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Portable fluorogenic probe for monitoring of volatile amine vapour and food spoilage

Chinese Chemical Letters 2024年第3期35卷 257-261页

作者： Jian-Hao Zhao Wen-Xing Xu Bin Li Wei Xu Wu-Kun Zhang Ming-Shuai Yuan Hui-Zi Li Qing-Guo He Xiang Ma Jian-gong cheng Yan-Yan Fu State key lab of Transducer technology Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China Center of materials Science and Optoelectronics Engineering University of the Chinese Academy of SciencesBeijing 100039China School of Physical Science and technology ShanghaiTech UniversityShanghai 201210China key laboratory for Advanced materials and Feringa Nobel Prize Scientist Joint Research Center Frontiers Science Center for Materiobiology and Dynamic Chemistry School of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China

There are urgent needs of volatile amine gas sensors with high-performance in food quality control,disease monitoring and environmental ***-film fluorescent probe is suitable for amine vapour sensing due to its high sensitivity,high selectivity,and no polluting ***,a novel fluorescent probe based on indacenodithiophene structure withπconjugated system was designed and *** experimental results show that the films prepared by this material exhibit rapid and distinct fluorescence quenching after being exposed to saturated vapours of primary amine,secondary amine and tertiary amine represented by n-propylamine,diethylamine and trimethylamine,*** quenching of fluorescence is 84%,87%and 96%,respectively,within 10 *** detection mechanism of probe for primary amine is based on specific chemical reaction,while the detection mechanism for secondary amine and tertiary amine is intramolecular charge *** experiments show that the detection limit of the fluorescent probe for trimethylamine,an important marker of food spoilage,could reach 4.610 ***-site detection based on spoilage of small yellow croaker suggests the material possesses the potential for food freshness *** simple fluorogenic probe is an original approach to simplify real-time visual monitoring of volatile amine vapour.

关键词： Fluorescent probe Volatile amine Gas sensing Trimethylamine Food spoilage

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Large low-field reversible magnetocaloric effect in K_(3)Gd(PO_(4))_(2) at sub-kelvin temperature

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Journal of Rare Earths 2024年第6期42卷 1087-1092,I0003页

作者： Haojie Wang Zhaojun Mo Jianjian gong Heng Tu Guochun Zhang Jun Shen School of Rare Earths University of Science and Technology of ChinaHefei230026China Ganjiang Innovation Academy Chinese Academy of SciencesGanzhou341119China Center for Crystal Research and Development Key Laboratory of Functional Crystals and Laser TechnologyKey Laboratory of CryogenicsTechnical Institute of Physics and ChemistryChinese Academy of SciencesBeijing100190China Department of Energy and PowerEngineering School of Mechanical EngineeringBeijing Institute of TechnologyBeijing100081China

We synthesized a potassium gadolinium phosphate K3Gd(PO_(4))_(2)with monoclinic structure(P2_(1/m))by the high-temperature solid-state reaction *** lattice constants obtained by Rietveld refinements of XRD curve are a=0.7411 nm,b=0.5624 nm,and c=0.9433 *** and magnetocaloric properties of K_(3)Gd(PO_(4))_(2)were investigated in *** magnetic phase transition temperature of K3Gd(PO_(4))2 was determined by ultra-low temperature testing to be 0.58 K.K_(3)Gd(PO_(4))2 exhibits large magnetic entropy changes(-ΔSM).The maximum-ΔSM are 20.2 and 29.4 J/(kg·K)in the magnetic field variation(ΔH)of 1 and 2 T,respectively,which are larger than that of the commercial Gd_(3)Ga_(5)O_(12)(GGG).The maximum adiabatic temperature change(ΔT_(ad))reaches 5.91 K under a magnetic field change(ΔH)of 1 T.K_(3)Gd(PO_(4))_(2)is a potential magnetic refrigeration material for obtaining sub-kelvin temperatures.

关键词： Ultra-low temperature Magnetocaloric effect Magnetic entropy change Magnetic refrigeration Rare earths

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Study of the blocking mechanism in gravel packing based on CFD-DEM

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Particuology 2024年第7期90卷 164-178页

作者： Fucheng Deng Lei Wen Gang Li Baitao Fan Ning gong Shenghong Chen Yangtze university Jingzhou434023China guangzhou institute of Energy Conversion Chinese Academy of Sciences510640China CNOOC Research institute Ltd Beijing100028China Tianjin Branch of CNOOC Ltd Tianjin300459China CNOOC Ener Tech-Drilling&Production Co Tianjin300457China

Gravel packing sand control(GPSC),as the optimization of mechanical sand control technology,is widely used in the deep water completion and sand control of loose sandstone heavy oil reservoirs and highly *** explore the blocking mechanism of GPSC,the influence of its structural parameters on the blocking of GPSC is *** paper establishes a particle element model based on computational fluid dynamics-discrete element method coupling using the discrete element method and establishes a fluid flow model combined with computational fluid dynamics to realize their full coupling *** sand control experiments were carried out using a micro visual sand control simulation device to verify the blocking *** blocking mechanism is analyzed from the microscopic point of view,and then,the influence of sand control structure parameters on the blocking in GPSC design is *** results show the following:(1)the blocking process of GPSC can be divided into three stages:an initial stage,sand accumulation stage,and equilibrium stage.(2)There are two main types of gravel packing *** first type of blocking is blocking on the surface of the gravel *** particles on the surface of gravel layer mainly exist in the form of large particle size blocking gravel pores and sand particles bridging each *** second type of blockage is the blockage inside the gravel *** particles mainly exist in the form of internal mud cakes and adsorption on gravels inside the gravel layer.(3)To ensure the sand control performance of the gravel layer,the gravel layer thickness is designed between 23 and 28 *** displacement or pressure of the on-site packing pump should be increased to ensure that the gravel layer packing solidity ranges between 59%and 62%.In the design of GPSC,it should be ensured that the median particle size of gravel is 5–6 times the median particle size of *** study provides an effective technical reference for the

关键词： CFD-DEM Blocking the process Blocking mechanism Structural parameter

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Dynamical Dark Energy in Light of Cosmic Distance Measurements.Ⅰ.A Demonstration Using Simulated Datasets

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Research in Astronomy and Astrophysics 2024年第6期24卷 7-14页

作者： Gan Gu Xiaoma Wang Xiaoyong Mu Shuo Yuan gong-Bo Zhao National Astronomical Observatories Chinese Academy of SciencesBeijing 100101China university of Chinese Academy of Sciences Beijing 100049China institute for Frontiers in Astronomy and Astrophysics Beijing Normal UniversityBeijing 102206China

We develop methods to extract key dark energy information from cosmic distance measurements including the BAO scales and supernova(SN) luminosity *** using simulated data sets of the complete DESI,LSST and Roman surveys designed for BAO and SN distance measurements,we show that using our method,the dynamical behavior of the energy,pressure,equation of state(with its time derivative) of dark energy and the cosmic deceleration function can all be accurately recovered from high-quality data,which allows for robust diagnostic tests for dark energy models.

关键词： (cosmology:)dark energy (cosmology:)large scale structure of universe (cosmology:)cosmic background radiation (cosmology:)cosmological parameters

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Novel Vesicular Aqueous Two-Phase Systems

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Chinese Chemical Letters 1998年第11期9卷 0-0,0-0页

作者： Guo Xi ZHAO Wang Lin YU Yu Jun gong Bu Yao ZHU (institute of Physical Chemistry, Peking university, beijing 100871) institute of Physical Chemistry Peking University Beijing 100871 China

The interesting phenopmena of two aqueous phases coexisting in dilute aqueous solutions of sodium undecenoate-dodecyltrimethylammo brodride ndxture and sodium laurate-dodecyltrimethylammonium brondde mixture were investigated. Vesicles existing in both phases were shown by TEM images. The vesicles are dispersed in lower phase and flocculated in upper phase. Multilamellar structure of vesicles was found in the upper phase of sodium laurate-dodecyltrimethylammonium bromide system.

关键词： Vesicular aqueous two phase catanionic surfactants sodium carboxylates alkyltrimethylarnmonium bromide

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Crystal structure of human eIF2B alpha subunit

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生物物理学报 2009年第S1期25卷 327-328页

作者： cheng Zhang1,2, Zhiyi Wei1,2, Hang Xu1, Weimin gong1,2 1 institute of Biophysics, CAS, 15 Datun-Road, Chaoyang District, beijing, 100101 2 School of Life Sciences, university of Science and technology of china, Hefei, Anhui, 230026

In translation initiation, eIF2 is responsible for delivering initiator tRNA to ribosome, and such delivery only occurs when GTP is bound to eIF2. eIF2B, a guanine nucleotide

关键词： eIF2Bα crystal structure Rossmann fold

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Regulating Oxygen Vacancy Defects in Heterogeneous NiO-CeO_(2)−δ Hollow Multi-shelled structure for Boosting Oxygen Evolution Reaction

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Chemical Research in Chinese Universities 2024年第3期40卷 475-483页

作者： WANG Huan gong Guannan SUN Guohua QI Jian YU Ranbo WANG Dan Hebei key laboratory of Flexible Functionals materials School of Materials Science and EngineeringHebei University of Science and TechnologyShijiazhuang 050000P.R.China Department of Physical Chemistry School of Metallurgical and Ecological EngineeringUniversity of Science&Technology BejingBeijing 100083P.R.China State key laboratory of Biochemical Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190P.R.China

CeO_(2) with excellent oxygen storage-exchange capacity and NiO with excellent surface activity were used to construct a heterogeneous NiO-CeO_(2)−δhollow multi-shelled structure(HoMS)by spray *** turned out that as the proportion of CeO_(2) increases,the overpotential and Tafel slope of NiO-CeO_(2)−δHoMSs first decreased and then *** is mainly because the construction of the NiO-CeO_(2)−δHoMSs not only increases the specific surface area,but also introduces oxygen vacancy defects,thus improving the interface charge transfer capability of the materials and further improving the oxygen evolution reaction(OER)***,the increase of the calcination temperature will induce the decay of the OER performance of NiO-CeO_(2)−δHoMSs,which is mainly due to the decrease of the specific surface area,the reduction of oxygen vacancy defects,and the weakening of interface charge transfer ***,a series of heterogeneous composite HoMSs,such as Ni/Co,Mo/Ni,Al/Ni and Fe/Ni oxides was successfully constructed by spray drying,which enriched the diversity of HoMSs.

关键词： Heterogeneous composite structure Hollow multishelled structure Oxygen vacancy defect Oxygen evolution reaction

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High-efficiency crystalline carbon nitride photocatalysts:Status and perspectives

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Nano Research 2024年第9期17卷 7840-7863页

作者： Wenji Pu Yunqiao Zhou Lingfeng Yang Haifeng gong Yuhan Li Qingyu Yang Dieqing Zhang Engineering Research Center for Waste Oil Recovery technology and Equipment Ministry of EducationChongqing Key Laboratory of Catalysis and New Environmental MaterialsChongqing Technology and Business UniversityChongqing 400067China The Education Ministry key lab of Resource Chemistry Joint International Research Laboratory of Resource Chemistry of Ministry of EducationShanghai Key Laboratory of Rare Earth Functional Materialsand Shanghai Frontiers Science Center of Biomimetic CatalysisShanghai Normal UniversityShanghai 200234China State key laboratory of Tibetan Plateau Earth System Resources and EnvironmentInstitute of Tibetan Plateau ResearchChinese Academy of SciencesBeijing 100101China

Crystallinity and crystal structure greatly influence the photocatalytic behavior of *** g-C3N4 produced by traditional thermal-induced polycondensation reaction bears low crystallinity and thus poor photoactivity,which originates from the incomplete polymerization of the precursor containing amine groups,abundant hydrogen bonds,and unreacted amino,as well as cyanide functional groups in the *** photocatalytic process,these residual functional groups often work as electron trap sites,which may hinder the transfer of electrons on the plane,resulting in low ***,crystalline carbon nitride(CCN)was reported as a promising photocatalyst because its increased crystallinity not only reduces the number of carriers recombination centers,but also increases charge conductivity and improves light utilization due to extendedπ-conjugated systems and delocalizedπ-*** such,we summarize the recent studies on CCN-based photocatalysts for the photoactivity ***,the unique structure and properties of CCN materials are ***,the preparation methods and modification strategies are well *** also sum up the applications of CCN-based materials in the environmental purification and energy ***,this review concerning CNN materials ends with prospects and challenges in the obtainment of high crystallinity by effective techniques,and the deep understanding of photocatalytic mechanism.

关键词： crystalline carbon nitride preparation method modification strategy photocatalytic application

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A Shift-Share Analysis on the Regional Industry Growth in the Northeast Area of china

A Shift-Share Analysis on the Regional Industry Growth in th...

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2012 IEEE International Conference on Engineering technology and Economic Management（ICETEM2012）

作者： She Yanshuang china Center for Industrial Security Research beijing Jiaotong university beijing P.R.china Sha Jinghua School of humanities and Economic Management china university of Geosciences (beijing) beijing P.R.china Lv Xiaolan china Center for Industrial Security Research beijing Jiaotong university beijing P.R.china

this paper analyzed the growth of industry in the northeast area of china by the method of Shift-Share Analytical *** national growth component,the industrial structure effect and the regional competition effect were used to explain the growth of regional industry in shiftshare analysis *** results showed that the industrial structure effect and regional competition of Liaoning and Jilin province are more positive than the average level of the *** province’s industrial composition and industrial structure is negative which compared with the country’s *** author believe it is necessary that make more plans to accelerate industrialization in this ***,the local economy’s competitive industries in different provinces were identified in this *** of those industries should be target as leading industries in different provinces,and should be paid more attention in the formulation of regional economic policy is in future.

关键词： the northeast area of china Shift-share analysis industrial structure regional competition

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Development of Diapirs and Accumulation of Natural Gases in Yinggehai Basin

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Journal of china university of Geosciences 2001年第2期12卷 127-131页

作者： gong Zaisheng china National Offshore Oil Corporation, beijing 100029 Yang Jiaming institute of Petroleum Exploration and Development, china National Offshore Oil Corporation, Gaobeidian 074010 Hu Jianwu Hao Fang Faculty of Earth Resources, china National Offshore Oil Corporation institute of Petroleum Exploration and Development China National Offshore Oil Corporation Faculty of Earth Resources China University of Geosciences

Overpressure developed throughout most of the Yinggehai basin. The burial depth to top overpressure varied from about 1 600 m to 4 500 m, with the shallowest top overpressure occurring in the depocenter. The main cause of the overpressure was disequilibrium compaction resulting from rapid sedimentation of fine grained sediments. The overpressure was strengthened by the retention of fluids including gases due to lack of faults before diapir development. The diapirism in the Yinggehai basin was a combined result of the strong overpressure and the tensile stress field caused by the right lateral slip of the boundary fault. The diapirism, a product of the movement of overpressured fluids and plastic shales, shaped the vertical conduits from source to traps that would be absent without overpressured fluid release. Natural gas accumulation in traps in the diapir structure zones was also intermittent, which can be inferred from the inter reservoir compositional heterogeneity, transient thermal effect of fluid flow and migration fractionation.

关键词： Yinggehai basin overpressure diapirism episodic natural gas accumulation.

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