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High-performance of sodium carboxylate-derived materials for electrochemical energy storage

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Science China Materials 2018年第5期61卷 707-718页

作者： Yong Xu1 jun chen1 Caijian Zhu1 Pengwei Zhang1 Guoxiang Jiang1 Chunxiang Wang1 Qian Zhang1 Nengwen Ding1 Yaxiang Huang2 Shengwen Zhong1 School of Materials Science and Engineering Key Laboratory of power battery and materials Jiangxi University of Science and Technology Ganzhou 341000 China Guangdong Jiana Energy Technology Co Ltd Guangzhou 511495 China

Four types of sustainable sodium carboxylate- derived materials are investigated as novel electrodes with high performance for lithium-ion batteries. Benefiting from the porous morphology provided by their intermolecular in- teractions, increasing capacity, excellent cycle stability and superior rate performance are observed for the sodium car- boxylate-derived materials. The sodium oxalate （SO） electro- des displayed an increasing discharging capacity at a current density of 50 mA g-1 with maximum values of 242.9 mA h g-1 for SO-631 and 373.9 mA h g-1 for SO-541 during the 100th cycle. In addition, the SO-541, SC-541 （sodium citrate）, ST- 541 （sodium tartrate） and SP-541 （sodium pyromellitate） electrode materials displayed high initial capacities of 619.6-392.3, 403.7 and 278.1 mA h g-1, respectively, with capacity retentions of 179%, 148%, 173% and 108%, respectively, after 200 cycles at 50 mA g-1. Even at a high current density of 2,000 mA g-1, the capacities remain 157.6, 131.3, 146.6 and 137.0mAhg-1, respectively. With these superior electro- chemical properties, the sodium carboxylate-derived materials could be considered as promising organic electrode materials for large-scale sustainable lithium-ion batteries.

关键词： sodium carboxylate lithium-ion batteries organicelectrode electrochemical performance green and sustainable

集胞藻PCC 6803中丝氨酸/苏氨酸激酶SpkC对高温胁迫的响应

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微生物学报 2018年第10期58卷 1732-1742页

作者：赵佳琳陈军崔玉琳于淑贤陈高秦松中国科学院烟台海岸带研究所山东烟台264003 中国科学院大学北京100049 山东省农业科学院生物技术研究中心山东济南250100 山东省作物遗传改良与生态生理重点实验室山东济南250100

丝氨酸/苏氨酸激酶是蓝藻感知和转导外界刺激的重要元件,但至今蓝藻中很多丝氨酸/苏氨酸激酶的功能尚属未知。【目的】研究集胞藻PCC6803中的丝氨酸/苏氨酸激酶Spk C是否参与对高温胁迫的响应。【方法】本研究采用同源重组的方法构建sp... 详细信息

丝氨酸/苏氨酸激酶是蓝藻感知和转导外界刺激的重要元件,但至今蓝藻中很多丝氨酸/苏氨酸激酶的功能尚属未知。【目的】研究集胞藻PCC6803中的丝氨酸/苏氨酸激酶Spk C是否参与对高温胁迫的响应。【方法】本研究采用同源重组的方法构建spC基因完全敲除突变株,检测突变株与野生株在高温胁迫下的生长状况、色素组成,并对高温胁迫下叶绿素荧光参数差异进行分析,比较光合系统Ⅱ活性差异。此外,通过测定生长速率来判断高温胁迫后藻株的恢复情况。【结果】经过42℃高温胁迫后,与野生株相比,突变株ΔspkC生长减缓,光合色素(叶绿素、类胡萝卜素和藻胆色素)的含量降低;45℃高温胁迫下突变株ΔspkC的光合系统Ⅱ活性下降幅度更大;经过5 d 42℃高温处理后,突变株生长几乎停滞,存活率较野生株明显降低。【结论】集胞藻PCC 6803中spkC基因的缺失导致突变株对高温胁迫响应出现缺陷,提示丝氨酸/苏氨酸激酶SpkC参与响应高温胁迫。

关键词：集胞藻PCC 6803 丝氨酸/苏氨酸激酶SpkC 高温胁迫

A Review of Contact Electrification at Diversified Interfaces and Related Applications on Triboelectric Nanogenerator

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Nano-Micro Letters 2024年第1期16卷 106-130页

作者： jun Hu Mitsumasa Iwamoto Xiangyu chen CAS Center for Excellence in Nanoscience Beijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 100083People’s Republic of China School of Nanoscience and Engineering University of Chinese Academy of SciencesBeijing 100049People’s Republic of China Department of Physical Electronics Tokyo Institute of Technology2‑12‑1 S3‑33 O‑OkayamaMeguro‑KuTokyo 152‑8552Japan

The triboelectric nanogenerator(TENG)can effectively collect energy based on contact electrification(CE)at diverse interfaces,including solid–solid,liquid–solid,liquid–liquid,gas–solid,and gas–*** enables energy harvesting from sources such as water,wind,and *** this review,we provide an overview of the coexistence of electron and ion transfer in the CE *** elucidate the diverse dominant mechanisms observed at different interfaces and emphasize the interconnectedness and complementary nature of interface *** review also offers a comprehensive summary of the factors influencing charge transfer and the advancements in interfacial modification ***,we highlight the wide range of applications stemming from the distinctive characteristics of charge transfer at various ***,this review elucidates the future opportunities and challenges that interface CE may *** anticipate that this review can offer valuable insights for future research on interface CE and facilitate the continued development and industrialization of TENG.

关键词： Contact electrification Interfaces Triboelectric nanogenerators Diversified applications

Vision-based survey method for extraordinary loads on buildings

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Frontiers of Structural and Civil Engineering 2024年第6期18卷 815-831页

作者： Yang LI jun chen Pengcheng WANG College of Civil Engineering Tongji UniversityShanghai 200092China China United Engineering Co.Ltd. Hangzhou 310052China State Key Laboratory of Disaster Reduction in Civil Engineering Tongji UniversityShanghai 200092China Shanghai Key Laboratory of Engineering Structure Safety Shanghai Research Institute of Building Sciences Co.Ltd.Shanghai 200032China

The statistical modeling of extraordinary loads on buildings has been stagnant for decades due to the laborious and error-prone nature of existing survey methods,such as questionnaires and verbal *** study proposes a new vision-based survey method for collecting extraordinary load data by automatically analyzing surveillance *** this purpose,a crowd head tracking framework is developed that integrates crowd head detection and reidentification models based on convolutional neural networks to obtain head trajectories of the crowd in the survey *** crowd head trajectories are then analyzed to extract crowd quantity and velocities,which are the essential factors for extraordinary *** survey areas with frequent crowd movements during temporary events,the equivalent dynamic load factor can be further estimated using crowd velocity to consider dynamic effects.A crowd quantity investigation experiment and a crowd walking experiment are conducted to validate the proposed survey *** experimental results prove that the proposed survey method is effective and accurate in collecting load data and reasonable in considering dynamic effects during extraordinary *** proposed survey method is easy to deploy and has the potential to collect substantial and reliable extraordinary load data for determining design load on buildings.

关键词： load survey extraordinary load live load object detection multiple-object tracking

Cybersecurity Landscape on Remote State Estimation:A Comprehensive Review

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IEEE/CAA Journal of Automatica Sinica 2024年第4期11卷 851-865页

作者： Jing Zhou jun Shang Tongwen chen the Department of Electrical and Computer Engineering University of AlbertaEdmonton AB T6G 1H9Canada the Department of Control Science and Engineering and Shanghai Research Institute for Intelligent Autonomous Systems Tongji UniversityShanghai 200092China

Cyber-physical systems(CPSs)have emerged as an essential area of research in the last decade,providing a new paradigm for the integration of computational and physical units in modern control *** state estimation(RSE)is an indispensable functional module of ***,it has been demonstrated that malicious agents can manipulate data packets transmitted through unreliable channels of RSE,leading to severe estimation performance *** paper aims to present an overview of recent advances in cyber-attacks and defensive countermeasures,with a specific focus on integrity attacks against ***,two representative frameworks for the synthesis of optimal deception attacks with various performance metrics and stealthiness constraints are discussed,which provide a deeper insight into the vulnerabilities of ***,a detailed review of typical attack detection and resilient estimation algorithms is included,illustrating the latest defensive measures safeguarding RSE from ***,some prevalent attacks impairing the confidentiality and data availability of RSE are examined from both attackers'and defenders'***,several challenges and open problems are presented to inspire further exploration and future research in this field.

关键词： Cyber-attacks Kalman filtering remote state estimation unreliable transmission channels

Volume of fluid simulation of single argon bubble dynamics in liquid steel under RH vacuum conditions

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Journal of Iron and Steel Research International 2024年第4期31卷 828-837页

作者： Gu-jun chen Sheng-ping He College of Materials Science and Engineering Yangtze Normal UniversityChongqing 400044China College of Materials Science and Engineering Chongqing UniversityChongqing 400044China

Single argon bubble dynamics in liquid steel under Ruhrstahl-Heraeus(RH)vacuum conditions were simulated using the volume of fluid method,and the ideal gas law was used to consider bubble growth due to heat transfer and pressure *** simulation with a constant bubble density was also performed to validate the numerical method,and the predicted terminal bubble shape and velocity were found to agree with those presented in the Grace diagram and calculated by drag correlation,*** simulation results under RH conditions indicate that the terminal bubble shape and velocity cannot be *** primary bubble growth occurs within a rising distance of 0.3 m owing to heating by the high-temperature liquid steel;subsequently,the bubble continues to grow under equilibrium with the hydrostatic *** the initial diameter is 8-32 mm,the bubble diameter and rising velocity near the liquid surface are 80-200 mm and 0.5-0.8 m/s,*** bubble rises rectilinearly with an axisymmetric shape,and the shape evolution history includes an initial sphere,(dimpled)ellipsoid,and spherical cap with satellite bubbles.

关键词： Bubble dynamics Liquid steel Volume of fluid Bubble growth Bubble shape Rising velocity

Prediction of liquid circulation flow rate in RH degasser:improvement of decarburization at low atmospheric pressure

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Journal of Iron and Steel Research International 2024年第7期31卷 1661-1667页

The two-fluid model coupled with population balance model was used for simulating the gas-liquid flow in the Ruhrstahl-Heraeus(RH)*** predicted circulation flow rate was compared with that measured from a water model experiment to validate the mathematical ***,influence of snorkel immersion depth on liquid circulation flow rate was numerically investigated under an atmospheric pressure of 101 and 84 kPa,*** result indicates that the circulation flow rate of the RH degasser in the high-altitude area was severely reduced because of the decrease in atmospheric ***,increasing the snorkel immersion depth from 0.5 to 0.7 m can compensate for the decrease in atmospheric *** test result indicates that decarburization rate is significantly enhanced by increasing the snorkel immersion *** optimization,the percentage of heats with a final carbon content less than 0.002 wt.%is significantly increased from 22.0%to 96.4%.

关键词： RH degasser Two-fluid model Population balance model-Circulation flow rate Decarburization Snorkel immersion depth

A modern survey method for determining live loads based on multi-source and open-access data on the Internet

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Frontiers of Structural and Civil Engineering 2024年第8期18卷 1135-1147页

作者： Chi XU jun chen Jie LI School of Civil Engineering Tongji UniversityShanghai 200092China The State Key Laboratory on Disaster Reduction in Civil Engineering Tongji UniversityShanghai 200092China

Sufficient survey data are required to describe the stochastic behaviors of live ***,due to manual and on-site operation required by traditional survey methods,traditional surveys face challenges like occupant resistance,high costs,and long implementation *** study proposes a new survey method to access live load data online and *** samples are acquired from multi-source,open-access and dynamically updated data on the *** change intervals,geometrical dimensions and object quantities are obtained from transaction information,building attributes and virtual reality models on real estate websites,*** object weights are collected from commodity information on e-commerce *** integration of the aforementioned data allows for the extraction of necessary statistics to describe a live load *** proposed method is applied to a live load survey in China,covering 20040 m^(2),with around 90000 samples acquired for object weights and load *** survey results reveal that about 70%−80%of the amplitude statistics are attributable to 1/6 of the total object types.

关键词： live load online survey method data acquisition data integration

Effect of Epoxy Resin on the Properties of Recycled Asphalt

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Journal of Wuhan University of Technology(Materials Science) 2024年第5期39卷 1149-1155页

作者： YANG Ruochong chen Huimin YANG jun School of Transportation Southeast UniversityNanjing 211189China

To promote the recycling of reclaimed asphalt pavement(RAP),epoxy resin was used to prepare the epoxy-recycled asphalt *** effect of epoxy resin on the properties of aged asphalt binder was investigated based on the tensile test,flexural creep test,and laser scanning confocal *** curing characteristics and the mechanical performance of recycled asphalt with different epoxy contents were *** results show that the low-temperature performance,ductility,and strength of the aged asphalt binder were significantly improved when the epoxy content reached 40%.The curing time of epoxy-recycled asphalt should be at least 4 d to ensure the formation of good internal spatial network structure.

关键词： RAP epoxy resin aged asphalt mechanical performance