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Porous poly（triazine-heptazine）s:low-temperature solvothermal synthesis,*HCO intermediate activation and photocatalytic COreduction to CH

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Science China Chemistry 2024年

作者： Zhu Gao Zhiwei Jiang Min Liu Yumin Yang Shahzad Ali Qiujian Xie Yuqiang Li Shuai Gu Younian Liu juntao tang Chunyue Pan Jiayin Yuan Guipeng Yu Department of Chemistry and Chemical Engineering Central South University Hunan Joint International Research Center for Carbon Dioxide Resource Utilization School of Physics and ElectronicsCentral South University State Key Laboratory of Superlattices and Microstructures Institute of Semiconductors Chinese Academy of Sciences Department of Materials and Environmental Chemistry Stockholm University

High-temperature ionothermal synthesis has been proven effective in preparing environment-friendly carbon nitride （CN）-based photocatalysts in either triazine or heptazine form for CO2reduction reaction （CO2RR）.However,such a process is usually energy-intensive and suffers from partial carbonization that results in non-porous catalysts and degenerating their ***,we report the preparation of highly porous CN polymers (porous C6N7,C3N3,C4.5N5) through a low-temperature solvothermal polymerization of cyameluric chloride itself or cyanuric chloride itself,or both,*** such,it avoids unfavorable carbonization and allows for fine control of its chemical structure and significantly enlarged surface area (up to669 m2g-1).The pincer-like 2,2′-bipyridine sites of porous C6N7alter the photocatalytic CO2reduction pathways via stabilizing the*HCO intermediates,which promotes further hydrogenation to produce CH4in a high *** from the carbonization-free polymerization,high porosity,and*HCO intermediate activation,porous C6N7gave a superior CO2RR to CH4performance (17.18μmol g-1h-1) as well as high stability （5 successive cycles）,outperforming the bulk and state-of-the-art counterparts of *** opens an avenue for the rational construction of efficient porous CN-based photocatalytic systems,demonstrating their great potential in energy conversion reactions.

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共价有机框架材料用于光催化产过氧化氢

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化学进展 2024年第3期36卷 357-366页

作者：陈安淇蒋智威唐俊涛喻桂朋中南大学化学化工学院长沙410083

过氧化氢(H_(2)O_(2))是一种重要的绿色氧化剂,然而其主流生产方法蒽醌法具有耗能高、安全隐患大等缺点。以水和氧气为原料,通过人工光合作用合成H_(2)O_(2)具有安全、环保和节能等特点,已成为当前研究热点。共价有机框架(COFs)因其结... 详细信息

过氧化氢(H_(2)O_(2))是一种重要的绿色氧化剂,然而其主流生产方法蒽醌法具有耗能高、安全隐患大等缺点。以水和氧气为原料,通过人工光合作用合成H_(2)O_(2)具有安全、环保和节能等特点,已成为当前研究热点。共价有机框架(COFs)因其结构可调性、高比表面积、良好光催化性能等优点被广泛应用于光催化生产H_(2)O_(2)中。本文归纳了近年来COFs光催化产H_(2)O_(2)领域研究进展,分别论述了通过氧还原、水氧化以及双通道过程产生H_(2)O_(2)的反应机理。综述了通过结构设计、官能团修饰等调控COFs光学带隙、提升电荷分离能力和载流子迁移率,从而提高光催化产H_(2)O_(2)性能的方法,有助于设计出高效、稳定、可持续生产的COFs应用于光催化产H_(2)O_(2)。

关键词：共价有机框架过氧化氢光催化氧还原水氧化

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基于电荷泵的燃料电池有源网络升压变换器

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电工技术学报 2022年第4期37卷 905-917页

作者：唐钧涛戚志东裴进单梁南京理工大学自动化学院南京210094

高增益DC-DC变换器是燃料电池发电技术的关键环节,有利于改善燃料电池小电压、大电流特性。但是由于传统Boost变换器存在电压增益有限、电感电流纹波大、功率器件应力高的缺陷,无法满足燃料电池发电系统并网运行的需求。该文提出一种基... 详细信息

高增益DC-DC变换器是燃料电池发电技术的关键环节,有利于改善燃料电池小电压、大电流特性。但是由于传统Boost变换器存在电压增益有限、电感电流纹波大、功率器件应力高的缺陷,无法满足燃料电池发电系统并网运行的需求。该文提出一种基于电荷泵的燃料电池有源网络升压变换器,将有源网络变换器中输入侧的电感用电荷泵结构代替。该变换器结合电荷泵电压倍增能力强和有源网络结构输入电流纹波小的优势,具有电压增益高、电感电流平均值小、开关器件电压/电流应力低、鲁棒性强的特点。最后搭建一套燃料电池前级功率变换实验样机,验证了变换器的高效率与有效性,当输入电压为20V、输出电流为1.25A时,系统整体效率可以达到94.1%。

关键词：燃料电池发电技术高增益DC-DC变换器有源网络电荷泵

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Validation of proposed diagnostic criteria for allergic bronchopulmonary aspergillosis

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Chinese Medical Journal 2024年第9期137卷 1132-1134页

作者： Runjin Cai Yifei Yang Huan Ge Xuemei Chen Xinyue Hu Yuanyuan Jiang Lisha Luo Shuanglinzi Deng Jiale tang Chendong Wu Huan tang Xiaoxiao Gong Xiaozhao Li juntao Feng Department of Respiratory Medicine National Key Clinical SpecialtyBranch of National Clinical Research Center for Respiratory DiseaseXiangya HospitalCentral South UniversityChangshaHunan 410008China National Clinical Research Center for Geriatric Disorders Xiangya HospitalCentral South UniversityChangshaHunan 410008China Department of Nephrology Xiangya HospitalCentral South UniversityChangshaHunan 410008China

To the Editor:Allergic bronchopulmonary aspergillosis(ABPA)is an allergic lung disease caused by hypersensitivity to antigens from Aspergillus,and it most commonly occurs in patients with asthma or cysticbrosis.[1]The main clinical characteristics of the disease are those related to elevated serum immunoglubulin(Ig)E level,positive Aspergillus fumigatus(***)specic IgE/IgG,repeated pulmonary inltration,and ***,due to the lack of unied diagnostic criteria and screening methods,ABPA is always *** 2021,new diagnostic criteria were proposed for allergic bronchopulmonary mycosis(ABPM)in the Japanese population.

关键词： allergic elevated aspergillosis

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Topologically protected entanglement switching around exceptional points

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Light(Science & Applications) 2024年第8期13卷 1631-1644页

作者： Zan tang Tian Chen Xing tang Xiangdong Zhang Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurements of Ministry of Education Beijing Key Laboratory of Nanophotonics&Ultrafine Optoelectronic SystemsSchool of PhysicsBeijing Institute of Technology100081 BeijingChina

The robust operation of quantum entanglement states is crucial for applications in quantum information,computing,and communications^(1–3).However,it has always been a great challenge to complete such a task because of decoherence and ***,we propose theoretically and demonstrate experimentally an effective scheme to realize robust operation of quantum entanglement states by designing quadruple degeneracy exceptional *** encircling the exceptional points on two overlapping Riemann energy surfaces,we have realized a chiral switch for entangled states with high *** to the topological protection conferred by the Riemann surface structure,this switching of chirality exhibits strong robustness against perturbations in the encircling ***,we have experimentally validated such a scheme on a quantum walk *** work opens up a new way for the application of non-Hermitian physics in the field of quantum information.

关键词： exceptional quantum Riemann

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重型半挂汽车列车防侧翻分层递阶控制

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汽车安全与节能学报 2019年第4期10卷 474-482页

作者：赵树恩张雄唐俊涛重庆交通大学机电与车辆工程学院中国重庆400074 重庆青山工业有限责任公司中国重庆402761 华东交通大学机电与车辆工程学院中国南昌330013

为提高重型半挂汽车列车在极限工况下的防侧翻稳定性,建立了侧向、横摆、侧倾运动的牵引车和挂车5自由度动力学模型。运用模型预测控制方法,决定目标控制横摆力矩。以车辆实时横摆角速度和轮胎载荷转移率为决策依据,对主动转向和直接横... 详细信息

为提高重型半挂汽车列车在极限工况下的防侧翻稳定性,建立了侧向、横摆、侧倾运动的牵引车和挂车5自由度动力学模型。运用模型预测控制方法,决定目标控制横摆力矩。以车辆实时横摆角速度和轮胎载荷转移率为决策依据,对主动转向和直接横摆力矩控制两子系统,进行协调控制。用TruckSim/Simulink平台,进行联合仿真分析。结果表明:在相同工况下,牵引车、挂车的侧向加速度最大值分别改善了7.76%、12.29%;横摆角速度最大绝对值分别改善了23.88%、3.39%;重型半挂半挂汽车列车的最大铰接角减小了19.87%。因而,相对于传统方法,该防侧翻分层递阶控制,提高了重型半挂汽车列车的防侧翻稳定性。

关键词：重型半挂汽车列车防侧翻分层递阶控制主动前轮转向直接横摆力矩控制

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An economic way to achieve all-weather CO2 reduction

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National Science Review 2024年第3期11卷 46-47页

作者： Junwang tang Department of Chemical Engineering University College London

Utilising solar power to convert carbon dioxide（CO2） into hydrocarbon fuels presents an eco-friendly method to address dependence on fossil fuels and contribute to a net-zero CO2emission goal[1,2].

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UAV-assisted data collection for wireless sensor networks with dynamic working modes

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Digital Communications and Networks 2024年第3期10卷 805-812页

作者： Jie Chen Jianhua tang Shien-Ming Wu School of Intelligent Engineering South China University of TechnologyGuangzhou511442China

Wireless Sensor Network(WSN)is a cornerstone of Internet of Things(IoT)and has rich application *** this work,we consider a heterogeneous WSN whose sensor nodes have a diversity in their Residual Energy(RE).In this work,to protect the sensor nodes with low RE,we investigate dynamic working modes for sensor nodes which are determined by their RE and an introduced energy ***,we employ an Unmanned Aerial Vehicle(UAV)to collect the stored data from the heterogeneous *** aim to jointly optimize the cluster head selection,energy threshold and sensor nodes’working mode to minimize the weighted sum of energy con-sumption from the WSN and UAV,subject to the data collection rate *** this end,we propose an efficient search method to search for an optimal energy threshold,and develop a penalty-based successive convex approximation algorithm to select the cluster *** we present a low-complexity iterative approach to solve the joint optimization problem and discuss the implementation *** results justify that our proposed approach is able to reduce the energy consumption of the sensor nodes with low RE significantly and also saves energy for the whole WSN.

关键词： Unmanned aerial vehicle Wireless sensor networks Cluster heads Dynamic working modes

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Highly effective design of high GFA alloys with different metalbased and various components by machine learning

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Science China(Technological Sciences) 2024年第5期67卷 1431-1442页

作者： tang YiChuan HE YiFan FAN ZhuoQun WANG ZhongQi tang ChengYing Guangxi Key Laboratory for Informational Materials School of Materials Science and EngineeringGuilin University of Electronic TechnologyGuilin541004China

The glass-forming ability(GFA)is of great significance for the development of novel functional metal-based metallic *** this study,seven popular machine learning(ML)algorithms were employed to design novel M-based(M=Fe,Co,Ni,Ti,Zr,and rare earth metal(RE))and X-component(X=2,3,4,5,6,and>6)alloys with excellent GFA.A GFA containing 6957 data points with structural analysis was *** engineering was used to analyze the importance and correlation of *** algorithms were utilized for GFA prediction,revealing that Xtreme Gradient Boosting Trees exhibited the strongest predictive capability,achieving a high accuracy of 94.0%,a true positive rate of 97.6%,and a root mean squared error of 0.3705 across the entire ***,the GFA of ternary to hexahydroxy alloys based on Fe,Co,Ni,Zr,Ti,and Y was predicted using all possible compositions generated through ***,a series of alloys with good GFA was successfully designed and *** present work suggests that the proposed ML method can be utilized to design novel multiple-M-based amorphous alloys with high GFA.

关键词： machine learning amorphous alloy feature engineering materials design glass forming ability

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Nuclear charge radius predictions by kernel ridge regression with odd-even effects

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Nuclear Science and Techniques 2024年第2期35卷 94-102页

作者： Lu tang Zhen-Hua Zhang Mathematics and Physics Department North China Electric Power UniversityBeijing 102206China Hebei Key Laboratory of Physics and Energy Technology North China Electric Power UniversityBaoding 071000China

The extended kernel ridge regression(EKRR)method with odd-even effects was adopted to improve the description of the nuclear charge radius using five commonly used nuclear *** are:(i)the isospin-dependent A^(1∕3) formula,(ii)relativistic continuum Hartree-Bogoliubov(RCHB)theory,(iii)Hartree-Fock-Bogoliubov(HFB)model HFB25,(iv)the Weizsacker-Skyrme(WS)model WS*,and(v)HFB25**** the last two models,the charge radii were calculated using a five-parameter formula with the nuclear shell corrections and deformations obtained from the WS and HFB25 models,*** each model,the resultant root-mean-square deviation for the 1014 nuclei with proton number Z≥8 can be significantly reduced to 0.009-0.013 fm after considering the modification with the EKRR *** best among them was the RCHB model,with a root-mean-square deviation of 0.0092 *** extrapolation abilities of the KRR and EKRR methods for the neutron-rich region were examined,and it was found that after considering the odd-even effects,the extrapolation power was improved compared with that of the original KRR *** strong odd-even staggering of nuclear charge radii of Ca and Cu isotopes and the abrupt kinks across the neutron N=126 and 82 shell closures were also calculated and could be reproduced quite well by calculations using the EKRR method.

关键词： Nuclear charge radius Machine learning Kernel ridge regression method

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