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Driving inward growth of lithium metal in hollow microcapsule hosts by heteroatom‐controlled nucleation

Carbon Energy 2024年第8期6卷 262-272页

作者： Siwon Kim Hong Rim Shin Ki Jae Kim Min‐Sik Park jong‐won lee Division of Materials Science and Engineering Hanyang UniversitySeoulRepublic of Korea Department of Energy Science and Engineering Daegu Gyeongbuk Institute of Science and Technology(DGIST)DaeguRepublic of Korea Department of Energy Science Sungkyunkwan UniversitySuwonRepublic of Korea Department of Advanced Materials Engineering for Information and Electronics Integrated Education for Frontier Science and Technology(BK21 Four)Kyung Hee UniversityYonginRepublic of Korea

The application of Li metal anodes in rechargeable batteries is impeded by safety issues arising from the severe volume changes and formation of dendritic Li ***‐dimensional hollow carbon is receiving increasing attention as a host material capable of accommodating Li metal inside its cavity;however,uncontrollable and nonuniform deposition of Li remains a *** this study,we synthesize metal–organic framework‐derived carbon microcapsules with heteroatom clusters(Zn and Ag)on the capsule walls and it is demonstrated that Ag‐assisted nucleation of Li metal alters the outward‐to‐inward growth in the microcapsule ***‐incorporated microcapsules are prepared via chemical etching of zeolitic imidazole framework‐8 polyhedra and are subsequently decorated with Ag by a galvanic displacement reaction between Ag^(+)and metallic *** introduced Ag significantly reduces the energy barrier and increases the reaction rate for Li nucleation in the microcapsule host upon Li *** combined electrochemical,microstructural,and computational studies,we verify the beneficial role of Ag‐assisted Li nucleation in facilitating inward growth inside the cavity of the microcapsule host and,in turn,enhancing electrochemical *** study provides new insights into the design of reversible host materials for practical Li metal batteries.

关键词： hollow carbon hosts lithium metal batteries lithium plating metal-organic frameworks nucleation

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Permeability evaluation for artificial single rock fracture according to geometric aperture variation using electrical resistivity

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Journal of Rock Mechanics and Geotechnical Engineering 2021年第4期13卷 787-797页

作者： Hangbok lee jong-won lee Tae-Min Oh Deep Subsurface Research Center Korea Institute of Geoscience and Mineral ResourcesDaejeon34132Republic of Korea Department of Civil and Environmental Engineering Pusan National UniversityBusan46241Republic of Korea

A convenient approach was proposed by which to evaluate and monitor the permeability of a rock fracture by verifying the quantitative correlation between the electrical resistivity and permeability at laboratory *** this purpose,an electrical resistivity measurement system was applied to the laboratory experiments using artificial cells with the shape of a single rock *** experiments were conducted using rock fractures according to the geometry,aperture sizes,wavelengths,and roughness *** overall negative relationship between the normalized electrical resistivity values and the aperture sizes directly linked with the permeability,was well fitted by the power-law function with a large determination coefficient(≈0.86).The effects of wavelength and roughness amplitude of the rock fracture on the electrical resistivity were also *** showed that the electrical resistivity was slightly increased with decreasing wavelength and increasing roughness *** empirical model for evaluating the permeability of a rock fracture was proposed based on the experimental *** the field,if the electrical resistivity of pore groundwater could be measured in advance,this empirical model could be applied effectively for simple,quick monitoring of the fracture *** uncertainty may be associated with the permeability estimation due to the limited control parameters considered in this research,this electrical resistivity approach could be helpful to monitor the rock permeability in deep underground facilities such as those used for radioactive waste repositories or forms of energy storage.

关键词： Permeability Rock fracture Electrical resistivity Fracture geometry Long-term monitoring

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Detection of damage locations and damage steps in pile foundations using acoustic emissions with deep learning technology

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Frontiers of Structural and Civil Engineering 2021年第2期15卷 318-332页

作者： Alipujiang JIERULA Tae-Min OH Shuhong WANG Joon-Hyun lee Hyunwoo KIM jong-won lee School of Resource&Civil Engineering Northeastern UniversityShenyang110819China School of Mechanical Engineering Pusan National UniversityBusan46241Korea Department of Civil and Environmental Engineering Pusan National UniversityBusan46241Korea Korea Institute of Geoscience and Mineral Resource(KIGAM) Daejeon34132Korea

The aim of this study is to propose a new detection method for determining the damage locations in pile foundations based on deep learning using acoustic emission ***,the damage location is simulated using a back propagation neural network deep learning model with an acoustic emission data set acquired from pile hit *** particular,the damage location is identified using two parameters:the pile location(PL)and the distance from the pile cap(DS).This study investigates the influences of various acoustic emission parameters,numbers of sensors,sensor installation locations,and the time difference on the prediction accuracy of PL and *** addition,correlations between the damage location and acoustic emission parameters are ***,the damage step condition is determined using a classification model with an acoustic emission data set acquired from uniaxial compressive strength ***,a new damage detection and evaluation method for pile foundations is *** new method is capable of continuously detecting and evaluating the damage of pile foundations in service.

关键词： pile foundations damage location acoustic emission deep learning damage step

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Low-temperature synthesis of Fe_(2)(MoO_(4))_(3) nanosheets: A cathode for sodium ion batteries with kinetics enhancement

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Nano Research 2021年第11期14卷 3977-3987页

作者： Ha Tran Huu N.S.M.Viswanath Ngoc Hung Vu jong-won lee won Bin Im Division of Materials Science and Engineering Hanyang University222Wangsimni-roSeongdong-guSeoul04763Republic of Korea School of Materials Science and Engineering Chonnam National University77 Yongbong-roBuk-guGwangju61186Republic of Korea Falcuty of Biotechnology Chemistry and Environmental EngineeringPhenikaa UniversityHanoi10000Vietnam A&A Green Phoenix Group Phenikaa Research and Technology Institute(PRATI)167 Hoang NganHanoi10000Vietnam Department of Energy Science and Engineering Daegu Gyeongbuk Institute of Science and Technology(DGIST)333 Techno Jungang-daeroHyeonpung-eupDalseonggunDaegu42988Republic of Korea

Sodium ion batteries (SIBs) are alternatives to lithium ion batteries (LIBs), and offer some significant benefits such as cost reduction and a lower environmental impact;however, to compete with LIBs, further research is required to improve the performance of SIBs. In this study, an orthorhombic Na super ionic conductor structural Fe_(2)(MoO_(4))_(3) nanosheet with amorphous-crystalline core-shell alignment was synthesized using a facile low-temperature water-vapor-assisted solid-state reaction and applied as a cathode material for SIBs. The obtained material has a well-defined three-dimensional stacking structure, and exhibits a high specific capacity of 87.8 mAh·g^(−1) at a current density of 1 C = 91 mA·g^(−1) after 1,000 cycles, which is due to the considerable contribution of extra surface-related reaction such as the pseudo-capacitive process. This material shows significantly improved cycling and rated behavior as well as enhanced performance under high- and low-temperature conditions, as compared to the same materials prepared by the conventional high-temperature solid-state reaction. This enhancement is explained by the unique morphology in combination with the improved kinetics of the electrochemical reaction due to its lower charge transfer resistance and higher sodium ion conductivity.

关键词： low-temperature synthesis cathode sodium ion batteries kinetics Na+super ionic conductor(NASICON)

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Porously Reduced 2-Dimensional Bi2O2CO3 Petals for Strain-Mediated Electrochemical CO2 Reduction to HCOOH

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Energy & Environmental Materials 2024年第1期7卷 219-225页

作者： won Seok Cho Dae Myung Hong Wan Jae Dong Tae Hyung lee Chul jong Yoo Donghwa lee Ho won Jang jong-Lam lee Department of Materials Science and Engineering Pohang University of Science and Technology (POSTECH) Department of Materials Science and Engineering Research Institute of Advanced Materials Seoul National University

Here we introduce bismuth-based catalysts for the efficient electrochemical reduction of CO2to formic acid（HCOOH）,which are composed of petalshaped Bi2O2CO3（BOC） that spontaneously formed from Bi thin film in aqueous carbonate solution at room *** the electrochemical reduction process,the BOC petals transform to reduced BOC（R-BOC）consisting of individual BOC and Bi domains.

关键词： bismuth carbon dioxide reduction formic acid heterointerfaces strain

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Overcoming the fundamental light-extraction efficiency limitations of deep ultraviolet light-emitting diodes by utilizing transverse-magnetic-dominant emission

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Light(Science & Applications) 2015年第1期4卷 422-429页

作者： Dong Yeong Kim Jun Hyuk Park jong won lee Sunyong Hwang Seung Jae Oh Jungsub Kim Cheolsoo Sone EFred Schubert jong Kyu Kim Department of Materials Science and Engineering Pohang University of Science and TechnologyPohang 790-784Korea LED Business Samsung ElectronicsYongin 446-920Korea Future Chips Constellation Department of ElectricalComputerand Systems EngineeringRensselaer Polytechnic InstituteTroyNY 12180USA

While the demand for deep ultraviolet(DUV)light sources is rapidly growing,the efficiency of current AlGaN-based DUV light-emitting diodes(LEDs)remains very low due to their fundamentally limited light-extraction efficiency(lee),calling for a novel lee-enhancing approach to deliver a real ***,we propose sidewall emission-enhanced(SEE)DUV LEDs having multiple light-emitting mesa stripes to utilize inherently strong transverse-magnetic polarized light from the AlGaN active region and three-dimensional reflectors between the *** SEE DUV LEDs show much enhanced light output power with a strongly upward-directed emission due to the exposed sidewall of the active region and Al-coated selective-area-grown n-type GaN *** devices also show reduced operating voltage due to better n-type ohmic contact formed on the regrown n-GaN stripes when compared with conventional ***,the proposed approach simultaneously improves optical and electrical *** addition,strategies to further enhance the lee up to the theoretical optimum value and control emission directionality are discussed.

关键词： deep ultraviolet light-emitting diodes light-extraction efficiency

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Benefit in physical function and quality of life to nonsurgical treatment of varicose veins: Pilot study

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World Journal of Clinical Cases 2024年第3期12卷 517-524页

作者： Gwon-Min Kim BoKun Kim Minwoo Jang jong-Hwan Park Miju Bae Chung won lee jong won Kim Up Huh Medical Research Institute Pusan National University School of MedicineYangsan 50612South Korea Future Convergence Research Institute Changwon National UniversityChangwon 51140South Korea Department of Convergence Medical Science School of MedicinePusan National UniversityYangsan 50612South Korea Health Convergence Medicine Laboratory Biomedical Research InstitutePusan National University HospitalBusan 49241South Korea Department of Thoracic and Cardiovascular Surgery Pusan National University School of MedicineBiomedical Research InstitutePusan National University HospitalBusan 49241South Korea

BACKGROUND Studies on varicose veins have focused its effects on physical function;however,whether nonsurgical treatments alter muscle oxygenation or physical function remains ***,the differences in such functions between individuals with varicose veins and healthy individuals remain *** To investigate changes in physical function and the quality of life(QOL)following nonsurgical treatment of patients with varicose veins and determine the changes in their muscle oxygenation during *** We enrolled 37 participants(those with varicose veins,n=17;healthy individuals,n=20).We performed the following measurements pre-and post-nonsurgical treatment in the varicose vein patients and healthy individuals:Calf muscle oxygenation during the two-minute step test,open eyes one-leg stance,30 s sit-to-stand test,visual analog scale(VAS)for pain,Pittsburgh sleep quality index,physical activity assessment,and QOL *** Varicose veins patients and healthy individuals differ in most variables(physical function,sleep quality,and QOL).Varicose veins patients showed significant differences between pre-and post-nonsurgical treatment—results in the 30 sit-to-stand test[14.41(2.45)to 16.35(4.11),P=0.018],two-minute step test[162.29(25.98)to 170.65(23.80),P=0.037],VAS for pain[5.35(1.90)to 3.88(1.73),P=0.004],and QOL[39.34(19.98)to 26.69(17.02),P=0.005];however,no significant difference was observed for muscle *** Nonsurgical treatment improved lower extremity function and QOL in varicose veins patients,bringing their condition close to that of healthy *** studies should include patients with severe varicose veins requiring surgery to confirm our findings.

关键词： Varicose vein Nonsurgical treatment Physical function Quality of life Near infrared spectroscopy

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Pyrometallurgical recycling of end-of-life lithium-ion batteries

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International Journal of Minerals,Metallurgy and Materials 2024年第7期31卷 1554-1571页

作者： Juheon lee Kwang won Park Il Sohn Sanghoon lee Department of Materials Science and Engineering Seoul 03722Korea Yonsei Industry Cooperation Center Yonsei UniversitySeoul 03722Korea RD Solution Wanju gunJeollabuk do 55365Korea

The global importance of lithium-ion batteries(LIBs)has been increasingly underscored with the advancement of high-performance energy storage ***,the end-of-life of these batteries poses significant challenges from environmental,economic,and resource management *** review paper focuses on the pyrometallurgy-based recycling process of lithium-ion batteries,exploring the fundamental understanding of this process and the importance of its *** on the high energy consumption and emission gas issues of the pyrometallurgical recycling process,we systematically analyzed the capital-intensive nature of this process and the resulting technological ***,we conducted an in-depth discussion on the future research directions to overcome the existing technological barriers and *** review will provide valuable insights for researchers and industry stakeholders in the battery recycling field.

关键词： spent lithium-ion batteries recycling sustainability lithium valuable metal

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Realizing High Thermoelectric Performance in n-Type Se-Free Bi2Te3 Materials by Spontaneous Incorporation of FeTe2 Nanoinclusions

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Energy & Environmental Materials 2024年第4期7卷 344-354页

作者： Jamil Ur Rahman Woo Hyun Nam Yong-Jae Jung jong Ho won jong-Min Oh Nguyen Van Du Gul Rahman Víctor M.García-Suárez Ran He Kornelius Nielsch Jung Young Cho won-Seon Seo jong Wook Roh Sang-il Kim Soonil lee Kyu Hyoung lee Hyun Sik Kim Weon Ho Shin Leibniz Institute for Solid State and Materials Research Advanced Materials Convergence R&D Division Korea Institute of Ceramic Engineering & Technology Department of Electronic Materials Engineering Kwangwoon University Department of Energy Engineering Dankook University Faculty of Fundamental Science Phenikaa University Department of Physics Quaid-i-Azam University Departamento de Física Universidad de Oviedo Nanomaterials and Nanotechnology Research Center-CINN Department of Materials Science and Engineering Yonsei University School of Nano & Materials Science and Engineering Kyungpook National University Department of Materials Science and Engineering University of Seoul School of Materials Science and Engineering Changwon National University

Bi2Te3-based materials have drawn much attention from the thermoelectric community due to their excellent thermoelectric performance near room ***,the stability of existing n-type Bi2（Te,Se）3materials is still low due to the evaporation energy of Se (37.70 kJ mol-1) being much lower than that of Te (52.55 kJ mol-1).The evaporated Se from the material causes problems in interconnects of the module while degrading the efficiency.

关键词： Bi2Te3 energy harvesting FeTe2 nanoinclusion n-type materials thermoelectric

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Occlusal Forces on Implant Prosthesis at Various Occlusal Heights

Occlusal Forces on Implant Prosthesis at Various Occlusal He...

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第八次全国口腔修复学学术年会

作者： jong-won lee Ji-Man Park Department of Prosthodontics Ewha Womans University

Purpose:The purpose of this study was to evaluate and compare the strain development at different occlusal hei ghts of the implant prosthesis and adjacent teeth by using strain *** and Methods:The test model was constructed using auto-polymerizing polyurethane resin,artificial re sin teeth and an implant gold crown(#46i).Group function occlusal scheme was established using a Hanau articulat *** resin block containina implant fixture and implant gold crown was sectioned and 2

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