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Graphene-like two-dimensional nanosheets-based anticorrosive coatings: A review

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Journal of Materials Science & Technology 2022年第34期129卷 139-162页

作者： Yumin Zhang jiulong sun Xinzhe Xiao Ning Wang Guozhe Meng Lin Gu School of Chemical Engineering and Technology Sun Yat-sen UniversityZhuhai 519082China Shenzhen Institute of Advanced Electronic Materials Shenzhen 518100China Shenzhen Institute of Advanced Technology Chinese Academy of SciencesShenzhen 518055China

In recent years, graphene has been widely employed in the field of metal corrosion protection owing to its outstanding impermeability and chemical stability, with examples of such metal protection including pure graphene coatings and graphene-based composite coatings. But the conductive graphene could promote the electrochemical reaction at the interface and accelerate the corrosion of metal substrates. More emerging graphene-like 2D nanosheets are attracting research attention for the application of metal anticorrosion, because of their barrier properties and poor conductivity, mainly including boron nitride(BN),molybdenum disulfide(MoS_(2)), zirconium phosphate(ZrP), and titanium carbide(MXene). In this review,the application of these graphene-like 2D nanosheets to metal protection is comprehensively reviewed.First, the general preparation methods of 2D nanosheets are briefly introduced. Second, surface functionalization of 2D nanosheets, including covalent and non-covalent modification, is described in detail.Third, the anticorrosion performance and optimization measures of pure 2D nanosheets coatings are summarized. Next, the protection performance, anticorrosive mechanism, and optimizations of 2D nanosheets composite coatings are presented. Finally, the future development of 2D nanosheets-based anticorrosive coatings has been prospected, and the challenges in the industrial application are discussed.

关键词： Two-dimensional nanomaterials Surface functionalization Polymer composite coatings Metal Corrosion protection

Location and Capacity Determination Method of Electric Vehicle Charging Station Based on Simulated Annealing Immune Particle Swarm Optimization

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Energy Engineering 2023年第2期120卷 367-384页

作者： jiulong sun Yanbo Che Ting Yang Jian Zhang Yibin Cai Key Laboratory of Smart Grid of Education Ministry Tianjin UniversityTianjin300072China Tianjin Electric Power Company State GridTianjin300010China

As the number of electric vehicles(EVs)continues to grow and the demand for charging infrastructure is also increasing,how to improve the charging infrastructure has become a bottleneck restricting the development of EVs.In other words,reasonably planning the location and capacity of charging stations is important for development of the EV industry and the safe and stable operation of the power system.Considering the construction and maintenance of the charging station,the distribution network loss of the charging station,and the economic loss on the user side of the EV,this paper takes the node and capacity of charging station planning as control variables and the minimum cost of system comprehensive planning as objective function,and thus proposes a location and capacity planning model for the EV charging station.Based on the problems of low efficiency and insufficient global optimization ability of the current algorithm,the simulated annealing immune particle swarm optimization algorithm(SA-IPSO)is adopted in this paper.The simulated annealing algorithm is used in the global update of the particle swarm optimization(PSO),and the immune mechanism is introduced to participate in the iterative update of the particles,so as to improve the speed and efficiency of PSO.Voronoi diagram is used to divide service area of the charging station,and a joint solution process of Voronoi diagram and SA-IPSO is proposed.By example analysis,the results show that the optimal solution corresponding to the optimisation method proposed in this paper has a low overall cost,while the average charging waiting time is only 1.8 min and the charging pile utilisation rate is 75.5%.The simulation comparison verifies that the improved algorithm improves the operational efficiency by 18.1%and basically does not fall into local convergence.

关键词： Electric vehicle charging station location selection and capacity configuration loss of distribution system simulated annealing immune particle swarm optimization Voronoi diagram

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用氢氟酸从白云鄂博矿中浸出铌及动力学研究

湿法冶金 2024年第3期43卷 236-241页

作者：孙盘石赵增武贾艳贺宇龙崔久龙张文迪汪文清内蒙古科技大学矿业与煤炭学院内蒙古包头014000 内蒙古工业大学材料科学与工程学院内蒙古呼和浩特010051 内蒙古科技大学内蒙古自治区碳中和协同创新中心内蒙古包头014000 内蒙古科技大学白云鄂博共伴生矿废弃物资源综合利用国家地方联合工程研究中心内蒙古包头014000

针对白云鄂博尾矿中含铌矿物综合回收利用中存在的问题,研究了用氢氟酸浸出含铌矿物中的铌,确定了最佳工艺条件,并探讨了浸出动力学。结果表明:在反应温度90℃、液固体积质量比7/1、氢氟酸浓度20 mol/L、反应时间2 h、搅拌速率300 r/mi... 详细信息

针对白云鄂博尾矿中含铌矿物综合回收利用中存在的问题,研究了用氢氟酸浸出含铌矿物中的铌,确定了最佳工艺条件,并探讨了浸出动力学。结果表明:在反应温度90℃、液固体积质量比7/1、氢氟酸浓度20 mol/L、反应时间2 h、搅拌速率300 r/min条件下,铌浸出率达90.91%;铌的浸出过程符合核收缩模型,浸出过程由化学反应和扩散混合控制,表观活化能为35.459 kJ/mol。该法能有效提取尾矿中的铌,有利于后续分离提纯。

关键词：白云鄂博尾矿含铌矿物铌氢氟酸浸出动力学

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Combining immune checkpoint blockade with ATP-based immunogenic cell death amplifier for cancer chemo-immunotherapy

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Acta Pharmaceutica Sinica B 2022年第9期12卷 3694-3709页

作者： jiulong Zhang Xiaoyan sun Xiufeng Zhao Chunrong Yang Menghao Shi Benzhuo Zhang Haiyang Hu Mingxi Qiao Dawei Chen Xiuli Zhao School of Pharmacy Shenyang Pharmaceutical UniversityShenyang 110016China Department of Oncology Affiliated Hongqi Hospital of Mudanjiang Medical CollegeMudanjiang 157011China Department of Pharmacy Shantou University Medical CollegeShantou 515041China Department of Neurology The Second Affiliated Hospital of Mudanjiang Medical CollegeMudanjiang 157009China

Amplifying“eat me signal”during tumor immunogenic cell death(ICD)cascade is crucial for tumor immunotherapy.Inspired by the indispensable role of adenosine triphosphate(ATP,a necessary“eat me signal”for ICD),a versatile ICD amplifier was developed for chemotherapy-sensitized immunotherapy.Doxorubicin(DOX),ATP and ferrous ions(Fe^(2+))were co-assembled into nanosized amplifier(ADO-Fe)throughπ‒πstacking and coordination effect.Meanwhile,phenylboric acid-polyethylene glycol-phenylboric acid(PBA-PEG-PBA)was modified on the surface of ADO-Fe(denoted as PADO-Fe)by the virtue of d-ribose unit of ATP.PADO-Fe could display active targetability against tumor cells via sialic acid/PBA interaction.In acidic microenvironment,PBA-PEG-PBA would dissociate from amplifier.Moreover,high H_(2)O_(2)concentration would induce hydroxyl radical(·OH)and oxygen(O_(2))generation through Fenton reaction by Fe^(2+).DOX and ATP would be released from the amplifier,which could induce ICD effect and“ICD adjuvant”to amplify this process.Together with programmed death ligands 1(PD-L1)checkpoint blockade immunotherapy,PADO-Fe could not only activate immune response against primary tumor,but also strong abscopal effect against distant tumor.Our simple and multifunctional ICD amplifier opens a new window for enhancing ICD effect and immune checkpoint blockade therapy.

关键词： Immunogenic cell death amplifier ATP Fenton reaction Immune checkpoint blockade Coordination polymer nanoparticles pH/ROS sensitive Phenylboric acid

Flexible optoelectronic neural transistors with broadband spectrum sensing and instant electrical processing for multimodal neuromorphic computing

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SmartMat 2023年第2期4卷 120-130页

作者： Yao Ni Lu Yang jiulong Feng Jiaqi Liu Lin sun Wentao Xu Institute of Photoelectronic Thin Film Devices and Technology Nankai UniversityTianjinChina Key Laboratory of Optoelectronic Thin Film Devices and Technology of Tianjin Nankai UniversityTianjinChina Engineering Research Center of Thin Film Photoelectronic Technology Ministry of EducationNankai UniversityTianjinChina Shenzhen Research Institute of Nankai University Nankai UniversityShenzhenChina

A flexible optoelectronic neural transistor(OENT)that consists of a one‐step spin‐coated tri‐blend film composed of 2,7‐dioctyl[1]benzothieno[3,2‐b][1]benzothiophene(C8‐BTBT),poly(3‐hexylthiophene‐2,5‐diyl)(P3HT),and poly(methyl methacrylate)(PMMA)is demonstrated.The C8‐BTBT and P3HT phases in the film partially segregate into distinct domains,which combine to provide broadband spectrum sensing,and instant electrical‐processing capabilities dominated by C8‐BTBT.The OENT is sensitive to solar radiation from the near‐ultraviolet(NUV)and to visible(Vis)radiation from blue to red.When exposed to NUV radiation,the OENT responds sensitively and retains the memory of the exposure for over 10^(3 )s.The OENT provides a warning of excessive chronic exposure to harmful NUV.These properties allow high‐pass filtering with different cut‐off frequencies fc that can restrict the reception of blue,green,or red.These switchable fc enables sensitive image reconstruction and multitarget monitoring.The device combined with a chitosan gel achieves strictly defined short‐range plasticity of<1 s that can achieve diverse instant‐computing applications such as spatiotemporally correlated coding and logic functions.Stable real‐time signal processing facilitates the realization of a Morse‐code recognition system constructed using neuro‐morphological hardware,achieving highly accurate character recognition.This study provides a useful resource that can have applications in wearable biomedical electronics and multimodal neuromorphic computing.

关键词： flexible optoelectronic neural transistor high‐pass filtering Morse‐code recognition system sensitive image reconstruction and multitarget monitoring spatiotemporally correlated coding and logic function

Research Developments and Prospects on Microseismic Source Location in Mines

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Engineering 2018年第5期4卷 653-660页

作者： jiulong Cheng Guangdong Song Xiaoyun sun Laifu Wen Fei Li State Key Laboratory of Coal Resources and Safe Mining China University of Mining and Technology Beijing 100083 China Laser Institute Qilu University of Technology (Shandong Academy of Sciences) Jinan 250014 China School of Electrical and Electronic Engineering Shijiazhuang Tiedao University Shijiazhuang 050043 China

Microseismic source location is the essential factor in microseismic monitoring technology, and its location precision has a large impact on the performance of the technique. Here, we discuss the problem of low-precision location identification for microseismic events in a mine, as may be obtained using conventional location methods that are based on arrival time. In this paper, microseismic location characteristics in mining are analyzed according to the characteristics of the mine's microseismic wavefield. We review research progress in mine-related microseismic source location methods in recent years, including the combination of the Geiger method with the linear method, combined microseismic event location method, optimization of relative location method, location method without pre-measured velocity, and location method without arrival time picking. The advantages and disadvantages of these methods are discussed, along with their feasible conditions. The influences of geophone distribution, first arrival time picking, and the velocity model on microseismic source location are analyzed, and measures are proposed to influence these factors. Approaches to solve the problem under study include adopting information fusion, combining and optimizing existing methods, and creating new methods to realize highprecision microseismic source location. Optimization of the velocity structure, along with applications of the time-reversal imaging technique, passive time-reversal mirror, and relative interferometric imaging, are expected to greatly improve microseismic location precision in mines. This paper also discusses the potential application of information fusion and deep learning methods in microseismic source location in mines. These new and innovative location methods for microseismic source location have extensive prospects for development.

关键词：微震源定位微震监测技术矿山技术创新

DEVELOPMENT OF SINGLE-PHASED WATER-COOLING RADIATOR FOR COMPUTER CHIP

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Chinese Journal of Mechanical Engineering 2007年第2期20卷 77-81页

作者： ZENG Ping CHENG Guangming LIU jiulong YANG Zhigang sun Xiaofeng PENG Taijiang College of Mechanical Engineering and Automatization Jilin University Changchun 130022 China Department of Mechettonics Jilin InsUtute of Chemical Technolgy Jilin 132022 China

In order to cool computer chip efficiently with the least noise, a single phase water-cooling radiator for computer chip driven by piezoelectric pump with two parallel-connection chambers is developed. The structure and work principle of this radiator is described. Material, processing method and design principles of whole radiator are also explained. Finite element analysis （FEA） software, ANSYS, is used to simulate the heat distribution in the radiator. Testing equipments for water-cooling radiator are also listed. By experimental tests, influences of flowrate inside the cooling system and fan on chip cooling are explicated. This water-cooling radiator is proved more efficient than current air-cooling radiator with comparison experiments. During cooling the heater which simulates the working of computer chip with different power, the water-cooling radiator needs shorter time to reach lower steady temperatures than current air-cooling radiator.

关键词： Computer chip Water-cooling Piezoelectric pump Radiator ANSYS simulation Simulative heater

Defect passivation by nontoxic biomaterial yields 21% efficiency perovskite solar cells

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Journal of Energy Chemistry 2021年第4期30卷 265-271页

作者： Shaobing Xiong Tianyu Hao Yuyun sun Jianming Yang Ruru Ma jiulong Wang Shijing Gong Xianjie Liu Liming Ding Mats Fahlman Qinye Bao Key Laboratory of Polar Materials and Devices Department of Electronic ScienceSchool of Physics and Electronic ScienceEast China Normal UniversityShanghai 200241China School of Chemistry and Chemical Engineering Shanghai Jiao Tong UniversityShanghai 200025China Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuan 030006ShanxiChina Laboratory of Organic Electronics ITNLinköping UniversitySE-60174 NorrköpingSweden Wallenberg Wood Science Center Linköping UniversitySE-60174 NorrköpingSweden Center for Excellence in Nanoscience(CAS) Key Laboratory of Nanosystem and Hierarchical Fabrication(CAS)National Center for Nanoscience and TechnologyBeijing 100190China

Defect passivation is one of the most important strategies to boost both the efficiency and stability of perovskite solar cells(PSCs).Here,nontoxic and sustainable forest-based biomaterial,betulin,is first introduced into perovskites.The experiments and calculations reveal that betulin can effectively passivate the uncoordinated lead ions in perovskites via sharing the lone pair electrons of hydroxyl group,promoting charge transport.As a result,the power conversion efficiencies of the p-i-n planar PSCs remarkably increase from 19.14%to 21.15%,with the improvement of other parameters.The hydrogen bonds of betulin lock methylamine and halogen ions along the grain boundaries and on the film surface and thus suppress ion migration,further stabilizing perovskite crystal structures.These positive effects enable the PSCs to maintain 90%of the initial efficiency after 30 days in ambient air with 60%±5%relative humidity,75%after 300 h aging at 85℃,and 55%after 250 h light soaking,respectively.This work opens a new pathway for using nontoxic and low-cost biomaterials from forest to make highly efficient and stable PSCs.

关键词： Perovskite solar cells Defect passivation Nontoxic biomaterial Efficiency

江西九龙山铁尾矿区3种树木对土壤重金属质量分数及微生物群落组成的影响

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林业科学 2024年第3期60卷 78-86页

作者：王文正宋立国王钱刘相荣孙启武厚凌宇中国林业科学研究院林业研究所、国家林业和草原局森林培育重点实验室、林木遗传育种国家重点实验室北京100091

【目的】探究种植湿地松、杉木、桤木对江西九龙山铁尾矿区土壤重金属质量分数及微生物群落组成的影响,为该矿区及相似立地区域植被恢复提供可靠的科学数据和理论依据。【方法】采用微波消解法处理湿地松、杉木、桤木的根际、非根际土... 详细信息

【目的】探究种植湿地松、杉木、桤木对江西九龙山铁尾矿区土壤重金属质量分数及微生物群落组成的影响,为该矿区及相似立地区域植被恢复提供可靠的科学数据和理论依据。【方法】采用微波消解法处理湿地松、杉木、桤木的根际、非根际土壤样品和根、茎、叶样品,通过ICP、AAS测定样品重金属质量分数,依据测定结果计算3种树木的生物富集和转移系数,分析其对不同重金属的富集和转移能力。应用宏基因组学测序分析3种树木根际、非根际土壤样品,探究各树种对应土壤中的微生物群落组成。【结果】1)3种树木对Hg、Cu、Pb、Zn的生物转移系数(BTF)均大于1,对Cr的BTF小于1,表明其对Hg、Cu、Pb、Zn的转移能力强,对Cr的转移能力弱。杉木的BTF(As)大于1,表明杉木对As的转移能力强。2)杉木对Hg、Pb的生物富集系数(BCF)均大于1,表明杉木对Hg、Pb的富集能力强。相较于其他重金属,湿地松对Hg、Pb的生物富集系数最高,桤木对Zn的生物富集系数最高,表明湿地松对Hg、Pb的富集能力强,桤木对Zn的富集能力强。3)在门水平上,对照组(J1)中酸杆菌门相对丰度最高(45.55%),其次为变形菌门(12.11%)。在湿地松根际土壤(J2)和非根际土壤(J3)、杉木根际土壤(J4)、桤木根际土壤(J5)和非根际土壤(J6)中变形菌门相对丰度最高(22.72%~44.56%),其次为酸杆菌门(13.49%~16.56%)。在属水平上,对照组优势属为短根瘤菌属和纤线杆菌属,J2、J3、J4、J5、J6中相对丰度占比最高的优势属为短根瘤菌属和鞘氨醇单胞菌属。【结论】1)根据3种树木对重金属的转移和富集能力评估结果,杉木、湿地松可作为Hg、Pb修复的先锋树种,桤木可作为Zn的修复树种与其间作。2)基于门、属2分类等级水平的分析,3种树木根际、非根际土壤中优势微生物群落均为变形菌门,3种树木种植均促进土壤中变形菌门微生物相对丰度增加,变形菌门可提高植物对重金属的吸收并对植物生长有促进作用,二者相辅相成,可有效提高植物吸收重金属的效率。

关键词：宏基因组学铁尾矿重金属污染植物修复效果微生物群落组成