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Graphitic carbon nitride (g-C3N4)-based nanosized heteroarrays: Promising materials for photoelectrochemical water splitting

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Carbon Energy 2020年第2期2卷 223-250页

作者： Liqun Wang Wenping Si Yueyu Tong Feng hou Daniele Pergolesi jungang hou Thomas Lippert Shi Xue Dou Ji Liang Applied Physics Department College of Physics and Materials ScienceTianjin Normal UniversityTianjinChina Key Laboratory of Advanced Ceramics and Machining Technology Ministry of EducationSchool of Materials Science and EngineeringTianjin UniversityTianjinChina Institute for Superconducting and Electronic Materials Australian Institute of Innovative MaterialsUniversity of WollongongNorth WollongongNSWAustralia Laboratory for Multiscale Materials Experiments Paul Scherrer InstituteVilligenPSISwitzerland State Key Laboratory of Fine Chemicals DUT-KTH Joint Education and Research Center on Molecular DevicesInstitute of Energy Science and TechnologyDalian University of Technology(DUT)DalianChina

Photoelectrochemical(PEC)water splitting is recognized as a sustainable strategy for hydrogen generation due to its abundant hydrogen source,utilization of inexhaustible solar energy,high-purity product,and environment-friendly *** actualize a practical PEC water splitting,it is paramount to develop efficient,stable,safe,and low-cost photoelectrode ***,graphitic carbon nitride(g-C3N4)has aroused a great interest in the new generation photoelectrode materials because of its unique features,such as suitable band structure for water splitting,a certain range of visible light absorption,nontoxicity,and good *** inherent defects of g-C3N4,however,seriously impair further improvement on PEC performance,including low electronic conductivity,high recombination rate of photogenerated charges,and limited visible light absorption at long wavelength *** of g-C3N4-based nanosized heteroarrays as photoelectrodes has been regarded as a promising strategy to circumvent these inherent limitations and achieve the high-performance PEC water splitting due to the accelerated exciton separation and the reduced combination of photogenerated electrons/***,we summarize in detail the latest progress of g-C3N4-based nanosized heteroarrays in PEC water-splitting ***,the unique advantages of this type of photoelectrodes,including the highly ordered nanoarray architectures and the heterojunctions,are ***,different g-C3N4-based nanosized heteroarrays are comprehensively discussed,in terms of their fabrication methods,PEC capacities,and mechanisms,*** conclude,the key challenges and possible solutions for future development on g-C3N4-based nanosized heteroarray photoelectrodes are discussed.

关键词： graphitic carbon nitride heterojunctions nanoarrays photoelectrochemical water splitting

Simultaneously Effi cient Solar Light Harvesting and Charge Transfer of Hollow Octahedral Cu_(2)S/CdS p-n Heterostructures for Remarkable Photocatalytic Hydrogen Generation

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Transactions of Tianjin University 2021年第4期27卷 348-357页

作者： Yanting Zhang Lei Ran Zhuwei Li Panlong Zhai Bo Zhang Zhaozhong Fan Chen Wang Xiaomeng Zhang jungang hou Licheng Sun State Key Laboratory of Fine Chemicals School of Chemical EngineeringDalian University of TechnologyDalian 116024China Center of Artifi cial Photosynthesis for Solar Fuels School of ScienceWestlake UniversityHangzhou 310024China Department of Chemistry School of Engineering Sciences in ChemistryBiotechnology and HealthKTH Royal Institute of Technology10044 StockholmSweden

Solar-driven water splitting is a promising alternative to industrial hydrogen *** study reports an elaborate design and synthesis of the integration of cadmium sulfi de(CdS)quantum dots and cuprous sulfi de(Cu_(2)S)nanosheets as three-dimensional(3D)hollow octahedral Cu_(2)S/CdS p-n heterostructured architectures by a versatile template and one-pot sulfi dation strategy.3D hierarchical hollow nanostructures can strengthen multiple refl ections of solar light and provide a large specifi c surface area and abundant reaction sites for photocatalytic water *** to the construction of the p-n heterostructure as an ideal catalytic model with highly matched band alignment at Cu_(2)S/CdS interfaces,the emerging internal electric fi eld can facilitate the space separation and transfer of photoexcited charges between CdS and Cu_(2)S and also enhance charge dynamics and prolong charge ***,the unique hollow Cu_(2)S/CdS architectures deliver a largely enhanced visible-light-driven hydrogen generation rate of 4.76 mmol/(g·h),which is nearly 8.5 and 476 times larger than that of pristine CdS and Cu_(2)S catalysts,*** work not only paves the way for the rational design and fabrication of hollow photocatalysts but also clarifi es the crucial role of unique heterostructure in photocatalysis for solar energy conversion.

关键词： Hollow octahedrons P-n heterostructure Charge separation Photocatalytic water splitting

Engineering single–atom active sites anchored covalent organic frameworks for efficient metallaphotoredox C-N cross–coupling reactions

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Science Bulletin 2022年第19期67卷 1971-1981页

作者： Zhuwei Li Shi Qiu Yurou Song Shiyu Huang Junfeng Gao Licheng Sun jungang hou State Key Laboratory of Fine Chemicals Frontiers Science Center for Smart Materials Oriented Chemical EngineeringSchool of Chemical EngineeringDalian University of TechnologyDalian 116024China Laboratory of Materials Modification by Laser Ion and Electron BeamsDalian University of TechnologyDalian 116024China Center of Artificial Photosynthesis for Solar Fuels and Department of Chemistry School of ScienceWestlake UniversityHangzhou 310024China Department of Chemistry School of Engineering Sciences in ChemistryBiotechnology and HealthKTH Royal Institute of TechnologyStockholm 10044Sweden

Photoredox catalysis has become an indispensable solution for the synthesis of small organic ***,the precise construction of single-atomic active sites not only determines the catalytic performance,but also avails the understanding of structure–activity ***,we develop a facile approach to immobilize single-atom Ni sites anchored porous covalent organic framework(COF)by use of 4,4',4''-(1,3,5-triazine-2,4,6-triyl)trianiline and 2,6-diformylpyridine(Ni SAS/TD-COF).Ni SAS/TDCOF catalyst achieves excellent catalytic performance in visible-light-driven catalytic carbon–nitrogen cross-coupling reaction between aryl bromides and amines under mild *** reaction provides amine products in excellent yields(71%–97%)with a wide range of substrates,including aryl and heteroaryl bromides with electron-deficient,electron-rich and neutral ***,Ni SAS/TD-COF could be recovered from the reaction mixture,corresponding to the negligible loss of photoredox performance after several *** work provides a promising opportunity upon rational design of single-atomic active sites on COFs and the fundamental insight of photoredox mechanism for sustainable organic transformation.

关键词： Single–atom active sites Covalent organic frameworks Photocatalysis C–N cross–coupling reaction Heterogeneous catalyst

Preparation of Laser Cladding Coating Undercooling Cu-based Alloy and Co on Non-equilibrium Solidification Structure

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Journal of Wuhan University of Technology(Materials Science) 2024年第2期39卷 463-472页

作者：田徐铭 CAO Shichao hou Kai hou Xiaopeng WANG Hongfu 张煜 Department of Outpatient Xinzhou People’s HospitalXinzhou 034099China School of Mechanical Engineering North University of ChinaTaiyuan 030051China Department of Neurosurgery Xinzhou People’s HospitalXinzhou 034099China Department of Orthopedics Xinzhou People’s HospitalXinzhou 034099China

The effect of the gradient content of Co element on the solidification process of Cu-based alloy under deep under cooling conditions was *** non-equilibrium solidification structure of the under cooled alloy samples were *** is found that the rapidly solidified alloy has undergone twice grain refinement during the undercooling *** and significance of the maximum undercooling refinement structure of Cu60Ni35Co5 at T=253 K were ***-density defects were observed,such as dislocations,stacking faults networks,and twinning *** standard FCC diffraction pattern represents that it is still a single-phase *** on the metallographic diagram,EBSD and TEM data analysis,it is illustrated that the occurrence of grain refinement under high undercooling is due to stress induced *** addition,the laser cladding technology is used to coat Co-based alloy(Stellite12) coating on 304 stainless steel substrate;the microstructure of the coating cross-section was *** was found that the microstructure of the cross-section is presented as columnar crystals,planar crystals,and disordered growth direction,so that the coating has better hardness and wear *** electrochemical corrosion of the substrate and coating,it can be seen that the Co and Cr elements present in the coating are more likely to form a dense passivation film,which improved the corrosion resistance of the coating.

关键词： non-equilibrium solidification structure undercooling recrystallization laser cladding coating

Integral Operators Between Fock Spaces

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Chinese Annals of Mathematics,Series B 2024年第2期45卷 265-278页

作者： Yongqing LIU Shengzhao hou School of Mathematics and Statistics Changshu Institute of TechnologySuzhou 215006JiangsuChina School of Mathematical Sciences Soochow UniversitySuzhou 215006JiangsuChina

In this paper,the authors study the integral operator■induced by a kernel functionφ(z,·)∈F_α~∞between Fock *** 1≤p≤∞,they prove that S_φ:F_α^(1)→F_α^(p)is bounded if and only if■where k_(a)is the normali... 详细信息

关键词： Fock spaces Integral operators Normalized reproducing kernel

Herbivore and native plant diversity synergistically resist alien plant invasion regardless of nutrient conditions

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Plant Diversity 2024年第5期46卷 640-647页

作者： Liping Shan Meng hou Key Laboratory of Wetland Ecology and Environment State Key Laboratory of Black Soils Conservation and UtilizationNortheast Institute of Geography and AgroecologyChinese Academy of SciencesChangchun 130102China

Alien plant invasion success can be inhibited by two key biotic factors:native herbivores and plant ***,few studies have experimentally tested whether these factors interact to synergistically resist invasion success,especially factoring in changing global environments(*** enrichment).Here we tested how the synergy between native herbivores and plant diversity affects alien plant invasion success in various nutrient *** this purpose,we exposed alien plant species in potmesocosms to different levels of native plant diversity(4 vs.8 species),native generalist herbivores,and high and low soil nutrient *** found that generalist herbivores preferred alien plants to native plants,inhibiting invasion success in a native *** inhibition was amplified by highly diverse native ***,the amplified effect between herbivory and native plant diversity was independent of nutrient *** results suggest that a higher diversity of native communities can strengthen the resistance of native generalist herbivores to alien plant invasions by enhancing herbivory *** synergistic effect remains in force in nutrient-enriched habitats that are always invaded by alien plant *** results shed light on the effective control of plant invasions using multi-trophic means,even in the face of future global changes.

关键词： Biological invasion Biotic resistance Diversity conservation Plant-herbivore interactions Resource availability Global change

Fractures interaction and propagation mechanism of multi-cluster fracturing on laminated shale oil reservoir

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Petroleum Science 2024年第4期21卷 2600-2613页

作者： Jia-Xin Lv Bing hou Key Laboratory of Petroleum Engineering Ministry of Education China University of Petroleum (Beijing) State Key Laboratory of Petroleum Resources and Engineering China University of Petroleum (Beijing) Department of Petroleum Engineering China University of Petroleum (Beijing) at Karamay

The continental shale reservoirs of Jurassic Lianggaoshan Formation in Sichuan Basin contain thin lamina, which is characterized by strong plasticity and developed longitudinal shell limestone *** improve the production efficiency of reservoirs by multi-cluster fracturing, it is necessary to consider the unbalanced propagation of hydraulic fractures and the penetration effect of fractures. This paper constructed a numerical model of multi-fracture propagation and penetration based on the finite element coupling cohesive zone method; considering the construction cluster spacing, pump rate,lamina strength and other parameters studied the influencing factors of multi-cluster fracture interaction propagation; combined with AE energy data and fracture mode reconstruction method, quantitatively characterized the comprehensive impact of the strength of thin interlayer rock interfaces on the initiation and propagation of fractures that penetrate layers, and accurately predicted the propagation pattern of hydraulic fractures through laminated shale oil reservoirs. Simulation results revealed that in the process of multi-cluster fracturing, the proportion of shear damage is low, and mainly occurs in bedding fractures activated by outer fractures. Reducing the cluster spacing enhances the fracture system's penetration ability, though it lowers the activation efficiency of lamina. The high plasticity of the limestone interlayer may impact the vertical propagation distance of the main fracture. Improving the interface strength is beneficial to the reconstruction of the fracture height, but the interface communication effect is limited. Reasonable selection of layers with moderate lamina strength for fracturing stimulation, increasing the pump rate during fracturing and setting the cluster spacing reasonably are beneficial to improve the effect of reservoir stimulation.

关键词： Laminated shale Multi-cluster fracturing Cross-layer Cohesive zone model Acoustic emission technique

In-Plane Dynamic Crushing Behaviors of a Vertex-Based Hierarchical Auxetic Honeycomb

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Acta Mechanica Solida Sinica 2024年第1期37卷 53-62页

作者： Yichen Zan Xiuhui hou Zichen Deng School of Mechanics Civil Engineering and ArchitectureNorthwestern Polytechnical UniversityXi'an 710072China MIIT Key Laboratory of Dynamics and Control of Complex Systems Northwestern Polytechnical UniversityXi'an 710072China School of Aeronautics Northwestern Polytechnical UniversityXi'an 710072China State Key Laboratory of Structural Analysis Optimization and CAE Software for Industrial EquipmentDalian University of TechnologyDalian 116024China

Auxetic metamaterials,which exhibit the negative Poisson’s ratio(NPR)effect,have found wide applications in many engineering ***,their high porosity inevitably weakens their bearing capacity and impact *** improve the energy absorption efficiency of auxetic honeycombs,a novel vertex-based hierarchical star-shaped honeycomb(VSH)is designed by replacing each vertex in the classical star-shaped honeycomb(SSH)with a newly added self-similar *** analytical model is built to investigate the Young’s modulus of VSH,which shows good agreement with experimental results and numerical *** in-plane dynamic crushing behaviors of VSH at three different crushing velocities are investigated,and empirical formulas for the densification strain and plateau stress are *** results reveal more stable deformation modes for VSH,attributed to the addition of self-similar star-shaped ***,compared with SSH under the same relative densities,VSH exhibits better specific energy absorption and higher plateau ***,VSH is verified to be a better candidate for energy absorption while maintaining the auxetic *** study is expected to provide a new design strategy for auxetic honeycombs.

关键词： Vertex-based hierarchical star-shaped honeycomb Auxetic honeycomb Energy absorption Plateau stress Negative Poisson's ratio

An Improved Method for Approximating the Infinite-Horizon Value Function of the Discrete-Time Switched LQR Problem

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Journal of Systems Science & Complexity 2024年第1期37卷 22-39页

作者： hou Tan LI Yuanlong LIN Zongli Department of Automation Shanghai Jiao Tong UniversityShanghai 200240China Key Laboratory of System Control and Information Processing Ministry of Education of ChinaShanghai 200240China Shanghai Engineering Research Center of Intelligent Control and Management Shanghai 200240China Charles L.Brown Department of Electrical and Computer Engineering University of VirginiaCharlottesvilleVA 22904-4743USA

This paper considers the problem of approximating the infinite-horizon value function of the discrete-time switched LQR *** particular,the authors propose a new value iteration method to generate a sequence of monotonically decreasing functions that converges exponentially to the value *** method facilitates us to use coarse approximations resulting from faster but less accurate algorithms for further value iteration,and thus,the proposed approach is capable of achieving a better approximation for a given computation time compared with the existing *** numerical examples are presented in this paper to illustrate the effectiveness of the proposed method.

关键词： Optimal control switched linear systems switched LQR problem.