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Assessing the range of blasting-induced cracks in the surrounding rock of deeply buried tunnels based on the unified strength theory

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Journal of Central South University 2024年第7期31卷 2341-2364页

作者： LI Liang CHEN Jia-jun zhao Lian-heng HE ke-pei HU Shi-hong LI Hua-long School of Civil Engineering Central South UniversityChangsha 410075China key Laboratory of Heavy-haul Railway Engineering Structure Ministry of EducationCentral South UniversityChangsha 410075China Hunan Provincial key Laboratory for Disaster Prevention and Mitigation of Rail Transit Engineering Structure Central South UniversityChangsha 410075China

Blasting-induced cracks in the rock surrounding deeply buried tunnels can result in water gushing and rock mass collapse,posing significant safety ***,previous theoretical studies on the range of blasting-induced cracks often ignore the impact of the in-situ stress,especially that of the intermediate principal *** particle displacement−crack radius relationship was established in this paper by utilizing the blasthole cavity expansion equation,and theoretical analytical formulas of the stress−displacement relationship and the crack radius were derived with unified strength theory to accurately assess the range of cracks in deep surrounding rock under a blasting *** analysis showed that the crushing zone size was positively correlated with in-situ stress,intermediate principal stress,and detonation pressure,whereas negatively correlated with Poisson ratio and decoupling *** dilatancy angle-crushing zone size relationship exhibited nonmonotonic *** relationships in the crushing zone and the fracture zone exhibited opposite trends under the influence of only in-situ stress or intermediate principal *** the in-situ stress increased from 0 to 70 MPa,the rate of change in the crack range and the attenuation rate of the peak vibration velocity gradually slowed.

关键词： deep drilling and blasting cracks in surrounding rock unified strength theory intermediate principle stress in-situ stress cavity expansion dilatancy characteristics

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SnO_(2)/metal organic complex composite derived from low-temperature activated metal organic complex for advanced lithium storage

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Rare Metals 2024年第7期43卷 3032-3043页

作者： Gui-Long Liu Zi-Han zhao Jin-ke Shen Zi-Bo zhao Nai-Teng Wu Dong-Lei Guo Wei-Wei Yuan Yong Liu Ye-Hua Su Xian-Ming Liu Luoyang key Laboratory of Green Energy Materials College of Chemistry and Chemical EngineeringLuoyang Normal UniversityLuoyang 471934China School of Materials Science and Engineering Henan University of Science and TechnologyLuoyang 471023China Inner Mongolia Shijie Chemical Co. Ltd.Alxa League 737300

Sn-based metal organic complexes with coordination bonds,multi-active sites,and high theoretical capacity have attracted much attention as promising anodes for lithium ion ***,the low electrical conductivity and huge volume changes restricted their electrochemical stability and practical ***,Snbased anode with superior electrochemical performance,including a high reversible capacity of 1050.1 mAh·g^(-1)at 2 A·g^(-1)and a stable capacity of 1105.5 mAh·g^(-1)after 500 cycles at 1 A·g^(-1),was fabricated via a low-temperature calcination strategy from Sn metal organic *** low-temperature calcination process regulates Sn-O bond and prevents the agglomeration of SnO_(2),generating highly dispersed SnO_(2) decorated metal organic complexes and providing sufficient active sites for ion *** situ characterizations expound that the undecomposed Sn-based metal organic complexes could be transformed into SnO_(2) during lithiation and delithiation,which enhances the electrical conductivity and induces a strong pseudo-capacitive behavior,accelerating the electrochemical kinetics;the multiple solid electrolyte interface with inflexible LiF and flexible ROCO_(2)Li buffers the volume variation of the electrode,resulting in its high electrochemical *** work provides a simple strategy for preparing excellent Sn-based anodes from metal organic complexes and reveals the lithium storage mechanism of the prepared Snbased anode.

关键词： Metal organic complex Lithium ion battery Electrochemical activation Low-temperature activation Partial decomposition

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Beyond microbial carbon use efficiency

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National Science Review 2024年第04期11卷 33-35页

作者： ke-Qing Xiao Chao Liang Zimeng Wang Jingjing Peng Yao zhao Ming Zhang Mingyu zhao Shuiqing Chen Yong-Guan Zhu Caroline L.Peacock State key Lab of Urban and Regional Ecology Research Center for Eco-Environmental SciencesChinese Academy of Sciences University of Chinese Academy of Sciences Institute of Applied Ecology Chinese Academy of Sciences Department of Environmental Science and Engineering Fudan University College of Resources and Environmental Sciences China Agricultural University State key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental Sciences State key Laboratory of Agricultural Microbiology College of Resources and Environment Huazhong Agricultural University key Laboratory of Cenozoic Geology and Environment Institute of Geology and Geophysics Chinese Academy of Sciences School of Earth and Environment University of Leeds

Microbial carbon use efficiency (CUE)is defined as the proportion of microbial biomass growth C versus substrate C uptake, and thus provides a useful measure of microbially driven accumulation and loss of soil organic carbon (SOC)[1]. In a recent study published in Nature [2],the authors used a data-driven machinelearning approach to conclude that CUE promotes global SOC storage based on a positive correlation between CUE and SOC content and that, based on sensitivity analysis, CUE is at least four times as important as six other evaluated factors,namely plant C inputs, C input allocation, non-microbial C transfer, substrate decomposability, environmental modifications and vertical transport.

关键词： SOIL-CARBON ORGANIC-MATTER

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Enhancing the deep-red/near-infrared fluorescence of higher rylene diimides via the chalcogen-annulation strategy

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Science China Chemistry 2024年第4期67卷 1324-1333页

作者： Kai Chen Xiao Chen ke Hu Yilun zhao Yujian Liu Guogang Liu Jinquan Chen Wei Jiang Zhigang Shuai Da-Hui Qu zhaohui Wang key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering Feringa Nobel Prize Scientist Joint Research CenterFrontiers Science Center for Materiobiology and Dynamic ChemistryInstitute of Fine ChemicalsSchool of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China key Laboratory of Organic Optoelectronics and Molecular Engineering Department of ChemistryTsinghua UniversityBeijing 100084China State key Laboratory of Precision Spectroscopy East China Normal University500 Dongchuan RoadShanghai 200241China

Deep-red/near-infrared fluorescence is highly suitable for bioimaging owing to its ability to deeply penetrate tissues,organs,and live ***,developing organic fluorophores with high deep-red/near-infrared fluorescence quantum yield(Φ_(FL))and fluorescent brightness remain a significant challenge owing to the energy gap ***,we developed a straightforward and effective chalcogen-annulation strategy by introducing O,S and Se into the bay region of TDI and QDI fluorophores,realizing the increase ofΦFLand fluorescent brightness up to 10 *** our best knowledge,this study potentially stands as the pioneering instance showcasing the anti-heavy-atom effect of chalcogens,and the absoluteΦFL(93%)and fluorescent brightness(128,200 cm^(-1)mol^(-1)L)of Se-TDI is among top deep-red/near-infrared organic fluorophores currently *** femtosecond transient absorption(fs-TA)measurements show the absence of obvious changes of the excited state lifetime after the introduction of chalcogens in TDI and QDI fluorophores,indicating that intersystem crossing(ISC)can be neglected in TDI and QDI *** calculations further reveal the chalcogen-annulation strategy increase the radiative rates and reduce the reorganization energy of several accepting modes at the ground state in TDI fluorophores,leading to the suppression of internal conversion(IC)*** chalcogen-annulation strategy,which effectively increases the Φ_(FL)and restricts the IC processes,while remaining unaffected by the heavy-atom effect,offers novel insights and theoretical support for the design and synthesis of deep-red/near-infrared organic fluorophores with high Φ_(FL)and fluorescent brightness.

关键词： π-extended rylene diimides chalcogen-annulation strategy deep-red/near-infrared fluorescence

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Genomic analysis provides insights into the westward expansion of domesticated peaches in China

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Horticultural Plant Journal 2024年第2期10卷 367-375页

作者： Wenqing Li Yong Li Xinwei Wang Guoqing zhao Gengrui Zhu ke Cao Weichao Fang Jinlong Wu Kai Ma Changwen Chen Lirong Wang Zhengzhou Fruit Research Institute CAASZhengzhouHennan 450009China Xinjiang Academy of Agricultural Sciences UrumqiXinjiang 830091China Western Research Institute CAASChangjiXinjiang 831100China

Peach, an economically important model plant of the Rosaceae family, has been domesticated and cultivated in China for approximately5 000 years. The Hexi Corridor, an important corridor connecting east-central China and the Tarim Basin, is the starting point of the Silk Road that links China and the Eurasian region. As a globally distributed fruit tree, the spread of peach was accomplished through historical trade routes in the Hexi Corridor and the Tarim Basin. However, knowledge of peach genetic diversity in these regions remains limited. In this study,we examined the relationships and the spread history of domesticated peaches through sequencing and genomic analysis of 161 peach accessions collected from Northwest China, including 43 from the Hexi Corridor and 104 from the Tarim Basin. The results indicate that peach landraces in the Hexi Corridor and the Tarim Basin are derivatives of peaches from the east and south of China (ESC). Notably, the genetic diversity of accessions from both the Hexi Corridor and the Tarim Basin was lower than that of ESC accessions. Reduction of diversity (ROD) and linkage disequilibrium (LD) analyses detected a genetic bottleneck in peaches from these regions. Additionally, these peaches have undergone varying degrees of selection from natural environment. Moreover, genes responsive to biotic and abiotic stresses were under selection, which could be the result of the climate change of Northwest China after the Last Glacial Maximum (LGM). Our findings provide a better understanding of the genetic basis of peach migration in Northwest China. Furthermore, this study expands the available genomic data for peaches and provides critical information for future peach breeding programs.

关键词： Peach Hexi corridor Tarim Basin Genetic diversity Gene flow

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Recent advances in core-shell organic framework-based photocatalysts for energy conversion and environmental remediation

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Journal of Energy Chemistry 2024年第8期95卷 168-199,I0004页

作者： Qibing Dong Ximing Li Yanyan Duan Qingyun Tian Xinxin Liang Yiyin Zhu Lin Tian Junjun Wang Atif Sial Yongqian Cui ke zhao Chuanyi Wang School of Environmental Science and Engineering Shaanxi University of Science and TechnologyXi’an 710021ShaanxiChina Guangdong Engineering Technology Research Center for Environmental Purification and Functional Materials Guangzhou Institute of Industrial IntelligenceGuangzhou 511400GuangdongChina Jiangxi key Lab of Flexible Electronics Flexible Electronics Innovation InstituteJiangxi Science and Technology Normal UniversityNanchang 330013JiangxiChina Helmholtz-Zentrum Berlin für Materialien und Energie Kekuléstraße 512489 BerlinGermany

Direct conversion of solar energy into chemical energy in an environmentally friendly manner is one of the most promising strategies to deal with the environmental pollution and energy *** a variety of materials developed as photocatalysts,the core-shell metal/covalent-organic framework(MOF or COF)photocatalysts have garnered significant attention due to their highly porous structure and the adjustability in both structure and *** existing reviews on core-shell organic framework photocatalytic materials have mainly focused on core-shell MOF ***,there is still a lack of indepth reviews specifically addressing the photocatalytic performance of core-shell COFs and MOFs@***,there is an urgent need for a comprehensive review encompassing these three types of core-shell *** on this,this review aims to provide a comprehensive understanding and useful guidelines for the exploration of suitable core-shell organic framework photocatalysts towards appropriate photocatalytic energy conversion and environmental ***,the classification,synthesis,formation mechanisms,and reasonable regulation of core-shell organic framework were ***,the photocatalytic applications of these three kinds of core-shell structures in different areas,such as H_(2)evolution,CO_(2)reduction,and pollutants degradation are ***,the main challenges and development prospects of core-shell organic framework photocatalysts were *** review aims to provide insights into the development of a novel generation of efficient and stable core-shell organic framework materials for energy conversion and environmental remediation.

关键词： Organic framework Core-shell structure Photocatalysis Energy conversion Environmental remediation

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Support design method for deep soft-rock tunnels in non-hydrostatic high in-situ stress field

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Journal of Central South University 2024年第7期31卷 2431-2445页

作者： ZHENG ke-yue SHI Cheng-hua zhao Qian-jin LEI Ming-feng JIA Chao-jun PENG Zhu National Engineering Research Center of High-speed Railway Construction Technology Changsha 410075China School of Civil Engineering Central South UniversityChangsha 410075China China Railway Group Co. Ltd.Beijing 100039China

Due to the long-term plate tectonic movements in southwestern China,the in-situ stress field in deep formations is *** passing through deep soft-rock mass under non-hydrostatic high in-situ stress field,tunnels will suffer serious asymmetric *** is no available support design method for tunnels under such a situation in existing studies to clarify the support time and support *** study first analyzed the mechanical behavior of tunnels in non-hydrostatic in-situ stress field and derived the theoretical equations of the ground squeezing curve(GSC)and ground loosening curve(GLC).Then,based on the convergence confinement theory,the support design method of deep soft-rock tunnels under non-hydrostatic high in-situ stress field was established considering both squeezing and loosening *** addition,this method can provide the clear support time and support stiffness of the second layer of initial *** proposed design method was applied to the Wanhe tunnel of the China-Laos railway in *** data indicated that the optimal support scheme had a good effect on controlling the tunnel deformation in non-hydrostatic high in-situ stress *** applications showed that the secondary lining could be constructed properly.

关键词： non-hydrostatic stress field high in-situ stress deep soft-rock tunnel squeezing pressure loosening pressure support design method

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Clinical observation of extraction-site incisional hernia after laparoscopic colorectal surgery

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World Journal of Gastrointestinal Surgery 2024年第3期16卷 710-716页

作者： Bao-Hang Fan ke-Li Zhong Li-Jin Zhu zhao Chen Fang Li Wen-Fei Wu Second Clinical Medical College of Jinan University Jinan UniversityShenzhen 518020Guangdong ProvinceChina Department of Gastrointestinal Surgery Shenzhen People’s Hospital(The Second Clinical Medical CollegeJinan UniversityThe First Affiliated HospitalSouthern University of Science and Technology)Shenzhen 518020Guangdong ProvinceChina Department of Radiation Oncology Shenzhen People’s Hospital(The Second Clinical Medical CollegeJinan UniversityThe First Affiliated HospitalSouthern University of Science and Technology)Shenzhen 518020Guangdong ProvinceChina

BACKGROUND Laparoscopic colorectal cancer surgery increases the risk of incisional hernia(IH)at the tumor extraction *** To investigate the incidence of IH at extraction sites following laparoscopic colo-rectal cancer surgery and identify the risk factors for IH *** This study retrospectively analyzed the data of 1614 patients who underwent la-paroscopic radical colorectal cancer surgery with tumor extraction through the abdominal wall at our center between January 2017 and December ***-rences in the incidence of postoperative IH at different extraction sites and the risk factors for IH incidence were *** Among the 1614 patients who underwent laparoscopic radical colorectal cancer surgery,303(18.8%),923(57.2%),171(10.6%),and 217(13.4%)tumors were ex-tracted through supraumbilical midline,infraumbilical midline,umbilical,and off-midline *** these,52 patients developed IH in the abdominal wall,with an incidence of 3.2%.The incidence of postoperative IH was significantly higher in the off-midline incision group(8.8%)than in the middle incision groups[the supraumbilical midline(2.6%),infraumbilical midline(2.2%),and umbilical incision(2.9%)groups](χ^(2)=24.985;P<0.05).Univariate analysis showed that IH occurrence was associated with age,obesity,sex,chronic cough,incision infection,and combined diabetes,anemia,and hypopro-teinemia(P<0.05).Similarly,multivariate analysis showed that off-midline incision,age,sex(female),obesity,incision infection,combined chronic cough,and hypoproteinemia were independent risk factors for IH at the site of laparoscopic colorectal cancer surgery(P<0.05).CONCLUSION The incidence of postoperative IH differs between extraction sites for laparoscopic colorectal cancer *** infraumbilical midline incision is associated with a lower hernia rate and is thus a suitable tumor extraction site.

关键词： Incisional hernia Laparoscopy Colorectal cancer Incision infection

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嵌入多阶泰勒微分知识的多尺度注意力循环网络深度时空序列预测方法

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电子与信息学报 2024年第6期46卷 2605-2618页

作者：孙强赵珂西安理工大学自动化与信息工程学院通信工程系西安710048

融合先验物理知识的深度时空序列预测方法通常使用偏微分方程(PDE)进行建模,这种做法通常存在两大问题:(1)偏微分方程的近似精度低;(2)无法在循环网络中有效捕捉多种空间尺度的时空特征和时空序列的边缘相关空间信息。为此,该文提出了... 详细信息

融合先验物理知识的深度时空序列预测方法通常使用偏微分方程(PDE)进行建模,这种做法通常存在两大问题:(1)偏微分方程的近似精度低;(2)无法在循环网络中有效捕捉多种空间尺度的时空特征和时空序列的边缘相关空间信息。为此,该文提出了融合泰勒微分的卷积循环神经网络(TDI-CRNN)。首先,为了提高高阶偏微分方程的近似精度并缓解偏微分方程应用的局限性,设计了一种多阶泰勒近似物理模块。该模块首先使用泰勒展开式对输入序列作微分逼近,再将不同阶数之间的微分卷积层使用微分系数耦合,最后动态调整泰勒展开结果的截断阶数与微分项数。其次,为了捕获循环网络隐藏状态的多种空间尺度特征并更好地捕捉时空序列的边缘相关空间信息,设计了一种多尺度注意力循环模块(MSARM),在该模块的多尺度卷积空间注意力UNet(即MCSA-UNet)的卷积层中使用了多尺度卷积和空间注意力机制,目的是关注时空序列的局部空间区域。在Moving MNIST,KTH以及CIKM数据集上开展了大量实验,Moving MNIST数据集的均方误差(MSE)指标下降到42.7,结构相似性指数(SSIM)提高到0.912;KTH数据集的SSIM和峰值信噪比(PSNR)分别提高到0.882和29.03;CIKM数据集上的临界成功指数(CSI)提高到0.515。最终的可视化和定量预测结果均验证了TDI-CRNN模型的合理性和有效性。

关键词：时空序列预测长短期记忆网络知识引导偏微分方程泰勒展开式

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Atomic-resolution Interfacial Microstructure and Thermo-electro-magnetic Energy Conversion Performance of Gd/Bi0.5Sb1.5Te3 Composites

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Energy & Environmental Materials 2024年第4期7卷 355-363页

作者： Chengshan Liu Wenjie Xu Ping Wei Shaoqiu ke Wenjun Cui Longzhou Li Dong Liang Xianfeng Ye Tiantian Chen Xiaolei Nie Wanting Zhu Wenyu zhao Qingjie Zhang State key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory

Thermo-electro-magnetic materials with simultaneously large magnetocaloric(MC) and thermoelectric (TE) effects are the core part for designing TE/MC all-solid-state cooling *** MC phase with TE material is an effective ***,the elemental diffusion and chemical reaction occurring at the two-phase interfaces could significantly impair the cooling performance.

关键词： interfacial reaction magnetocaloric performance thermoelectric performance thermo-electro-magnetic materials

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