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Improved Reall-Santos method for AdS black holes in general 4-derivative gravities

Science China(Physics,Mechanics & Astronomy) 2024年第8期67卷 74-86页

作者： peng-ju Hu Liang Ma Hong Lü Yi Pang Center for Joint Quantum Studies and Department of Physics School of ScienceTianjin UniversityTianjin 300350China Joint School of National University of Singapore and Tianjin University International Campus of Tianjin UniversityFuzhou 350207China peng Huanwu Center for Fundamental Theory Hefei 230026China

For asymptotically flat black holes,Reall-Santos method is a convenient tool to compute leading higher derivative corrections to the thermodynamic quantities without actually solving the modified field ***,there are subtleties in its generalization to asymptotically AdS black holes with general higher derivative *** of all,it is necessary to know all the higher derivative holographic counterterms and the surface terms implementing the variational principle and subtracting the *** then needs to solve for the modified AdS radius and rescale the time coordinate in an appropriate way such that the induced metric on the conformal boundary of AdS black hole is not *** observe that Reall-Santos method can be directly applied to a particular 4-derivative gravity model,known as the Einstein-Weyl gravity,which does not modify the AdS radius and requires only the Gibbons-Hawking-York term and holographic counterterms for the 2-derivative *** thus suggest that to compute the thermodynamic quantities of AdS black holes in general 4-derivative theories of gravity,one simply needs to transform it to a Einstein-Weyl gravity with identical thermodynamic variables by appropriate field *** explicitly verify this proposal with spherically-symmetric and static charged black holes in Einstein-Maxwell theory extended with generic 4-derivative interactions.

关键词： black holes thermodynamics higher-derivative corrections effective theories higher dimensional black holes quantum gravity

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Double enzyme mimetic activities of multifunctional Ag nanoparticle-decorated Co_(3)V_(2)O_(8)hollow hexagonal prismatic pencils for application in colorimetric sensors and disinfection

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Nano Materials Science 2024年第2期6卷 244-255页

作者： Ying Gao peng ju Yu Zhang Yuxin Zhang Xiaofan Zhai Jizhou Duan Baorong Hou Key Laboratory of Marine Environmental Corrosion and Bio-fouling Institute of OceanologyChinese Academy of SciencesQingdao266071PR China Key Laboratory of Marine Eco-Environmental Science and Technology Marine Bioresource and Environment Research CenterFirst Institute of OceanographyMinistry of Natural ResourcesQingdao266061PR China University of Chinese Academy of Sciences Beijing100049PR China Open Studio for Marine Corrosion and Protection Pilot National Laboratory for Marine Science and Technology(Qingdao)Qingdao266071PR China Center for Ocean Mega-Science Chinese Academy of SciencesQingdao266071PR China College of Materials Science and Engineering Chongqing UniversityChongqing400044China

Since the catalytic activity of most nanozymes is still far lower than the corresponding natural enzymes,there is urgent need to discover novel highly efficient enzyme-like *** this work,Co_(3)V_(2)O_(8)with hollow hexagonal prismatic pencil structures were prepared as novel artificial enzyme *** were then decorated by photo-depositing Ag nanoparticles(Ag NPs)on the surface to further improve its catalytic *** Ag NPs decorated Co_(3)V_(2)O_(8)(ACVPs)showed both excellent oxidase-and peroxidase-like catalytic *** can oxidize the colorless 3,3’,5,5’-tetramethylbenzidine rapidly to induce a blue *** enhanced enzyme mimetic activities can be attributed to the surface plasma resonance(SPR)effect of Ag NPs as well as the synergistic catalytic effect between Ag NPs and Co_(3)V_(2)O_(8),accelerating electron transfer and promoting the catalytic *** were applied in constructing a colorimetric sensor,validating the occurrence of the Fenton reaction,and disinfection,presenting favorable catalytic *** enzyme-like catalytic mechanism was studied,indicating the chief role of⋅O_(2)-radicals in the catalytic *** work not only discovers a novel functional material with double enzyme mimetic activity but also provides a new insight into exploiting artificial enzyme mimics with highly efficient catalytic ability.

关键词： Co_(3)V_(2)O_(8) Ag NPs Enzyme mimetic Colorimetric sensor Disinfection

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Seismic response and correlation analysis of a pile-supported wharf to near-fault pulse-like ground motions

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Earthquake Engineering and Engineering Vibration 2024年第4期23卷 883-897页

作者： Wang Jianfeng Su Lei Xie Libo Ling Xianzhang ju peng School of Civil Engineering Qingdao University of TechnologyQingdao 266500China School of Civil Engineering Harbin Institute of TechnologyHarbin 150006China No.2 Engineering Company Ltd.of CCCC First Harbor Engineering Company Ltd Qingdao 266071China

Earthquake investigations have shown that near-fault pulse-like(NF-P)ground motions have unique characteristics compared to near-fault non-pulse-like(NF-NP)and far-field(FF)ground *** is necessary to study the seismic response of pile-supported wharf(PSW)structures under NF-P ground *** this study,a three-dimensional finite element numerical model is created to simulate a *** imparting three types of ground motion,the engineering demand parameters(EDPs)of PSW under NF-P ground motions were analyzed and compared,in which EDPs are the maximum displacement and bending moment of the *** intensity measures(IMs)were selected to characterize the properties of ground *** correlation between IMs and EDPs was *** results show that the piles present larger displacement and bending moment under NF-P ground motions compared to NF-NP and FF ground *** of the IMs have a high correlation with EDPs under NF-P ground motions,and these IMs are more applicable to FF ground *** correlation coefficients between EDPs and IMs under three types of ground motion were obtained,which will provide a valuable reference for the seismic design of PSWs.

关键词： pile-supported wharf correlation analysis near-fault pulse-like ground motion intensity measure seismic response

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Photocatalytic vinyl radical-mediated multicomponent 1,4-/1,8-carboimination across alkynes and olefins/(hetero)arenes

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Science China Chemistry 2024年第2期67卷 558-567页

作者： Shan-Shan Li Yu-Shi Jiang Xue-Ling Luo Xuming Ran Yuqiang Li Dong Wu Cheng-Xue Pan peng-ju Xia School of Chemistry and Pharmaceutical Sciences Guangxi Normal UniversityGuilin541004China Shanghai Artificial Intelligence Laboratory Shanghai200433China The Institute for Advanced Studies Wuhan UniversityWuhan430064China

We developed a highly selective and efficient multicomponent transformation by utilizing alkynes and olefins/(hetero)arenes through photoinduced energy-transfer *** reaction involves the formation of three distinct chemical bonds,namely C(sp~3)–C(sp~2),C(sp~2)–C(sp~3),and C(sp~3)–N,in a single coordinated *** strategy used a vinyl radical-mediated radical relay approach under mild conditions,exhibiting a broad substrate scope(>70 examples),excellent functional-group tolerance,and remarkable regio-and *** the utilization of a combination of experimental techniques and density functional theory(DFT),we delved deeper into the mechanistic intricacies of this distinctive *** revealed that the selective radical addition to electron-deficient alkynes,rather than olefins,was governed by the inherent reactivity of alkyl *** discovery presented a highly effective approach for the synthesis of stereodefined multisubstituted alkenes.

关键词： alkyne-olefin coupling DFT studies regio-and anti-stereoselectivity multisubstituted alkenes

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Multiple factors influencing high-purity indium electrolytic refining

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Chinese Journal of Chemical Engineering 2024年第7期71卷 148-160页

作者： Hong-Qiang Fan Fei Li Hong-Xing Zheng Wu-ji Pan Mei-Zhen Wu Yashar Behnamian ju-Bo peng Dong-Hai Lin State Key Laboratory of Advanced Special Steel&School of Materials Science and Engineering Shanghai UniversityShanghai 200444China Shanghai Engineering Research Center for Integrated Circuits and Advanced Display Materials Shanghai UniversityShanghai 200444China Research&Development Center Yunnan Tin Group(Holding)Limited CompanyKunming 650032China Department of Chemical and Materials Engineering University of AlbertaEdmonton T6G 2V4AlbertaCanada School of Energy and Materials Shanghai Key Laboratory of Engineering Materials Application and EvaluationShanghai Polytechnic UniversityShanghai 201209China

The effects of various contaminants in the electrolytic refinement of indium were investigated using a glow discharge mass spectrometer(GDMS).The effects of several factors such as the indium ion(In3+)concentration,the sodium chloride(NaCl)concentration,the current density,the gelatin concentration,the pH,and the electrode distance,were *** variations in impurity levels concerning gelatin concentration were *** the gelatin and In3+concentration were moderately positively correlated with the Pb *** Sb concentration was associated positively with the NaCl concentration,while the Ti concentration had an adverse correlation with the NaCl *** Bi element content was positively linked to the electrode *** the current density increased,Cu,Pb,and Bi impurities initially rose and then eventually ***,a critical current density of 45 A·m^(-2) was identified in this behavior.

关键词： High-purity indium Electrolysis Multiple factors Electrochemistry Purification

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Drug delivery with Mn-doped MoO_(2) for photothermalenhanced chemotherapy in fighting cancers

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Rare Metals 2024年第5期43卷 2230-2240页

作者： Ping Zhao Hai-Fa Zheng ju peng Xing-Long Li Fazal Raziq Xiao-jun Liu Hao-Quan Yu Jin-Lu Tang Yi-Fan Kang Wen-Huan Huang School of Chemistry and Chemical Engineering Guangdong Pharmaceutical UniversityGuangzhou 510006China KAUST Catalysis Center King Abdullah University of Science and Technology23955-6900 ThuwalKingdom of Saudi Arabia Key Laboratory of Chemical Additives for China National Light Industry College of Chemistry and Chemical EngineeringShaanxi University of Science and TechnologyXi'an 710021China

Although chemotherapy has been intensively applied in cancer treatments,its inadequate therapeutic efficacy and severe side effects are still under constant *** used as anti-tumor drug delivery system(DDS)have attracted tremendous attentions owing to their various intriguing ***,Mn-doped MoO_(2)nanoparticles coated with ZrO_(2)and capped with Bi_(2)O_(3)have been designed as a DDS,namely *** possesses good magnetic properties,great photothermal conversion ability,sensitive tumor microenvironment(TME)responsiveness,and good biocompatibility in hemocompatibility in ***,MMZB has been utilized to load the chemotherapeutic agent daunomycin(DNM)(MMZB@DNM)for chemo-photothermal combined ***@DNM demonstrates a more impressive anti-cancer effect than the individual photothermal or chemotherapy both in vitro and in ***,the analysis of tumor specimen sections and serum levels after the treatment indicates negligible side effects for MMZB@DNM in *** contribution provides a valuable concept in designing therapeutic agents for achieving significantly enhanced tumor treatments,which benefits from the synergistic combination of chemotherapy and photothermal therapy in one single nanoagent.

关键词： Mn-doped MoO_(2) Bi_(2)O_(3) Nanocarrier Photothermal Chemotherapy

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Enhancing Storage Efficiency and Performance: A Survey of Data Partitioning Techniques

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Journal of Computer Science & Technology 2024年第2期39卷 346-368页

作者：刘鹏举李翠平陈红 Distinguished Member CCF 1.School of InformationRenmin University of ChinaBeijing 100872China Key Laboratory of Data Engineering and Knowledge Engineering of the Ministry of Education Beijing 100872China

Data partitioning techniques are pivotal for optimal data placement across storage devices,thereby enhancing resource utilization and overall system ***,the design of effective partition schemes faces multiple challenges,including considerations of the cluster environment,storage device characteristics,optimization objectives,and the balance between partition quality and computational ***,dynamic environments necessitate robust partition detection *** paper presents a comprehensive survey structured around partition deployment environments,outlining the distinguishing features and applicability of various partitioning strategies while delving into how these challenges are *** discuss partitioning features pertaining to database schema,table data,workload,and runtime *** then delve into the partition generation process,segmenting it into initialization and optimization stages.A comparative analysis of partition generation and update algorithms is provided,emphasizing their suitability for different scenarios and optimization ***,we illustrate the applications of partitioning in prevalent database products and suggest potential future research directions and *** survey aims to foster the implementation,deployment,and updating of high-quality partitions for specific system scenarios.

关键词： data partitioning survey partitioning feature partition generation partition update

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LLM-105的分子间相互作用和热力学性质

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物理学报 2024年第4期73卷 235-244页

作者：范俊宇高楠王鹏举苏艳太原师范学院物理系晋中030619 台州学院材料科学与工程学院台州318000 之江实验室杭州311100 大连理工大学三束材料改性教育部重点实验室大连116024

应用第一性原理可以计算含能材料0 K下的结构和物理性质,但温度效应的缺失通常会导致计算数据与实验结果产生偏差.同时,与温度相关的热力学参数是含能材料在宏观和介观尺度下建模的关键输入.为此,本文以高能低感炸药1-氧-2,6-二氨基-3,5... 详细信息

应用第一性原理可以计算含能材料0 K下的结构和物理性质,但温度效应的缺失通常会导致计算数据与实验结果产生偏差.同时,与温度相关的热力学参数是含能材料在宏观和介观尺度下建模的关键输入.为此,本文以高能低感炸药1-氧-2,6-二氨基-3,5-二硝基吡嗪(LLM-105)为研究体系,基于准简谐近似,采用色散修正的密度泛函理论研究温度加载下LLM-105的分子间相互作用和热力学性质.晶格参数和热膨胀系数的演化表明LLM-105分子间相互作用具有强烈的各向异性,其中b轴方向(分子层间)的膨胀率远高于ac平面(分子层内).Hirshfeld表面及其指纹图分析进一步证实LLM-105的分子间相互作用主要取决于O···H构成的氢键.结合Mulliken布居数和结构分析,温度加载下氢键相互作用的变化可诱发硝基旋转,并使得C—NO_(2)键的强度明显减弱,为高温分解反应的触发键提供了理论依据.此外,本文计算了等容和等压条件下的热容、熵以及等温和绝热条件下的体模量等基础热力学参数.其中绝热条件下的体模量与实验值吻合,同时体模量随温度的演化反映了LLM-105在温度加载下的软化行为.上述理论研究可用于构建含能材料在介观和宏观尺度下的模型,也为测量原子分子水平下的热力学性质提供了重要的参考价值.

关键词： LLM-105 热力学性质分子间相互作用准简谐近似

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衡先培辨治垂体瘤术后持续性高钠血症临床经验

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中国中西医结合杂志 2024年第5期44卷 619-622页

作者：全鹏举衡先培福建中医药大学附属人民医院内分泌代谢病科福州350004

位于鞍区的下丘脑—垂体是人体水钠调节中枢。垂体瘤手术损伤导致该中枢受损,进而水钠失衡,发生高钠血症^([1])。多数鞍区术后渴感正常的高钠血症患者可在1周内恢复^([2]),属于短暂性高钠血症。但是,有部分鞍区术后患者高钠血症持续两... 详细信息

位于鞍区的下丘脑—垂体是人体水钠调节中枢。垂体瘤手术损伤导致该中枢受损,进而水钠失衡,发生高钠血症^([1])。多数鞍区术后渴感正常的高钠血症患者可在1周内恢复^([2]),属于短暂性高钠血症。但是,有部分鞍区术后患者高钠血症持续两周以上,常可造成严重后果^([3])。这种持续性高钠血症又分为两种情况:一种去氨加压素有反应;另一种对去氨加压素无明显反应,仅能采取限盐、强制补液来治疗。目前现代医学对第一种情况研究相对较多,有许多案例报道,且相应的评估、治疗均有文献详细记录,医师治疗有据可循^([4,5])。

关键词：高钠血症去氨加压素垂体瘤手术案例报道现代医学衡先培持续性有据可循

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起伏地形下基于非结构网格模型降维的重力三维密度反演

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地球物理学报 2024年第1期67卷 379-393页

作者：高新宇鲁宝亮安国强巨鹏长安大学地质工程与测绘学院西安710054 海洋油气勘探国家工程研究中心北京100028 长安大学西部矿产资源与地质工程教育部重点实验室西安710054

复杂起伏地形以及剖分方式对重力反演解释具有重要影响.目前重力密度反演研究主要基于直立长方体模型,这显著降低了对起伏地形和复杂地质体的拟合程度,对重力反演解释易产生较大影响.四面体非结构网格能够更加精细地模拟起伏地形及复杂... 详细信息

复杂起伏地形以及剖分方式对重力反演解释具有重要影响.目前重力密度反演研究主要基于直立长方体模型,这显著降低了对起伏地形和复杂地质体的拟合程度,对重力反演解释易产生较大影响.四面体非结构网格能够更加精细地模拟起伏地形及复杂地质体,为此本文研究了起伏地形条件下基于四面体非结构网格剖分的重力三维密度反演.首先基于Delaunay方法将地下区域剖分为四面体非结构网格,引入垂向导数和相关系数两种方法进行模型降维技术从而减小解的空间,通过添加最小长度约束,深度加权约束,物性范围约束构建目标函数,并采用预条件共轭梯度法求解.为了提高反演效率在计算过程引入OpenMP并行算法.并研究了各项约束以及两种模型降维方法在四面体非结构网格正则化反演中的效果.通过不同深度直立长方体模型以及起伏地形下组合模型试验,基于四面体非结构网格的重力密度反演可以清晰地反映异常体位置.将本文提出的方法应用于美国密苏里州东南部的氧化铁矿床,反演结果与已知岩体具有较好的一致性,进一步证明该方法的正确性和有效性.

关键词：非结构网格起伏地形密度反演模型降维正则化

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