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High Efficiency Mixed Amine Adsorbents for Directly Capturing Carbon Dioxide from Air

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Chemical Research in Chinese Universities 2025年第1期41卷 138-145页

作者： WU Yilu ZHENG Haolong XIA Zihan fu Chengmin XU Feng YAN Jian School of Environment and Chemical Engineering Foshan UniversityFoshan528000P.R.China Guangzhou Zhixin High School Guangzhou510080P.R.China

The development of effective adsorbents with high amine efficiency and CO_(2)adsorption almost unaffected by humidity is extremely *** this study,we introduce an innovative solid amine adsorbent,TETA/DEA@FS,composed of triethylenetetramine(TETA)and diethanolamine(DEA)functionalized fumed silica(FS),which exhibits exceptional capability in selectively capturing trace CO_(2)from N_(2).TETA/DEA@FS shows an exceptionally high capacity of CO_(2)adsorption of 1.13 mmol/g at the temperature of 298 K and the pressure of 0.0004 bar(1 bar=100 kPa),and achieves an unprecedented CO_(2)/N_(2)IAST selectivity of 1.70×10^(12).TETA/DEA@FS exhibits high amine efficiency,with breakthrough experiments demonstrating that CO_(2)adsorption remains nearly unaffected by ***,TETA/DEA@FS demonstrates rapid CO_(2)adsorption kinetics and outstanding cyclic stability.

关键词： Direct air capture(DAC) CO_(2) N_(2) Triethylenetetramine Diethanolamine

Unsupervised multiplex graph diffusion networks with multi-level canonical correlation analysis for multiplex graph representation learning

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Science China(Information Sciences) 2025年第03期68卷 66-79页

作者： Sichao fu Qinmu PENG Yange HE Baokun DU Bin ZOU Xiao-Yuan JING Xinge YOU School of Electronic Information and Communications Huazhong University of Science and Technology Platform Operation and Marketing Center JD Retail Faculty of Mathematics and Statistics Hubei Key Laboratory of Applied Mathematics Hubei University School of Computer Science Wuhan University

In recent years, unsupervised multiplex graph representation learning(UMGRL) has received increasing research interest, which aims to learn discriminative node features from the multiplex graphs supervised by data without the guidance of labels. Although these designed UMGRL methods have obtained great success in various graph-related tasks, most existing UMGRL models still have the following issues: highly depending on complex self-supervised strategies(i.e., data augmentation,pretext tasks, and negative pairs sampling), restricted receptive fields, and only aggregating low-frequency information between nodes. In this paper, we propose a simple unsupervised multiplex graph diffusion network(UMGDN) with the aid of multi-level canonical correlation analysis to solve the above issues. Specifically, we first decouple the feature transform and propagation processes of the graph convolution layer to further improve the generalization of the learnable parameters. And then, we propose adaptive diffusion propagation to capture long-range dependency relationships between nodes, not the local neighborhood interactions. Finally, a multi-level canonical correlation analysis loss on both the feature transform and propagation processes is proposed to maximize the correlation of the same node features from multiple graphs for guiding model optimization. Compared to the existing UMGRL models, our proposed UMGDN does not need to introduce any data augmentation, negative pairs sampling techniques, complex pretext tasks, and also adaptively aggregates the optimal frequency information between nodes to generate more robust node embeddings. Extensive experiments on four popular datasets and two graph-related tasks demonstrate the effectiveness of the proposed method.

关键词： unsupervised multiplex graph representation learning graph neural networks node classification node clustering

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Bioenergy recovery and carbon emissions benefits of short-term bio-thermophilic pretreatment on low organic sewage sludge anaerobic digestion:A pilot-scale study

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Journal of Environmental Sciences 2025年第2期148卷 321-335页

作者： Hui Wang Xiang fu Haozhe Huang Danni Shen Dongdong Fan Liming Zhu Xiaohu Dai Bin Dong College of Environmental Science and Engineering Tongji UniversityShanghai 200092China Yangtze Eco-Environment Engineering Research Center China Three Gorges CorporationBeijing 100038China Yangtze River Eco-Environmental Engineering Research Center Shanghai InvestigationDesign and Research Institute Co.LTDShanghai 200092China China Construction Third Engineering Bureau First Engineering Co. Ltd.Wuhan 430000China

Sewage sludge in cities of Yangzi River Belt,China,generally exhibits a lower organic content and higher silt contentdue to leakage of drainage system,which caused low bioenergy recovery and carbon emission benefits in conventional anaerobic digestion(CAD).Therefore,this paper is on a pilot scale,a bio-thermophilic pretreatment anaerobic digestion(BTPAD)for low organic sludge(volatile solids(VS)of 4%)was operated with a long-term continuous flow of 200 *** VS degradation rate and CH_(4) yield of BTPAD increased by 19.93%and 53.33%,respectively,compared to those of *** analysis of organic compositions in sludge revealed that BTPAD mainly improved the hydrolysis of proteins in *** analysis of microbial community proportions by high-throughput sequencing revealed that the short-term bio-thermophilic pretreatment was enriched in Clostridiales,Coprothermobacter and Gelria,was capable of hydrolyzing acidified proteins,and provided more volatile fatty acid(VFA)for the subsequent *** combined with fluorescence quantitative polymerase chain reaction(PCR)analysis showed that the number of bacteria with high methanogenic capacity in BTPAD was much higher than that in CAD during the medium temperature digestion stage,indicating that short-term bio-thermophilic pretreatment could provide better methanogenic conditions for ***,the greenhouse gas emission footprint analysis showed that short-term bio-thermophilic pretreatment could reduce the carbon emission of sludge anaerobic digestion system by 19.18%.

关键词： Sludge Anaerobic digestion Bio-thermophilic pretreatment Pilot scale Molecular microbiology Carbon emissions

PS-CoT-Adapter: adapting plan-and-solve chain-of-thought for ScienceQA

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Science China(Information Sciences) 2025年第1期68卷 392-393页

作者： Qun LI Haixin SUN fu XIAO Yiming WANG Xinping GAO Bir BHANU School of Computer Science Nanjing University of Posts and Telecommunications Purple Mountain Laboratories Department of Electrical and Computer Engineering University of California at Riverside

Large language models (LLMs) have recently shown remarkable performance in a variety of natural language processing (NLP) *** further explore LLMs'reasoning abilities in solving complex problems,recent research [1-3]has investigated chain-of-thought (CoT) reasoning in complex multimodal scenarios,such as science question answering (ScienceQA) tasks [4],by fine-tuning multimodal models through human-annotated CoT ***,collected CoT rationales often miss the necessary rea-soning steps and specific expertise.

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The crosstalk between cellular survival pressures and N6-methyladenosine modification in hepatocellular carcinoma

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Hepatobiliary & Pancreatic Diseases International 2025年第1期24卷 67-75页

作者： Chu-Li fu Zheng-Wei Zhao Qiang-Nu Zhang Department of Hematology and Oncology Guangzhou Women and Children's Medical Center Guangzhou Medical University Biomedicine Research Center Guangdong Provincial Key Laboratory of Major Obstetric Disease Guangdong Provincial Clinical Research Center for Obstetrics and Gynecology the Third Affiliated Hospital of Guangzhou Medical University

Background:Within the tumor microenvironment, survival pressures are prevalent with potent drivers of tumor progression, angiogenesis, and therapeutic resistance. N6-methyladenosine (m6 A) methylation has been recognized as a critical post-transcriptional mechanism regulating various aspects of mRNA metabolism. Understanding the intricate interplay between survival pressures and m6 A modification provides new insights into the molecular mechanisms underlying hepatocellular carcinoma (HCC) progression and highlights the potential for targeting the survival pressures-m6 A axis in HCC diagnosis and *** sources:A literature search was conducted in Pub Med, MEDLINE, and Web of Science for relevant articles published up to April 2024. The keywords used for the search included hepatocellular carcinoma,cellular survival, survival pressure, N6-methyladenosine, tumor microenvironment, stress response, and ***:This review delves into the multifaceted roles of survival pressures and m6 A RNA methylation in HCC, highlighting how survival pressures modulate the m6 A landscape, the impact of m6 A modification on survival pressure-responsive gene expression, and the consequent effects on HCC cell survival,proliferation, metastasis, and resistance to treatment. furthermore, we explored the therapeutic potential of targeting this crosstalk, proposing strategies that leverage the understanding of survival pressures and m6 A RNA methylation mechanisms to develop novel, and more effective treatments for ***:The interplay between survival pressures and m6 A RNA methylation emerges as a complex regulatory network that influences HCC pathogenesis and progression.

关键词： Hepatocellular carcinoma N6-methyladenosine methylation Hypoxia Target therapy Survival pressure

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摩擦式离合器滑摩过程及温度场分析

计算机辅助工程 2010年第4期19卷 70-73页

作者：陈惠亮武秀根付昆昆莘明星同济大学航空航天与力学学院上海200092 同济大学土木工程学院上海200092 中国船舶重工集团公司第七〇四研究所上海200031

为更真实地反映摩擦式离合器滑摩过程中的温度场,提出1种利用动力学软件与有限元软件相互辅助分析的方法.在试验测得的负载扭矩的基础上,建立摩擦片和内鼓轮及气胎的模型;利用MSC Adams对摩擦式离合器进行动力学仿真,通过对摩擦片加压... 详细信息

为更真实地反映摩擦式离合器滑摩过程中的温度场,提出1种利用动力学软件与有限元软件相互辅助分析的方法.在试验测得的负载扭矩的基础上,建立摩擦片和内鼓轮及气胎的模型;利用MSC Adams对摩擦式离合器进行动力学仿真,通过对摩擦片加压计算出滑摩时间和主、从动端的相对转速;将该相对转速用于有限元热机耦合场分析,通过摩擦片和内鼓轮的相对转动形成滑摩、生成热量,得离合器各时刻的温度场.结果表明:离合器在接触后3.064 s时主、从动端接合完毕,且摩擦片瞬态最高温度只有65.83℃.该方法对摩擦式离合器滑摩过程及温度场分析具有一定的实际意义.

关键词：摩擦式离合器滑摩时间热机耦合温度场

Removal of arsenic from water by silver nanoparticles and Fe-Ce mixed oxide supported on polymeric anion exchanger

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Journal of Environmental Sciences 2025年第5期151卷 540-549页

作者： Li Li Su-juan Yu Rong-gang Zheng Qing-cun Li Rui Liu Jing-fu Liu State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Hubei Key Laboratory of Environmental and Health Effects of Persistent Toxic Substances Institute of Environment and HealthJianghan UniversityWuhan 430056China University of Chinese Academy of Sciences Beijing 100049China Department of Ecology and Resources Engineering He Tao CollegeInner Mongolia 015000China

By encapsulating nanoscale particles of goethite(α-FeO(OH)),hydrous ceric oxide(CeO_(2)·H_(2)O,HCO)and silver nanoparticles(AgNPs)in the pores of polystyrene anion exchanger D201,a novel nanocomposite FeO(OH)-HCO-Ag-D201 was prepared for the effective removal of arsenic from *** isotherm study shows that FeO(OH)-HCO-Ag-D201 has excellent adsorption performance for As(III)and As(V),with an increased adsorption capacity of As(III)to 40.12 mg/g compared to that of 22.03 mg/g by the composite adsorbent without AgNPs(FeO(OH)-HCO-D201).The adsorption kinetics data showed that the sorption rate of FeO(OH)-HCO-Ag-D201 for As(III)is less than that for As(V),and the adsorption of As(III)and As(V)were consistent with the pseudo-second-order model and the pseudofirst-order model,*** or basic conditions are favored for the adsorption of As(III/V)by FeO(OH)-*** with nitrate/chloride/bicarbonate,sulfate/silicate/phosphate showed more remarkable inhibition of arsenic removal by FeO(OH)-HCO-Ag-D201,whereas natural organic matter showed no interference to the arsenic *** As(V)adsorption involved different interactions such as electrostatic attraction and surface complexation,while the adsorption of As(III)involved the part oxidization of As(III)to As(V)and the simultaneous adsorption of As(III)and As(V).In addition to the Ce(IV)in CeO_(2)·H_(2)O acted as an oxidant,the synergistic effect ofα-FeO(OH)and AgNPs also contributed to the oxidization of As(III)to As(V).Moreover,the reusable property suggested that this FeO(OH)-HCO-Ag-D201 nanocomposite has great potential for arsenic-contaminated water purification.

关键词： FeO(OH)-HCO-Ag-D201 Arsenic removal Synergistic effect Oxidation Electrostatic attraction Surface complexation

Joint Retrieval of PM_(2.5) Concentration and Aerosol Optical Depth over China Using Multi-Task Learning on FY-4A AGRI

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Advances in Atmospheric Sciences 2025年第1期42卷 94-110页

作者： Bo LI Disong fu Ling YANG Xuehua FAN Dazhi YANG Hongrong SHI Xiang’ao XIA Electronic Engineering College Chengdu University of Information TechnologyChengdu 610225China Tianjin Meteorological Radar Research Trial Center Tianjin Meteorological BureauTianjin 300074China Key Laboratory of Middle Atmosphere and Global Environment Observation Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Research Centre on Meteorological Observation Engineering Technology China Meteorological AdministrationBeijing 100081China Key Laboratory of Atmospheric Environment and Extreme Meteorology Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China School of Electrical Engineering and Automation Harbin Institute of TechnologyHarbin 150001China University of Chinese Academy of Sciences Beijing 100049China

Aerosol optical depth(AOD)and fine particulate matter with a diameter of less than or equal to 2.5μm(PM_(2.5))play crucial roles in air quality,human health,and climate ***,the complex correlation of AOD–PM_(2.5)and the limitations of existing algorithms pose a significant challenge in realizing the accurate joint retrieval of these two parameters at the same *** this point,a multi-task learning(MTL)model,which enables the joint retrieval of PM_(2.5)concentration and AOD,is proposed and applied on the top-of-the-atmosphere reflectance data gathered by the Fengyun-4A Advanced Geosynchronous Radiation Imager(FY-4A AGRI),and compared to that of two single-task learning models—namely,Random Forest(RF)and Deep Neural Network(DNN).Specifically,MTL achieves a coefficient of determination(R^(2))of 0.88 and a root-mean-square error(RMSE)of 0.10 in AOD *** comparison to RF,the R^(2)increases by 0.04,the RMSE decreases by 0.02,and the percentage of retrieval results falling within the expected error range(Within-EE)rises by 5.55%.The R^(2)and RMSE of PM_(2.5)retrieval by MTL are 0.84 and 13.76μg m~(-3)*** with RF,the R^(2)increases by 0.06,the RMSE decreases by 4.55μg m~(-3),and the Within-EE increases by 7.28%.Additionally,compared to DNN,MTL shows an increase of 0.01 in R^(2)and a decrease of 0.02 in RMSE in AOD retrieval,with a corresponding increase of 2.89%in *** PM_(2.5)retrieval,MTL exhibits an increase of 0.05 in R^(2),a decrease of 1.76μg m~(-3)in RMSE,and an increase of 6.83%in *** evaluation suggests that MTL is able to provide simultaneously improved AOD and PM_(2.5)retrievals,demonstrating a significant advantage in efficiently capturing the spatial distribution of PM_(2.5)concentration and AOD.

关键词： AOD PM_(2.5) FY-4A multi-task learning joint retrieval

“Sergeants-and-soldiers” effect and modified Ising model in chiral polymer materials

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Science China Chemistry 2025年

作者： Liyuan Shi fu Tian Sheng Wang Jiangsu Key Laboratory of Advanced functional Polymer Design and Application College of Chemistry Chemical Engineering and Materials Science Soochow University

The “sergeants-and-soldiers” effect is a significant feature of helical copolymers, where a small fraction of chiral components can endow the copolymers with an intense optical activity close to that of chiral homopolymer. With the development of helical polymers, some abnormal examples have also been discovered, in which the twisting sense of main chain can be inversed with the increment of chiral unit content, termed as abnormal “sergeants-and-soldiers” effect. In this review, we detailedly summarize the development of “sergeants-and-soldiers” effect and its theoretical model in chiral polymer systems, including normal and abnormal “sergeants-and-soldiers” effects, modification of Ising model, dynamic transformation of the above two chiral amplification effects, as well as their applications in chiral separation, asymmetric catalysis, and circularly polarized ***, the remaining challenges are discussed to provide an outlook on the future directions.

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