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Electrocatalytic performance of CNTs/graphene composited rare earth phthalocyanines(M=La,Y,Yb,Sc)

Journal of Rare earths 2024年第2期42卷 323-333,I0004页

作者： Tingting jiang Caixia Ou Luyi wang jun Chen Sydorov Dmytro Qian Zhang Jintian Luo hua wang jiangxi Key Laboratory of Power Batteries and Materials Faculty of Materials Metallurgy and ChemistryJiangxi University of Science and TechnologyGanzhou341000China Joint Department of Electrochemical Energy Systems Institute of Bioorganic Chemistry and PetrochemistryNational Academy of Sciences of Ukraine38A VernadskyAveKiev03142Ukraine Guangdong Jiana Energy Technology Co. Ltd.Qingyuan511500China

In this study,a class of rare earth composite sandwich phthalocyanines(MPcs,M=La,Y,Yb,Sc) were prepared and compounded with graphene and carbon nanotubes to obtain MPc/Gr and MPc/CNTs *** electrocatalytic behaviors of MPc/Gr and MPc/CNTs electrodes were further *** results show that the central rare earth metal has a large influence on the electrocatalytic *** the MPcs/Gr samples,ScPc with the smallest ionic radius and molecular size can be more uniformly dispersed in graphene,and the hydrogen precipitation overpotential of ScPc/Gr electrode is514 mV,corresponding to a Tafel slope of 148 mV/dec,with better electrocatalytic performance than other rare earth metal *** for the MPc/CNTs composites,LaPc,which has the largest ionic radius and molecular size,is more uniformly dispersed on the surface of CNTs,so that the LaPc/CNT electrode exhibits the best LSV performance with the smallest corresponding Tafel slope(176 mV/dec).The main reason is the different binding modes of MPcs molecules in Gr and *** rare earth phthalocyanine is combined with layered graphene,the smallest size of rare earth phthalocyanine(ScPc)is more easily embedded in the graphene layer,resulting in better homogeneity of the composite,larger effective contact area and better electrocatalytic *** contrast,when rare earth phthalocyanine is bound to carbon nanotubes in a tubular structure,it is mainly bound by attaching to the surface or being entangled by the carbon *** this case,the rare-earth phthalocyanine molecules(LaPc)with larger layer spacing can provide more contact area with CNTs,forming a more uniform and effective composite,which eventually provides more active sites and better electrocatalytic performance.

关键词： Electrocatalysis Rare earth phthalocyanines Graphene(Gr) Carbon nanotubes(CNTs) Composite

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Hydrocarbon Accumulation Condition and Exploration Direction in the Deepwater Area of Qiongdongnan Basin,Northern South china.Sea

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地学前缘 2009年第S1期16卷 147-148页

作者： jun xiao,hua wang,hua jiang faculty of earth resources,china university of geosciences(wuhan),wuhan 43.074,china.

The deepwater area of southern Qiongdongnan Basin is a hydrocarbon exploration frontier and mainly located on the continental slope in the northwestern South china.*** tectonic and depositional evolution is similar to the typical marginal deepwater areas abroad where oils have been *** hydrocarbon conditions in this area are as follows:(1) three sets of source rocks (including lacustrine mudstone of Eocene,coastal plain coal-bearing strata and semi-closed shallow sea mudstone of Oligocene,and marine mudstone

关键词： Qiongdongnan Basin deepwater area condition of hydrocarbon reservoir forming hydrocarbon exploration

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The energy response of LaBr_(3)(Ce),LaBr_(3)(Ce,Sr),and NaI(Tl)crystals for GECAM

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Nuclear Science and Techniques 2024年第2期35卷 110-122页

作者： Pei-Yi Feng Xi-Lei Sun Zheng-hua An Yong Deng Cheng-Er wang huang jiang jun-Jie Li Da-Li Zhang Xin-Qiao Li Shao-Lin Xiong Chao Zheng Ke Gong Sheng Yang xiao-Jing Liu Min Gao Xiang-Yang Wen Ya-Qing liu Yan-Bing Xu xiao-Yun Zhao Jia-Cong Liu Fan Zhang Hong Lu Particle and Astrophysics Center Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China Key Laboratory of Particle Astrophysics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China university of Chinese Academy of Sciences Chinese Academy of SciencesBeijing 100049China Experimental Physics Center Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China State Key Laboratory of Particle Detection and Electronics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China School of Nuclear Science and Technology University of South ChinaHengyang 421001China National Engineering Research Center for Rare earth Grirem Advanced Materials Co.Ltd.and General Research Institute for Nonferrous MetalsBeijing 100088China

The GECAM series of satellites utilizes LaBr_(3)(Ce),LaBr_(3)(Ce,Sr),and NaI(Tl)crystals as sensitive materials for gamma-ray detectors(GRDs).To investigate the nonlinearity in the detection of low-energy gamma rays and address the errors in the calibration of the E-C relationship,comprehensive tests and comparative studies of the three aforementioned crystals were conducted using Compton electrons,radioactive sources,and mono-energetic *** nonlinearity test results of the Compton electrons and X-rays demonstrated substantial differences,with all three crystals presenting a higher nonlinearity for X/-rays than for Compton *** the LaBr_(3)(Ce)and LaBr_(3)(Ce,Sr)crystals having higher absolute light yields,they exhibited a noticeable nonlinear decrease in the light yield,especially at energies below 400 *** NaI(Tl)crystal demonstrated an"excess"light output in the 6-200 keV range,reaching a maximum"excess"of 9.2%at 30 keV in the X-ray testing and up to 15.5%at 14 keV during Compton electron testing,indicating a significant advantage in the detection of low-energy gamma ***,we explored the underlying causes of the observed nonlinearity in these *** study not only elucidates the detector responses of GECAM,but also initiates a comprehensive investigation of the nonlinearity of domestically produced lanthanum bromide and sodium iodide crystals.

关键词： LaBr_(3)(Ce)detector LaBr_(3)(Ce,Sr)detector NaI(Tl)detector GECAM Energy response Light yield nonlinearity

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Bone Research 2024年第1期12卷 122-136页

作者： Nan-Yu Zou Ran Liu Mei huang Yu-Rui Jiao Jie Wei Yangzi jiang Wen-Zhen He Min huang Yi-Li Xu Ling Liu Yu-Chen Sun Mi Yang Qi Guo Yan huang Tian Su Ye xiao Wei-Shan wang Chao Zeng Guang-hua Lei Xiang-Hang Luo Chang-jun Li Department of Endocrinology Endocrinology Research CenterXiangya Hospital of Central South UniversityChangshaHunan 410008China Department of Orthopaedics Xiangya Hospital of Central South UniversityChangshaHunan 410008China Department of Epidemiology and Health Statistics Xiangya School of Public HealthCentral South UniversityChangshaChina Hunan Key Laboratory of Joint Degeneration and Injury ChangshaHunan 410008China Key Laboratory of Aging-related Bone and Joint Diseases Prevention and Treatment Ministry of EducationXiangya HospitalCentral South UniversityChangshaChina School of Biomedical Sciences Institute for Tissue Engineering and Regenerative MedicineFaculty of MedicineThe Chinese University of Hong KongHong Kong SARChina Department of Orthopaedics The First Affiliated Hospital of Shihezi UniversityShiheziXinjiangChina National Clinical Research Center for Geriatric Disorders Xiangya HospitalCentral South UniversityChangshaHunan 410008China

Skeletal stem/progenitor cell(SSPC)senescence is a major cause of decreased bone regenerative potential with aging,but the causes of SSPC senescence remain *** this study,we revealed that macrophages in calluses secrete prosenescent factors,including grancalcin(GCA),during aging,which triggers SSPC senescence and impairs fracture *** injection of human rGCA in young mice induced SSPC senescence and delayed fracture *** deletion of Gca in monocytes/macrophages was sufficient to rejuvenate fracture repair in aged mice and alleviate SSPC ***,GCA binds to the plexin-B2 receptor and activates Arg2-mediated mitochondrial dysfunction,resulting in cellular *** of Plxnb2 in SSPCs impaired fracture *** of GCA-neutralizing antibody enhanced fracture healing in aged ***,our study revealed that senescent macrophages within calluses secrete GCA to trigger SSPC secondary senescence,and GCA neutralization represents a promising therapy for nonunion or delayed union in elderly individuals.

关键词： healing union senescence

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Sedimentary Characteristics and Model of Gravity Flow Depositional System for the First Member of Upper Miocene huangliu Formation in Dongfang Area, Yinggehai Basin, Northwestern South china.Sea

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Journal of earth Science 2014年第3期25卷 506-518页

作者： Ming Sun hua wang Jihua Liao huajun Gan jun xiao Jinfeng Ren Shu'e Zhao Key Laboratory of Tectonics and Petroleum resources Ministry of Education China University of Geosciences Guangzhou Marine Geological Survey faculty of earth resources China University of Geosciences CNOOC Research Institute

The gravity flow deposit were mainly developed in the lowstand systems tract（LST） of the first member of Upper Miocene huangliu Formation（Ehl1） in Dongfang area, Yinggehai Basin, has become a valuable target for gas exploration and production. The gravity flow sedimentary characteristics of lithofacies associations, sedimentary texture, seismic facies and logging facies were described in detail on the basis of integrated analysis of cores, logging and seismic data. The sedimentary microfacies types composed of neritic sandbar, continental shelf mud, main channel, bifurcated or cross-cutting distributary channel, overspill, and natural levee are revealed under the constraint of high resolution sequence stratigraphic framework in the Ehl1. The gravity flow deposit system in the LST is divided into three evolution stages corresponding to periods of three parasequence sets. The gravity flow deposit was induced in the early LST, expanded rapidly in the middle LST and decreased slightly in the late LST. But its developing scale decreased sharply in the transgression systems tract（TST） and finally vanished in the highstand systems tract（HST）. This spatial evolution rule is constrained by the integrated function of sediments supply of the Vietnam Blue River in the LST, the development of local gradient change in sea floor（micro-topography, i.e., flexure slope break）, and the fall in relative sea level. On the basics of the deep study of the coupling relationship among the three main control factors, the sedimentary model is established as an optimal component of ＂source-channel-sink＂ for shallow marine turbidite submarine fan.

关键词： Yinggehai Basin Dongfang area the first member of Upper Miocene huangliu Formation(Ehl1) sedimentation characteristics gravity flow sedimentary model.

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Ground- and Space-Based Observation of Kordylewski Clouds

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Space(Science & Technology) 2021年第1期2021卷 299-308页

作者： Peng wang xiao-jun jiang Xi-Yun Hou Li-hua Zhang Li-Xiang jiang Jia-Qi wang Hui Zhi Zi-Long Jiao Tao Li Ming-He Liu Jian-Feng wang DFH Satellite Co. Ltd.Beijing 100094China School of Aerospace Engineering Beijing Institute of TechnologyBeijing 100081China National Astronomical Observatories Chinese Academy of SciencesBeijing 100101China School of Astronomy and Space Science University of Chinese Academy of SciencesBeijing 100101China Nanjing university Nanjing 210023China Beijing Institute of Spacecraft Environment Engineering Beijing 100094China

The ghost dust clouds in the vicinity of earth-Moon triangular libration points are known as the“Kordylewski clouds”(KDCs).Objects in the KDCs may give hints to the physical,chemical,and dynamical properties of the solar *** a result,in situ exploration of the KDCs can help us understand the evolution of our solar *** paper first summarizes the observation history of the *** on the properties of the KDCs,a ground-and space-based observation concept is proposed,using the CAST 100 platform developed by DFH and ground *** details of the concept are exploited.

关键词： ghost system details

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Upregulation of β-catenin signaling represents a single common pathway leading to the various phenotypes of spinal degeneration and pain

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Bone Research 2023年第2期11卷 316-327页

作者： Ke Lu Qingyun wang hua jiang jun Li Zhou Yao Yongcan huang Jianquan Chen Yejia Zhang Guozhi xiao Xueyu Hu Zhuojing Luo Liu Yang Liping Tong Di Chen Research Center for Computer-aided Drug Discovery Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhenChina faculty of Pharmaceutical Sciences Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhenChina Division of Spine Surgery the First Affiliated Hospital of Guangxi Medical UniversityNanningGuangxiChina Department of Orthopedic Surgery Perelman School of MedicineUniversity of PennsylvaniaPhiladelphiaPAUSA Institute of Orthopedics Xijing Hospitalthe Fourth Military Medical UniversityXi’anChina Department of Spine Surgery Peking University Shenzhen HospitalShenzhenChina Department of Clinical Medicine School of MedicineZhejiang University City CollegeHangzhouZhejiangChina Departments of Physical Medicine&Rehabilitation Perelman School of MedicineUniversity of PennsylvaniaPAUSA School of Medicine Southern University of Science and TechnologyShenzhenChina

Spine degeneration is an aging-related disease,but its molecular mechanisms remain unknown,although elevatedβ-catenin signaling has been reported to be involved in intervertebral disc ***,we determined the role ofβ-catenin signaling in spinal degeneration and in the homeostasis of the functional spinal unit(FSU),which includes the intervertebral disc,vertebra and facet joint and is the smallest physiological motion unit of the *** showed that pain sensitivity in patients with spinal degeneration is highly correlated withβ-catenin protein *** then generated a mouse model of spinal degeneration by transgenic expression of constitutively activeβ-catenin in Col2^(+) *** found thatβ-catenin-TCF7 activated the transcription of CCL2,a known critical factor in osteoarthritic *** a lumbar spine instability model,we showed that aβ-catenin inhibitor relieved low back *** study indicates thatβ-catenin plays a critical role in maintaining spine tissue homeostasis,its abnormal upregulation leads to severe spinal degeneration,and its targeting could be an avenue to treat this condition.

关键词： degeneration smallest homeostasis

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CEPC Technical Design Report

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Radiation Detection Technology and Methods 2024年第1期8卷 I0003-I0016,1-1091页

作者： Waleed Abdallah Tiago Carlos Adorno de Freitas Konstantin Afanaciev Shakeel Ahmad Ijaz Ahmed xiaocong Ai Abid Aleem Wolfgang Altmannshofer Fabio Alves Weiming An Rui An Daniele Paolo Anderle Stefan Antusch Yasuo Arai Andrej Arbuzov Abdesslam Arhrib Mustafa Ashry Sha Bai Yu Bai Yang Bai Vipul Bairathi Csaba Balazs Philip Bambade Yong Ban Tripamo Bandyopadhyay Shou-Shan Bao Desmond P.Barber Ayse Bat Varvara Batozskaya Subash Chandra Behera Alexander Belyaev Michele Bertucci xiao-jun Bi Yuanjie Bi Tianjian Bian Fabrizio Bianchi Thomas Biekotter Michela Biglietti Shalva Bilanishvili Deng Binglin Denis Bodrov Anton Bogomyagkov Serge Bondarenko Stewart Boogert Maarten Boonekamp Marcello Borri Angelo Bosotti Vincent Boudry Mohammed Boukidi Igor Boyko Ivanka Bozovic Giuseppe Bozzi Jean-Claude Brient Anastasiia Budzinskaya Masroor Bukhari Vladimir Bytev Giacomo Cacciapaglia hua Cai Wenyong Cai Wujun Cai Yijian Cai Yizhou Cai Yuchen Cai Haiying Cai huacheng Cai Lorenzo Calibbi junsong Cang Guofu Cao Jianshe Cao Antoine Chance Xuejun Chang Yue Chang Zhe Chang Xinyuan Chang Wei Chao Auttakit Chatrabhuti Yimin Che Yuzhi Che Bin Chen Danping Chen Fuqing Chen Fusan Chen Gang Chen Guoming Chen hua-Xing Chen Huirun Chen Jinhui Chen Ji-Yuan Chen Kai Chen Mali Chen Mingjun Chen Mingshui Chen Ning Chen Shanhong Chen Shanzhen Chen Shao-Long Chen Shaomin Chen Shiqiang Chen Tianlu Chen Wei Chen Xiang Chen xiaoyu Chen Xin Chen Xun Chen Xurong Chen Ye Chen Ying Chen Yukai Chen Zelin Chen Zilin Chen Gang Chen Boping Chen Chunhui Chen Hok Chuen Cheng huajie Cheng Shan Cheng Tongguang Cheng Yunlong Chi Pietro Chimenti Wen Han Chiu Guk Cho Ming-Chung Chu xiaotong Chu Ziliang Chu Guglielmo Coloretti Andreas Crivellin Hanhua Cui xiaohao Cui Zhaoyuan Cui Brunella D'Anzi Ling-Yun Dai Xinchen Dai Xuwen Dai Antonio De Maria Nicola De Filippis Christophe De La Taille Francesca De Mori Chiara De Sio Elisa Del Core Shuangxue Deng Wei-Tian Deng Zhi Deng Ziyan Deng Bhupal Dev Tang Dewen Biagio Di Micco Ran Ding Siqin Dingl Yadong Ding Haiyi Dong Jianin AGH university of Science and Technology Faculty of Physics and Applied Computer ScienceKrakow Anhui university HefeiAnhui Applied Physics Department Federal Urdu University of ArtsScience and TechnologyIslamabad Banaras Hindu university Institute of ScienceVaranasi Bandirma Onyedi Eylul university Bandirma Beihang university Beijing Beijing Computational Science Research Center Beijing Beijing Conveyi LTD Beijing Beijing Glass Research Institute Co. LtdBeijing Beijing Institute of Technology Beijing Beijing Normal university Beijing Brown university ProvidenceRI Budker Institute of Nuclear Physics Novosibirsk Cadi Ayyad university Laboratory of Fundamental and Applied PhysicsPolydisciplinary FacultyMarrakech Cairo university Giza Center for Theory and Computation National Tsing Hua UniversityHsinchu Central china.Normal university WuhanHubei Central South university ChangshaHunan Centro de Fisica Teorica de Particulas Universidade Tecnica de LisboaLisboa Chengdu KaitengSifang Digital Radio&TV Equipment Co. LtdChengduSichuan china.academy of engineering physics MianyangSichuan china.building materials academy Beijing china.Center of Advanced Science and Technology Beijing china.Institute of Atomic Energy Beijing china.Jiliang university HangzhouZhejiang china.Nuclear Instrument CO. LTDBeijing china university of geosciences Beijing china university of geosciences WuhanHubei china.university of Mining and Technology XuzhouJiangsu china.West Normal university NanchongSichuan Chongqing university Department of PhysicsChongqing Chulalongkorn university Bangkok City university of Hong Kong Department of PhysicsHong Kong Cockcroft Institute Daresbury Cornell university IthacaNY CPPM(AMU/IPhU&CNRS/INP) Marseille Dalian Minzu university DalianLiaoning Dalian university of Technology Department of PhysicsDalian Deutsches Elektronen-Synchrotron DESY Hamburg Dzhelepov Laboratory of Nuclear Problems of Joint Institute for Nuclear Research(DLNP JINR) Dubna East china.university Of Science And Technol

The Circular Electron Positron Collider(CEPC)is a large scientific project initiated and hosted by china.fostered through extensive collaboration with international *** complex comprises four accelerators:a 30 GeV Linac,a 1.1 GeV Damping Ring,a Booster capable of achieving energies up to 180 GeV,and a Collider operating at varying energy modes(Z,W,H,and tt).The Linac and Damping Ring are situated on the surface,while the subterranean Booster and Collider are housed in a 100 km circumference underground tunnel,strategically accommodating future expansion with provisions for a potential Super Proton Proton Collider(SPPC).The CEPC primarily serves as a Higgs *** its baseline design with synchrotron radiation(SR)power of 30 MW per beam,it can achieve a luminosity of 5×10^(34)cm^(-2)s^(-1)per interaction point(IP),resulting in an integrated luminosity of 13 ab^(-1)for two IPs over a decade,producing 2.6 million Higgs *** the SR power to 50 MW per beam expands the CEPC's capability to generate 4.3 million Higgs bosons,facilitating precise measurements of Higgs coupling at sub-percent levels,exceeding the precision expected from the HL-LHC by an order of *** Technical Design Report(TDR)follows the Preliminary Conceptual Design Report(Pre-CDR,2015)and the Conceptual Design Report(CDR,2018),comprehensively detailing the machine's layout,performance metrics,physical design and analysis,technical systems design,R&D and prototyping efforts,and associated civil engineering ***,it includes a cost estimate and a preliminary construction timeline,establishing a framework for forthcoming engineering design phase and site selection *** is anticipated to begin around 2027-2028,pending government approval,with an estimated duration of 8 *** commencement of experiments and data collection could potentially be initiated in the mid-2030s.

关键词： initiated exceeding precise

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Ore-forming environment of Pb−Zn mineralization related to granite porphyry at huangshaping skarn deposit,Nanling Range,South china

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Transactions of Nonferrous Metals Society of china 2022年第9期32卷 3015-3035页

作者： Da-peng ZHU huan LI Wei-cheng jiang Chong wang xiao-jun HU hua KONG Key Laboratory of Metallogenic Prediction of Nonferrous Metals and Geological Environment Monitoring Ministry of EducationSchool of Geosciences and Info-PhysicsCentral South UniversityChangsha 410083China Department of earth and Environmental Sciences Macquarie UniversityNSW2109Australia

Multiple metallogenic types(skarn-type and vein-type)related to hypabyssal granites are found at the huangshaping polymetallic deposit in the Nanling Range,South *** constrain the crystallization and mineralization processes of skarn formation,three generations of magnetite and pyrrhotite from the hydrous silicate stage,oxide stage,early quartz–sulfide stage,and late quartz–sulfide stage were *** geochemical compositions of magnetite and pyrrhotite were obtained by electron probe microanalyzer(EPMA)and in-situ ablation-inductively coupled plasma-mass spectrometry(LA‒ICP‒MS).The results show that there may be silicate inclusions in magnetite and interaction of wall rock occurred in the mineralization *** geochemical trends recorded in pyrrhotite show the influence of limestone during the crystallization of *** re-equilibration temperatures of Po I,Po II,and Po III are 420.46,380.45,and 341.81°C,respectively,which suggests a continuous evolution following the high-temperature W–Sn mineralized *** content change of Ni and V reflects a gradual decrease of oxygen fugacity from Mag I to Mag III,while the sulfur fugacity calculated from pyrrhotite gradually *** continuous skarn mineralization evolution process helps us to better understand the change of metallogenic environment in the retrograde stage of the huangshaping deposit.

关键词： trace elements magnetite pyrrhotite geochemistry

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北部湾盆地涠西南凹陷W61潜山油气成藏条件分析

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新疆石油学院学报 2003年第4期15卷 30-33,37页

作者：肖军王华马丽娟甘华军刘君荣陈亮中国地质大学资源学院湖北武汉430074

W61潜山区块已发现了岩性—古潜山风化带叠合型、岩性与古潜山风化带分离型和单纯的古潜山风化带型三类油气藏。W61潜山由于处在构造高部位 ,受多期构造运动影响 ,断层及不整合面发育 ,具有良好的油气运移通道 ,其西南生油洼陷内的流沙... 详细信息

W61潜山区块已发现了岩性—古潜山风化带叠合型、岩性与古潜山风化带分离型和单纯的古潜山风化带型三类油气藏。W61潜山由于处在构造高部位 ,受多期构造运动影响 ,断层及不整合面发育 ,具有良好的油气运移通道 ,其西南生油洼陷内的流沙港组烃源岩生成的油气多沿此运移至潜山成藏。石炭系碳酸盐岩风化壳及其上覆的碎屑岩为主要的储集层 ,储集空间主要为裂缝、溶孔、溶洞及原、次生孔隙。区域盖层为流沙港组和角尾组厚层泥、页岩。在本区 ,古潜山风化带。

关键词：涠西南凹陷石炭系潜山油气藏类型

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