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Stable Zn Metal Anodes with Limited Zn-Doping in Mgf_(2) Interphase for fast and Uniformly Ionic flux

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Nano-Micro Letters 2022年第3期14卷 169-183页

作者： Ji Young Kim Guicheng Liu Ryanda Enggar Anugrah Ardhi Jihun Park Hansung Kim Joong kee Lee Energy Storage Research Center Korea Institute of Science and TechnologyHwarang‑ro 14‑gil 5Seongbuk‑guSeoul 02792Republic of Korea Department of Chemical and Biomolecular Engineering Yonsei University50 Yonsei‑roSeodaemun‑guSeoul 03722Republic of Korea Department of Physics Dongguk UniversitySeoul 04620Republic of Korea APC Technology 10868 Gangbyeonyeok‑ro‑4‑gilGwangjin‑guSeoul 05116Republic of Korea Department of Energy and Environmental Engineering KIST SchoolKorea University of Science and TechnologyHwarang‑ro 14‑gil 5Seongbuk‑guSeoul 02792Republic of Korea

The practical applications of aqueous Zn metal batteries are currently restricted by the inherent drawbacks of Zn such as the hydrogen evolution reaction,sluggish kinetics,and dendrite *** address these problems,herein,a limitedly Zn-doped Mgf_(2)interphase comprising an upper region of pure,porous Mgf_(2)and a lower region of gradient Zn-doped Mgf_(2)is achieved via radio frequency sputtering *** porous Mgf_(2)region is a polar insulator whose high corrosion resistance facilitates the de-solvation of the solvated Zn ions and suppression of hydrogen evolution,resulting in Zn metal electrodes with a low interfacial *** Zn-doped Mgf_(2)region facilitates fast transfer kinetics and homogeneous deposition of Zn ions owing to the interfacial polarization between the Zn dopant and Mgf_(2)matrix,and the high concentration of the Zn dopant on the surface of the metal substrate as fine ***,a symmetric cell incorporating the proposed Zn metal exhibits low overpotentials of~27.2 and~99.7 mv without Zn dendrites over 250 to 8000 cycles at current densities of 1.0 and 10.0 mA cm−2,*** developed Zn/MnO2 full cell exhibits superior capacity retentions of 97.5%and 84.0%with average Coulombic efficiencies of 99.96%after 1000 and 3000 cycles,respectively.

关键词： Zinc metal battery Mgf_(2)layer Limited zinc doping Ion-transfer kinetic Deposition guidance

Reversible Zn/polymer heterogeneous anode

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Carbon Energy 2023年第6期5卷 82-91页

作者： Lingyun Xiong Hao fu Kai Yang Ji Young Kim Ren Ren Joong kee Lee Woochul Yang Guicheng Liu Department of Physics Dongguk UniversitySeoulRepublic of Korea School of Energy Power and Mechanical Engineering North China Electric Power UniversityBeijingChina Energy Storage Research Center Clean Energy InstituteKorea Institute of Science and Technology(KIST)Seongbuk‐guSeoulRepublic of Korea Department of Materials Science and Engineering City University of Hong KongKowloonHong KongChina

Commercialization of Zn-metal anodes with low cost and high theoretical capacity is hindered by the poor reversibility caused by dendrites growth,side reactions,and the slow Zn^(2+)-transport and reaction ***,a reversible heterogeneous electrode of Zn-nanocrystallites/polyvinylphosphonic acrylamide(Zn/PPAm)with fast electrochemical kinetics is designed for the first time:phosphonic acid groups with strong polarity and chelation effect ensure structural reversibility and stability of the threedimensional Zn-storage-host PPAm network and the Zn/PPAm hybrid;hydrophobic carbon chains suppress side reactions such as hydrogen evolution and corrosion;weak electron-donating amide groups constitute Zn^(2+)-transport channels and promote“desolvation”and“solvation”effects of Zn^(2+)by dragging the PPAm network on the Zn-metal surface to compress/stretch during Zn plating/stripping,respectively;and the heterostructure and Zn nanocrystallites suppress dendrite growth and enhance electrochemical reactivity,***,the Zn/PPAm electrode shows cycle reversibility of over 6000 h with a hysteresis voltage as low as 31 mv in symmetrical cells and excellent durability and flexibility in fiber-shaped batteries.

关键词： dendrite-free electrode process kinetics fiber-shaped battery reversible metal/polymer heterostructure Zn-metal anode

Performance and calibration of quark/gluon-jet taggers using 140 fb^(-1) of pp collisions at √s=13 Tev with the ATLAS detector

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Chinese Physics C 2024年第2期48卷 1-25页

作者： G. Aad B. Abbott K. Abeling N.J. Abicht S.H. Abidi A. Aboulhorma H. Abramowicz H. Abreu Y. Abulaiti B.S. Acharya C. Adam Bourdarios L. Adamczyk S.v. Addepalli M.J. Addison J. Adelman A. Adiguzel T. Adye A.A. Affolder Y. Afik M.N. Agaras J. Agarwala A. Aggarwal C. Agheorghiesei A. Ahmad f. Ahmadov W.S. Ahmed S. Ahuja X. Ai G. Aielli A. Aikot M. Ait Tamlihat B. Aitbenchikh I. Aizenberg M. Akbiyik T.P.A. Åkesson A.v. Akimov D. Akiyama N.N. Akolkar K. Al Khoury G.L. Alberghi J. Albert P. Albicocco G.L. Albouy S. Alderweireldt M. Aleksa I.N. Aleksandrov C. Alexa T. Alexopoulos f. Alfonsi M. Algren M. Alhroob B. Ali H.M.J. Ali S. Ali S.W. Alibocus M. Aliev G. Alimonti W. Alkakhi C. Allaire B.M.M. Allbrooke J.f. Allen C.A. Allendes flores P.P. Allport A. Aloisio f. Alonso C. Alpigiani M. Alvarez Estevez A. Alvarez fernandez M. Alves Cardoso M.G. Alviggi M. Aly Y. Amaral Coutinho A. Ambler C. Amelung M. Amerl C.G. Ames D. Amidei S.P. Amor Dos Santos K.R. Amos v. Ananiev C. Anastopoulos T. Andeen J.K. Anders S.Y. Andrean A. Andreazza S. Angelidakis A. Angerami A.v. Anisenkov A. Annovi C. Antel M.T. Anthony E. Antipov M. Antonelli f. Anulli M. Aoki T. Aoki J.A. Aparisi Pozo M.A. Aparo L. Aperio Bella C. Appelt A. Apyan N. Aranzabal S.J. Arbiol val C. Arcangeletti A.T.H. Arce E. Arena J-f. Arguin S. Argyropoulos J.-H. Arling O. Arnaez H. Arnold G. Artoni H. Asada K. Asai S. Asai N.A. Asbah J. Assahsah K. Assamagan R. Astalos S. Atashi R.J. Atkin M. Atkinson H. Atmani P.A. Atmasiddha K. Augsten S. Auricchio A.D. Auriol v.A. Austrup G. Avolio K. Axiotis G. Azuelos D. Babal H. Bachacou K. Bachas A. Bachiu f. Backman A. Badea P. Bagnaia M. Bahmani A.J. Bailey v.R. Bailey J.T. Baines L. Baines O.K. Baker E. Bakos D. Bakshi Gupta v. Balakrishnan R. Balasubramanian E.M. Baldin P. Balek E. Ballabene f. Balli L.M. Baltes W.K. Balunas J. Balz E. Banas M. Bandieramonte A. Bandyopadhyay S. Bansal L. Barak M. Barakat E.L. Barberio D. Barberis M. Barbero M.Z. Barel K.N. Barends T. Barillari M-S. Barisits T. Barklow P. Baron D.A. Baron Mo The ATLAS Collaboration

The identification of jets originating from quarks and gluons,often referred to as quark/gluon tagging,plays an important role in various analyses performed at the Large Hadron Collider,as Standard Model measurements and searches for new particles decaying to quarks often rely on suppressing a large gluon-induced *** paper describes the measurement of the efficiencies of quark/gluon taggers developed within the ATLAS Collaboration,using √s=13 Tev proton–proton collision data with an integrated luminosity of 140 fb^(-1) collected by the ATLAS *** taggers with high performances in rejecting jets from gluon over jets from quarks are studied:one tagger is based on requirements on the number of inner-detector tracks associated with the jet,and the other combines several jet substructure observables using a boosted decision tree.A method is established to determine the quark/gluon fraction in data,by using quark/gluon-enriched subsamples defined by the jet *** in tagging efficiency between data and simulation are provided for jets with transverse momentum between 500 Gev and 2 Tev and for multiple tagger working points.

关键词： ATLAS JET QUARK GLUON TAGGING

ST2可能并非心血管事件、心力衰竭和死亡有用的预测因子

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中华高血压杂志 2014年第8期22卷 736-736页

作者：赵狄叶鹏 Hughes Mf Appelbaum S Havulinna AS Jagodzinski A Zeller T2 kee f Blankenberg S salomaa v

研究人员假设可溶性ST2（soluble ST2,sST2）水平可识别出心血管疾病（cardiovascular disease,CvD）风险较高的人群,应将其纳入风险预测计算指标。ST2是炎症性细胞因子白细胞介素33的受体。sST2水平增加与急性心肌梗死患者和一般人群... 详细信息

研究人员假设可溶性ST2（soluble ST2,sST2）水平可识别出心血管疾病（cardiovascular disease,CvD）风险较高的人群,应将其纳入风险预测计算指标。ST2是炎症性细胞因子白细胞介素33的受体。sST2水平增加与急性心肌梗死患者和一般人群的心力衰竭及死亡相关。方法：研究人员测定fINRISK97前瞻性研究人群队列中的8444名男性和女性（25-74岁）的高敏sST2水平,应用Cox比例风险模型评估在15年的随访中,sST2对致命性或非致命性心力衰竭、CvD（冠状动脉性心脏病和脑卒中）、糖尿病和死亡情况的预测能力。研究者获取10年绝对风险识别和重新分类的统计数据,

关键词：心力衰竭死亡情况 ST2 心血管事件预测因子细胞因子白细胞介素 Cox比例风险模型冠状动脉性心脏病

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氨基末端脑钠尿肽前体与脑卒中风险的关系

中华高血压杂志 2019年第5期27卷 409-409页

作者：刘莉叶鹏 Di Castelnuovo A veronesi G Costanzo S Zeller T Schnabel RB de Curtis A salomaa v Borchini R ferrario M Giampaoli S kee f S?derberg S Niiranen T Kuulasmaa K de Gaetano G Donati MB Blankenberg S Iacoviello L 不详

氨基末端脑钠尿肽前体(N-terminal pro-B-type natriuretic peptide,NT-proBNP)是心房颠动的危险因素,是用于检测心力衰竭的心脏功能标志物。鉴于心脏功能障碍与脑卒中之间的关系,NT-proBNP是脑卒中风险的候选标志物。该研究旨在评估NT-... 详细信息

氨基末端脑钠尿肽前体(N-terminal pro-B-type natriuretic peptide,NT-proBNP)是心房颠动的危险因素,是用于检测心力衰竭的心脏功能标志物。鉴于心脏功能障碍与脑卒中之间的关系,NT-proBNP是脑卒中风险的候选标志物。该研究旨在评估NT-proBNP与脑卒中的相关性。方法:基于欧洲联盟心血管病风险评估研究的生物标志物,研究人员分析了来自6个社区队列无脑卒中的58173名参与者(50%男性;平均年龄52岁)数据。NT-proBNP测量在欧洲心血管病风险评估中心生物标志物实验室中进行。主要观察结果是脑卒中和脑卒中的亚型(缺血/出血)。结果显示,在随访7.9年(中位数)期间,共观察到1550例脑卒中事件(1176例为缺血性)。NT-proBNP四分位数增加与脑卒中风险增加相关(调整风险因素和心脏病后行多因素Cox回归分析显示趋势P<0.01)。

关键词：风险评估脑卒中脑钠尿肽 NT-proBNP 前体 N-terminal 心脏功能障碍生物标志物

酒精摄入、心脏生物标志物和心房颤动风险与不良结局

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中华高血压杂志 2021年第2期29卷 103-103页

作者：陈嘉睿(译) 练桂丽((审校) Csengeri D Sprünker NA Di Castelnuovo A Niiranen T vishram-Nielsen JK Costanzo S S derberg S Jensen SM vartiainen E Donati MB Magnussen C Camen S Gianfagna f L chen ML kee f Kontto J Mathiesen EB Koenig W Stefan B de Gaetano G J rgensen T Kuulasmaa K Zeller T salomaa v Iacoviello L Schnabel RB 不详

酒精摄入和新发心房颤动相关性证据不一,尤其是在低剂量下。该研究评估欧洲队列在整个饮酒范围内酒精摄入、生物标志物和新发心房颤动的关系。方法和结果:在一个以社区为基础的汇集队列中,研究者随访107845人,以评估酒精摄入(酒精种类... 详细信息

酒精摄入和新发心房颤动相关性证据不一,尤其是在低剂量下。该研究评估欧洲队列在整个饮酒范围内酒精摄入、生物标志物和新发心房颤动的关系。方法和结果:在一个以社区为基础的汇集队列中,研究者随访107845人,以评估酒精摄入(酒精种类和饮酒方式)与新发心房颤动的关系。研究者收集经典心血管病危险因素和新发心力衰竭的信息,并检测生物标记物氨基末端脑钠肽前体和高敏肌钙蛋白I。

关键词：氨基末端脑钠肽前体酒精摄入心血管病危险因素生物标记物心房颤动饮酒方式不良结局生物标志物

双胞胎中第二个新生儿的发病率与出生时的孕龄和分娩方式相关

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世界核心医学期刊文摘（妇产科学分册） 2005年第2期1卷 11-11页

作者： Karen fung kee f. Lawrence O. 程广艳

Objective This study was undertaken to assess the risk of neonatal morbidity in the second twi *** design We carried out a cohort study of 128,219live born second twins in the United States,1995thro ugh *** study subjects were divided into 3groups:second twins delivered by cesarean section after vaginal delivery of the first twin(v -C),both twins delivered vaginally(v -v),and both twins delivered by cesarean section(C -C).Results The rates of low 5-minute Apgar score,me chanical ventila-tion,and seizure were higher in the v-C group(8.27%,13.39%,and 0.31%)than in the v -v(3.07%,7.51%,and 0.08%)and the C -C(2.66%,8.53%,and 0.06%)*** v -C associated increase in risk remained after adjustment for confo unding factors and was more evident at term than *** nclusion The risk of neonatal morbidity is increased in s econd twins who had a cesarean section after vaginal delivery of the first twin,especially at term.

关键词：生时剖宫产分娩中第患病风险阴道分娩分率活产队列研究混杂因素发病风险