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Dispersive Ability of Carboxylated Cellulose Nanofibrils for Aqueous Monolayer Montmorillonite Dispersion:Influence of Na^(+) and Ca^(2+) Concentrations

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Paper And Biomaterials 2022年第1期7卷 28-37页

作者： kaihuang chen Chuan Sun Guanhui Li Jinhao Huang Zhiqiang Fang Xueqing Qiu School of Chemistry and Chemical Engineering South China University of TechnologyGuangzhouGuangdong Province510640China State Key Laboratory of Pulp and Paper Engineering South China University of TechnologyGuangzhouGuangdong Province510640China School of Chemical Engineering and Light Industry Guangdong Provincial Key Laboratory of Plant Resources BiorefineryGuangdong University of TechnologyGuangzhouGuangdong Province510006China

Carboxylated cellulose nanofibrils(CNFs)have emerged as effective green dispersants for monolayer montmorillonite(MMT)***,their dispersion capability is sensitive to the metal ion concentration in aqueous ***,this study investigated the effects of Na^(+) and Ca^(2+) concentrations on the dispersive ability of carboxylated CNFs for monolayer MMTs in *** crystal microbalance with dissipation monitoring(QCM-D)and atomic force microscopy(AFM)were utilized to explore the interfacial interactions between the carboxylated CNFs and monolayer MMTs under different Na^(+) and Ca^(2+) *** the concentration of Na^(+) reached 0.1 mmol/L,the adhesion mass of carboxylated CNFs on MMT-coated wafer peaked at 24.47 mg/m^(2),higher than control sample(carboxylated CNF-dispersed monolayer MMT dispersion without metal ions,16.03 mg/m^(2)).Moreover,the electrostatic shielding effect promoted a better dispersion of monolayer MMTs by carboxylated CNF *** a further increase in the Na^(+) concentration,the surface charge of CNFs and MMTs would be reversed resulting from the improved electrostatic shielding effect,which weaken the dispersive ability of carboxylated *** addition of Ca^(2+) reduced the dispersive ability of carboxylated CNFs for monolayer MMTs,because Ca^(2+) required a lower concentration for the onset of charge reversal compared to Na^(+).This study provides interfacial scale insights into the influence of metal ion concentration on carboxylated CNF-dispersed monolayer MMT *** also provides a strategy to enhance the dispersive ability of carboxylated CNFs for monolayer MMTs.

关键词： monolayer montmorillonite carboxylated cellulose nanofibrils dispersion mechanism metal ion

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滇黔桂盆地碎屑物源的变化及其对古特提斯洋演化历史的启示

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山东国土资源 2021年第3期37卷 11-21页

作者：陈开煌皮桥辉桂林理工大学地球科学学院广西桂林541004

古特提斯洋的构造与演化过程一直是研究热点,很多学者在其产生、扩张、俯冲及闭合的时间上持有不同观点。本次研究中,运用LA-ICP-MS锆石U-Pb测年技术对滇黔桂盆地三叠纪罗楼组碎屑锆石、泥盆纪坡松冲组碎屑独居石进行分析测试,同时结合... 详细信息

古特提斯洋的构造与演化过程一直是研究热点,很多学者在其产生、扩张、俯冲及闭合的时间上持有不同观点。本次研究中,运用LA-ICP-MS锆石U-Pb测年技术对滇黔桂盆地三叠纪罗楼组碎屑锆石、泥盆纪坡松冲组碎屑独居石进行分析测试,同时结合古生代以来碎屑物源的演化历史,以期确定出古特提斯洋开启与闭合的时间。锆石测试结果显示:者桑地区罗楼组碎屑锆石U-Pb年龄主要集中在308-396 Ma,440-680 Ma,727-930 Ma,1004-1266 Ma,1400-1880 Ma,2360-2724 Ma;老寨湾地区坡松冲组碎屑独居石U-Pb年龄则主要集中在657-460 Ma和998-798 Ma。通过对比研究区与周围地块的年龄分布特征,联系研究区岩相古地理、古海流以及古流向等地质证据,发现滇黔桂盆地古生代时期碎屑物源在460 Ma左右发生了变化,460 Ma以前碎屑物源主要来自印度北部、喜马拉雅、拉萨、羌塘、海南岛、澳大利亚西部及江南造山带,460 Ma以后碎屑物源主要来自越北古陆、湘粤桂构造山系,云开地区也可能提供了碎屑物源。

关键词：古特提斯洋碎屑物源锆石U-Pb定年独居石U-Pb定年滇黔桂盆地

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纳米纤维素/纳米铜复合材料制备及应用研究进展

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中国造纸 2021年第10期40卷 88-99页

作者：熊梓航方志强杨东杰周杰陈开湟邱学青华南理工大学化学与化工学院广东广州510641 华南理工大学制浆造纸工程国家重点实验室广东广州510641 广东工业大学轻工化工学院广东广州510006

纳米纤维素/纳米铜复合材料兼顾了纳米纤维素的优异力学和光学性能、高比表面积、低热膨胀系数、环境友好等特性以及铜的导电、导热、抗菌等性能,近年来在锂离子电池、多相催化、抗菌领域有广泛的应用。本文首先分别介绍了纳米纤维素和... 详细信息

纳米纤维素/纳米铜复合材料兼顾了纳米纤维素的优异力学和光学性能、高比表面积、低热膨胀系数、环境友好等特性以及铜的导电、导热、抗菌等性能,近年来在锂离子电池、多相催化、抗菌领域有广泛的应用。本文首先分别介绍了纳米纤维素和纳米铜的制备方法和理化特性;重点阐述了纳米纤维素/纳米铜复合材料的制备方法(物理沉积法和化学还原法)、理化特性(导电性能、催化性能和抗菌性能)及其在电子器件、催化剂和抗菌材料的应用进展;最后总结了纳米纤维素/纳米铜复合材料存在的问题并展望了未来的发展趋势。

关键词：纳米复合材料纳米铜纳米纤维素

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Role of the Greenland Sea ice anomaly in the late-spring drought over Northwest China

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Atmospheric and Oceanic Science Letters 2025年第1期18卷 1-5页

作者： Yang Liu Huopo chen Nansen-Zhu International Research Centre Institute of Atmospheric Physics Chinese Academy of SciencesBeijingChina Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters Nanjing University for Information Science and TechnologyNanjingChina

Drought across Northwest China in late spring has exerted a vital effect on the local climate and agricultural production,and has been alleviated during the past *** study explored the influence of the preceding Arctic sea ice on the May drought in Northwest China caused by the precipitation *** analysis indicated that when the Greenland Sea ice concentration is abnormally high during February to April,the dry conditions in Northwest China tend to be *** increase of sea ice in the Greenland Sea can excite a meridional circulation,which causes sea surface temperature(SST)anomalies in the North Atlantic via the sea-air interaction,manifested as significant warm SST anomalies over the south of Greenland and the subtropical North Atlantic,but negative SST anomalies over the west of the *** abnormal SST pattern maintains to May and triggers a zonal wave train from the North Atlantic through Scandinavia and Central Asia to Northwest China,leading to abnormal cyclones in Northwest ***,Northwest China experiences a more humid climate than usual.

关键词： Arctic sea ice Greenland Sea North Atlantic SST Drought Northwest China

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Cell polarization in ischemic stroke: molecular mechanisms and advances

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Neural Regeneration Research 2025年第3期20卷 632-645页

作者： Yuanwei Li Xiaoxiao Xu Xuan Wu Jiarui Li Shiling chen Danyang chen Gaigai Li Zhouping Tang Department of Neurology Tongji HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhanHubei ProvinceChina

Ischemic stroke is a cerebrovascular disease associated with high mortality and disability rates. Since the inflammation and immune response play a central role in driving ischemic damage, it becomes essential to modulate excessive inflammatory reactions to promote cell survival and facilitate tissue repair around the injury site. Various cell types are involved in the inflammatory response, including microglia, astrocytes, and neutrophils, each exhibiting distinct phenotypic profiles upon stimulation. They display either proinflammatory or anti-inflammatory states, a phenomenon known as ‘cell polarization.’ There are two cell polarization therapy strategies. The first involves inducing cells into a neuroprotective phenotype in vitro, then reintroducing them autologously. The second approach utilizes small molecular substances to directly affect cells in vivo. In this review, we elucidate the polarization dynamics of the three reactive cell populations(microglia, astrocytes, and neutrophils) in the context of ischemic stroke, and provide a comprehensive summary of the molecular mechanisms involved in their phenotypic switching. By unraveling the complexity of cell polarization, we hope to offer insights for future research on neuroinflammation and novel therapeutic strategies for ischemic stroke.

关键词： astrocyte polarization immune regulation inflammation ischemic injury microglia polarization neutrophil polarization signaling pathways stroke

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Engineering atomic Rb-N configurations to tune radical pathways for highly selective photocatalytic H2O2 synthesis coupled with biomass valorization

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Journal of Energy Chemistry 2025年第1期100卷 215-225页

作者： Jiaye Li Shuang Pan Yihuang chen Qiong Liu College of Chemistry and Materials Engineering Wenzhou University Guangdong Provincial Key Laboratory of Chemical Measurement and Emergency Test Technology (China) Institute of Analysis Guangdong Academy of Sciences (China National Analytical CenterGuangzhou)

Photocatalytic oxygen reduction for hydrogen peroxide （H2O2） synthesis presents a green and costeffective production ***,achieving highly selective H2O2synthesis remains challenging,necessitating precise control over free radical reaction pathways and minimizing undesirable oxidative ***,we report for the visible light-driven simultaneous co-photocatalytic reduction of O2to H2O2and oxidation of biomass using the atomic rubidium-nitride modified carbon nitride（CNRb）.The optimized CNRb catalyst demonstrates a record photoreduction rate of 8.01 mM h-1for H2O2generation and photooxidation rate of 3.75 mM h-1for furfuryl alcohol to furoic acid,achieving a remarkable solar-to-chemical conversion （SCC） efficiency of up to 2.27%.Experimental characterizations and DFT calculation disclosed that the introducing atomic Rb–N configurations allows for the high-selective generation of superoxide radicals while suppressing hydroxyl free radical *** is because the Rb–N serves as the new alternative site to perceive a stronger connection position for O2adsorption and reinforce the capability to extract protons,thereby triggering a high selective redox product *** study holds great potential in precisely regulating reactive radical processes at the atomic level,thereby paving the way for efficient synthesis of H2O2coupled with biomass valorization.

关键词： Atomic economy Radical pathway regulation Rubidium atom coordination Biomass valorization

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Cyano migration-mediated radical-polar crossover cyclopropanation

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Science China Chemistry 2025年第01期 241-248页

作者： Ziqiang Wang Yasu chen Jie Li chen Zhu Key Laboratory of Organic Synthesis of Jiangsu Province College of Chemistry Chemical Engineering and Materials ScienceSoochow University Frontiers Science Center for Transformative Molecules Zhangjiang Institute for Advanced Study and Shanghai Key Laboratory for Molecular Engineering of Chiral Drugs Shanghai Jiao Tong University

We report a novel cyano migration-mediated radical-polar crossover process, whereby both the sulfonylcyanation of aliphatic alkenes and the formation of cyclopropanes are concurrently achieved. This transformation yields a diverse array of multisubstituted cyclopropanes under mild photocatalytic conditions. Mechanistic studies elucidate that the reaction proceeds via intramolecular nucleophilic substitution, leading to the formation of the cyclopropane derivatives.

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Brain region-specific roles of brain-derived neurotrophic factor in social stress-induced depressive-like behavior

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Neural Regeneration Research 2025年第1期20卷 159-173页

作者： Man Han Deyang Zeng Wei Tan Xingxing chen Shuyuan Bai Qiong Wu Yushan chen Zhen Wei Yufei Mei Yan Zeng Brain Science and Advanced Technology Institute Wuhan University of Science and TechnologyWuhanHubei ProvinceChina Geriatric Hospital Affiliated to Wuhan University of Science and Technology WuhanHubei ProvinceChina School of Public Health Wuhan University of Science and TechnologyWuhanHubei ProvinceChina

Brain-derived neurotrophic factor is a key factor in stress adaptation and avoidance of a social stress behavioral *** studies have shown that brain-derived neurotrophic factor expression in stressed mice is brain region–specific,particularly involving the corticolimbic system,including the ventral tegmental area,nucleus accumbens,prefrontal cortex,amygdala,and *** how brain-derived neurotrophic factor participates in stress processing in different brain regions will deepen our understanding of social stress *** this review,we discuss the expression and regulation of brain-derived neurotrophic factor in stress-sensitive brain regions closely related to the pathophysiology of *** focused on associated molecular pathways and neural circuits,with special attention to the brain-derived neurotrophic factor–tropomyosin receptor kinase B signaling pathway and the ventral tegmental area–nucleus accumbens dopamine *** determined that stress-induced alterations in brain-derived neurotrophic factor levels are likely related to the nature,severity,and duration of stress,especially in the above-mentioned brain regions of the corticolimbic ***,BDNF might be a biological indicator regulating stress-related processes in various brain regions.

关键词： amygdala chronic mild stress chronic social defeat stress corticolimbic system depression hippocampus medial prefrontal cortex nucleus accumbens social stress models ventral tegmental area

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A Novel Self-Supervised Learning Network for Binocular Disparity Estimation

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Computer Modeling in Engineering & Sciences 2025年第1期142卷 209-229页

作者： Jiawei Tian Yu Zhou Xiaobing chen Salman A.AlQahtani Hongrong chen Bo Yang Siyu Lu Wenfeng Zheng Department of Computer Science and Engineering Major in Bio Artificial IntelligenceHanyang UniversityAnsan-si15577Republic of Korea School of Electrical and Computer Engineering Louisiana State UniversityBaton RougeLA 70803USA Department of Computer Engineering College of Computer and Information SciencesKing Saud UniversityRiyadh11574Saudi Arabia School of Automation University of Electronic Science and Technology of ChinaChengdu610054China

Two-dimensional endoscopic images are susceptible to interferences such as specular reflections and monotonous texture illumination,hindering accurate three-dimensional lesion reconstruction by surgical *** study proposes a novel end-to-end disparity estimation model to address these *** approach combines a Pseudo-Siamese neural network architecture with pyramid dilated convolutions,integrating multi-scale image information to enhance robustness against lighting *** study introduces a Pseudo-Siamese structure-based disparity regression model that simplifies left-right image comparison,improving accuracy and *** model was evaluated using a dataset of stereo endoscopic videos captured by the Da Vinci surgical robot,comprising simulated silicone heart sequences and real heart video *** results demonstrate significant improvement in the network’s resistance to lighting interference without substantially increasing ***,the model exhibited faster convergence during training,contributing to overall performance *** study advances endoscopic image processing accuracy and has potential implications for surgical robot applications in complex environments.

关键词： Parallax estimation parallax regression model self-supervised learning Pseudo-Siamese neural network pyramid dilated convolution binocular disparity estimation

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Two paths, one goal: mechanism of calcium homeostasis to balance plant growth and immunity

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Science China Life Sciences 2025年第1期 306-308页

作者： Aziz Ul Ikram Yanping Jing Huan chen Jian chen International Genome Center Jiangsu University Joint Center for Single Cell Biology School of Agriculture and BiologyShanghai Jiao Tong University

Calcium(Ca2+) is an essential nutrient and a cellular signal in plants. The level of free Ca2+in the apoplast is ～10,000-fold higher than that in the cytoplasm at the resting state. This large Ca2+level gradient across the membrane between the interior and exterior can cause Ca2+overload and toxicity. Plants have evolved mechanisms to export Ca2+out of the cytoplasm or store it in intracellular organelles, such as endoplasmic reticulum（ER）, mitochondria, and vacuole.

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