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Phosphorous-doped carbon nanotube/reduced graphene oxide aerogel cathode enabled by pseudocapacitance for high energy and power zinc-ion hybrid capacitors

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Chinese Chemical Letters 2024年第2期35卷 570-576页

作者： junjun yao Fuzhi Li Ruyi Zhou Chenchen Guo Xinru Liu Yirong Zhu Hunan Key Laboratory of Green Metallurgy and New Energy Materials College of Materials and Advanced ManufacturingHunan University of TechnologyZhuzhou 412007China College of packaging and Material Engineering Hunan University of TechnologyZhuzhou 412007China

The design and development of energy storage device with high energy/power density has become a research ***-ion hybrid capacitors(ZHCs)are considered as one of the most promising ***,the application of ZHCs is hindered by their low energy density at high power density due to the unsatisfactory cathode *** this study,a novel 3D phosphorus-doped carbon nanotube/reduced graphene oxide(P-CNT/rGO)aerogel cathode is synthesized through a synergistic modification strategy of CNT insertion and P doping modification combined with 3D porous *** as-obtained P-CNT/rGO aerogel cathode manifests significantly increased surface aera,expanded interlayer spacing,and enhanced pseudocapacitance behavior,thus leading to significantly enhanced specific capacitance and superb ions transport *** as-assembled ZHC based on P-CNT/rGO cathode delivers a superior energy density of 42.2 Wh/kg at an extreme-high power density of 80 kW/kg and excellent cycle ***-depth kinetic analyses are undertaken to prove the enhanced pseudocapacitance behavior and exceptional power output capability of ***,the reaction mechanism of physical and chemical adsorption/desorption of electrolyte ions on the P-CNT/rGO cathode is revealed by systematic ex-situ *** work can provide a valuable reference for developing advanced graphene-based cathode for high energy/power density ZHCs.

关键词： Graphene aerogel Phosphorus doping Pseudocapacitance Zinc-ion hybrid capacitors Energy storage mechanism

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Copper-induced formation of heterostructured Co_(3)O_(4)/CuO hollow nanospheres towards greatly enhanced lithium storage performance

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Chinese Chemical Letters 2024年第2期35卷 594-598页

作者： junjun Zhang Huiying Lu Tianhao yao Xin Ji Qingmiao Zhang Lingjie Meng Jianmin Feng Hongkang Wang College of Geography & Environment Xianyang Normal UniversityXianyang 712000China State Key Lab of Electrical Insulation and Power Equipment Center of Nanomaterials for Renewable Energy (CNRE)School of Electrical EngineeringXi'an Jiaotong UniversityXi'an 710049China School of Chemistry Xi'an Key Laboratory of Sustainable Energy Material Chemistryand Instrumental Analysis CenterXi'an Jiaotong UniversityXi'an 710049China

We report a facile template-free fabrication of heterostructured Co_(3)O_(4)/CuO hollow nanospheres using pre-synthesized Co/Cu-glycerate as conformal *** introduction of copper nitrate in the solvothermal reaction system of glycerol/isopropanol/cobalt nitrate readily induces the conversion from solid Co-glycerate to hollow Co/Cu-glycerate nanospheres,and the effect of the Co/Cu atomic ratio on the structure evolution of the metal glycerates as well as their corresponding oxides were *** examined as anode materials for lithium-ion batteries,the well-defined Co_(3)O_(4)/CuO hollow nanospheres with Co/Cu molar ratio of 2.0 demonstrate excellent lithium storage performance,delivering a high reversible capacity of 930 mAh/g after 300 cycles at a current density of 0.5 A/g and a stable capacity of 650 mAh/g after 500 cycles even at a higher current density of 2.0 A/g,which are much better than their counterparts of bare CuO and Co_(3)O_(4).The enhanced lithium storage performance can be attributed to the synergistic effect of the CuO and Co_(3)O_(4)heterostructure with hollow spherical morphology,which greatly enhances the charge/electrolyte transfer and effectively buffers the volume changes upon lithiation/delithiation cycling.

关键词： Lithium-ion batteries Co/Cu-glycerate Hollow nanospheres Co_(3)O_(4)/CuO heterostructure Electrochemical properties

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Enhancement of CH_(3)CO^(*) adsorption by editing d-orbital states of Pd to boost C–C bond cleavage of ethanol eletrooxidation

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Science China Chemistry 2024年第2期67卷 696-704页

作者： Yuchen Qin Fengqi Wang Pei Liu Jinyu Ye Qian Wang yao Wang Guangce Jiang Lijie Liu Pengfang Zhang Xiaobiao Liu Xin Zheng Yunlai Ren junjun Li Zhicheng Zhang College of Sciences Henan Agricultural UniversityZhengzhou450000China Tianjin Key Laboratory of Molecular Optoelectronic Sciences Department of ChemistrySchool of ScienceTianjin University&Collaborative Innovation Center of Chemical Science and EngineeringTianjin300072China College of Chemistry and Chemical Engineering Xiamen UniversityXiamen361005China Department of Analysis Sinopec Engineering Group Luoyang R&D Center of TechnologyLuoyang471000China School of Chemical and Material Engineering Jiangnan UniversityWuxi214211China Shandong Provincial Key Laboratory of Chemical Energy Storage and Novel Cell Technology Liaocheng UniversityLiaocheng252000China

Improving the complete ethanol electrooxidation on Pd-based catalysts in alkaline media has drawn widely attention due to the high mass energy ***,the weak adsorption energy of CH_(3)CO^(*) on Pd restricts the C–C bond *** by the molecular orbital theory,we proposed the d-state-editing strategy to construct more unoccupied d-states of Pd for the enhanced interaction with CH_(3)CO^(*) to break C–C *** expected,the reduced number of e_g electrons and more unoccupied d-states of Pd successfully formed on as-prepared porous Rh Au–Pd Cu nanosheets(PNSs).Theoretical calculations show that the optimized d-states of Rh Au–Pd Cu PNS can effectively improve the adsorption of CH_(3)CO^(*) and drastically reduce the energy barrier of C–C bond cleavage,thus boosting the complete oxidation of *** charge ratio of C_1 pathway on Rh Au–Pd Cu PNSs is 51.5%,more than 2 times higher than that of Pd *** finding provides an innovative perspective for the design of highly-efficient noble-based electrocatalysts.

关键词： C–C bond cleavage CH_(3)CO^(*)adsorption unoccupied d-states ethanol oxidation reaction RhAu–PdCu porous nanosheets

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Morphological disruption and visual tuning alterations in the primary visual cortex in glaucoma(DBA/2J)mice

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Neural Regeneration Research 2024年第1期19卷 220-225页

作者： Yin Yang Zhaoxi Yang Maoxia Lv Ang Jia junjun Li Baitao Liao Jing’an Chen Zhengzheng Wu Yi Shi Yang Xia Dezhong yao Ke Chen Department of Ophthalmology Sichuan Provincial People’s HospitalMedical SchoolUniversity of Electronic Science and Technology of ChinaChengduSichuan ProvinceChina The Clinical Hospital of Chengdu Brain Science Institute MOE Key Lab for NeuroInformationSchool of Life Science and TechnologyUniversity of Electronic Science and Technology of ChinaChengduSichuan ProvinceChina Research Unit of NeuroInformation Chinese Academy of Medical SciencesChengduSichuan ProvinceChina Institute of Basic Medical Sciences Chinese Academy of Medical Sciences School of Basic Medicine Peking Union Medical CollegeBeijingChina Health Management Center Sichuan Provincial Key Laboratory for Human Disease Gene StudySichuan Provincial People’s HospitalUniversity of Electronic Science and Technology of ChinaChengduSichuan ProvinceChina Research Unit for Blindness Prevention of Chinese Academy of Medical Sciences(2019RU026) Sichuan Academy of Medical SciencesChengduSichuan ProvinceChina School of Electrical Engineering Zhengzhou UniversityZhengzhouHenan ProvinceChina

Glaucoma is a leading cause of irreve rsible blindness wo rldwide,and previous studies have shown that,in addition to affecting the eyes,it also causes abnormalities in the ***,it is not yet clear how the primary visual cortex(V1)is altered in *** study used DBA/2J mice as a model for spontaneous secondary *** aim of the study was to compare the electrophysiological and histomorphological chara cteristics of neurons in the V1between 9-month-old DBA/2J mice and age-matched C57BL/6J *** conducted single-unit recordings in the V1 of light-anesthetized mice to measure the visually induced responses,including single-unit spiking and gamma band *** morphology of layerⅡ/Ⅲneurons was determined by neuronal nuclear antigen staining and Nissl staining of brain tissue ***-seven neurons from eight DBA/2J mice and eighty-one neurons from eight C57BL/6J mice were *** with the C57BL/6J group,V1 neurons in the DBA/2J group exhibited weaker visual tuning and impaired spatial *** r,fewer neuro ns were observed in the V1 of DBA/2J mice compared with C57BL/6J *** findings suggest that DBA/2J mice have fewer neurons in the VI compared with C57BL/6J mice,and that these neurons have impaired visual *** findings provide a better understanding of the pathological changes that occur in V1 neuron function and morphology in the DBA/2J mouse *** study might offer some innovative perspectives regarding the treatment of glaucoma.

关键词： DBA/2J degeneration gamma band oscillations glaucoma primary visual cortex(V1) retina single-unit recording tuning curve

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高校巡察与其他监督贯通融合路径研究

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国家教育行政学院学报 2022年第7期295卷 81-87页

作者：姚君君王瓅苑刘东晓上海外国语大学党委巡察工作办公室上海200083 上海外国语大学纪委办公室上海200083

高校巡察是巡视向基层的延伸和拓展,是学校党委落实全面从严治党主体责任的重要抓手。高校巡察与其他监督贯通融合对提升各类监督整体效能起到重要作用,其实现路径可以“思想、责任、机制、组织”四个要素为核心,即通过筑牢贯通融合的... 详细信息

高校巡察是巡视向基层的延伸和拓展,是学校党委落实全面从严治党主体责任的重要抓手。高校巡察与其他监督贯通融合对提升各类监督整体效能起到重要作用,其实现路径可以“思想、责任、机制、组织”四个要素为核心,即通过筑牢贯通融合的思想基础、强化贯通融合的责任抓手、建构贯通融合的有效机制和夯实贯通融合的组织保障来实现。

关键词：高校巡察监督贯通融合

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大体积墩身混凝土施工裂缝控制

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铁道建筑 2005年第3期45卷 12-14页

作者：姚军军中铁十二局集团公司一公司太原030024

以兰武二线龙沟 3号特大桥墩身混凝土施工为背景 ,探讨墩身大体积混凝土内部温度控制及混凝土表面开裂等问题 ,提出大体积墩身混凝土裂缝控制措施。实践证明 ,采取这些措施可取得较好的裂缝控制效果。

关键词：桥墩施工大体积混凝土温度施工裂缝控制

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钻孔桩穿越溶洞地层的施工

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铁道建筑 2005年第5期45卷 19-21页

作者：姚军军姚辉中铁十二局集团一公司太原030024

结合白杨河大桥和小驻马高架桥桩基施工实例,介绍在溶洞地层中施工长度为2 0～4 0m的钻孔灌注桩的地质情况、施工常见问题处理及施工体会。

关键词：钻孔桩溶洞施工

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大体积混凝土温度监控技术总结

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铁道建筑 2005年第4期45卷 12-14页

作者：姚军军姚辉中铁十二局集团公司一公司太原030024

阐述在大体积混凝土施工中 ,通过从选料、配比、拌制到入模浇筑的温度控制 ,减少引起混凝土内部温升的因素 ,降低混凝土中心温度峰值 ;在混凝土浇筑完毕后立即保温养护 ,掌握混凝土温度变化情况 ,预防混凝土因温度应力引起的开裂。采取... 详细信息

阐述在大体积混凝土施工中 ,通过从选料、配比、拌制到入模浇筑的温度控制 ,减少引起混凝土内部温升的因素 ,降低混凝土中心温度峰值 ;在混凝土浇筑完毕后立即保温养护 ,掌握混凝土温度变化情况 ,预防混凝土因温度应力引起的开裂。采取这些措施后 ,混凝土再也没有出现裂缝 ,提高了整个工程的质量。

关键词：大体积混凝土温度监控选料施工养护

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温室环境多参数自动监测仪的设计

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农机化研究 2010年第1期32卷 143-145页

作者：侯波姚军军陕西理工学院电气系陕西汉中723003 012基地军事代表室陕西汉中723100

设计了以AT89C52单片机为核心的温室环境多参数自动监测仪。采用传感器HIH-3610,DS18B20,TSL2561以及AM-4模块对多个环境参数检测,通过TLC1549模数转换器或I2C总线与单片机接口相连;实现了温室环境多参数动态采集与显示、数据USB存储、... 详细信息

设计了以AT89C52单片机为核心的温室环境多参数自动监测仪。采用传感器HIH-3610,DS18B20,TSL2561以及AM-4模块对多个环境参数检测,通过TLC1549模数转换器或I2C总线与单片机接口相连;实现了温室环境多参数动态采集与显示、数据USB存储、参数在线修改和4～20mA远程传输等功能。现场运行表明:监测仪运行可靠,检测精度高,数据传输实时性好,具有很好的实用价值。

关键词：温室环境监测仪单片机传感器

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基于ASNLS算法的智能浮标浮潜模型参数辨识

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中国舰船研究 2024年第2期19卷 13-20页

作者：钟一鸣于曹阳曹军军姚宝恒连琏上海交通大学海洋学院上海200030 上海交通大学海洋工程全国重点实验室上海200240

[目的]针对智能浮标大深度浮潜模型难以精确量化的问题,提出一种抗数据饱和及测量噪声的最小二乘算法(ASNLS),以实现浮潜多参数识别及深度预测。[方法]首先,在智能浮标浮潜运动灰箱模型中引入其执行机构的非线性动作特性以契合实际模型... 详细信息

[目的]针对智能浮标大深度浮潜模型难以精确量化的问题,提出一种抗数据饱和及测量噪声的最小二乘算法(ASNLS),以实现浮潜多参数识别及深度预测。[方法]首先,在智能浮标浮潜运动灰箱模型中引入其执行机构的非线性动作特性以契合实际模型,并将连续型浮潜运动方程转化为离散模式以匹配实际离散的数据采样方式;然后,将离散型运动方程构造为基于相关函数的表达形式,以减弱噪声对参数辨识的影响;最后,通过调整协方差矩阵的取值,实现该浮潜参数辨识算法的抗数据饱和功能。[结果]基于2021年智能浮标在南海的大深度试验数据,开展了浮潜运动模型参数辨识及深度预测,验证结果表明:相较于传统的最小二乘算法及支持向量机算法,ASNLS算法的收敛速度更快(较最小二乘算法提高了31.8%)、深度预测误差更小(不同深度下的平均绝对百分比误差均小于9%)。[结论]ASNLS算法可为智能浮标的深度控制和预报提供有效的浮潜模型支撑。

关键词：智能浮标参数辨识抗数据饱和及测量噪声的最小二乘算法运动预测数据饱和

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