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Rational Design of Ruddlesden-Popper Perovskite Ferrites as Air Electrode for Highly Active and Durable Reversible Protonic Ceramic Cells

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nano-Micro letters 2024年第9期16卷 308-324页

作者： na Yu Idris Temitope Bello Xi chen Tong liu Zheng li Yufei Song Meng ni Department of Building and Real Estate Research Institute for Sustainable Urban Development(RISUD)and Research Institute for Smart Energy(RISE)The Hong Kong Polytechnic UniversityHung HomKowloonHong KongPeople’s Republic of China the Hong kong Polytechnic University Shenzhen Research Institute Shenzhen 518057GuangdongPeople’s Republic of China Department of Mechanical and Aerospace Engineering The Hong Kong University of Science and TechnologyClear Water BayHong KongPeople’s Republic of China

Reversible protonic ceramic cells(RePCCs)hold promise for efficient energy storage,but their practicality is hindered by a lack of high-performance air electrode ***-Popper perovskite Sr_(3)Fe_(2)O_(7−δ)(SF)exhibits superior proton uptake and rapid ionic conduction,boosting ***,excessive proton uptake during RePCC operation degrades SF’s crystal structure,impacting *** study introduces a novel A/B-sites co-substitution strategy for modifying air electrodes,incorporating Sr-deficiency and Nb-substitution to create Sr_(2.8)Fe_(1.8)Nb_(0.2)O_(7−δ)(D-SFN).Nb stabilizes SF’s crystal,curbing excessive phase formation,and Sr-deficiency boosts oxygen vacancy concentration,optimizing oxygen *** D-SFN electrode demonstrates outstanding activity and durability,achieving a peak power density of 596 mw cm^(−2)in fuel cell mode and a current density of−1.19 A cm^(−2)in electrolysis mode at 1.3 V,650℃,with excellent cycling *** approach holds the potential for advancing robust and efficient air electrodes in RePCCs for renewable energy storage.

关键词： Reversible protonic ceramic cells Air electrode Ruddlesden-Popper perovskite Hydration Oxygen reduction reaction

STATNet:One-stage coal-gangue detector based on deep learning algorithm for real industrial application

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Energy and AI 2024年第3期17卷 113-125页

作者： kefei Zhang a Teng wang Xiaolin Yang liang Xu Jesse thé Zhongchao Tan Hesheng Yu key laboratory of Coal Processing and Efficient Utilization of Ministry of Education School of Chemical Engineering and TechnologyChina University of Mining and TechnologyXuzhouJiangsu 221116China Department of Mechanical&Mechatronics Engineering University of Waterloo200 University Avenue WestWaterlooOntario N2L 3G1Canada lakes Environmental Research Inc. 170 Columbia St.W.Suite 1WaterlooOntarioN2L 3L3 Canada Eastern Institute for Advanced Study Eastern Institute of TechnologyNingboZhejiang 315200China Department of Energy and Power Engineering Tsinghua UniversityBeijing 100084China

Coal-gangue object detection has attracted substantial attention because it is the core of realizing vision-based intelligent and green coal separation. However, most existing studies have been focused on laboratory datasets and prioritized model lightweight. this makes the coal-gangue object detection challenging to adapt to the complex and harsh scenes of real production environments. therefore, our project collected and labeled image datasets of coal and gangue under real production conditions from a coal preparation plant. we then designed a one-stage object model, named STATNet, following the “backbone-neck-head” architecture with the aim of enhancing the detection accuracy under industrial coal preparation scenarios. the proposed model utilizes Swin Transformer as backbone module to extract multi-scale features, improved path augmentation feature pyramid network (iPAFPN) as neck module to enrich feature fusion, and task-aligned head (TAH) as head module to mitigate conflicts and misalignments between classification and localization tasks. Experimental results on a real-world industrial dataset demonstrate that the proposed STATNet model achieves an impressive AP50 of 89.27 %, significantly surpassing several state-of-the-art baseline models by 2.02 % to 5.58 %. Additionally, it exhibits stronger robustness in resisting image corruption and perturbation. these findings demonstrate its promising prospects in practical coal and gangue separation applications.

关键词： Coal-gangue detection Swin transformer Impr oved path augmentation feature pyranid network Task-aligned head Object detection

Nonaqueous potassium-ion full-cells:Mapping the progress and identifying missing puzzle pieces

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Journal of Energy chemistry 2024年第6期93卷 384-399,I0010页

作者： Badre larhrib louiza larbi lénaïc Madec Universite de Pau et des Pays de l’Adour E2S UPPACNRSIPREMPauFrance Universitéde Haute-Alsace Institut de Science des Matériaux de Mulhouse(IS2M)CNRS UMR 7361F-68100 MulhouseFrance Universitéde Strasbourg F-67081 StrasbourgFrance Réseau sur le Stockage Electrochimique de l’Energie CNRS FR3459AmiensFrance Institut des Matériaux Jean Rouxel(IMN) CNRS UMR 6502Univ.Nantes44322 Cedex 3 NantesFrance

this review addresses the growing interest for potassium-ion full-cells(kIFCs)in view of the transition from potassium-ion half-cells(kIHCs)toward commercial k-ion batteries(kIBs).It focuses on the key parameters of kIFCs such as the electrode/electrolyte interfaces challenge,major barriers,and recent advancements in *** strategies for enhancing kIFC performance,including interfaces co ntrol,electrolyte optimization,electrodes capacity ratio,electrode material screening and electrode design,are *** review highlights the need to evaluate kIBs in full-cell configurations as half-cell results are strongly impacted by the k metal *** also emphasizes the importance of understanding solid electrolyte interphase(SEI)formation in kIFCs and explores promising nonaqueous as well as quasiand all-solid-state electrolytes *** review thus paves the way for practical,cost-effective,and scalable kIBs as energy storage systems by offering insights and guidance for future research.

关键词： k-ion full-cells Potassium-ion batteries Cross-talk Solid-state batteries Potassium reactivity Electrolyte design Electrode design

Toughened (Ti_(0.2)Zr_(0.2)Hf_(0.2)Nb_(0.2)Ta_(0.2))B_(2)–SiC composites fabricated by one-step reactive sintering with a unique SiB_(6) additive

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Journal of Advanced Ceramics 2024年第1期13卷 86-100页

作者： wei Hao Xinzhe lu ling li Tao wang Guoliang Ren Huangyue Cai Xiaofeng Zhao Dongyun wang na ni Zhejiang Provincial key laboratory of Urban Rail Transit Intelligent Operation and Maintenance Technology&Equipment Zhejiang Normal UniversityZhejiang 321004China key lab of Education Ministry for Power Machinery and Engineering School of Mechanical EngineeringShanghai Jiao Tong UniversityShanghai 200240China School of Materials Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China

High-entropy diboride has been arousing considerable interest in recent ***,the low toughness and damage tolerance limit its applications as ultra-high-temperature structural *** we report that a unique SiB_(6) additive has been first incorporated as boron and silicon sources to fabricate a high-entropy boride(Ti_(0.2)Zr_(0.2)Hf_(0.2)Nb_(0.2)Ta_(0.2))B_(2)–SiC composite though one-step boro/carbothermal reduction reactive sintering.A synergetic effect of high-entropy sluggish diffusion and SiC secondary phase retarded the grain growth of the(Ti_(0.2)Zr_(0.2)Hf_(0.2)Nb_(0.2)Ta_(0.2))B_(2)–51SiC *** small grain size was beneficial to shorten the diffusion path for mass transport,thereby enhancing the relative density to~99.3%.these results in an increase of fracture toughness from~5.2 in HEBS-1900 to~7.7 MPa·m^(1/2) in HEBS-2000,which corresponded to a large improvement of 48%.the improvement was attributed to a mixed mode of intergranular and transgranular cracking for offering effective pinning in crack propagation,resulting from balanced grain boundary strength collectively affected by improved densification,solid solution strengthening,and incorporation of SiC secondary phase.

关键词： high-entropy diboride silicon hexaboride boro/carbothermal reduction reactive sintering fracture toughness

Exploring the mechanical behavior and microstructure of compacted loess subjected to dry-wet cycles and chemical contamination

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第9期16卷 3673-3695页

作者： Yongpeng nie wankui ni Xiangfei lü wenxin Tuo College of Geological Engineering and Geomatics Chang'an UniversityXi'an710054China Department of Civil Engineering Nagoya Institute of TechnologyNagoya466-8555Japan School of water and Environment Chang'an UniversityXi'an710054China

Due to climatic factors and rapid urbanization,the soil in the loess Plateau,china,experiences the coupled effects of dry-wet cycles and chemical *** the mechanical behavior and corresponding microstructural evolution of contaminated loess subjected to dry-wet cycles is essential to elucidate the soil degradation ***,direct shear and consolidation tests were performed to investigate the variations in mechanical properties of compacted loess contaminated with acetic acid,sodium hydroxide,and sodium sulfate during dry-wet *** mechanical response mechanisms were investigated using zeta potential,mineral chemical composition,and scanning electron microscopy(SEM)*** results indicate that the mechanical deterioration of sodium hydroxidecontaminated loess during dry-wet cycles decreases with increasing contaminant concentration,which is mainly attributed to the thickening of the electrical double layer(EDl)by nat and the precipitation of calcite,as well as the formation of colloidal flocs induced by OH,thus inhibiting the development of large pores during the dry-wet *** contrast,the attenuation of mechanical properties of both acetic acid-and sodium sulfate-contaminated loess becomes more severe with increasing contaminant concentration,with the latter being more particularly *** is primarily due to the reduction of the EDl thickness and the erosion of cement in the acidic environment,which facilitates the connectivity of pores during dry-wet ***,the salt expansion generated by the drying process of saline loess further intensifies the structural ***,the mechanical performance of compacted loess is sensitive to both pollutant type and concentration,exhibiting different response patterns in the dry-wet cycling condition.

关键词： Contaminated loess Dry-wet cycles Compressibility Shear strength Microstructural evolution

Recent progress in MnBi2nTe3n+1 intrinsic magnetic topological insulators: crystal growth, magnetism and chemical disorder

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national Science Review 2024年第2期11卷 65-80页

作者： chaowei Hu Tiema Qian ni ni Department of Physics and Astronomy and California nano Systems Institute University of California-Los Angeles

the search for magnetic topological materials has been at the forefront of condensed matter research for their potential to host exotic states such as axion insulators, magnetic weyl semimetals, chern insulators,etc. To date, the MnBi2nTe3n+1family is the only group of materials showcasing van der waals-layered structures, intrinsic magnetism and non-trivial band topology without trivial bands at the Fermi level. the interplay between magnetism and band topology in this family has led to the proposal of various topological phenomena, including the quantum anomalous Hall effect, quantum spin Hall effect and quantum magnetoelectric effect. Among these, the quantum anomalous Hall effect has been experimentally observed at record-high temperatures, highlighting the unprecedented potential of this family of materials in fundamental science and technological innovation. In this paper, we provide a comprehensive review of the research progress in this intrinsic magnetic topological insulator family, with a focus on single-crystal growth, characterization of chemical disorder, manipulation of magnetism through chemical substitution and external pressure, and important questions that remain to be conclusively answered.

关键词： MnBi2Te4 magnetic topological insulator magnetism tuning antiferromagnetism ferromagnetism pressure chemical doping

Some Mean Convergence theorems for the Maximum of Normed Double Sums of Banach Space Valued Random Elements

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Acta Mathematica Sinica,English Series 2024年第7期40卷 1727-1740页

作者： Andrew ROSAlSkY le Van thANH Nguyen thi thUY Department of Statistics University of FloridaGainesvilleFL 32611-8545USA Department of Mathematics Vinh UniversityVinhNghe AnViet Nam High School for Gifted Students Vinh UniversityVinhNghe AnViet Nam

In this correspondence,we establish mean convergence theorems for the maximum of normed double sums of Banach space valued random *** of the results pertain to random elements which are *** expand and improve a number of particular cases in the literature on mean convergence of random elements in Banach *** of the main contributions of the paper is to simplify and improve a recent result of li,Presnell,and Rosalsky[Journal of Mathematical Inequalities,16,117–126(2022)].A new maximal inequality for double sums of M-dependent random elements is proved which may be of independent *** sharpness of the results is illustrated by four examples.

关键词： Double sum mean convergence Rademacher type p Banach space Banach space valued random element M-dependent random elements

Vitamin D and selenium for type 2 diabetes mellitus with Hashimoto’s thyroiditis:Dosage and duration insights

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world Journal of Diabetes 2024年第8期15卷 1824-1828页

作者： Yun-Feng Yu Xue-li Shangguan Dan-ni Tan li-na Qin Rong Yu School of Traditional chinese Medicine Hunan University of Chinese MedicineChangsha 410208Hunan ProvinceChina

this letter discusses the publication by Feng et ***,selenium,and vitamin D are closely associated with thyroid hormone production in humans;however,the efficacy of selenium and vitamin D supplementation for type 2 diabetes mellitus(T2DM)patients with Hashimoto’s thyroiditis(HT)remains *** the retrospective study we discuss herein,the authors highlighted significant improvements in thyroid function,thyroid antibodies,blood glucose,and blood lipid in T2DM patients with HT following addition of vitamin D and selenium to their antidiabetic regimens,underscoring the value of these *** team is currently engaged in research exploring the relationship between micronutrients and HT,and we have obtained invaluable insights from the aforementioned *** on this research and current literature,we recommend a regimen of 4000 IU/day of vitamin D and 100-200μg/day of selenium for over three months to six months for patients with HT,particularly for those with concurrent T2DM.

关键词： Vitamin D Selenium Type 2 diabetes mellitus Hashimoto’s thyroiditis Dosage Duration

Regional features of pollen R-values in china

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Science china Earth Sciences 2024年第1期67卷 295-308页

作者： Jie XIA Jian ni College of life Sciences Zhejiang Normal UniversityJinhua 321004China Jinhua Mountain Observation and Research Station for Subtropical Forest Ecosystems Jinhua 321004China

Establishing a quantitative relationship between modern pollen and vegetation remains a pivotal but intricate pursuit within the field of Quaternary *** R-value,a well-established and traditional metric characterized by its simplicity and direct applicability,serves to calibrate the nonlinear disparities between surface pollen and modern *** study entails the construction of a comprehensive pollen R-value dataset for china derived from R-values published between 1987 and *** dataset,compiled after rigorous screening,calibration,and standardization processes,encompasses 898 modern pollen sampling sites and 2115 pollen R-value data entries,encapsulating 152 pollen taxa spanning 65 families and 113 *** the extracted R-values yielded the following insights:(1)A macrospatial analysis validates previously established knowledge at a site-specific ***,pollen R-value variations across china are statistically *** two-thirds of pollen taxa exhibit underrepresentation(e.g.,Taxodiaceae,Corylus,nitraria,Tamarix,Cyperaceae,Poaceae,and Fabaceae),while the remaining one-third display overrepresentation(e.g.,Pinus,Picea,Betula,Ephedra,chenopodiaceae,and Artemisia).the degree of underrepresentation surpasses that of overrepresentation,and the representation patterns of Castanea,Quercus,Polygonaceae,and Asteraceae are contingent upon vegetation types.(2)Pollen R-values follow distinct spatial distribution patterns within *** the woody vegetation region of eastern china,R-values progressively decline from north to south,correlating with rising temperatures and ***,in herbaceous vegetation regions of northern and western china,R-values decrease from east to west and from northeast to southwest,corresponding to increased ***,pollen R-values manifest variation contingent on pollen taxa,vegetation types,and climatic regions,even differing for the same taxa across varying

关键词： Pollen R-value Modern pollen-vegetation relationship Regional pattern Variability Paleovegetation reconstruction