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From concept to commercialization:A review of tubular solid oxide fuel cell technology

Journal of Energy Chemistry 2024年第10期97卷 79-109页

作者： Ruyan Chen Yuan gao jiutao gao Huiyu Zhang Martin Motola Muhammad Bilal Hanif Cheng-Xin Li State Key Laboratory for Mechanical Behavior of Materials School of Materials Science and Engineering Xi'an Jiaotong University Department of Inorganic Chemistry Faculty of Natural Sciences Comenius University Bratislava

The reduced sealing difficulty of tubular solid oxide fuel cells(SOFCs) makes the stacking of tubular cell groups relatively easy,and the thermal stress constraints during stack operation are smaller,which helps the stack to operate stably for a long *** special design of tubular SOFC structures can completely solve the problem of high-temperature sealing,especially in the design of multiple single-cell series integrated into one tube,where each cell tube is equivalent to a small electric stack,with unique characteristics of high voltage and low current output,which can significantly reduce the ohmic polarization loss of tubular *** paper provides an overview of typical tubular SOFC structural designs both domestically and *** on the geometric structure of tubular SOFCs,they can be divided into bamboo tubes,bamboo flat tubes,single-section tubes,and single-section flat tube ***,this article provides an overview of commonly used materials and preparation methods for tubular SOFCs,including commonly used materials and preparation methods for support and functional layers,as well as a comparison of commonly used preparation methods for microtubule SOFCs,It introduced the three most important parts of building a fuel cell stack:manifold,current collector,and ceramic adhesive,and also provided a detailed introduction to the power generation systems of different tubular SOFCs,Finally,the development prospects of tubular SOFCs were discussed.

关键词： Geometric structure Preparation methods Stack Support material Tubular solid oxide fuel cell

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管式固体氧化物燃料电池技术进展

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硅酸盐学报 2024年第6期52卷 1900-1916页

作者：陈汝妍高九涛高圆张惠宇李成新西安交通大学金属材料强度国家重点实验室西安710049 山东冰轮海卓氢能技术研究院有限公司山东烟台264002

管式固体氧化物燃料电池(SOFC)的结构特征决定了其高温密封难度低于板式结构,特殊的管式SOFC结构设计可以完全解决高温密封难题,尤其是在一个管上进行多个单电池串联集成设计的管式SOFC结构,其一个电池管相当于一个小型电堆,具有独特的... 详细信息

管式固体氧化物燃料电池(SOFC)的结构特征决定了其高温密封难度低于板式结构,特殊的管式SOFC结构设计可以完全解决高温密封难题,尤其是在一个管上进行多个单电池串联集成设计的管式SOFC结构,其一个电池管相当于一个小型电堆,具有独特的高电压小电流的输出特征,可显著降低管式电池的欧姆极化损失。管式SOFC的密封难度降低使得管式电池组堆相对容易,且电堆运行中的热应力约束较小,有助于电堆长期稳定运行。与板式电池相比,其体积功率密度和输出电流密度在同等条件下相对较低。本文综述了国内外管式SOFC的典型结构设计,通过管式SOFC的几何结构与电池支撑体的材料类型进行了分类,包括按电池支撑材料分类的阳极支撑型、阴极支撑型、陶瓷管支撑型、金属/金属陶瓷支撑型,按照管式SOFC的几何形状分类的圆管多节、扁管多节,单节圆管及单节扁管结构。同时综述了管式SOFC的常用材料及常用制备方法,最后对管式SOFC的发展进行了展望。

关键词：管式固体氧化物燃料电池支撑材料几何结构制备方法电堆

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Record-high efficiency perovskite LEDs achieved by accelerating radiative recombination

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Science China Materials 2024年第9期67卷 3039-3040页

作者： Feng gao Department of Physics Chemistry and BiologyLinköping UniversityLinköping58183Sweden

Light-emitting diodes(LEDs)have revolutionized the lighting and displays due to their superior energy *** increasing demand for more efficient and brighter thin-film LEDs in flat-panel displays and solid-state lighting applications has driven extensive research into perovskite materials,which show great promise for high brightness and efficiency.

关键词： lighting radiative high

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Stress tensor determination by modified hydraulic tests on pre-existing fractures:Method and stress constraints

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第5期16卷 1637-1648页

作者： Guiyun gao Chenghu Wang Ke gao National Institute of Natural Hazards Ministry of Emergency Management of ChinaBeijing100085China Beijing Engineering Research Center of Earthquake Observation Beijing100085China Key Laboratory of Compound and Chained Natural Hazards Dynamics Ministry of Emergency Management of ChinaBeijing100085China Department of Earth and Space Sciences Southern University of Science and TechnologyShenzhen518055China

The hydraulic testing of pre-existing fractures(HTPF)is one of the most promising in situ stress measurement methods,particularly for three-dimensional stress tensor ***,the stress tensor determination based on the HTPF method requires at least six tests or a minimum of 14-15 tests(under different conditions)for reliable *** this study,we modified the HTPF method by considering the shear stress on each pre-existing fracture,which increased the number of equations for the stress tensor determination and decreased the number of tests *** shear stresses were attributed to different fractures by random sampling;therefore,the stress tensors were obtained by searching for the optimal solution using the least squares criterion based on the Monte Carlo ***,we constrained the stress tensor based on the tensile strength criterion,compressive strength criterion,and vertical stress *** inverted stress tensors were presented and analyzed based on the tensorial nature of the stress using the Euclidean mean stress *** stress-measurement campaigns in Weifang(Shandong Province,China)and Mercantour road tunnel(France)were implemented to highlight the validity and efficiency of the modified HTPF(M-HTPF)*** results showed that the M-HTPF method can be applied for stress tensor inversion using only three to four tests on pre-existing fractures,neglecting the stress *** inversion results were confined to relatively small distribution dispersions and were significantly reliable and stable due to the shear stresses on the fractures and the stress constraints *** M-HTPF method is highly feasible and efficient for complete stress tensor determination in a single borehole.

关键词： Stress tensor Hydraulic tests on pre-existing fractures Mean stress Stress constraint Hydraulic fracturing

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Thermal and mechanical behavior of casting copper alloy wheel during wheel and belt continuous casting process

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China Foundry 2024年第1期21卷 82-90页

作者： Kun gao Yan Peng School of Mechanical Engineering Yanshan UniversityQinhuangdao 066004HebeiChina

To investigate the thermal and mechanical behavior of casting wheel,a two-dimensional thermoelastic-plastic finite element model was used to predict the temperature,stress and distortion distribution of the casting wheel during the wheel and belt continuous casting *** effects of grinding thickness and casting speed on the thermal and mechanical behaviors of the center of the hot face of the casting wheel were discussed in *** each rotation,the casting wheel passes through four different spray *** results show that the temperature distribution of the casting wheel in different spray zones is similar,the temperature of the hot face is the highest and the temperature reaches the peak in the spray zoneⅢ.The stress and distortion depend on the temperature distribution,and the maximum stress and distortion of the hot face are 358.2 MPa and 1.82 mm,*** temperature at the center of the hot face decreases with increasing grinding thickness and increases with increasing casting speed.

关键词： casting wheel finite element model grinding thickness casting speed hot face spray zones

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Durable poly(binaphthyl-co-p-terphenyl piperidinium)-based anion exchange membranes with dual side chains

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Journal of Energy Chemistry 2024年第2期89卷 324-335,I0008页

作者： Weiting gao Xuelang gao Qiugen Zhang Aimei Zhu Qinglin Liu Department of Chemical&Biochemical Engineering Fujian Provincial Key Laboratory of Theoretical and Computational ChemistryThe College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005FujianChina Department of Chemistry Pohang University of Science and Technology(POSTECH)Pohang 790-784South Korea

Building well-developed ion-conductive highways is highly desirable for anion exchange membranes(AEMs).Grafting side chain is a highly effective approach for constructing a well-defined phaseseparated morphological structure and forming unblocked ion pathways in AEMs for fast ion *** of side chains can further enhance phase separation due to the superhydrophobic nature of fluorine ***,their electronic effect on the alkaline stability of side chains and membranes is rarely ***,fluorine-containing and fluorine-free side chains are introduced into the polyaromatic backbone in proper configuration to investigate the impact of the fluorine terminal group on the stability of the side chains and membrane *** poly(binaphthyl-co-p-terphenyl piperidinium)AEM(QBNp TP)has the highest molecular weight and most dimensional stability due to its favorable backbone arrangement among ortho-and meta-terphenyl based ***,by introducing both a fluorinated piperidinium side chain and a hexane chain into the p-terphenyl-based backbone,the prepared AEM(QBNp TP-QFC)presents an enhanced conductivity(150.6 m S cm^(-1))and a constrained swelling at 80℃.The electronic effect of fluorinated side chains is contemplated by experiments and *** results demonstrate that the presence of strong electro-withdrawing fluorine groups weakens the electronic cloud of adjacent C atoms,increasing OH^(-)attack on the C atom and improving the stability of piperidinium *** QBNp TP-QFC possesses a robust alkaline stability at 80℃(95.3%conductivity retention after testing in 2 M Na OH for 2160 h).An excellent peak power density of 1.44 W cm^(-2)and a remarkable durability at 80℃(4.5%voltage loss after 100 h)can be observed.

关键词： Anion exchange membranes Backbone structure Fluorinated side chain Alkaline stability

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On the core entropy of Newton maps

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Science China Mathematics 2024年第1期67卷 77-128页

作者： Yan gao Department of Mathematics Shenzhen UniversityShenzhen 518060China

In this paper,we define the core entropy for postcritically-finite Newton maps and study its continuity within this *** show that the entropy function is not continuous in this family,which is different from the polyn... 详细信息

关键词： core entropy extended Newton graph critical marking polynomial Newton map

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Segmental nature of the Red River fault revealed by seismic anisotropy and geological structures

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Science China Earth Sciences 2024年第8期67卷 2423-2443页

作者： Ying LI Yuan gao School of Earth and Space Sciences University of Science and Technology of ChinaHefei 230026China Key Laboratory of Earthquake Prediction Institute of Earthquake ForecastingChina Earthquake AdministrationBeijing 100036China

As the western boundary of the Sichuan-Yunnan block(SYB),the Red River fault(RRF)is a major fault that controls deep crustal movement and deformation in the southeast margin of the Tibetan Plateau and regulates middle-lower crustal *** data suggest that the RRF is segmented and exhibits distinct variations in seismicity,velocity structure and crustal deformation from north to *** anisotropy reveals a complex pattern of lateral spatial and vertical stratified distributions.(1)From the perspective of crustal stratification,in the upper crust,the fast wave polarization in the north segment of the RRF is complex and possibly influenced by the Sanjiang lateral collision zone and adjacent faults with varying *** fast wave polarization in the middle segment is in the NW-SE direction,indicating a localized area of closed down or locked up with consistent *** in the south segment,it presents a disordered pattern,signifying complex deep tectonics and stress conditions at the wedged intersection *** the middle-lower crust in the north and south segments of the RRF,the azimuthal anisotropy is strong and consistent with the spatial strike of the weak zone characterized by low-velocity and *** suggests a connection between the anisotropy and the material migration.(2)In the whole crustal scale,the fast wave directions in two sides of the RRF are consistent with the NW-SE tectonic *** indicates that the RRF,as a large fault potentially cutting through the whole crust,strongly controls the surrounding media.(3)In the lithospheric scale,the fast wave polarizations are oriented nearly E-W and independent of the fault strike,consistent with the low P-and S-wave velocity structures and positive radial anisotropy in the upper *** fast wave directions could be related to lithospheric olivine deformation and asthenospheric *** paper suggests a decoupling of deformation between the crust and the lithospheri

关键词： Red River fault Seismic anisotropy Geological structures Lithosphere Fault segmentation

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Effect of mesopore spatial distribution of HZSM-5 catalyst on zinc state and product distribution in 1-hexene aromatization

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Chinese Journal of Chemical Engineering 2024年第3期67卷 16-26页

作者： Chenhao Wei Di gao Guohao Zhang Liang Zhao Jinsen gao Chunming Xu The State Key Lab of Heavy Oil Processing China University of Petroleum(Beijing)Beijing 102249China SINOPEC Research Institute of Petroleum Processing Co. Ltd.Beijing 100083China

1-hexene aromatization is a promising technology to convert excess olefin in fluid catalytic cracking(FCC)gasoline to high-value benzene(B),toluene(T),and ***,the increasing market demand of xylene has put forward higher requirements for new generation of *** increasing xylene yield in 1-hexene aromatization,the effect of mesopore structure and spatial distribution on product distribution and Zn loading was *** with different mesopore spatial distribution were prepared by post-treatment of parent HZSM-5 zeolite,including NaOH treatment,tetra-propylammonium hydroxide(TPAOH)treatment,and *** was found the evenly distributed mesopore mainly prolongs the catalyst lifetime by enhancing diffusion properties but reduces the aromatics selectivity,as a result of damage of micropores close to the catalyst *** the selectivity of high-value xylene can be highly promoted when the mesopore is mainly distributed interior the ***,the state of loaded Zn was also affected by mesopores spatial *** the optimized catalyst,the xylene selectivity was enhanced by 12.4%compared with conventional Zn-loaded parent HZSM-5 catalyst at conversion over 99%.It was attributed to the synergy effect of mesopores spatial distribution and optimized acid *** work reveals the role of mesopores in different spatial positions of 1-hexene aromatization catalysts in the reaction process and the influence on metal distribution,as well as their synergistic effect two on the improvement of xylene selectivity,which can improve our understanding of catalyst pore structure and be helpful for the rational design of high-efficient catalyst.

关键词： 1-Hexene aromatization Alkali treatment Xylene selectivity Mesopores Zinc state

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Impacts of central-Pacific El Niño and physical drivers on eastern Pacific bigeye tuna

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Journal of Oceanology and Limnology 2024年第3期42卷 972-987页

作者： Peng LIAN Le gao Key Laboratory of Ocean Observation and Forecasting and Key Laboratory of Ocean Circulation and Waves Institute of OceanologyChinese Academy of SciencesQingdao 266071China University of Chinese Academy of Sciences Beijing 100049China

Bigeye tuna Thunnus obesus is an important migratory species that forages deeply,and El Niño events highly influence its distribution in the eastern Pacific *** sea surface temperature is widely recognized as the main factor affecting bigeye tuna(BET)distribution during El Niño events,the roles of different types of El Niño and subsurface oceanic signals,such as ocean heat content and mixed layer depth,remain *** conducted A spatial-temporal analysis to investigate the relationship among BET distribution,El Niño events,and the underlying oceanic signals to address this knowledge *** used monthly purse seine fisheries data of BET in the eastern tropical Pacific Ocean(ETPO)from 1994 to 2012 and extracted the central-Pacific El Niño(CPEN)indices based on Niño 3 and Niño ***,we employed Explainable Artificial Intelligence(XAI)models to identify the main patterns and feature importance of the six environmental variables and used information flow analysis to determine the causality between the selected factors and BET ***,we analyzed Argo datasets to calculate the vertical,horizontal,and zonal mean temperature differences during CPEN and normal years to clarify the oceanic thermodynamic structure differences between the two types of *** findings reveal that BET distribution during the CPEN years is mainly driven by advection feedback of subsurface warmer thermal signals and vertically warmer habitats in the CPEN domain area,especially in high-yield fishing *** high frequency of CPEN events will likely lead to the westward shift of fisheries centers.

关键词： bigeye tuna central-Pacific El Niño(CPEN) ocean heat content Argo explainable artificial intelligence(XAI) information flow

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