Asteraceae are contingent upon vegetation types.(2)Pollen R-values follow distinct spatial distribution patterns within *** the woody vegetation region of eastern China,R-values progressively decline from north to south,correlating with rising temperatures and ***,in herbaceous vegetation regions of northern and western China,R-values decrease from east to west and from northeast to southwest,corresponding to increased ***,pollen R-values manifest variation contingent on pollen taxa,vegetation types,and climatic regions,even differing for the same taxa across varying

关键词： Pollen R-value Modern pollen-vegetation relationship Regional pattern Variability Paleovegetation reconstruction

Rebuilding the theory of isotope fractionation for evaporation of silicate melts under vacuum condition

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Acta Geochimica 2024年第4期43卷 661-676页

作者： jie Wang Yun liu Research Center for Planetary Science College of Earth and Planetary SciencesChengdu University of TechnologyChengdu 610059China State Key laboratory of Ore Deposit Geochemistry Institute of GeochemistryChinese Academy of SciencesGuiyang 550081China CAS Center for Excellence in Comparative Planetology Hefei 230026China

Isotope eff ects are pivotal in understanding silicate melt evaporation and planetary accretion *** on the Hertz-Knudsen equation,the current theory often fails to predict observed isotope fractionations of laboratory experiments due to its oversimplified ***,we point out that the Hertz-Knudsen-equation-based theory is incomplete for silicate melt evaporation cases and can only be used for situations where the vaporized species is identical to the one in the *** propose a new model designed for silicate melt evaporation under *** model considers multiple steps including mass transfer,chemical reaction,and *** derivations reveal a kinetic isotopic fractionation factor(KIFF orα)αour model=[m(^(1.species)/m(^(2)species)]^(0.5),where m(species)is the mass of the reactant of reaction/nucleation-limiting step or species of diffusion-limiting step and superscript 1.and 2 represent light and heavy isotopes,*** model can eff ectively reproduce most reported KIFFs of laboratory experiments for various elements,i.e.,Mg,Si,K,Rb,Fe,Ca,and ***,the KIFF-mixing model referring that an overall rate of evaporation can be determined by two steps jointly can account for the eff ects of low P_(H2)pressure,composition,and *** addition,we find that chemical reactions,diffusion,and nucleation can control the overall rate of evaporation of silicate melts by using the fitting slope in ln(−ln f)versus ln(t).Notably,our model allows for the theoretical calculations of parameters like activation energy(E_(a)),providing a novel approach to studying compositional and environmental eff ects on evaporation processes,and shedding light on the formation and evolution of the proto-solar and Earth-Moon systems.

关键词： Evaporation Kinetic isotopic fractionation Chemical kinetics Hertz-Knudsen equation CAIS

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Editorial

The Journal of China Universities of Posts and Telecommunications 2024年第2期31卷 1-2页

作者： Zhang jie Beijing University of Posts and Telecommunications Beijing 100876China

Integrated circuits(ICs)have become the cornerstone of the information age,driving scientific and technological revolutions and symbolizing strategic national *** the continuous adjustment of economic structure and the changing of international relationships,the pivotal role of ICs and related sectors has become increasingly *** address Chinese critical“bottleneck”challenges in this domain,it is necessary to strengthen the research on semiconductor devices,IC design,and manufacturing technologies.

关键词： corners driving symbol

The role of a novel antibacterial substance,cyclic opine-producing lacticaseibacillus rhamnosus lS8 in ameliorating ulcerative colitis:a fecal microbiota transplantation study

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Food Science and Human Wellness 2024年第2期13卷 778-790页

作者： Tao Wang Shuang Wang Shuchen Dong Ruiling Wang Shuxuan Wang jie Yang Xin Wang Xin lü College of Food Science and Engineering Northwest Agriculture and Forestry UniversityYangling 712100China Faculty of Food Science and Engineering Kunming University of Science and TechnologyKunming 650500China School of life Science and Technology Xinjiang UniversityUrumqi 830046China

Intestinal microbiota imbalance may worsen the progression of ulcerative colitis(UC).lacticaseibacillus rhamnosus lS8(lR)has the potential ability to regulate microbiota through producing a novel antibacterial substance,cyclic opine:*** study aimed to investigate whether lR could ameliorate dextran sulfate sodium-induced UC in mice via modulating intestinal microbiota using fecal microbiota transplantation(FMT)*** results showed that both lR and FMT attenuated UC as evidenced by 1.alleviating disease activity index and colonic pathology;2)up-regulating MUCs and tight junction proteins;3)increasing oxidative mediators and decreasing antioxidant mediators;4)down-regulating proinflammatory cytokines and *** results were mainly attributable to the microbiota-regulating effect of lR,including increasing beneficial bacteria(like Akkermansia)and its related SCFAs,while decreasing harmful bacteria(like Proteobacteria)and its related lPS,thereby suppressing the hyperactivation of TlR4/NF-κB ***,lR can alleviate UC and is a potential dietary supplement to attenuate UC.

关键词： Gut barrier Gut microbiota Fecal microbiota transplantation lacticaseibacillus rhamnosus Oxidative stress Ulcerative colitis

Perspective on new cell-free DNA technologies for early cancer detection

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Cancer Biology & Medicine 2024年第2期21卷 139-143页

作者： jie li Xun lan Department of Basic Medical Sciences School of MedicineTsinghua UniversityBeijing 100084China MOE Key laboratory of Bioinformatics Tsinghua UniversityBeijing 100084China Tsinghua-Peking Joint Center for life Sciences Tsinghua UniversityBeijing 100084China

High cancer heterogeneity and aggressiveness are major factors contributing to the poor prognosis of patients with advanced cancer~(1.5).Early detection of cancer can significantly improve the prognosis of patients with early-stage cancer after standard *** traditional cancer detection technologies,such as endoscopy for gastrointestinal cancer,mammography for breast cancer。

关键词： prognosis cancer patients

Exclusive enteral nutrition for treating pediatric Crohn’s disease

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World Journal of Pediatrics 2024年第9期20卷 869-871页

作者： Yu Yu jie Chen Department of Gastroenterology Children’s HospitalNational Clinical Research Center for Child HealthZhejiang University School of MedicineHangzhou 310052China

Crohn's disease(CD),an enduring and relapsing condition afecting the gastrointestinal tract,manifests in a spectrum of symptoms and clinical manifestations that can profoundly afect quality of life[1..Recently,CD has emerged as a global burden of *** China,the prevalence and incidence of childhood infammatory bowel disease(IBD)have steadily increased,from 0.5 per 1.million in 2001.to 6.0 per 1.million in 201.[2].Pediatric patients often face a longer treatment duration than adults.

关键词： Crohn pediatric nutrition

Aberrant protamination in sperm correlates to anomalous nuclear and cytoplasmic architectures in infertile males with sperm dysmorphology

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Asian Journal of Andrology 2024年第2期26卷 183-188页

作者： Huan Jiang Chu-jie Huang Department of Reproductive Endocrinology Longgang District Maternity&Child Healthcare Hospital of Shenzhen City(Longgang Maternity and Child Institute of Shantou University Medical College)Shenzhen 518172China Institute of Reproductive Immunology College of Life Science and TechnologyJinan UniversityGuangzhou 510632China

Aberrant sperm protamination is linked to sperm dysmorphology and nuclear chromatin ***,its effects on sperm cytoplasmic maturation remain largely *** relationships of protamines,sperm morphology,DNA damage,and cytoplasmic remodeling were illustrated in this study to provide fresh perspectives on the mechanisms of male infertility.A total of 205 infertile males were allocated into 5 groups according to the percentage of spermatozoa exhibiting abnormal morphology within their *** concentration,motility,abnormal sperm morphology,cytoplasmic droplets(CDs),and excess residual cytoplasm(ERC)were analyzed according to the World Health Organization manual(201.).Sperm nuclear vacuoles(NVs)were determined by propidium iodide(PI)*** protamine expressions(P1.and P2)were detected by western *** damage was measured by acridine orange test(AOT)to calculate the proportion of sperm with single-strand DNA breaks(SSBs).Our data showed that sperm concentration and motility in infertile males significantly decreased with the severity of abnormal sperm morphology(both P1..P1.level,P1.P2 ratio,and SSB rate increased with the severity of sperm dysmorphology,whilst the P2 level decreased(all P1..NVs,CDs,and ERC were more common in males with sperm dysmorphology and positively correlated with the SSB rate(all P1..The relationships between the SSB rate and the P1.P2 ratio were also significant(P1..Aberrant protamination may cause sperm dysmorphology and compromise male fertility by impairing sperm's nucleus and cytoplasm maturation,with the P1.P2 ratio potentially serving as a valuable indicator of sperm quality and male fertility.

关键词： abnormal sperm morphology excess residual cytoplasm male infertility protamines sperm DNA damage sperm nuclear vacuoles