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Highly efficient and stable organic solar cells with SnO_(2)electron transport layer enabled by UV-curing acrylate oligomers

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Journal of Energy Chemistry 2024年第5期92卷 124-131页

作者： Mwende Mbilo Du Hyeon Ryu Seungjin Lee Muhammad Haris julius Mwakondo mwabora Robinson Juma Musembi Hang Ken Lee Sang Kyu Lee Chang Eun Song Won Suk Shin Department of Physics Faculty of Science and TechnologyUniversity of Nairobi(UoN)P.O.Box 30197-00100NairobiKenya Advanced Energy Materials Research Center Korea Research Institute of Chemical Technology(KRICT)Daejeon 34114Republic of Korea Advanced Materials and Chemical Engineering University of Science and Technology(UST)Daejeon 34113Republic of Korea

The interfaces between the inorganic metal oxide and organic photoactive layer are of outmost importance for efficiency and stability in organic solar cells(OSCs).Tin oxide(SnO_(2))is one of the promising candidates for the electron transport layer(ETL)in high-performance inverted *** a solution-processed SnO_(2)ETL is employed,however,the presence of interfacial defects and suboptimal interfacial contact can lower the power conversion efficiency(PCE)and operational stability of ***,highly efficient and stable inverted OSCs by modification of the SnO_(2)surface with ultraviolet(UV)-curable acrylate oligomers(SAR and OCS)are *** highest PCEs of 16.6%and 17.0%are achieved in PM6:Y6-BO OSCs with the SAR and OCS,respectively,outperforming a device with a bare SnO_(2)ETL(PCE 13.8%).The remarkable enhancement of PCEs is attributed to the optimized interfacial contact,leading to mitigated surface *** strikingly,improved light-soaking and thermal stability strongly correlated with the interfacial defects are demonstrated for OSCs based on SnO_(2)/UV cross-linked resins compared to OSCs utilizing bare SnO_(2).We believe that UV cross-linking oligomers will play a key role as interfacial modifiers in the future fabrication of large-area and flexible OSCs with high efficiency and stability.

关键词： Organic solar cells SnO_(2) Surface defects Ultraviolet resins Stability Cross-linking oligomers Non-halogenated solvent

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Light Soaking Induced Increase in Conversion Efficiency in Solar Cells Based on In(OH)xSy/Pb(OH)xSy

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Materials Sciences and Applications 2013年第11期4卷 718-722页

作者： Robinson Musembi Bernard Aduda julius mwabora Marin Rusu Kostantinos Fostiropoulos Martha Lux-Steiner Department of Physics School of Physical Sciences University of Nairobi Nairobi Kenya Solarenergieforsung (SE2) Lise- Meitner Campus Hermholtz-Zentrum Berlin für Materialien und Energie Berlin Germany

Light soaking characterization on complete SnO2:F/TiO2/In(OH)xSy/Pb(OH)xSy/PEDOT:PSS/Au, eta solar cell structure as well as on devices which do not include one or both TiO2 and/or PEDOT:PSS layers has been conducted. Additionally, studies of SnO2:F/In(OH)xSy/Pb(OH)xSy/PEDOT:PSS/Au solar cell have been performed. The power conversion efficiency and the short circuit current density have been found to increase with light soaking duration by a factor of about 1.6 - 2.7 and 2.1 - 3, respectively. The increase in these two parameters has been attributed to the filling up of trap states and/or charge-discharge of deep levels found in In(OH)xSy. These effects take place at almost fill factor and open circuit voltage being unaffected by the light soaking effects.

关键词： Eta Solar Cell Light Soaking Conversion Efficiency TiO2 In(OH)xSy Pb(OH)xSy

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Role of Bismuth and Substrate Temperature on the Optical Properties of Some Flash Evaporated Se100-XBiXGlassy System

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New Journal of Glass and Ceramics 2015年第2期5卷 16-24页

作者： Austine A. Mulama julius M. mwabora Andrew O. Oduor Cosmas M. Muiva Boniface Muthoka Betty N. Amukayia Drinold A. Mbete Department of Physics & Materials Science Maseno University Maseno Kenya Department of Physics University of Nairobi Nairobi Kenya Department of Physics Botswana International University of Science & Technology Palapye Botswana Department of Mathematics Masinde Muliro University of Science and Technology Kakamega Kenya

Chalcogenide glasses are very important in the modern technology especially selenium-based. These glasses are sensitive to electromagnetic radiation useful in the infrared optics. The study investigated the effect of substrate temperature on the as-deposited selenium-bismuth thin films in addition to bismuth content. The films were deposited by flash evaporation method. Thickness of the films was measured on a surface profiler and confirmed through calculation based on the Swanepoel method. The spectral range of study was between 200 - 3000 nm. It is found that the effect of increasing bismuth content on the as-deposited films led to increased absorption coefficient, reflectance, refractive index and extinction coefficient while transmittance and optical band gap energy decreased. On the other hand, reflectance, absorption coefficient, extinction coefficient, refractive index, real and imaginary parts of dielectric constant increased with increase in substrate temperature but transmittance and optical band gap energy decreased.

关键词： Chalcogenide Glass Selenium-Bismuth Alloy Substrate Temperature

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