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Energy Geoscience 2024年第2期5卷 1-13页

作者： Herong Zheng jun luo Petroleum Exploration and Production Research Institute SINOPECBeijing 102206China

Deep geothermal resources in the Fujian-Guangdong-Hainan region,China,offer significant potential for sustainable *** diverse igneous rock formations along the southeast coast present intricate geological challenges that impede exploration and evaluation *** this study,we address critical concerns related to the Fujian-Guangdong-Hainan region's deep geothermal resources,encompassing heat source composition,formation conditions,strategic favorable areas,and exploration *** methods involve the analysis of regional geothermal reservoirs and cap *** findings include:the primary heat sources in the Fujian-Guangdong-Hainan region consist of the radioactive heat generation from granites in the crust,heat conduction in the mantle,and,in specific areas like Yangjiang and Shantou,melts within the middle and lower crust;the deep,high-temperature geothermal resources in the region predominantly reside in basins'depressed *** areas are characterized by the confluence of triple heat sources:heat from the Earth's crust,mantle,and other supplementary sources;our analysis led to the identification of three strategic areas favorable for deep geothermal resources in the Fujian-Guangdong-Hainan *** are the Beibu Gulf Basin's continental area,the Yuezhong Depression,and the Fuzhou-Zhangzhou area.

关键词： Deep geothermal resources Geology of geothermal energy Strategic selection

Adaptive coupled-sliding-variable-based finite-time control of composite formation for multi-robot systems

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Science China(Information Sciences) 2024年第10期67卷 244-260页

作者： Xinru MA Hengyu LI jun LIU Yueying WANG Shaorong XIE jun luo School of Mechatronic Engineering and Automation Shanghai University School of Mathematics and Computer Application Technology Jining University School of Computer Science Shanghai University College of Mechanical and Vehicle Engineering Chongqing University

This paper focuses on the finite-time control(FTC) of the composite formation consensus(CFC)problems for multi-robot systems(MRSs). The CFC problems are firstly proposed for MRSs under the complex network topology of cooperative or cooperative-competitive networks. Regarding the problems of FTC and CFC on multiple Lagrange systems(MLSs), coupled sliding variables are introduced to deal with the robustness and consistent convergence. Then, the adaptive finite-time protocols are given based on the displacement approaches. With the premised FTC, tender-tracking methods are further developed for the problems of tracking information disparity. Stability analyses of those MLSs mentioned above are clarified with Lyapunov candidates considering the coupled sliding vectors, which provide new verification for tender-tracking systems. Under the given coupled-sliding-variable-based finite-time protocols, MLSs distributively adjust the local formation error to achieve global CFC and perform uniform convergence in time-varying tracking. Finally, simulation experiments are conducted while providing practical solutions for the theoretical results.

关键词： composite formation time-vary tracking information disparity tender-tracking finite-time control nonlinear robots complex networks symmetry consensus

Cl^(-)ions accelerating interface charge transfer in a Si/In_(2)S_(3) Faradaic junction photocathode for solar seawater splitting

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Science China Chemistry 2024年第9期67卷 2923-2929页

作者： jun luo Ruotong Bao Hongzheng Dong Ye Fu Dongjian Jiang Bo Wang Yuzhan Zheng Qiong Wang Wenjun luo Zhigang Zou Eco-materials and Renewable Energy Research Center(ERERC) Jiangsu Key Laboratory for Nano TechnologyNational Laboratory of Solid State MicrostructuresCollege of Engineering and Applied SciencesNanjing UniversityNanjing 210093China National Laboratory of Solid State Microstructures and Department of Physics Nanjing UniversityNanjing 210093China

Photoelectrocatalytic seawater splitting is a promising low-cost method to produce green hydrogen in a large *** effects of Cl^(-)ions in seawater on the performance of a photoanode have been reported in previous ***,few researches have been done on the roles of Cl^(-)ions in a ***,for the first time,we find that Cl^(-)ions in the electrolyte improve the photocurrent of a Si/In_(2)S_(3) photocathode by 50% at-0.6 V_(RHE).An in-situ X-ray photoelectron spectroscopy(XPS)characterization combined with the time-of-flight secondary-ion mass spectrometry by simulating photoelectrochemical conditions was used to investigate the interface charge transfer *** results suggest that there is an In_(2)^(+3)S_(3-x)(OH)_(2x)layer on the surface of In_(2)S_(3) in the phosphate buffer solution(PBS)electrolyte,which plays a role as an interface charge transfer mediator in the Si/In_(2)S_(3) *** In_(2)^(+3)S_(3-x)(OH)_(2x)surface layer becomes In_(2)^(+3)S_(3-x)(Cl)_(2x)in the PBS electrolyte with NaCl and accelerates the charge transfer rate at the In_(2)S_(3)/electrolyte *** results offer a new concept of regulating interface charge transfer mediator to enhance the performance of photoelectrocatalytic seawater splitting for hydrogen production.

关键词： solar hydrogen production interface charge transfer mechanism coupled electron and ion transfer in-situ XPS characterization In_(2)^(+3)S_(3-x)(OH)_(2x)surface layer

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BaCe_(0.8)Fe_(0.1)Ni_(0.1)O_(3−δ)-impregnated Ni-GDC by phase-inversion as an anode of solid oxide fuel cells with on-cell dry methane reforming

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Journal of Advanced Ceramics 2024年第6期13卷 834-841页

作者： Yanya Liu jun luo Cheng Li Bo Liu Dong Yan Jian Li Lichao Jia School of Materials Science and Engineering State Key Laboratory of Materials Processing and Die&Mould TechnologyHuazhong University of Science and TechnologyWuhan 430074China

BaCe_(0.8)Fe_(0.1)Ni_(0.1)O_(3−δ)(BCFN)in a perovskite structure is impregnated consecutively by BCFN solution and BCFN suspension into a phase-inversion prepared NiO–Gd_(0.1)Ce_(0.9)O_(2−δ)(GDC)scaffold as an anode for solid oxide fuel cells(SOFCs)with on-cell dry reforming of methane(DRM).The whole pore surface of the scaffold is covered by small BCFN particles formed by BCFN solution impregnation;the large pores near the scaffold surface are filled by BCFN aerogels with a high specific surface area produced by BCFN suspension impregnation,which act as a catalytic layer for on-cell *** reduction,the anode consists of a Ni–GDC scaffold and BCFN particles with exsolved FeNi3 *** BCFN-impregnated Ni–GDC anode has higher electrical conductivity,electrochemical activity,and resistance to carbon deposition,with which the cell shows maximum power densities between 1.44 and 0.92 W·cm^(−2) when using H_(2) and between 1.09 and 0.50 W·cm^(−2) when using CO_(2)–CH_(4) at temperatures ranging from 750 to 600℃.A stable performance at 400 mA·cm^(−2) and 700℃is achieved using 45%CO_(2)–45%CH_(4)–10%N_(2) for more than 400 h without carbon deposition,benefiting from the impregnated BCFN aerogel with a high specific surface area and water adsorbability.

关键词： aerogel solid oxide fuel cells(SOFCs) phase-inversion dry reforming of methane(DRM) carbon resistance

Structural engineering of hard carbon through spark plasma sintering for enhanced sodium-ion storage

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Rare Metals 2024年第9期43卷 4274-4285页

作者： Hao-Ming Xiao Heng Zheng Ping Yuan jun-Hui luo Lin-Lin Shen Jie-Feng Tan Xian-You luo De Li Yong Chen Guangdong Key Laboratory for Hydrogen Energy Technologies School of Materials Science and Hydrogen EnergyFoshan UniversityFoshan 528000China State Key Laboratory of Marine Resource Utilization in South China Sea Hainan Provincial Key Laboratory of Research on Utilization of Si-Zr-Ti ResourcesHainan UniversityHaikou 570228China

Hard carbon(HC)has emerged as one of the superior anode materials for sodium-ion batteries(SIBs),with its electrochemical performance significantly influenced by the presence of oxygen functional groups and its closed pore ***,current research on the structural adjustment of these oxygen functional groups and the closed pore architecture within HC remains ***,energy-efficient and contamination-free spark plasma sintering technology was employed to tune the structure of coconut-shell HC,resulting in significant adjustments to the content of carboxyl(decreasing from 5.71 at%to 2.12 at%)and hydroxyl groups(decreasing from 7.73 at%to 6.26 at%).Crucially,these modifications reduced the irreversible reaction of oxygen functional groups with Na^(+).Simultaneously,a substantial number of closed pores with an average diameter of 1.22 nm were generated within the HC,offering an ideal environment for efficient Na^(+)*** structural changes resulted in a remarkable improvement in the electrochemical performance of the modified *** reversible specific capacity of the modified HC surged from 73.89 mAh·g^(-1)to an impressive 251.97 m Ah·g^(-1)at a current density of 50 mA·g^(-1).Even at 400 mA·g^(-1),the reversible specific capacity increased significantly from 14.55 to 85.44 mAh·g^(-1).Hence,this study provides a novel perspective for designing tailored HC materials with the potential to develop high-performance SIBs.

关键词： Hard carbon Spark plasma sintering Sodiumion batteries Closed pores Oxygen functional groups

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Construction of daily precipitation series and the observational characteristics of extreme precipitation in Tianjin,China during 1888-2022

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Advances in Climate Change Research 2024年第1期15卷 52-61页

作者： Peng SI Qing-Xiang LI Xiao-Yang CHEN Min WANG Chuan-jun luo Tianjin Meteorological Information Center Tianjin Meteorological BureauTianjin 300074China Research Centerfor Ecology and Environment of Central Asia Chinese Academy of SciencesWulumuqi 830011China School of Atmospheric Sciences Sun Yat-sen UniversityZhuhai 528478China Key Laboratory of Tropical Amosphere-Ocean System Ministry of EducationZhuhai 528478China Shaoguan Meteorological Service Shaoguan 512028China

Given the difficulties in rescuing and ensuring the quality of long-term climate data,current studies on century-scale climate change are usually limited to annual and monthly data,resulting in the poor detection of extreme climate events and their changes before *** this study,we reconstructed a daily precipitation series for Tianjin from 15 September 1887 to 31 December 2022 on the basis of the most comprehensive daily precipitation records collected from the Tianjin Meteorological Archive,China,and in reference to the precipitation analysis results based on the datasets developed by the Climatic Research Unit Time-Series version 4.06,Global Precipitation Climatology Centre and University of Delaware along with the application of various homogenisation methods for climate *** approach provides a complete and reliable century-long daily precipitation series for the study of regional or local extreme weather and climate *** reconstructed daily dataset reveals that the annual precipitation amount and R95 intensity in Tianjin during 1888-2022 lack significant trends and have values of 0.74±6.99 and-1.84±3.22 mm per decade,*** the annual and seasonal scales,the precipitation amount and R95 intensity,particularly those in autumn,have increased since the latter half of the 20th century relative to those in ***,the increase in precipitation amount and R95 intensity is relatively limited compared with that in atmospheric water vapour content due to surface warming,indicating the highly sensitive response of extreme precipitation events to *** addition,the estimates for the return periods of 5,10,20,50 and 100 years covering 1888-2022,1888-1950 and 1951-2022 depict that the intensity of heavy rain and above magnitude was highest in 1888-1950 and decreased in 1951-2022.

关键词： Over a century-long timescale Daily precipitation series Extreme precipitation Return period

Endoplasmic reticulum stress improved chicken tenderness,promoted apoptosis and autophagy during postmortem ageing

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Food Science and Human Wellness 2024年第4期13卷 2141-2151页

作者： Yuwei Chai Lin Chen Shuya Xiang Linxuan Wu Xuebo Liu jun luo Xianchao Feng College of Food Science and Engineering Northwest A&F UniversityYangling 712100China College of Animal Science and Technology Northwest A&F UniversityYangling 712100China

In this study,endoplasmic reticulum(ER)stress inducer tunicamycin(TM)and inhibitor 4-phenylbutyric acid(4-PBA)were used to treat postmortem chicken breast muscle to investigate changes in tenderness and effects on apoptosis and autophagy during 5 days ***-induced ER stress reduced shear force,enhanced myofibril fragmentation index(MFI),disrupted myofibril structure,increased desmin degradation,and activatedμ-calpain and *** addition,TM-induced ER stress increased the expression of Bax,Bim,and cytochrome c,and decreased the expression of Bcl-x ***,TM-induced ER stress improved the conversion of LC3I to LC3II,raised the expression of Beclin-1,and decreased the expression of p62,PI3K,and m *** opposite results were observed after 4-PBA *** results suggested that ER stress could improve chicken tenderness,promote apoptosis and autophagy during chicken postmortem ageing.

关键词： Endoplasmic reticulum stress Tenderness Apoptosis Autophagy Chicken

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Au nanoclusters anchored on TiO_(2) nanosheets for high-efficiency electroreduction of nitrate to ammonia

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Nano Research 2024年第3期17卷 1209-1216页

作者： Miaosen Yang Tianran Wei Jia He Qian Liu Ligang Feng Hongyi Li jun luo Xijun Liu School of Chemical Engineering Northeast Electric Power UniversityJilin 132012China Nanchang Institute of Technology Nanchang 330044China State Key Laboratory of Chemistry and Utilization of Carbon Based Energy Resources College of ChemistryXinjiang UniversityUrumqi 830017China State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures Guangxi Key Laboratory of Processing for Non-Ferrous Metals and Featured MaterialsSchool of ResourcesEnvironment and MaterialsGuangxi UniversityNanning 530004China Institute for New Energy Materials and Low-Carbon Technologies School of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China Institute for Advanced Study Chengdu UniversityChengdu 610106China School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhou 225002China Guangzhou Panyu Polytechnic Guangzhou 511483China ShenSi Lab Shenzhen Institute for Advanced StudyUniversity of Electronic Science and Technology of ChinaLonghua DistrictShenzhen 518110China

Electrocatalytic nitrate reduction reaction(NO_(3)RR)offers a unique rationale for green NH_(3) synthesis,yet the lack of high-efficiency NO_(3)RR catalysts remains a great *** this work,we show that Au nanoclusters anchored on TiO_(2) nanosheets can efficiently catalyze the conversion of NO_(3)RR-to-NH_(3) under ambient conditions,achieving a maximal Faradic efficiency of 91%,a peak yield rate of 1923μg·h^(-1)·mgcat.-1,and high durability over 10 consecutive cycles,all of which are comparable to the recently reported metrics(including transition metal and noble metal-based catalysts)and exceed those of pristine TiO_(2).Moreover,a galvanic Zn-nitrate battery using the catalyst as the cathode was proposed,which shows a power density of 3.62 mW·cm^(-2) and a yield rate of 452μg·h^(-1)·mgcat.-*** simulations further indicate that the atomically dispersed Au clusters can promote the adsorption and activation of NO_(3)-species,and reduce the NO_(3)RR-to-NH_(3) barrier,thus leading to an accelerated cathodic *** work highlights the importance of metal clusters for the NH_(3) electrosynthesis and nitrate removal.

关键词： NH3 electrosynthesis Zn-nitrate battery Au nanoclusters nitrate reduction reaction(NRR) TiO_(2)nanosheets

Adaptive Memetic Algorithm with Dual-Level Local Search for Cooperative Route Planning of Multi-Robot Surveillance Systems

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Complex System Modeling and Simulation 2024年第2期4卷 210-221页

作者： Hao Cheng Jin Yi Wei Xia Huayan Pu jun luo the State Key Laboratory of Mechanical Transmission for Advanced Equipment Chongqing UniversityChongqing 400044China the Department of Electronics Information and BioengineeringPolitecnico di MilanoMilano 20133Italy

The heightened autonomy and robust adaptability inherent in a multi-robot system have proven pivotal in disaster search and rescue,agricultural irrigation,and environmental *** study addresses the coordination of multiple robots for the surveillance of various key target positions within an *** involves the allocation of target positions among robots and the concurrent planning of routes for each *** tackle these challenges,we formulate a unified optimization model addressing both target allocation and route ***,we introduce an adaptive memetic algorithm featuring dual-level local search *** algorithm operates independently among and within robots to effectively solve the optimization problem associated with *** proposed method’s efficacy is substantiated through comparative numerical experiments and simulated experiments involving diverse scales of robot teams and different target positions.

关键词： multi-robot system surveillance memetic algorithm

Dealloyed TiCuMn efficiently catalyze the NO reduction and Zn-NO batteries

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Frontiers of Chemical Science and Engineering 2024年第9期18卷 51-59页

作者： Lang Zhang Tong Hou Weijia Liu Yeyu Wu Tianran Wei junyang Ding Qian Liu jun luo Xijun Liu State Key Laboratory of Featured Metal Materials and Life-Cycle Safety for Composite Structures MOE Key Laboratory of New Processing Technology for Nonferrous Metals and MaterialsSchool of ResourcesEnvironment and MaterialsGuangxi UniversityNanning 530004China Education Department of Guangxi Zhuang Autonomous Region Key Laboratory of Applied Analytical ChemistryGuangxi Collaborative Innovation Center for Chemistry and Engineering of Forest ProductsGuangxi Key Laboratory of Chemistry and Engineering of Forest ProductsKey Laboratory of Chemistry and Engineering of Forest ProductsState Ethnic Affairs CommissionSchool of Chemistry and Chemical EngineeringGuangxi Minzu UniversityNanning 530006China Institute for New Energy Materials&Low-Carbon Technologies School of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China Institute for Advanced Study Chengdu UniversityChengdu 610106China ShenSi Lab Shenzhen Institute for Advanced StudyUniversity of Electronic Science and Technology of ChinaShenzhen 518110China

Electrocatalytic NO reduction reaction offers a sustainable route to achieving environmental protection and NH3 production targets as *** this work,a class of dealloyed Ti_(60)Cu_(33)Mn_(7)ribbons with enough nanoparticles for the high-efficient NO reduction reaction to NH_(3)is fabricated,reaching an excellent Faradaic efficiency of 93.2%at–0.5 V vs reversible hydrogen electrode and a high NH3 synthesis rate of 717.4μmol·h^(-1)·mgcat.-1 at–0.6 V vs reversible hydrogen *** formed nanoparticles on the surface of the catalyst could facilitate the exposure of active sites and the transportation of various reactive ions and ***,the Mn content in the TiCuMn ribbons modulates the chemical and physical properties of its surface,such as modifying the electronic structure of the Cu species,optimizing the adsorption energy of N^(*)atoms,decreasing the strength of the NO adsorption,and eliminating the thermodynamic energy barrier,thus improving the NO reduction reaction catalytic ***,a Zn-NO battery was fabricated using the catalyst and Zn plates,generating an NH3 yield of 129.1µmol·h^(-1)·cm^(-2)while offering a peak power density of 1.45 mW·cm^(-2).

关键词： nitric oxide reduction NH3 electrosynthesis TiCuMn alloy Mn modulation Zn-NO battery