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Effect of early stepwise cardiopulmonary rehabilitation on function and quality of life in sepsis patients

World Journal of clinical cases 2024年第4期12卷 729-736页

作者： Ming-Hui Zheng Wen-Jun Liu juan Yang Division of cardiovascular First Ward Departments of Internal Medicine Liyuan HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhan 430077Hubei ProvinceChina Department of Respiratory Medicine PuRen Hospital Affiliated to Wuhan University of Science and Technology/Respiratory MedicineWuhan 430000Hubei ProvinceChina Department of cardiology Huanggang Central HospitalHuanggang 438000Hubei ProvinceChina

BAcKGROUND Sepsis,as a non-limiting host infection disease,can be accompanied by serious complications such as organ failure,which seriously threatens patient quality of *** To investigate the effect of early stepwise cardiopulmonary rehabilitation on cardiopulmonary function and quality of life in patients evacuated from mechanical ventilation with *** A total of 80 patients with sepsis who were hospitalized in our hospital from January 2021 to January 2022 were selected and divided into the observation group(n=40)and the control group(n=40)according to the random number table *** observation group was treated with early stepwise cardiopulmonary rehabilitation,and the control group was treated with a conventional treatment *** function indexes(central venous pressure,cardiac troponin I,B-type brain natriuretic peptide),lung function indicators(diaphragmatic mobility,changes in central venous oxygen saturation,oxygenation index),and quality of life(Quality of Life Evaluation Scale)were compared between the two groups after *** After treatment,the central venous pressure,diaphragm mobility,central venous oxygen saturation,oxygenation index,and Quality of Life Evaluation Scale scores in the observation group were higher than those in the control group,and the differences were statistically significant(Pcontrol group for other parameters,and the differences were statistically significant(PcONcLUSION Early stepwise cardiopulmonary rehabilitation can effectively enhance cardiac and pulmonary function and improve the quality of life in patients evacuated from mechanical ventilation with sepsis.

关键词： Stepwise cardiopulmonary rehabilitation Sepsis Evacuation of mechanical ventilation cardiopulmonary function Quality of life

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Porphyrinic Acceptors forFullerene-Free MolecularPhotovoltaics

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ccS chemistry 2024年第2期6卷 276-296页

作者： Jorge Labella juan Laforga-Martin Tomás Torres Department of Organic chemistry Universidad Aut´onoma de Madrid28049 Madrid Institute for Advanced Research in chemical Sciences Universidad Aut´onoma de MadridMadrid IMDEA—Nanociencia 28049 Madrid

Over the past few years,the development of nonfullerene acceptors(NFAs)has become a prominent focus in both organic and perovskite solar cell(OScs and PScs,respectively)research *** this context,porphyrinoids,compounds structurally related to porphyrins,have emerged as promising solar cell *** contrast to the widely used fullerene acceptors,porphyrinoids exhibit strong,broad absorption properties across the UV–vis/NIR spectrum,which can be easily tuned through chemical ***,they can be prepared and derivatized using cost-effective and straightforward methodologies,allowing for convenient adjustments in thin-film morphology,processability,supramolecular organization,and energy ***,these compounds offer higher thermal and photochemical stability,resulting in longer device lifetimes compared to their fullerene-based *** this review,we outline the utilization of porphyrinoids as NFAs in OScs and PScs,discussing essential aspects such as design guidelines,molecular properties,and device *** goal is to inspire and further promote the development of n-type porphyrinoids,which have not yet fully unleashed their potential.

关键词： fullerene-free molecular photovoltaics nonfullerene acceptors porphyrinic acceptors n-type porphyrinoids organic and perovskite solar cells

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The relationship between morphology and flight in Drosophila:a study of two pairs of sibling species from a natural population

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Insect Science 2024年第3期31卷 885-900页

作者： Nicolás Flaibani Victoría Estefania Ortiz juan JoséFanara Valeria Paula carreira Laboratorio de Evolucion Departamento de EcologiaGenética y Evolucion(DEGE)Facultad de Ciencias Exactas y Naturales(FCEN)Universidad de Buenos Aires(UBA)Instituto de GenéticaEcologia y Evolucion de Buenos Aires(IEGEBA)Consejo Nacional de Investigaciones Cientificasy Tecnicas(CONICET)-UBABuenos AiresArgentina

Insect flight is a complex trait involved in different behaviors,from the search for sexual partners,food,or breeding *** studies have postulated the adaptive advantages of certain morphological traits in relation to increased flight capacity,such as low values of wing loading or high values of wing:thorax ratio and wing-aspect ***,few studies have evaluated the relationship between variables related to flight and morphological traits in *** work aimed to study morphological traits in males and females of two pairs of sibling species:Drosophila buzzati Patterson and Wheeler-Drosophila koeferae Fontdevila and Wasserman,and Drosophila melanogaster Meigen-Drosophila simulans Sturtevant,and to analyze its relationship with *** detected the highest proportion of flight time in *** and *** compared to *** and ***,*** results also revealed sexual dimorphism,with males exhibiting a higher proportion of flight time than ***,we did not find a general pattern to explain the relationship between morphology and the proportion of flight time because associations varied depending upon the analyses(considering all groups together or each sex-species combination separately).Moreover,these associations explained a low percentage of variation,suggesting that other nonmorphological components related to flight,such as physiological variables,should be taken into *** work allowed us to show the variability and complexity of an aspect of flight,suggesting that the adaptive role of the morphological traits studied might have been overestimated.

关键词： morphological traits time in flight wing loading wing:thorax ratio wingaspect ratio wing second moment of area

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Synthesis of Planar-chiral[2.2]Paracyclophane-Based Oxazole-Pyrimidine Ligands and Application in Nickel-catalyzed 1,2-Reduction ofα,β-Unsaturated Ketones

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chinese Journal of chemistry 2024年第7期42卷 705-710页

作者： juan Wang Qing-Xian Xie Xiang Li chang-Bin Yu Yong-Gui Zhou School of chemistry Dalian University of Technology2 Linggong RoadDalianLiaoning 116024China State Key Laboratory of catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalianLiaoning 116023China

The planar-chiral ligands have been widely applied as a class of unique and significant ligands in asymmetric *** them,chiral[2.2]paracycyclophane has emerged as a privileged type of planar-chiral framework and has been utilized as an important toolbox due to their structural ***,we design and synthesize[2.2]paracyclophane-derived oxazole-pyrimidine ligands(abberviated as PYMcOX).These N,N-ligands with stable properties,rigid structure and large steric hindrance performed successfully in nickel-catalyzed asymmetric 1,2-reduction ofα,β-unsaturated ketones,affording the chiral allylic alcohols with up to 99%yield and 99%***,this reduction reaction could be conducted on gram-scale without loss of activity and enantioselectivity,and the chiral ligand could be conveniently recovered with high yield.

关键词： Oxazole-pyrimidine ligands Planar chirality Nickel Hydroboration Asymmetric synthesis

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A multi-stream network for retrosynthesis prediction

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Frontiers of computer Science 2024年第2期18卷 231-233页

作者： Qiang ZHANG juan LIU Wen ZHANG Feng YANG Zhihui YANG Xiaolei ZHANG Institute of Artificial Intelligence School of Computer ScienceWuhan UniversityWuhan 430072China college of Informatics Huazhong Agricultural UniversityWuhan 430072China

1 Introduction Retrosynthesis aims to predict a set of reactants for producing given molecules[1],which plays a significant part in the biochemistry field,such as molecular pathway design and drug *** existing methods perform better in solving this problem,most of these methods[2,3]only describe the molecules from one kind of perspective,such as they use Simplified Molecular Input Line Entry System(SMILES)strings[4]to represent the atomic components and the relationship between atoms of molecules or leverage Extended connectivity Fingerprints(EcFPs)represent the information of the molecular sub-structure composition via binary vectors[5].

关键词： synthesis reactant hough

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Paleoenvironmental changes recorded by grain size of loess/paleosol sequence from the chifeng city,Northeastern china since the Last Glacial

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Journal of Mountain Science 2024年第9期21卷 3068-3082页

作者： LI juan BRYE Kristofor R ZHANG Mengge JIANG Zhuodong WANG Qiubing college of Land and Environment Shenyang Agricultural UniversityShenyang 110866China Department of crop Soiland Environmental SciencesUniversity of ArkansasFayettevilleAR 72701USA

The accumulation processes of loess in northeastern(NE)china record the varying characteristics of the East Asian Monsoons(EAM)and the evolution of the local *** this study,grain size end-member analysis of the Dajiugang(DJG)section deposited since the Last Glacial in chifeng city,NE china was used to reveal the dynamic depositional characteristics of loess and environmental evolution of NE *** showed that the chifeng loess comprises three grain size end-members(EM),EM1(7.38μm),EM2(49.4μm)and EM3(90.00μm),indicating the three transport dynamics of dust delivered to the *** EM1 represents atmospheric dust as the *** EM2,mainly derived from relatively distant-sources deposition,and EM3,material transported over a short distance,correspond to the intensity of southwesterly winds and the East Asian Winter Monsoon(EAWM),*** of climate reconstruction,combined with other records,showed that the climate was generally cold and dry with a strong EAWM and a weak East Asian summer monsoon(EASM)during the stadial-period[Marine Isotope Stage(MIS)4 and MIS 2 stage].The climate was predominantly warm and humid,with weak EAWM and surface winds and strong EASM in interstadial-period(MIS 3 and MIS 1 stage).comparisons between indicators,e.g.,EM3,the LR04 benthicδ18O stack and summer insolation at 65°N suggest that the strong EAWM is induced by increasing the Northern Hemisphere ice volume and reduced summer solar radiation.

关键词： Loess deposit Grain size end-member Northeastern china Environmental change The Last Glacial

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Unlocking the Potential of Poly(butylene succinate)through Incorporation of Vitrimeric Network Based on Dynamic Imine Bonds

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chinese Journal of Polymer Science 2024年第10期42卷 1414-1424,I0006页

作者： Shan-Song Wu Hui-juan Lu Yi-Dong Li Shui-Dong Zhang Jian-Bing Zeng chongqing Key Laboratory of Soft-Matter Material Manufacturing School of Chemistry and Chemical EngineeringSouthwest UniversityChongqing400715China School of Mechanical and Automotive Engineering South China University of TechnologyGuangzhou510640China

Poly(butylene succinate)(PBS)exhibits many advantages,such as renewability,biodegradability,and impressive thermal and mechanical properties,but is limited by the low melt viscosity and strength resulted from the linear *** address this,vitrimeric network was introduced to synthesize PBS vitrimers(PBSVs)based on dynamic imine bonds through melt polymerization of hydroxyl-terminated PBS with vanillin derived imine containing compound and hexamethylene diisocyanate using trimethylolpropane as a crosslinking *** with different crosslinking degrees were synthesized through changing the content of the crosslinking *** effect of crosslinking degree on the thermal,theological,mechanical properties,and stress relaxation behavior of the PBSVs was studied in *** results demonstrated that the melt viscosity,melt strength,and heat resistance were enhanced substantially without obvious depression in crystallizability,thermal stability,and mechanical properties through increasing crosslinking *** addition,the PBSVs exhibit thermal reprocessability with mechanical properties recovered by more than 90%even after processing for three ***,PBSV with improved melt properties shows significantly improved foamability compared to commercial *** research contributes to the advancement of polymer technology by successfully developing PBS vitrimers with improved properties,showcasing their potential applications in sustainable and biodegradable materials.

关键词： Poly(butylene succinate) Vitrimer Imine bonds Foamability

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Langasite-based SAW high-temperature vibration sensor with temperature decoupling

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Science china(Technological Sciences) 2024年第6期67卷 1946-1956页

作者： ZHANG juan cHENG WenHua WANG Hao ZHANG Lei LI XiangRong MA HongShuai PANG JunQi TAN QiuLin State Key Laboratory of Dynamic Measurement Technology North University of ChinaTaiyuan030051China Department of Mechanical Engineering Taiyuan Institute of TechnologyTaiyuan030008China

Monitoring high-temperature vibrations is critical in aerospace engineering,industrial manufacturing,and energy production,where harsh conditions necessitate robust vibration sensors for detecting anomalous ***,the accuracy of such sensors is often compromised by crosstalk between temperature and vibration *** study introduces a high-temperature vibration sensor based on langasite(LGS)surface acoustic wave(SAW)technology,designed to withstand temperatures up to 500℃.The sensor demonstrates high sensitivity,ranging from 12.54 kHz/g at 25℃ to 15.63 k Hz/g at 500℃.A comprehensive mechanical and electrical coupling model for the SAW vibration sensor was developed by integrating theoretical equations with numerical simulations to optimize the sensor's ***,a novel decoupling algorithm for temperature and vibration was established,achieving thermomechanical decoupling with precise vibration *** results indicated a maximum relative deviation of 4.67%for the *** conclusion,the proposed LGS SAW vibration sensor emerges as a promising solution for the accurate detection of multiple parameters in high-temperature vibration monitoring.

关键词： high temperature langasite(LGS) surface acoustic wave(SAW) piezoelectric vibration sensor temperature decoupling

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Fabrication of amorphous FecoNicuMnP x high-entropy phosphide/carbon composites with a heterostructured fusiform morphology for efficient oxygen evolution reaction

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Journal of Materials Science & Technology 2024年第1期168卷 62-70页

作者： Yifan Zhou Longqing Gao Haoyuan chen Hao Wang juan Zhang Xiumin Li Fangfang Duo Guoqing Guan School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001China Graduate School of Sustainable community Studies Hirosaki University1-BunkyochoHirosaki 036-8560Japan Graduate School of Science and Technology Hirosaki University3-BunkyochoHirosaki 036-8561Japan Xinxiang University School of Chemistry&Materials EngineeringXinxiang 453003China Energy conversion Engineering Laboratory Institute of Regional InnovationHirosaki University3-BunkyochoHirosaki 036-8561Japan

Amorphous high-entropy materials with abundant defects,coordinatively unsaturated sites,and loosely bonded atoms could exhibit excellent electrocatalytic ***,how to fabricate such ma-terials with nanostructure as well as amorphous structure is still full of *** this work,high-entropy metal organic framework(HE-MOF)is employed as the self-sacrificial template to fabricate FecoNicuMnP x high-entropy phosphide/carbon(HEP/c)*** obtained composite shows a het-erostructured fusiform morphology,in which the HEP is encapsulated by a carbon layer,revealing high electron conductivity as well as rich catalytic active sites for oxygen evolution reaction(OER).Beside,it is found that there is a short-range ordered crystal structure in the amorphous phase,which is bene-ficial for revealing high OER catalytic activity as well as good *** a result,the optimum HEP/c composite shows an overpotential 239 mV@10 mA cm^(−2)with a small Tafel slope of 72.5 mV dec^(−1) for catalyzing OER in alkaline solution.

关键词： Water electrolysis Oxygen evolution reaction High-entropy MOFs High-entropy phosphides Amorphous structure

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A gas sensing neural circuit for an olfactory neuron

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communications in Theoretical Physics 2024年第10期76卷 26-40页

作者： Xi-Kui Hu Song Zhu juan Yang Zhao Yao Ping Zhou Jun Ma School of Science Chongqing University of Posts and Telecommunications School of Physics and Electronics Central South University Department of Physics Lanzhou University of Technology

A gas sensor can convert external gas concentration or species into electric voltage or current signals by physical adsorption or chemical changes. As a result, a gas sensor in a nonlinear circuit can be used as a sensitive sensor for detecting external gas signals from the olfactory system. In this paper, a gas sensor and a field-effect transistor are incorporated into a simple FithzHugh–Nagumo neural circuit for capturing and encoding external gas signals. An improved functional neural circuit is obtained, and the effect of gas concentration, gas species and neuronal activity can be discerned as the gate voltage, threshold voltage and activation coefficient of the field-effect transistor, respectively. The gas concentration can affect the neural activities from quiescent to normal working and, finally, to saturation state in bursting, spiking, periodic and chaotic firings with different frequencies. The effects of gas species and neuronal activity on the firing state can also be achieved in this functional neural circuit. In addition, variations in the gate voltage, threshold voltage and activation coefficient can cause switching between different firing modes. These results can be helpful in designing artificial olfactory devices for bionic gas recognition and other coupled systems arising in applied sciences.

关键词： bifurcation field-effect transistor gas sensor olfactory neural circuit

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