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Synthesis and applications of lanthanoid complexes of pentadentate and hexadentate N_(5) and N_(6) macrocycles:A review

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Journal of Rare Earths 2024年第1期42卷 1-15,I0001页

作者： julio Corredoira-vázquez Cristina González-Barreira Paula Oreiro-Martínez Ana M.García-Deibe Jesús Sanmartín-Matalobos Matilde Fondo Departamento de Química Inorganica Facultade de QuímicaUniversidade de Santiago de CompostelaCampus Vida15782Santiago de CompostelaSpain Phantom-g CICECO-Aveiro Institute of MaterialsDepartment of PhysicsUniversity of Aveiro3810-193AveiroPortugal Institute of Materials(iMATUS) Universidade de Santiago de Compostela15782Santiago de CompostelaSpain

In this paper,the lanthanoid complexes of N_(5) and N_(6) macrocycle ligands,without pendant arms or additional heteroatoms,are *** review covers the period from 2015 to the current date,since in 2014 Schiff base macrocyclic ligands incorporating the pyridine moiety,and their complexes,were revised,and in 2015 the chemistry of pentaaza macrocycle ligands with rare earth metals was also *** and phthalocyanine ligands are not included in this review,which primarily focuses on complexes with Schiff bases and amines without pendant arms or any additional donor other than *** synthetic methods,structural characterization,based on single X-ray crystal data,and properties of the lanthanoid complexes,with special attention to magneto-structural correlations,are presented herein.

关键词： Lanthanoid N_(5),N_(6)macrocycle Coordination chemistry Chirality Biological activity Molecule magnet

Genomic selection in plant breeding:Key factors shaping two decades of progress

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Molecular Plant 2024年第4期17卷 552-578页

作者： Admas Alemu Johanna Astrand Osval A.Montesinos-López julio Isidro y Sanchez Javier Fernandez-Gónzalez Wuletaw Tadesse Ramesh R.vetukuri Anders S.Carlsson Alf Ceplitis JoséCrossa Rodomiro Ortiz Aakash Chawade Department of Plant Breeding Swedish University of Agricultural SciencesAlnarpSweden Lantmannen Lantbruk SvalövSweden Facultad de Telematica University de ColimaColimaColima 28040Mexico Centro de Biotecnología y Genómica de Plantas(CBGP UPM-INIA)Universidad Politécnica de Madrid(UPM)-Instituto Nacional de Investigación y Tecnología Agraria y Alimentaria(INIA)Campus de Montegancedo-UPM28223 MadridSpain International Center for Agricultural Research in the Dry Areas(ICARDA) RabatMorocco International Maize and Wheat Improvement Center(CIMMYT) Km 45Carretera México-VeracruzTexcocoMéxico 52640Mexico

Genomic selection,the application of genomic prediction(GP)models to select candidate individuals,has significantly advanced in the past two decades,effectively accelerating genetic gains in plant *** article provides a holistic overview of key factors that have influenced GP in plant breeding during this *** delved into the pivotal roles of training population size and genetic diversity,and their relationship with the breeding population,in determining GP *** emphasis was placed on optimizing training population *** explored its benefits and the associated diminishing returns beyond an optimum *** was done while considering the balance between resource allocation and maximizing prediction accuracy through current optimization *** density and distribution of single-nucleotide polymorphisms,level of linkage disequilibrium,genetic complexity,trait heritability,statistical machine-learning methods,and non-additive effects are the other vital *** wheat,maize,and potato as examples,we summarize the effect of these factors on the accuracy of GP for various *** search for high accuracy in GP—theoretically reaching one when using the Pearson’s correlation as a metric—is an active research area as yet far from optimal for various *** hypothesize that with ultra-high sizes of genotypic and phenotypic datasets,effective training population optimization methods and support from other omics approaches(transcriptomics,metabolomics and proteomics)coupled with deep-learning algorithms could overcome the boundaries of current limitations to achieve the highest possible prediction accuracy,making genomic selection an effective tool in plant breeding.

关键词： genomic selection genetic gain genomic prediction optimization deep learning training population optimization

Exome sequencing identifies a likely causative variant in 53%of families with ciliopathy-related features on renal ultrasound after excluding NPHP1 deletions

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Genes & Diseases 2024年第5期11卷 40-43页

作者： Konstantin Deutsch verena Klambt Thomas M.Kitzler Tilman Jobst-Schwan Ronen schneider Florian Buerger Steve Seltzsam Sherif El Desoky Jameela A.Kari Farkhanda Hafeez Maria Szczepanska Loai A.Eid Hazem S.Awad Muna Al-Saffar Neveen A.Soliman velibor Tasic Camille Nicolas-Frank Kirollos Yousef Luca M.Schierbaum Sophia schneider Abdul Halawi Izzeldin Elmubarak Katharina Lemberg Shirlee Shril Shrikant M.Mane Nancy Rodig Friedhelm Hildebrandt Division of Nephrology Department of PediatricsBoston Children’s HospitalHarvard Medical SchoolBostonMA 02215USA Department of Pediatric Gastroenterology Nephrology and Metabolic DiseasesCharite Universitatsmedizin BerlinBerlin 13353Germany Berlin Institute of Health at Charitee Universitatsmedizin Berlin BIH Biomedical Innovation AcademyBIH Charite Clinician Scientist ProgramBerlin 10178Germany Department of Nephrology and Hypertension FriedrichAlexander-Universitat Erlangen-NurnbergErlangen 91054Germany Department of Pediatrics Faculty of Medicine King Abdulaziz UniversityPediatric Nephrology Center of ExcellenceKing Abdulaziz University HospitalJeddah 21589Saudi Arabia Department of Pediatric Nephrology The Children’s Hospital and Institute of Child HealthLahore 54000Pakistan Department of Pediatrics Faculty of Medical Sciences in ZabrzeMedical University of Silesia in KatowiceKatowice 40-752Poland Dubai Hospital and Al-Jalila Children’s Specialty Hospital Kidney Center of ExcellenceDubai 4545United Arab Emirates Department of Genetics and Genomics UAE UniversityAbu Dhabi 15551United Arab Emirates Department of Pediatrics Division of Genetics and GenomicsBoston Children’s HospitalHarvard Medical SchoolBostonMA 02215USA Department of Pediatrics Center of Pediatric Nephrology and TransplantationKasr Al Ainy School of MedicineCairo UniversityCairo 11562Egypt Egypt Center for Research and Regenerative Medicine(ECRRM) Cairo 11511Egypt Medical Faculty Skopje University Children’s HospitalSkopje 1000North Macedonia Department of Genetics Yale University School of MedicineNew HavenCT 06520USA

Nephronophthisis-related ciliopathies(NPHP-RC)represent one of the most common causes of chronic kidney disease in the first three decades of life and are characterized by a broad genetic and clinical heterogeneity.1 To date,more than 90 genes have been identified that cause autosomalrecessive NPHP-RC if mutated,accounting for up to 60%of cases.1 Among these,homozygous deletions of NPHP1 are the most common *** genes localize to primary cilia,basal bodies,or the centrosome and lead to a primary ciliary disruption if mutated,thereby causing a broad phenotypical spectrum.1 Patients that suffer from NPHP-RC can either have an isolated renal phenotype,such as polyuria,polydipsia,decreased urinary concentration ability,and secondary enuresis due to loss of tubular function,or present with extrarenal symptoms including retinal degeneration,cerebellar vermis hypoplasia,or hepatic *** are often diagnosed in early adolescence,reaching end-stage renal disease before 25 years of age,but early onset and rapidly progressive forms of NPHP-RC also exist.1 Renal ultrasound indicates kidneys of normal or reduced renal length with increased echogenicity and corticomedullary cysts.

关键词： degeneration urinary likely

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夜间观鸟

科技纵览 2024年第7期 18-20页

作者： David schneider 不详

观鸟正在谨勃兴起。你可能会感觉到,在鸟类迁徒的季节,当鸟类在夏季和冬季栖息地之间迁徙时,当地的自然观测景点尤其繁忙。你发现正在逐渐消失的物种可能已经被以前没有的物种取代了。或者,你可能看到过飞翔的候鸟,比如说一群野雁排成v... 详细信息

观鸟正在谨勃兴起。你可能会感觉到,在鸟类迁徒的季节,当鸟类在夏季和冬季栖息地之间迁徙时,当地的自然观测景点尤其繁忙。你发现正在逐渐消失的物种可能已经被以前没有的物种取代了。或者,你可能看到过飞翔的候鸟,比如说一群野雁排成v字形飞行。即使你不是专门的鸟类观测人员,你也可能曾经做过这样的观察。

关键词：观测人员观鸟栖息地候鸟迁徙鸟类 v字形物种

Survival and growth of dominant tree seedlings in seasonally tropical dry forests of Yucatan: site and fertilization effects

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Journal of Plant Ecology 2014年第5期7卷 470-479页

作者： Luis Salinas-Peba víctor Parra-Tabla julio Campo Miguel A.Munguía-Rosas Departamento de Ecología Tropical Campus de Ciencias Biológicas y AgropecuariasUniversidad Autónoma de YucatánKm.15.5 Carretera Mérida-XmatkuilYucatán 97000México Instituto de Ecología Universidad Nacional Autónoma de MéxicoA.p.70-275México D.F.04510México Departamento de Ecología Humana Centro de Investigación y de Estudios Avanzados del Instituto Politécnico Nacional(CINVESTAV)Km.6 Antigua carretera a ProgresoMérida 97310México

Aims Seasonally tropical dry forests of the Yucatan Peninsula are typically found in sites with nutrient-poor soils because of the recent geologi-cal origin of the *** landscape is dominated by extensive karstic plates that shape environments where vegetation regenera-tion through seed germination may be limited by the availability of suitable *** this study,we documented the survival and growth of seedlings from three dominant tree species(Bursera simaruba,Piscidia piscipula and Lysiloma latisiliquum)in seasonally tropical dry forests in ***,we evaluated the effect of nutrient addition(N and P,separately and in combination)on seedling survival and growth across three sites with differing levels of *** We conducted a nutrient addition experiment,whereby we estab-lished 12 plots of dimensions 10×10 m(100 m^(2))at each site,from which three plots were randomly selected to receive one of four treatments:N addition,P addition,N and P addition and no nutri-ent addition(controls).Prior to treatment application,in each plot,we planted 10 seedlings of each species in October 2010 and sub-sequently conducted surveys of plant growth and survival every 20 days from November 2010 to April *** Findings Overall,nutrient addition increased seedling survival and the mag-nitude of this effect was similar among *** did not observe an additive effect of the N+P treatment on ***,we observed a positive effect of nutrient addition on seedling growth,but this effect was contingent upon site;regarding survival,the effects of N and P on seedling growth were not *** results suggest that seedling recruitment and growth in the three dominant species of trees in Yucatan are limited by nutrient avail-ability but that the magnitude of this effect,particularly on seedling growth,is specific for species and site.

关键词： growth nitrogen nutrient addition phosphorus seedling survival seasonally tropical dry forest

miniSCIDOM: a scintillator-based tomograph for volumetric dose reconstruction of single laser-driven proton bunches

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High Power Laser Science and Engineering 2024年第2期12卷 41-50页

作者： A.Corvino M.Reimold E.Beyreuther F.-E.Brack F.Kroll J.Pawelke J.D.Schilz M.schneider U.Schramm M.E.P.Umlandt K.Zeil T.Ziegler J.Metzkes-Ng Helmholtz-Zentrum Dresden–Rossendorf DresdenGermany Technische Universität Dresden DresdenGermany OncoRay–National Center for Radiation Research in Oncology Faculty of Medicine and University Hospital Carl Gustav CarusTUD Dresden University of TechnologyHelmholtz-Zentrum Dresden–RossendorfDresdenGermany Current affiliation:Institut Curie UniversitéPSLCNRS UMR3347OrsayFrance Current affiliation:Universitätsklinikum Freiburg FreiburgGermany

Laser plasma accelerators(LPAs)enable the generation of intense and short proton bunches on a micrometre scale,thus offering new experimental capabilities to research fields such as ultra-high dose rate radiobiology or material *** spectrally broadband,laser-accelerated proton bunches allow for tailored volumetric dose deposition in a sample via single bunches to excite or probe specific sample *** rising number of such experiments indicates a need for diagnostics providing spatially resolved characterization of dose distributions with volumes of approximately 1 cm^(3) for single proton bunches to allow for fast online *** we present the scintillator-based miniSCIDOM detector for online single-bunch tomographic reconstruction of dose distributions in volumes of up to approximately 1 cm^(3).The detector achieves a spatial resolution below 500μm and a sensitivity of 100 *** detector performance is tested at a proton therapy cyclotron and an LPA proton *** experiments’primary focus is the characterization of the scintillator’s ionization quenching behaviour.

关键词： beam monitoring detectors laser-driven proton beams scintillator-based diagnostics ultra-high dose rate

Cardiorespiratory fitness measured with cardiopulmonary exercise testing and mortality in patients with cardiovascular disease:A systematic review and meta-analysis

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Journal of Sport and Health Science 2021年第6期10卷 609-619,F0003页

作者： Yasmin Ezzatvar MikelIzquierdo julio Núñez Joaquín Calatayud Robinson Ramírez-vélez Antonio García-Hermoso Exercise Intervention for Health Research Group(EXINH-RG) Department of PhysiotherapyUniversitat de ValènciaValencia 46010Spain Navarrabiomed Navarra Hospital Complex(CHN)Public University of Navarra(UPNA)Navarra Medical Research Institute(IdiSNA)Pamplona 31008Spain CIBER of Frailty and Healthy Aging(CIBERFES) Instituto de Salud Carlos IIIMadrid 28029Spain Department of Cardiology Valencia University HospitalBiomedical Research Institute(INCLIVA)Valencia 46010Spain CIBER in Cardiovascular Diseases(CIBERCv) Madrid 28029Spain Sciences of Physical Activity Sports and Health SchoolUniversity of Santiago of Chile(USACH)Santiago 71783-5Chile

Background Cardiorespiratory fitness(CRF)is inversely associated with mortality in apparently healthy subjects and in some clinical populations,but evidence for the association between CRF and all-cause and/or cardiovascular disease(CvD)mortality in patients with established CvD is *** study aimed to quantify this *** We searched for prospective cohort studies that measured CRF with cardiopulmonary exercise testing in patients with CvD and that examined all-cause and CvD mortality with at least 6 months of *** hazard ratios(HRs)were calculated using random-effect inverse-variance *** Data were obtained from 21 studies and included 159,352 patients diagnosed with CvD(38.1%female).Pooled HRs for all-cause and CvD mortality comparing the highest *** category of CRF were 0.42(95%confidence interval(95%CI):0.28–0.61)and 0.27(95%CI:0.16–0.48),*** HRs per 1 metabolic equivalent(1-MET)increment were significant for all-cause mortality(HR=0.81;95%CI:0.74–0.88)but not for CvD mortality(HR=0.75;95%CI:0.48–1.18).Coronary artery disease patients with high CRF had a lower risk of all-cause mortality(HR=0.32;95%CI:0.26–0.41)than did their unfit *** 1-MET increase was associated with lower all-cause mortality risk among coronary artery disease patients(HR=0.83;95%CI:0.76–0.91)but not lower among those with heart failure(HR=0.69;95%CI:0.36–1.32).Conclusion A better CRF was associated with lower risk of all-cause mortality and *** study supports the use of CRF as a powerful predictor of mortality in this population.

关键词： Cardiopulmonary fitness Coronary artery disease Exercise capacity Heart failure Survival

Surface-plasmonic sensor using a columnar thin film in the grating-coupled configuration [Invited]

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Chinese Optics Letters 2021年第8期19卷 121-129页

作者： Kiran Mujeeb Muhammad Faryad Akhlesh Lakhtakia julio v.Urbina Department of Electronics Quaid-i-Azam UniversityIslamabad 45320Pakistan Department of Physics Lahore University of Management SciencesLahore 54792Pakistan Department of Engineering Science and Mechanics The Pennsylvania State UniversityUniversity ParkPennsylvania 16802USA Department of Electrical Engineering The Pennsylvania State UniversityUniversity ParkPennsylvania 16802USA

The excitation of a surface-plasmon-polariton(SPP) wave guided by a columnar thin film(CTF) deposited on a one-dimensional metallic surface-relief grating was investigated for sensing the refractive index of a fluid infiltrating that CTF. The Bruggemann homogenization formalism was used to determine the relative permittivity scalars of the CTF infiltrated by the fluid. The change in the refractive index of the fluid was sensed by determining the change in the incidence angle for which an SPP wave was excited on illumination by a p-polarized plane wave, when the plane of incidence was taken to coincide with the grating plane but not with the morphologically significant plane of the CTF. Multiple excitations of the same SPP wave were found to be possible, depending on the refractive index of the fluid, which can help increase the reliability of results by sensing the same fluid with more than one excitation of the SPP wave.

关键词： metal grating multiple excitation rigorous coupled-wave approach sensitivity surface-plasmon-polariton wave

Methodology for ranking controllable parameters to enhance operation of a steam generator with a combined Artificial Neural Network and Design of Experiments approach

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能源与人工智能(英文) 2021年第1期3卷 9-21页

作者： Lara Werncke vieira Augusto Delavald Marques Paulo Smith schneider Antônio Joseda Silva Neto Felipe Antonio Chegury viana Madhat Abdel-jawad Julian David Hunt julio Cezar Mairesse Siluk Federal University of Rio Grande do Sul-UFRGS Porto AlegreBrazil State University of Rio de Janeiro-UERJ Nova FriburgoBrazil University of Central Florida OrlandoUCFUnited States Advanced Analysis Australia-AAA PerthAustralia International Institute for Applied Systems Analysis-IIASA ViennaAustria Federal University of Santa Maria-UFSM Santa MariaBrazil

The operation of complex systems can drift away from the initial design conditions,due to environmental condi-tions,equipment wear or specific *** generators are complex equipment and their proper opera-tion relies on the identification of their most relevant *** approach to rank the operational parameters of a subcritical steam generator of an actual 360 MW power plant is *** Artificial Neural Network-ANN delivers a model to estimate the steam generator efficiency,electric power generation and flue gas outlet temperature as a function of seven input *** ANN is trained with a two-year long database,with training errors of 0.2015 and 0.2741(mean absolute and square error)and validation errors of 0.32%and 2.350(mean percent and square error).That ANN model is explored by means of a combination of situations proposed by a Design of Experiment-DoE *** seven controlled parameters showed to be relevant to express both steam generator efficiency and electric power generation,while primary air flow rate and speed of the dynamic classifier can be neglected to calculate flue gas temperature as they are not statistically *** also shows the prominence of the primary air pressure in respect to the steam generator efficiency,electric power generation and the coal mass flow rate for the calculation of the flue gas outlet *** ANN and DoE combined methodology shows to be promising to enhance complex system efficiency and helpful whenever a biased behavior must be brought back to stable operation.

关键词： Coal-fired power plant Artificial Neural Network Design of Experiments Response surface methodology Steam generator