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Natural high-porous diatomaceous-earth based self-floating aerogel for efficient solar steam power generation

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Green Energy & Environment 2024年第2期9卷 378-389页

作者： Aitang Zhang kai Wang md Julker Nine Mengyu Cao Hanwen Zong Zhiqiang Liu Hanwen Guo Jingquan Liu Dusan Losic College of Materials Science and Engineering Institute for Graphene Applied Technology InnovationCollaborative Innovation Center for Marine Biomass Fibers Materials and Textiles of Shandong ProvinceQingdao UniversityQingdao266071China The University of Adelaide School of Chemical Engineering and Advanced MaterialsARC Graphene Research HubNorth Engineering BuildingN206 AdelaideSA 5005Australia

The application of solar steam generation in seawater desalination is an effective way to solve the shortage of fresh water *** present,many kinds of photothermal conversion materials have been developed and used as evaporators in seawater ***,some evaporators need additional thermal insulation or water supply devices to achieve efficient photothermal *** addition,their complex,time consuming and no scalable preparation process,high cost of raw materials and poor salt resistance hinder the practical application of these *** to its distinctive nanoporous structure,diatomite as fossilized single-cells algae diatoms is a promising natural silica-based material for seawater *** are taken from sea and that makes true sense to use them in the ***,we report the first example of synthesis robust three-dimensional(3D)natural-diatomite composite by assembling polyaniline nanoparticles covered diatomite into the polyvinyl alcohol pre-treated melamine foam frameworks and demonstrate its application as new evaporator for seawater *** porous framework does not only improve the sunlight scattering efficiency,but also offer large network of channels for water *** inherent mechanism behind salt desalination process involves the absorption of water molecules on the surface of the internal silica micro-nano pores,and evaporation under the heat induced by the polyaniline absorbed ***,the metal ions are segregated by many available pores and channels to achieve the self-desalting *** developed evaporator possesses the superiority of multi-stage pore structure,strong hydrophilicity,low thermal conductivity,excellent light absorption,fast water transportation and salt-resistant crystallization as well as good *** evaporation rate without an additional device is found to be 1.689 kg m^(-2)h^(-1)under 1-Sun irradiation,and the energy conversion efficiency is as

关键词： Diatomite Micro/nanopores Polyaniline Three-dimensional composite Solar steam generation

An Efficient Approach to Narrow the Emission Band of Pyrene-Based Emitters

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有机化学 2024年第8期44卷 2504-2512页

作者： Xie Zhixin Li Shaoling Liu Wei Yan kai Jiang Tao Liu Yiwei Islam md.Monarul Feng Xing School of Materials and Energy Guangdong University of TechnologyGuangzhou 510006 b Analysis and Test Center Guangdong University of TechnologyGuangzhou 510006 Synthesis Laboratory Chemical Research DivisionBangladesh Council of Scientific and Industrial Research(BCSIR)DhanmondiDhaka-1205Bangladesh

The construction of high color purity and high resolution organic light-emitting diodes(OLEDs)is facilitated by the development of highly-efficient organic luminescent materials with narrow-band ***,in order to address the problem of broad emission spectra of organic luminescent materials,an effective molecular design strategy is presented to reduce the full width at half maximum(FWHM)of emission by integrating the steric hindrance effect in the pyrene *** the bulky group was introduced into the 2-position,compounds 5 not only show a relative high quantum yield(>0.31)in the solid state,but also can suppress the molecular rotation of triphenylamine(TPA)at the 3-position to narrow the FWHM in the solid state compared to that in *** 5c containing biphenyl units exhibits a maximum emission peak at 484 nm with a quantum yield of 0.38 and FWHM value of 49 nm in the solid state.

关键词： aggregation-induced emission pyrene narrow-band emission steric effect

Electrolyte Design for Low‑Temperature Li‑Metal Batteries:Challenges and Prospects

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Nano-Micro Letters 2024年第2期16卷 365-382页

作者： Siyu Sun Kehan Wang Zhanglian Hong Mingjia Zhi kai Zhang Jijian Xu Department of Chemistry City University of Hong KongHong Kong 999077People’s Republic of China State Key Laboratory of Silicon Materials School of Materials Science and EngineeringZhejiang UniversityHangzhou 310027People’s Republic of China State Key Laboratory of Advanced Chemical Power Sources Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education)Haihe Laboratory of Sustainable Chemical TransformationsCollaborative Innovation Center of Chemical Science and Engineering(Tianjin)College of ChemistryNankai UniversityTianjin 300071People’s Republic of China Department of Chemical and Biomolecular Engineering University of Maryland College ParkCollege ParkMD 20742USA

Electrolyte design holds the greatest opportunity for the development of batteries that are capable of sub-zero temperature *** get the most energy storage out of the battery at low temperatures,improvements in electrolyte chemistry need to be coupled with optimized electrode materials and tailored electrolyte/electrode ***,this review critically outlines electrolytes’limiting factors,including reduced ionic conductivity,large de-solvation energy,sluggish charge transfer,and slow Li-ion transportation across the electrolyte/electrode interphases,which affect the low-temperature performance of Li-metal *** theoretical derivations that explain the explicit influence of temperature on battery performance are presented to deepen *** improvement strategies from the aspects of electrolyte design and electrolyte/electrode interphase engineering are summarized and rigorously *** on future research are proposed to guide the ongoing exploration for better low-temperature Li-metal batteries.

关键词： Solid electrolyte interphase Li metal Low temperature Electrolyte design Batteries

Deep learning CNN-APSO-LSSVM hybrid fusion model for feature optimization and gas-bearing prediction

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Petroleum Science 2024年第4期21卷 2329-2344页

作者： Jiu-Qiang Yang Nian-Tian Lin kai Zhang Yan Cui Chao Fu Dong Zhang College of Earth Sciences and Engineering Shandong University of Science and Technology Laboratory for Marine Mineral Resources Qingdao National Laboratory for Marine Science and Technology Transportation Institute of Inner Mongolia University Key Laboratory of Gas Hydrate Qingdao Institute of Marine Geology Ministry of Natural Resources

Conventional machine learning(CML) methods have been successfully applied for gas reservoir prediction. Their prediction accuracy largely depends on the quality of the sample data; therefore, feature optimization of the input samples is particularly important. Commonly used feature optimization methods increase the interpretability of gas reservoirs; however, their steps are cumbersome, and the selected features cannot sufficiently guide CML models to mine the intrinsic features of sample data efficiently. In contrast to CML methods, deep learning(DL) methods can directly extract the important features of targets from raw data. Therefore, this study proposes a feature optimization and gas-bearing prediction method based on a hybrid fusion model that combines a convolutional neural network(CNN)and an adaptive particle swarm optimization-least squares support vector machine(APSO-LSSVM). This model adopts an end-to-end algorithm structure to directly extract features from sensitive multicomponent seismic attributes, considerably simplifying the feature optimization. A CNN was used for feature optimization to highlight sensitive gas reservoir information. APSO-LSSVM was used to fully learn the relationship between the features extracted by the CNN to obtain the prediction results. The constructed hybrid fusion model improves gas-bearing prediction accuracy through two processes of feature optimization and intelligent prediction, giving full play to the advantages of DL and CML methods. The prediction results obtained are better than those of a single CNN model or APSO-LSSVM model. In the feature optimization process of multicomponent seismic attribute data, CNN has demonstrated better gas reservoir feature extraction capabilities than commonly used attribute optimization methods. In the prediction process, the APSO-LSSVM model can learn the gas reservoir characteristics better than the LSSVM model and has a higher prediction accuracy. The constructed CNN-APSO-LSSVM mode

关键词： Multicomponent seismic data Deep learning Adaptive particle swarm optimization Convolutional neural network Least squares support vector machine Feature optimization Gas-bearing distribution prediction

Simultaneously enhancing erosion and compression resistance:designing AlCoCrFeNi high-entropy alloy strengthened Ag-based contacts

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Rare Metals 2024年第9期43卷 4476-4492页

作者： Xiao-Yang Xue Zhe Wang Hui-Ling Nie Zhao Yuan Jun Wang Chang-Hu Xu kai Wen Cong-Hao Yu School of Materials Science and Engineering Xi’an Polytechnic UniversityXi’an 710048China School of Physics Xi’an Jiaotong UniversityXi’an 710049China Key Laboratory of Pulsed Power Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China

Designing microstructures and unveiling dynamic erosion mechanisms remain important challenges for Ag-based *** simultaneously enhance erosion and compression resistance,an Al Co Cr Fe Ni high-entropy alloy(HEA)is introduced into Ag-based materials to fabricate novel Ag-HEA contacts with island-and skeletonrestricted *** arc erosion experimental results reveal that the skeleton-restricted HEA microstructure is the key factor in reducing the hill and crater morphologies of the contact surface,effectively delaying material transfer between the movable and stationary *** molten bridge evolution and compressive deformation behavior of Ag-HEA contacts with various microstructures are investigated using molecular dynamics(md)*** results indicate that the constraint of Ag atom diffusion in the molten pool and the involvement of HEA atoms in the molten bridge are the primary mechanisms for improving erosion *** skeleton-restricted HEA microstructure reduces the total energy and structural stability of the molten bridge system and promotes its fracture and ***,the synergistic effect of the twin and Lomerz–Cottrell lock structures can hinder dislocation glide,generating dispersed and small-area stacking faults in the Ag matrix and mitigating the concentration of shear ***,the skeleton-restricted HEA microstructure contributes positively to compression *** study presents a novel approach to designing Ag-based contacts.

关键词： Electrical contact materials High entropy alloys Arc erosion Molecular dynamics Microstructures

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窄化芘基发光分子半峰宽的合成策略（英文）

有机化学 2024年第8期44卷 2504-2512页

作者：谢志鑫黎少玲刘威严楷蒋涛刘一苇 md.Monarul Islam 冯星广东工业大学材料与能源学院广东工业大学分析测试中心孟加拉国科学和工业研究理事会(BCSIR)化学研究部

开发高效窄带发射的有机发光材料是实现有机发光二极管高色纯度、高分辨的关键.针对有机发光分子的发射光谱谱较宽的问题,基于芘基发光材料体系,提出了利用空间立体效应窄化发光分子的半峰宽的分子设计策略.利用空间位阻效应,通过在芘... 详细信息

开发高效窄带发射的有机发光材料是实现有机发光二极管高色纯度、高分辨的关键.针对有机发光分子的发射光谱谱较宽的问题,基于芘基发光材料体系,提出了利用空间立体效应窄化发光分子的半峰宽的分子设计策略.利用空间位阻效应,通过在芘的2-位引入大位阻的取代基团,降低了3-位取代基团三苯胺的分子转动,设计合成的芘基发光分子5具有相对高的固态量子产率(>0.31)和固态下较窄的半峰宽(相较于溶液态和没有立体效应存在下).特别的,制备的化合物5c在固态下显示出最大的发射峰位于484 nm,量子产率较高(0.38)和发射半峰宽较窄(49 nm).

关键词：聚集诱导发光芘窄带发射立体效应

Milling degree affects the fermentation properties of rice:perspectives from the composition of nutrients and gut microbiota via in vitro fermentation

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Food Science and Human Wellness 2024年第3期13卷 1578-1588页

作者： Yu Zhang Fan Li Shutong Pan Bing Bai kai Huang Sen Li Hongwei Cao Tian Xie Jian Xie Xiao Guan School of Health Science and Engineering University of Shanghai for Science and TechnologyShanghai 200093China National Grain Industry(Urban Grain and Oil Security)Technology Innovation Center Shanghai 200093China Nutrition&Health Research Institute Co.Ltd. COFCO CorporationBeijing 102209China China Grain Wuhan Scientific Research&Design Institute Co.Ltd. Wuhan 430079China

Fermentation substrates of rice with different milling degrees(mds) were prepared and fermented with human feces to compare their fermentation properties and effects on gut *** 0s,md 5s and md 60s represented brown rice,moderately-milled rice and white rice,*** in vitro fermentation,the md 5s group showed higher starch utilization,compared with the md 0s and 60s groups evaluated by Fourier transform infrared spectrometer,and confocal laser scanning *** of fermentation substrates of rice with different mds on gut microbiota were evaluated by 16S rDNA *** the sample groups reduced the pH and produced short-chain fatty acids(SCFAs) and branched-chain fatty *** md 5s group exhibited higher α-diversity than the md 0s and 60s *** of Phascolarctobacterium,Blautia and norank_f_Ruminococcaceae were higher in the md 0s and 5s groups,compared with the md 60s *** bacteria were also positively correlated with the SCFAs production via Spearman correlation *** vitro culture assay revealed that fermentation substrates of md 0s and 5s promoted the growth of two probiotics(Akkermansia muciniphila and Bifidobacterium adolescentis).Our results showed that moderate milling might be an appropriate way to produce rice products with richer nutrients and better fermentation properties.

关键词： Rice processing Milling Whole grains Gut microbiota

21世纪全球新建水库编目:丰度、热点区及总蓄水量

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Science Bulletin 2024年第14期69卷 2179-2182页

作者：范晨雨宋春桥 Jida Wang Yongwei Sheng 蔺亚玲苑春雨 md Safat Sikder Jean-Francois Crétaux 刘凯陈探曾繁轩柯灵红 Key Laboratory of Watershed Geographic Sciences Nanjing Institute of Geography and LimnologyChinese Academy of SciencesNanjing 210008China University of Chinese Academy of Sciences Beijing 100049China University of Chinese Academy of Sciences Nanjing(UCASNJ)Nanjing 211135China Department of Geography and Geographic Information Science University of Illinois Urbana-ChampaignUrbana IL 61801USA Department of Geography and Geospatial Sciences Kansas State UniversityManhattan KS 66506USA Department of Geography University of CaliforniaLos Angeles CA 90095USA Laboratoire d’Études en Géophysique et Océanographie Spatiales(LEGOS) CNES-IRD-CNRS-UT3Universitéde ToulouseToulouse 31401France College of Hydrology and Water Resources Hohai UniversityNanjing 210098China State Key Laboratory of Hydrology-Water Resources and Hydraulic Engineering Hohai UniversityNanjing 210098China

Dams and reservoirs play an essential role in regulating and managing water *** the middle of the 20th century,the growing demand for water and hydropower has led to an unprecedented boom in reservoir construction worldwide[1,2].Meanwhile,reservoir construction has also resulted in a variety of ecological and socioeconomic impacts[3–5].Reservoirs transform natural flow regimes into conditions favored by human *** associated flow regulations,especially in reservoirs constructed in recent decades(e.g.,after 2000)with greater seasonal variability[6,7],represent a strong human-induced alteration of the hydrologic *** reservoir construction continues to boom in many parts of the world,an up-to-date and openaccess inventory of reservoirs worldwide remains critically desired.

关键词： reservoir reservoirs alteration

Outcomes of liver resection in hepatitis C virus-related intrahepatic cholangiocarcinoma:A systematic review and meta-analysis

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World Journal of Virology 2024年第1期13卷 107-119页

作者： Feng Yi Cheo kai Siang Chan Vishal G Shelat Yong Loo Lin School of Medicine National University of SingaporeSingapore 117597Singapore Department of General Surgery Tan Tock Seng HospitalSingapore 308433Singapore

BACKGROUND Cholangiocarcinoma is the second most common primary liver *** incidence and mortality rates have been increasing in recent *** C virus(HCV)infection is a risk factor for development of cirrhosis and ***,surgical resection remains the only curative treatment option for *** aim to study the impact of HCV infection on outcomes of liver resection(LR)in intrahepatic cholangiocarcinoma(ICC).AIM To study the outcomes of curative resection of ICC in patients with HCV(i.e.,HCV+)compared to patients without HCV(i.e.,HCV-).METHODS We conducted a systematic review and meta-analysis of randomized controlled trials(RCTs)and observational studies to assess the outcomes of LR in ICC in HCV+patients compared to HCV-patients in tertiary care ***,EMBASE,The Cochrane Library and Scopus were systematically searched from inception till August *** studies were RCTs and non-RCTs on patients≥18 years old with a diagnosis of ICC who underwent LR,and compared outcomes between patients with HCV+vs HCV-.The primary outcomes were overall survival(OS)and recurrence-free *** outcomes include perioperative mortality,operation duration,blood loss,intrahepatic and extrahepatic *** Seven articles,published between 2004 and 2021,fulfilled the selection *** of the studies were retrospective ***,incidence of male patients,albumin,bilirubin,platelets,tumor size,incidence of multiple tumors,vascular invasion,bile duct invasion,lymph node metastases,and stage 4 disease were comparable between HCV+and *** transaminase[md 22.20,95%confidence interval(CI):13.75,30.65,Pmd 27.27,95%CI:20.20,34.34,P<0.00001)were significantly higher in HCV+group compared to *** of cirrhosis was significantly higher in HCV+group[odds ratio(OR)5.78,95%CI:1.38,24.14,P=0.02]compared to *** of poorly

关键词： Cholangiocarcinoma Bile duct cancer Hepatitis C Surgical resection Hepatectomy