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Cu/TiO_(2)adsorbents modified by air plasma for adsorption-oxidation of H_(2)S

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Journal of Environmental Sciences 2025年第2期148卷 476-488页

作者： Yongqi Yan Xinyu Yang Ping Ning Chi wang Xin Sun Fei wang Peng Gao kai Li Faculty of Environmental Science and Engineering Kunming University of Science and TechnologyKunming 650500China National-Regional Engineering Center for Recovery of Waste Gases from Metallurgical and Chemical Industries Kunming University of Science and TechnologyKunming 650500China Faculty of Chemical Engineering Kunming University of Science and TechnologyKunming 650500China City College Kunming University of Science and TechnologyKunming 650500China

In this study,non-thermal plasma(NTP)was employed to modify the Cu/TiO_(2)adsorbent to efficiently purify H_(2)S in low-temperature and micro-oxygen *** effects of Cu loading amounts and atmospheres of NTP treatment on the adsorption-oxidation performance of the adsorbents were *** NTP modification successfully boosted the H_(2)S removal capacity to varying degrees,and the optimized adsorbent treated by air plasma(Cu/TiO_(2)-Air)attained the best H_(2)S breakthrough capacity of 113.29 mg H_(2)S/gadsorbent,which was almost 5 times higher than that of the adsorbent without NTP *** studies demonstrated that the superior performance of Cu/TiO_(2)-Air was attributed to increased mesoporous volume,more exposure of active sites(CuO)and functional groups(amino groups and hydroxyl groups),enhanced Ti-O-Cu interaction,and the favorable ratio of active oxygen ***,the X-ray diffraction(XRD)and X-ray photoelectron spectroscopy(XPS)results indicated the main reason for the deactivationwas the consumption of the active components(CuO)and the agglomeration of reaction products(CuS and SO_(4)^(2−))occupying the active sites on the surface and the inner pores of the adsorbents.

关键词： Non-thermal plasma(NTP) Surface modification Simultaneous adsorption-oxidation Cu/TiO_(2)(TiO_(2)loaded with copper) H_(2)S

A smart finger patch with coupled magnetoelastic and resistive bending sensors

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Journal of Semiconductors 2025年第1期46卷 194-203页

作者： Ziyi Dai Mingrui wang Yu wang Zechuan Yu Yan Li Weidong Qin kai Qian School of Integrated Circuits Shandong UniversityJinan 250100China Department of Mechanical Engineering University of AucklandAuckland 1010New Zealand Department of Urology Qilu Hospital of Shandong UniversityJinan 250100China Shenzhen Research Institute of Shandong University Shenzhen 518000China Department of Critical Care Medicine Qilu hospital of Shandong universityJinan 250100China

In the era of Metaverse and virtual reality(VR)/augmented reality(AR),capturing finger motion and force interactions is crucial for immersive human-machine *** study introduces a flexible electronic skin for the index finger,addressing coupled perception of both state and process in dynamic tactile *** device integrates resistive and giant magnetoelastic sensors,enabling detection of surface pressure and finger joint *** e-skin identifies three phases of finger action:bending state,dynamic normal force and tangential force(sweeping).The system comprises resistive carbon nanotubes(CNT)/polydimethylsiloxane(PDMS)films for bending sensing and magnetoelastic sensors(NdFeB particles,EcoFlex,and flexible coils)for pressure *** inward bending resistive sensor,based on self-assembled microstructures,exhibits directional specificity with a response time under 120 ms and bending sensitivity from 0°to 120°.The magnetoelastic sensors demonstrate specific responses to frequency and deformation magnitude,as well as sensitivity to surface roughness during sliding and material *** system’s capability is demonstrated through tactile-based bread type and condition recognition,achieving 92%*** intelligent patch shows broad potential in enhancing interactions across various fields,from VR/AR interfaces and medical diagnostics to smart manufacturing and industrial automation.

关键词： human machine interface flexible sensor wearable sensor giant magnetoelastic effect inward bending sensor

Response properties of geometries of coal penetrating fracture on seepage behavior

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International Journal of Mining Science and Technology 2025年第2期35卷 191-211页

作者： Penghua Han kai wang Jiewen Pang Xiaofeng Ji Cun Zhang College of Engineering for Safety and Emergency Management Taiyuan University of Science and TechnologyTaiyuan 030024China School of Energy and Mining Engineering China University of Mining and Technology-BeijingBeijing 100083China Engineering Research Center of Green and Intelligent Mining for Thick Coal Seam Ministry of EducationChina University of Mining and Technology-BeijingBeijing 100083China

The fracture surfaces of coal-rock masses formed under mining-induced stress generally exhibit complex geometries, and the fracture geometry is one of the primary factors affecting the seepage characteristics of coal-rock penetrating fracture. This paper investigates the seepage characteristics of 5 groups of coal penetrating fracture(CPF) with different joint roughness coefficients(JRCs). Based on 3D morphology scanner tests and hydraulic coupling tests, a characterization method of effective geometric parameters in fracture surfaces under various confining pressures was improved, and a relationship between effective geometric parameters and the confining pressure is established. The results indicate that the nonlinear flow behavior in a CPF primarily includes three types: non-Newtonian fluid seepage under high confining pressure and low JRC, non-Darcy seepage under low confining pressure and high JRC, and the whole process of seepage characteristics between these two conditions. Among them, nonNewtonian fluid seepage is caused by significant fracture expansion, while non-Darcy seepage can be attributed to turbulence effects. During the seepage process, the geometric parameters with different JRC fracture samples all exhibit exponential changes with the increase of confining pressure. In addition,under high confining pressure, the effective contact ratio, effective fracture aperture, and void deviation ratio with high JRC fracture samples under high confining pressure increase by 93.5%, 67.4%, and 24.9%,respectively, compared with those of low JRC fracture samples. According to the variation of geometric parameters in a CPF with external stress, a seepage model considering geometric parameters in a CPF is proposed. By introducing the root mean square error(RMSE) and coefficient of determination(R2) to evaluate the error and goodness of fit between model curves and experimental data, it is found that the theoretical curves of model in this paper have the best matchi

关键词： Coal penetrating fracture Roughness Geometries Seepage characteristics

Secure beamforming and deployment design for rate-splitting multiple access-based UAV communications

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Science China(Information Sciences) 2025年第1期68卷 342-356页

作者： Bing wang Xiaofeng TAO Shujun HAN Huici WU kai YANG Zhu HAN National Engineering Research Center of Mobile Network Technologies Beijing University of Posts and Telecommunications Peng Cheng Laboratory Department of Electrical and Computer Engineering University of Houston

Rate-splitting multiple access(RSMA) has recently gained attention as a potential robust multiple access(MA)scheme for upcoming wireless networks. Given its ability to efficiently utilize wireless resources and design interference management strategies, it can be applied to unmanned aerial vehicle(UAV) networks to provide convenient services for large-scale access ground users. However, due to the line-of-sight(LoS) broadcast nature of UAV transmission, information is susceptible to eavesdropping in RSMA-based UAV networks. Moreover, the superposition of signals at the receiver in such networks becomes complicated. To cope with the challenge, we propose a two-user multi-input single-output(MISO) RSMA-based UAV secure transmission framework in downlink communication networks. In a passive eavesdropping scenario, our goal is to maximize the sum secrecy rate by optimizing the transmit beamforming and deployment location of the UAV-base station(UAV-BS),while considering quality-of-service(QoS) constraints, maximum transmit power, and flight space limitations. To address the non-convexity of the proposed problem, the optimization problem is first decoupled into two subproblems. Then, the successive convex approximation(SCA) method is employed to solve each subproblem using different propositions. In addition, an alternating optimization(AO)-based location RSMA(L-RSMA) beamforming algorithm is developed to implement joint optimization to obtain the suboptimal solution. Numerical results demonstrate that(1) the proposed L-RSMA scheme yields a28.97% higher sum secrecy rate than the baseline L-space division multiple access(SDMA) scheme;(2) the proposed L-RSMA scheme improves the security performance by 42.61% compared to the L-non-orthogonal multiple access(NOMA) scheme.

关键词： rate-splitting multiple access UAV communication precoding optimization deployment location physical layer security

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Dynamic intelligent prediction approach for landslide displacement based on biological growth models and CNN-LSTM

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Journal of Mountain Science 2025年第1期22卷 71-88页

作者： wang Ziqian FANG Xiangwei ZHANG Wengang wang Luqi wang kai CHEN Chao School of Civil Engineering Chongqing UniversityChongqing 400045China Nanjiang Hydro-geology and Engineering Geology Team of Chongqing Geology Mineral Bureau Chongqing 401147China China Coal Technology and Engineering Chongqing Design and Research Institute(Group)Co. Ltd.Chongqing 400016China

Influenced by complex external factors,the displacement-time curve of reservoir landslides demonstrates both short-term and long-term diversity and dynamic *** is difficult for existing methods,including Regression models and Neural network models,to perform multi-characteristic coupled displacement prediction because they fail to consider landslide creep *** paper integrates the creep characteristics of landslides with non-linear intelligent algorithms and proposes a dynamic intelligent landslide displacement prediction method based on a combination of the Biological Growth model(BG),Convolutional Neural Network(CNN),and Long ShortTerm Memory Network(LSTM).This prediction approach improves three different biological growth models,thereby effectively extracting landslide creep characteristic ***,it integrates external factors(rainfall and reservoir water level)to construct an internal and external comprehensive dataset for data augmentation,which is input into the improved CNN-LSTM ***,harnessing the robust feature extraction capabilities and spatial translation invariance of CNN,the model autonomously captures short-term local fluctuation characteristics of landslide displacement,and combines LSTM's efficient handling of long-term nonlinear temporal data to improve prediction *** evaluation of the Liangshuijing landslide in the Three Gorges Reservoir Area indicates that BG-CNN-LSTM exhibits high prediction accuracy,excellent generalization capabilities when dealing with various types of *** research provides an innovative approach to achieving the whole-process,realtime,high-precision displacement predictions for multicharacteristic coupled landslides.

关键词： Reservoir landslides Displacement prediction CNN LSTM Biological growth model

Assessing the corrosion protection property of coatings loaded with corrosion inhibitors using the real-time atmospheric corrosion monitoring technique

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 119-126页

作者： Xiaoxue wang Lulu Jin Jinke wang Rongqiao wang Xiuchun Liu kai Gao Jingli Sun Yong Yuan Lingwei Ma Hongchang Qian Dawei Zhang School of Energy and Power Engineering Beihang UniversityBeijing 100191China Beijing Institute of Space Long March Vehicle Beijing 100076China National Materials Corrosion and Protection Data Center University of Science and Technology BeijingBeijing 100083China Institute of Materials Intelligent Technology Liaoning Academy of MaterialsShenyang 110004China Shanghai Spaceflight Precision Machinery Institute Shanghai 201600China

The atmospheric corrosion monitoring(ACM)technique has been widely employed to track the real-time corrosion behavior of metal ***,limited studies have applied ACM to the corrosion protection properties of organic *** study compared a bare epoxy coating with one containing zinc phosphate corrosion inhibitors,both applied on ACM sensors,to observe their corrosion protection properties over *** with artificial damage via scratches were exposed to immersion and alternating dry and wet environments,which allowed for monitoring galvanic corrosion currents in *** the corrosion tests,the ACM currents of the zinc phosphate/epoxy coating were considerably lower than those of the blank epoxy *** trend in ACM current variations closely matched the results obtained from regular electrochemical tests and surface *** alignment highlights the potential of the ACM technique in evaluating the corrosion protection capabilities of organic *** with the blank epoxy coating,the zinc phosphate/epoxy coating showed much-decreased ACM current values that confirmed the effective inhibition of zinc phosphate against steel corrosion beneath the damaged coating.

关键词： atmospheric corrosion monitoring technology corrosion inhibitor coating carbon steel corrosion protection

Research Progress of Chinese Medicine Monomers in Treatment of Cholangiocarcinoma

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Chinese Journal of Integrative Medicine 2025年第2期31卷 170-182页

作者： wang Xiang wang Xiao-qing LUO kai BAI He QU Jia-lin ZHANG Gui-xin Department of General Surgery the Second Hospital of Dalian Medical UniversityDalianLiaoning Province(116027)China Clinical Laboratory of Integrative Medicine First Affiliated Hospital of Dalian Medical UniversityDalianLiaoning Province(116021)China Hepatobiliary Surgery Department Shandong Provincial Third HospittalShandong UniversityJinan(250031)China Institute(College)of Integrative Medicine Dalian Medical UniversityDalianLiaoning Province(116044)China

Cholangiocarcinoma(CCA)is a malignant tumor originating from ***,it remains unclear about the pathogenesis of this carcinoma,which may be related to multiple ***,CCA is mainly treated by surgery,chemotherapy,and *** them,surgery is the only potentially curative option for ***,the high malignancy and asymptomatic nature of CCA may lead to poor treatment *** has been demonstrated that Chinese medicine(CM)plays a significant role in various antitumor ***,CM exhibits fewer side effects and high ***,the in vitro application of CM monomers has been explored in many domestic and foreign *** article mainly reviews the signaling pathways and molecular mechanisms of CM monomers in the treatment of CCA in recent *** findings are expected to provide new insights into the treatment of CCA.

关键词： cholangiocarcinoma Chinese medicine monomers antitumor signaling pathways molecular mechanisms review

Lattice-mismatch-induced formation of defect-rich Pd-Cu alloy nanocages for enhanced formic acid oxidation activity

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Science China Chemistry 2025年第2期68卷 481-491页

作者： Zhaojun Liu Zhengyan wang Zhaoyu wang Hao Yuan Yuke Bai Xiaoxiao wang Zerui Mu Chunxia Wu kai Liu Zhun Hu Chuanbo Gao Sate Key Laboratory of Multiphase Flow in Power Engineering Frontier Institute of Science and TechnologyXi’an Jiaotong UniversityXi’an 710049China Institute of Industrial Catalysis School of Chemical Engineering and TechnologyXi’an Jiaotong UniversityXi’an 710049China

Crystallographic defects in noble metal nanocrystals are recognized as highly active catalytic sites,significantly enhancing activities in many important *** their importance,synthesizing noble metal nanocrystals with a high density of defects poses a considerable synthetic ***,we present a novel lattice mismatch-induced formation mechanism to create high-density defects in noble metal *** approach takes advantage of lattice mismatch to enable nonepitaxial nucleation and growth of a noble metal on a foreign metal substrate,forming abundant noble metal crystallites with random lattice orientations not dictated by the substrate *** these crystallites grow extensively,they merge,forming numerous grain boundaries and yielding defect-rich noble metal ***-rich alloy nanocrystals can also be synthesized through a subsequent vacancy-diffusion alloying *** take defective PdCu alloy nanocages as an example and demonstrate the effectiveness of crystallographic defects in enhancing catalytic performance of noble metal *** nanocages exhibit superior activity in the electrocatalytic formic acid oxidation reaction,which is 1.6 times greater than their defect-free *** strategy offers a new avenue for creating defect-rich noble metal nanocrystals as highly efficient catalysts for a wide array of catalytic applications.

关键词： noble metal nanocrystals defects non-epitaxial growth electrocatalysis formic acid oxidation reaction

Statistical Research on Megahertz-peaked Spectra Pulsars

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Research in Astronomy and Astrophysics 2025年第1期25卷 116-134页

作者： Hong-Bing Cai Li Chen Shi-Dang Li kai wang Hang Liu JSNU SPBPU Institute of Engineering & SINO RUSSIAN Institute Jiangsu Normal University School of Physics and Electronic Engineering Jiangsu Normal University

Megahertz-peaked spectra(MPS) pulsars are referred as cases whose radio spectra turn over around 100 MHz. We identified 53 MPS pulsars based on the spectral data from the literature, and statistically analyzed the spatial location distribution, the magnetic field-period distribution, peak frequencies, spectral indices, and dispersion measures of these MPS pulsars. We found that there is a strong positive correlation between the dispersion measures and the peak frequencies of MPS pulsars, and negative correlations of the dispersion measures with spectral indices and the ages are also found. Such correlations suggest that the interstellar medium is an important factor that affects observational properties of MPS pulsars.

关键词： (stars:) pulsars: general ISM: general radio continuum: general