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Journal of Materials Science & Technology 2024年第1期168卷 62-70页

作者： Yifan Zhou Longqing Gao Haoyuan Chen Hao Wang juan Zhang Xiumin Li Fangfang Duo Guoqing Guan School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001China Graduate School of Sustainable Community Studies Hirosaki University1-BunkyochoHirosaki 036-8560Japan Graduate School of Science and Technology Hirosaki University3-BunkyochoHirosaki 036-8561Japan Xinxiang University School of Chemistry&Materials EngineeringXinxiang 453003China Energy Conversion Engineering Laboratory Institute of Regional InnovationHirosaki University3-BunkyochoHirosaki 036-8561Japan

Amorphous high-entropy materials with abundant defects,coordinatively unsaturated sites,and loosely bonded atoms could exhibit excellent electrocatalytic ***,how to fabricate such ma-terials with nanostructure as well as amorphous structure is still full of *** this work,high-entropy metal organic framework(HE-MOF)is employed as the self-sacrificial template to fabricate FeCoNiCuMnP x high-entropy phosphide/carbon(HEP/C)*** obtained composite shows a het-erostructured fusiform morphology,in which the HEP is encapsulated by a carbon layer,revealing high electron conductivity as well as rich catalytic active sites for oxygen evolution reaction(OER).Beside,it is found that there is a short-range ordered crystal structure in the amorphous phase,which is bene-ficial for revealing high OER catalytic activity as well as good *** a result,the optimum HEP/C composite shows an overpotential 239 mV@10 mA cm^(−2)with a small Tafel slope of 72.5 mV dec^(−1) for catalyzing OER in alkaline solution.

关键词： Water electrolysis Oxygen evolution reaction High-entropy MOFs High-entropy phosphides Amorphous structure

Development of the electric automatic steering system for agricultural vehicles

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International Journal of Agricultural and Biological Engineering 2024年第1期17卷 209-214页

作者： Guangshun An Chong Yu juan Du Xiang Yin Youliang Ni Chengqian Jin School of Agricultural Engineering and Food Science Shandong University of TechnologyZibo 255000ShandongChina Nanjing Research Institute for Agricultural Mechanization of Ministry of Agriculture and Rural Affairs Nanjing 210014China

Automatic guidance of agricultural vehicles requires automatic execution of operation commands received from the navigation controller by using electronically controlled mechanisms for wheel steering,speed changing and work *** steering contributes as a prerequisite technique in automatic and semi-automatic agricultural *** research aimed to develop an electric automatic steering system that was compact in its structure and integrated into original steering mechanism in a simply and convenient way for aftermarket modification.A brushless motor and reducer assembly was utilized to provide an adequate steering torque instead of manual maneuver.A rapid assembling approach was proposed by passing the steering shaft through the hollow output shaft.A digital proportional-integral-differential(PID)algorithm was implemented to calculate the rotation speeds and directions by comparing the desired angle and the actual angle,which was implemented in a printed circuit board with a microcontroller unit(MCU)and interface *** unmanned wheeled tractor was applied as test platform to integrate the newly developed electric automatic steering *** were conducted to evaluate its performance in terms of stability and *** autonomous navigation system guided the tractor along target paths in the field by sending steering commands to the electric automatic steering *** results show that the steering angle error was less than 0.81°when desired steering angle was less than 10°.The lateral error difference was no more than 4.76 cm when repeating following the same target path,which indicated that the electric automatic steering system responded accurately and robustly to steering commands.

关键词： automatic steering automatic navigation agricultural vehicles

Modeling Near-Field Impulsive Waves Generated by Deformable Landslide Using the HBP Model Based on the SPH Method

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Journal of Ocean University of China 2024年第2期23卷 328-344页

作者： WANG Wei WEI Weicheng CHAI Bo XIA Hao WANG Yang DU juan LIU Jizhixian School of Environmental Studies China University of GeosciencesWuhan 430078China Hubei Key Laboratory of Yangtze Catchment Environmental Aquatic Science Wuhan 430078China Faculty of Engineering China University of GeosciencesWuhan 430074China Research Center for Geohazards Monitoring and Warning in Three Gorges Reservoir Wanzhou 404000China

Landslide-generated impulsive waves(LGWs)in reservoir areas can seriously threaten waterway safety as well as hu-man life and properties around the two side *** risk reduction and mitigation of such a hazard require the accurate prediction of near-field wave characteristics,such as wave amplitude and ***,near-field LGW involves complicated fluid-solid ***,the wave characteristics are closely related to various aspects,including the geometry and physical features of the slide,river,and body of ***,the empirical or analytical methods used for rough estimation cannot derive accurate results,especially for deformable landslides,due to their significant geometry changes during the sliding *** this study,the near-field waves generated by deformable landslides were simulated by smoothed particle hydrodynamics(SPH)based on multi-phase *** deformable landslides were generalized as a kind of viscous flow by adopting the Herschel-Bulkley-Papanastasiou(HBP)-based nonNewtonian rheology *** HBP model is capable of producing deformable landslide dynamics even though the high-speed sliding process is *** this study,an idealized experiment case originating from Lituya LGW and a practical case of Gongjiafang LGW were reproduced for verification and *** simulation results of both cases show satisfactory consistency with the experiment/investigation data in terms of landslide movement and near-field impulsive wave characteristics,thus indicating the applicability and accuracy of the proposed ***,the effects of the HBP model’s rheological parameters on the landslide dynamics and near-field wave characteristics are discussed,providing a parameter calibration method along with sug-gestions for further applications.

关键词： deformable landslide impulsive waves near-field SPH nonNewtonian fluids

Core-shell design of UiO66-Fe_(3)O_(4) configured with EDTA-assisted washing for rapid adsorption and simple recovery of heavy metal pollutants from soil

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Journal of Environmental Sciences 2024年第5期139卷 556-568页

作者： Xi Wang Asif Hussain Qingqing Li Mingyu Ma juan Wu Mingqiang Deng Jie Yang Dengxin Li Department of Environmental Science and Engineering Donghua UniversityShanghai 201620China Department of Environmental Science Federal Urdu University of ArtsScience and Technology75300 KarachiPakistan Shanghai Academy of Environmental Sciences Shanghai 200233China

The coupling of washing with adsorption process can be adopted for the treatment of soils contaminated with heavy metals ***,the complex environment of soil and the competitive behavior of leaching chemicals considerably restrain adsorption capacity of adsorbent material during washing process,which demands a higher resistance of the adsorbents to *** this study,we synthesized strongly magnetic,high specific surface area(573.49 m^(2)/g)UiO66 composites(i.e.,UiO66-Fe_(3)O_(4))using hydrothermal *** UiO66-Fe_(3)O_(4) was applied as an adsorbent during the ethylene diamine tetraacetic acid(EDTA)-assisted washing process of contaminated *** incorporation of UiO66-Fe_(3)O_(4)results in rapid heavy metal removal and recovery from the soil under low concentrations of washing agent(0.001 mol/L)with reduced residual heavy metal mobility of soil after ***,UiO66-Fe_(3)O_(4)can quickly recollect by an external magnet,which offers a simple and inexpensive recovery method for heavy metals from contaminated ***,UiO66-Fe_(3)O_(4)configuration with EDTA-assisted washing process showed opportunities for heavy metals contaminated sites.

关键词： UiO66 composites Metal-EDTA complexes EDTA-assisted washing Heavy metals recovery Soil

Next‑Generation Green Hydrogen: Progress and Perspective from Electricity, Catalyst to Electrolyte in Electrocatalytic Water Splitting

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Nano-Micro Letters 2024年第11期16卷 274-322页

作者： Xueqing Gao Yutong Chen Yujun Wang Luyao Zhao Xingyuan Zhao juan Du Haixia Wu Aibing Chen College of Chemical and Pharmaceutical Engineering Hebei University of Science and TechnologyShijiazhuang 050018People’s Republic of China

Green hydrogen from electrolysis of water has attracted widespread attention as a renewable power *** several hydrogen production methods,it has become the most promising ***,there is no large-scale renewable hydrogen production system currently that can compete with conventional fossil fuel hydrogen *** energy electrocatalytic water splitting is an ideal production technology with environmental cleanliness protection and good hydrogen purity,which meet the requirements of future *** review summarizes and introduces the current status of hydrogen production by water splitting from three aspects:electricity,catalyst and *** particular,the present situation and the latest progress of the key sources of power,catalytic materials and electrolyzers for electrocatalytic water splitting are ***,the problems of hydrogen generation from electrolytic water splitting and directions of next-generation green hydrogen in the future are discussed and *** is expected that this review will have an important impact on the field of hydrogen production from water.

关键词： Hydrogen Electrolysis Hydrogen production Renewable energy Catalyst

Learning to bag with a simulation‐free reinforcement learning framework for robots

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IET Cyber-Systems and Robotics 2024年第2期6卷 52-66页

作者： Francisco Munguia-Galeano Jihong Zhu juan David Hernández Ze Ji Cooper Group University of LiverpoolLiverpoolUK School of Physics Engineering and Technology University of YorkYorkUK School of Computer Science and Informatics Cardiff UniversityCardiffUK School of Engineering Cardiff UniversityCardiffUK

Bagging is an essential skill that humans perform in their daily ***,deformable objects,such as bags,are complex for robots to manipulate.A learning-based framework that enables robots to learn bagging is *** novelty of this framework is its ability to learn and perform bagging without relying on *** learning process is accomplished through a reinforcement learning(RL)algorithm introduced and designed to find the best grasping points of the bag based on a set of compact state *** framework utilises a set of primitive actions and represents the task in five *** our experiments,the framework reached 60% and 80% success rates after around 3 h of training in the real world when starting the bagging task from folded and unfolded states,***,the authors test the trained RL model with eight more bags of different sizes to evaluate its generalisability.

关键词： reinforcement learning robot learning robotics

The guest CH_(3)CN molecule triggers solid-state photochromism in a Cu_(2)I_(2)-based MOF for advanced time-dependent encryption and inkless erasable printing

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Chinese Chemical Letters 2024年第3期35卷 532-537页

作者： Meng-juan Wang Bo Li Yong-Li Wei Shu-Na Zhao Shuang-Quan Zang Henan Key Laboratory of Crystalline Molecular Functional Materials Henan International Joint Laboratory of Tumor Theranostical Cluster MaterialsGreen Catalysis Centerand College of ChemistryZhengzhou UniversityZhengzhou 450001China College of Chemistry and Pharmaceutical Engineering Nanyang Normal UniversityNanyang 473061China

It remains a big challenge to develop solid-state stimuli-responsive materials for time-dependent information encryption and inkless erasable printing with long retention ***,a 2D Cu_(2)I_(2)-based MOF with photoresponsive spiropyran(SP)groups orderly installed on its skeleton is *** structural isomerization from SP to colored merocyanine(MC)form can be triggered by removing the CH_(3)CN ***,the degree of structural isomerization and the retention time can be adjusted by controlling the amount of CH_(3)CN guests,exhibiting dynamic photochromic behavior with multicolor states and tunable retention *** on these advantages,time-dependent information encryption is successfully ***,the long retention time(>72 h)of the MC form under daylight conditions in the CH_(3)CN-removed Cu_(2)I_(2)-based MOF and good repeatability make it promising in various applications,such as temporary calendars,price-cards,billboards,and reusable identity *** work provides a novel design strategy to fabricate multi-functional MOF-based smart materials for challenging applications of time-dependent information encryption and inkless erasable printing.

关键词： Stimuli-responsive materials Spiropyran Solid-state photochromism Time-dependent encryption Inkless erasable printing

Robot-assisted treatment of secondary epilepsy caused by parasitic infection:a case report

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Acta Epileptologica 2024年第2期7卷 143-150页

作者： juan Luo Xin Chen Sixun Yu Haifeng Shu Department of Neurosurgery Affiliated Hospital of Southwest Medical UniversityLuzhou Sichuan 646000China Department of Neurosurgery General Hospital of the Western Theater Command of the PLAChengdu Sichuan 610083China

Background Cerebral sparganosis represents the most severe manifestation of sparganosis,with a relatively low global *** cases of secondary epileptic seizures caused by sparganosis infection in the functional areas of the brain,what advanced neurosurgical techniques should be employed to precisely identify and excise the epi-leptic lesions in the deep functional areas of the brain,aiming to achieve maximal removal while minimising the risk of neurological deficits?This remains a current challenge for epilepsy *** presentation A 24-year-old Chinese male was admitted to our hospital,presenting with a history of left limb twitching persisting for over a *** main clinical symptoms presented twitching and numbness of his left limb without loss of *** the premise of inappropriate anti-seizure treatment,recurrent epilepsy attacked *** patient’s diagnosis was considered as“space-occupying lesions in the several lobes of brain,secondary epilepsy”after comprehensive assessment and *** experts considered that the patient’s space-occupying lesions in the right frontal and parietal lobes were highly suspected to be infected by *** report delved into the application of neurosurgery robot-assisted frameless stereotaxic technology and intraopera-tive stereotactic electroencephalography(SEEG)monitoring technology to accurately locate and optimize removal of parasite-related epileptic lesions situated in functional areas of the *** a result,the patient had achieved seizure freedom,leaving no symptoms of neurological *** With the highly integrated development of imaging technology,mechanical technology,computer control technology,and artificial intelligence,surgical robots are poised to play a larger role across various neurosur-gical specialties in the *** benefits for patients and the promising application of this technology,its utilization holds significant value.

关键词： Cerebral sparganosis Secondary epilepsy Robot Frameless stereotaxic technology

Strategies to advance thermoelectric performance of PbSe and PbS materials

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Rare Metals 2024年第9期43卷 4099-4114页

作者： Zheng-Hao Hou Xin Qian Qiu-juan Cui Shu-Fang Wang Li-Dong Zhao Shijiazhuang Key Laboratory of Low Carbon Energy Materials College of Chemical EngineeringShijiazhuang UniversityShijiazhuang 050035China Hebei Key Lab of Optic-Electronic Information and Materials College of Physics Science and TechnologyHebei UniversityBaoding 071002China School of Materials Science and Engineering Beihang UniversityBeijing 100191China

Thermoelectric materials possess the unique capability to convert thermal energy into electric energy and vice versa,making them promising for waste heat recovery and efficient cooling ***,extensively investigated thermoelectric materials such as Bi2Te3,PbTe and GeTe exhibit superior thermoelectric properties at room temperature and medium temperature ***,the broad application of these thermoelectric materials has been impeded by the high cost and restricted accessibility of Te and Ge in the earth's *** the past few years,researchers have shown increasing interest in PbSe-and PbS-based materials,primarily attributed to their abundant elemental supply and relatively low *** assessment of research progress and a comprehensive overview of optimization strategies in time can significantly contribute to further improving the thermoelectric *** strategies include optimizing carrier concentration(aliovalent doping,dynamic doping and defect state),enhancing density-of-state effective mass(band convergence,band flattening and energy filtering effect),optimizing carrier mobility(band sharpening and band alignment)and reducing lattice thermal conductivity(all-scale hierarchical defect structures designing).This systematic summary and analysis provide novel insights and perspectives for the development of thermoelectric materials.

关键词： PbSe and PbS thermoelectric materials Carrier concentration Density-of-state effective mass Carrier mobility Lattice thermal conductivity

A novel histone methyltransferase gene Cg SDG40 positively regulates carotenoid biosynthesis during citrus fruit ripening

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Journal of Integrative Agriculture 2024年第8期23卷 2633-2648页

作者： Jialing Fu Qingjiang Wu Xia Wang juan Sun Li Liao Li Li Qiang Xu National Key Laboratory for Germplasm Innovation&Utilization of Horticultural Crops College of Horticulture&Forestry ScienceHuazhong Agricultural UniversityWuhan 430070China Hubei Hongshan Laboratory Wuhan 430070China Institute of Horticultural Sciences Jiangxi Academy of Agricultural SciencesNanchang 330200China Plant Breeding and Genetics Section School of Integrative Plant ScienceCornell UniversityNew York 14853USA Robert W.Holley Center for Agriculture and Health USDA-Agricultural Research ServiceCornell UniversityNew York 14853USA

The flesh color of pummelo(Citrus maxima)fruits is highly diverse and largely depends on the level of carotenoids,which are beneficial to human *** is vital to investigate the regulatory network of carotenoid biosynthesis to improve the carotenoid content in ***,the molecular mechanism underlying carotenoid accumulation in pummelo is not fully *** this study,we identified a novel histone methyltransferase gene,CgSDG40,involved in carotenoid regulation by analyzing the flesh transcriptome of typical white-fleshed pummelo,red-fleshed pummelo and extreme-colored F1 hybrids from a segregated pummelo *** of CgSDG40 corresponded to flesh color change and was highly coexpressed with ***,CgSDG40 and CgPSY1 are located physically adjacent to each other on the chromosome in opposite directions,sharing a partially overlapping promoter *** localization analysis indicated that CgSDG40 localizes to the *** of CgSDG40 significantly increased the total carotenoid content in citrus calli relative to that in wild *** addition,expression of CgPSY1 was significantly activated in overexpression lines relative to wild *** together,our findings reveal a novel histone methyltransferase regulator,CgSDG40,involved in the regulation of carotenoid biosynthesis in citrus and provide new strategies for molecular design breeding and genetic improvement of fruit color and nutritional quality.

关键词： pummelo SET domain protein epigenetic regulation PSY1 lycopene fruit quality fruit color