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Fast UV-vis-NIR photoresponse of self-oriented F_(16)CuPc nanoribbons

Nano Research 2023年第7期16卷 9561-9568页

作者： Lingyu Zhang Xingyu Wang Wei Zhou Hao Wang Jiaxun Song Zihao Zhao Jihui Liao Jian Song Yajun Li jinyou xu Institute of Electronic Paper Displays South China Academy of Advanced OptoelectronicsSouth China Normal UniversityGuangzhou 510006China Department of Materials and Interfaces Weizmann Institute of ScienceRehovot 76100Israel

Controlling the vapor-deposited nanoribbons to grow along a consistent orientation will enable the desired in situ integration of functional devices,representing a major technological advance compared to post-growth processing strategies.In this work,ntype F_(16)CuPc molecules are self-assembled into horizontally-oriented nanoribbons with a consistent growth axis after creating periodic hydrophobic nanogrooves on a sapphire surface.Consequently,electrodes are deposited directly on the growth substrate to enable in situ fabrication of photodetectors.Depending on the deposited electrodes,these horizontally-oriented nanoribbons are connected to form a monolithic photodetector with a large sensing area or an on-chip array of photodetectors with multiple detector units.This in situ integration strategy avoids potential structural damage and contamination from impurities associated with post-growth processing steps.Therefore,the vapor-deposited nanoribbons can retain their high quality during the device manufacturing process,which contributes to performance improvement.As a result,the in-situ integrated F_(16)CuPc photodetectors exhibit a sensitive response in the ultraviolet-visible-near-infrared(UV-vis-NIR)region.The response time is on the order of tens of milliseconds,the fastest record ever for the F_(16)CuPc-based photodetectors.Furthermore,statistics from an array of 6×6 photodetectors show little variation in their sensitivity and response time,and hence this in situ fabrication scheme will contribute to the implementation of on-chip integrated photodetectors with consistent performance based on bottom-up nanoribbons.Overall,this self-oriented growth provides a versatile option to achieve desired in-situ integrated functional devices based on bottom-up nanoribbons.

关键词： fluorinated copper phthalocyanine nanoribbon planar array photodetector in situ integration

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一种双工位旋转式上甑机器人设计

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机械设计 2024年第5期41卷 76-83页

作者：徐进友邢恩宏张磊李彬董磊岳之斌天津理工大学天津市先进机电系统设计与智能控制重点实验室天津300384 天津理工大学机电工程国家级实验教学示范中心天津300384

上甑是白酒酿造的关键工序,为解决传统白酒酿造上甑过程中劳动强度大、酒质及产酒率不稳定等问题,依据上甑过程的工艺要求及标准,设计了一种双工位旋转式上甑机器人。该机器人采用3个旋转关节和撒料器实现上甑铺料的平面定位,平移关节... 详细信息

上甑是白酒酿造的关键工序,为解决传统白酒酿造上甑过程中劳动强度大、酒质及产酒率不稳定等问题,依据上甑过程的工艺要求及标准,设计了一种双工位旋转式上甑机器人。该机器人采用3个旋转关节和撒料器实现上甑铺料的平面定位,平移关节实现撒料高度的控制。对机器人的正、逆运动学进行了解析求解和验证,采用Monte⁃Carlo法模拟了上甑机器人的工作空间;基于有限元方法对关键部件进行了强度及模态分析。通过物理试验样机的现场测试,表明样机上甑相比于人工上甑的出酒率提高了10%左右,尾酒度数降低了5°~7°,有效提高了上甑的效率,验证了设计的可行性。模拟仿真与样机测试结果表明:文中上甑机器人的结构及功能满足设计要求,可为上甑机器人的设计及后续性能优化提供参考。

关键词：上甑机器人结构设计运动学分析工作空间模拟有限元分析

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Synthesis and Diameter-dependent Thermal Conductivity of InAs Nanowires

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Nano-Micro Letters 2014年第4期6卷 301-306页

作者： Pinyun Ren Xiaoli Zhu Jinyun Han jinyou xu Liang Ma Honglai Li Xiujuan Zhuang Hong Zhou Qinglin Zhang Minggang Xia Anlian Pan Key Laboratory for Micro-Nano Physics and Technology of Hunan Province State Key Laboratory of Chemo/Biosensing and Chemometrics College of Physics and Microelectronics Science Hunan University Condensed Matter Physics Laboratory Center on Experimental Physics School of Science Xi’an Jiaotong University

In this work, we synthesized high-quality In As nanowires by a convenient chemical vapor deposition method,and developed a simple laser heating method to measure the thermal conductivity of a single In As nanowire in air. During the measurement, a focused laser was used to heat one end of a freely suspended nanowire, with its other end embedded into a carbon conductive adhesive. In order to obtain the thermal conductivity of In As nanowires, the heat loss in the heat transfer process was estimated, which includes the heat loss through air conduction, the heat convection, and the radiation loss. The absorption ratio of the laser power in the In As nanowire was calculated. The result shows that the thermal conductivity of In As nanowires monotonically increases from 6.4 W m-1K-1to 10.5 W m-1K-1with diameters increasing from 100 nm to 190 nm, which is ascribed to the enhanced phonon-boundary scattering.

关键词： InAs nanowires Chemical vapor deposition Thermal conductivity Phonon-boundary scattering

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三维振动辅助铣削创成结构型表面的建模与振动参数影响仿真分析

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工具技术 2024年第6期58卷 110-115页

作者：肖蒙杰吝永红王启祥王桂莲徐进友天津市先进机电系统设计与智能控制重点实验室(天津理工大学) 机电工程国家级实验教学示范中心(天津理工大学) 建科机械(天津)股份有限公司天津中德应用技术大学

结构型表面因良好的表面特性被广泛应用于光学、生物以及航空航天等重要领域。提出三维振动辅助铣削制备结构型表面的方法,分析施加三维振动激励条件下的铣削加工轨迹。基于正交螺旋理论和空间矩阵变换建立三维振动辅助铣削模型,在正弦... 详细信息

结构型表面因良好的表面特性被广泛应用于光学、生物以及航空航天等重要领域。提出三维振动辅助铣削制备结构型表面的方法,分析施加三维振动激励条件下的铣削加工轨迹。基于正交螺旋理论和空间矩阵变换建立三维振动辅助铣削模型,在正弦函数曲面面型上预测生成的结构型表面微结构形态。探究了振幅以及振动频率对结构型表面微结构形貌的影响规律。

关键词：振动辅助铣削轨迹结构型表面表面形貌

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Riverine sulfate sources and behaviors in arid environment,Northwest China:Constraints from sulfur and oxygen isotopes

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Journal of Environmental Sciences 2024年第3期137卷 716-731页

作者： Yifu xu Wenjing Liu Bing xu Zhifang xu Key Laboratory of Cenozoic Geology and Environment Institute of Geology and GeophysicsChinese Academy of SciencesBeijing 100029China Innovation Academy for Earth Science Chinese Academy of SciencesBeijing 100029China University of Chinese Academy of Sciences Beijing 100049China

The fate of riverine sulfate ion (SO_(4)^(2-)) and its environmental effects in arid environment are difficult to evaluate due to its complicated sources and strongly coupled behaviors with water cycle which is significantly modified by humans.To understand the sulfur cycle in aquatic systems in arid environment,the chemical and sulfur and oxygen isotopic compositions (δ^(34)S_(SO4)and δ^(18)O_(SO4)) of major rivers around the Badain Jaran Desert,northwestern China,were investigated.These rivers had averaged SO_(4)^(2-)content at 1336μmol/L,over 10times higher than the global average.The δ^(34)S_(SO4)and δ^(18)O_(SO4)values ranged from-5.3‰to+11.8‰and+1.6‰to+12.8‰,respectively.The end-member analysis and the inverse model showed that riverine sulfate was mainly derived from evaporites dissolution (0-87%),sulfide oxidation (13%-100%) and precipitation (0-33%),indicating heterogeneity in sulfur sources and behaviors along the river drainage with the lithology variations and climate gradients.Multiple isotopic tools combining with hydro-chemistry compositions could be applied to reveal sulfur cycle in arid environment.Based on the calculation,sulfide oxidation plays the primary role in the headwater and upstream in the Qilian-Mountains area,where sulfide is widely exposed.While the proportion of evaporites dissolution contributing to riverine sulfate is much higher in downstream in a drier environment.Besides,less precipitation and higher temperature can lead to more intensive evaporation,affecting the process of sulfide oxidation and enhancing the rates of evaporites dissolution and sulfate precipitation in the basin.

关键词： Sulfur and oxygen isotopes Source apportionment Inverse model Arid environment Inland rivers Northwestern China

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城市轨道交通直流接触网残压形成原因探究

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电工技术 2022年第22期 183-185,188页

作者：许金友珠海优特电力科技股份有限公司广东珠海519000

城市轨道交通直流接触网停电后存在残压,残压高于验电器门槛值时会影响验电判别和接地操作,延误接触网检修作业。在不同天气状况下,对正线接触网和车辆段接触网做残压放电试验,测算出接触网分布参数等效值,找出了直流接触网残压形成的原... 详细信息

城市轨道交通直流接触网停电后存在残压,残压高于验电器门槛值时会影响验电判别和接地操作,延误接触网检修作业。在不同天气状况下,对正线接触网和车辆段接触网做残压放电试验,测算出接触网分布参数等效值,找出了直流接触网残压形成的原因,为降低残压影响提供依据。

关键词：城市轨道交通直流接触网残压

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Biohythane production from two-stage anaerobic digestion of food waste:A review

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Journal of Environmental Sciences 2024年第5期139卷 334-349页

作者： Xiaona An Ying xu Xiaohu Dai State Key Laboratory of Pollution Control and Resource Reuse School of Environmental Science and EngineeringTongji UniversityShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China

The biotransformation of food waste(FW)to bioenergy has attracted considerable research attention as a means to address the energy crisis and waste disposal problems.To this end,a promising technique is two-stage anaerobic digestion(TSAD),in which the FW is transformed to biohythane,a gaseous mixture of biomethane and biohydrogen.This review summarises the main characteristics of FW and describes the basic principle of TSAD.Moreover,the factors influencing the TSAD performance are identified,and an overview of the research status;economic aspects;and strategies such as pre-treatment,co-digestion,and regulation of microbial consortia to increase the biohythane yield from TSAD is provided.Additionally,the challenges and future considerations associated with the treatment of FW by TSAD are highlighted.This paper can provide valuable reference for the improvement and widespread implementation of TSAD-based FW treatment.

关键词： Two-stage anaerobic digestion(TSAD) Food waste(FW) Methane production Hydrogen production

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Identification of high oxygen-consuming substances in stormwater drainage systems illicitly connected with sewage system

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Journal of Environmental Sciences 2024年第4期138卷 132-140页

作者： Chen xu Zuxin xu Wenhai Chu Shanshan Wu Rong Xiao Lei Su State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Ministry of Education Key Laboratory of Yangtze River Water Environment Tongji UniversityShanghai 200092China Guangzhou Resource Environmental Protection Technology Co. Ltd.Guangzhou 510030China

The dissolved oxygen content in water is an important indicator for assessing the quality of the water environment,and maintaining a certain amount of dissolved oxygen is essential for the healthy development of the ecological environment.When a water body is anoxic,the activity of anaerobic microorganisms increases and organic matter is decomposed to produce a large number of blackening and odorizing substances,resulting in black and odorous water bodies,which is a very common and typical phenomenon in China.Presently,there is still a relatively universal occurrence of illicitly connected stormwater and sewage pipes in the urban drainage pipe network in China,which makes oxygen-consuming substances be directly discharged into rivers through stormwater pipes and consume the dissolved oxygen in the water bodies,resulting in an oxygen deficiency of the water.This induces seasonal or year-round black and stink phenomena in urban rivers.Hence,identifying high oxygen-consuming substances,which lays the foundation for the subsequent removal of oxygen-consuming substances,is essential.Through a series of comparisons of water quality indicators and analysis of organic characteristics,it was found that the oxygen consumption capacity of domestic sewage was higher than that of industrial wastewater in the selected area of this study,and the oxygen-consuming substances of domestic sewage were small molecular amino acids.By comparing 20 conventional free amino acids,it was found that seven of them consumed oxygen easily,and compared with chemical oxygen consumption,biological oxygen consumption was in a leading position.

关键词： Urban drainage system Oxygen-consuming substances Domestic sewage Amino acid

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Aldehyde oxidase mediated enantioselective metabolic health risk of dinotefuran

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Science China Chemistry 2024年第6期67卷 2079-2091页

作者： Liwei xu Xinxin xu Hua Kuang Chuanlai xu Xiaoling Wu State Key Laboratory of Food Science and Resources Jiangnan UniversityWuxi214122China International Joint Research Laboratory for Biointerface and Biodetection and School of Food Science and Technology Jiangnan UniversityWuxi214122China Collaborative Innovation center of Food Safety and Quality Control in Jiangsu Province Jiangnan UniversityWuxi214122China

Chiral pollutants often pose significant differential environmental health risks.In this study,the biotransformation of chiral dinotefuran(DIN)and its enantioselective metabolic toxicity mechanisms have been systemically investigated.Firstly,reversedphase chromatography-high resolution mass spectrometry was developed to quantify the content of DIN R/S chiral enantiomer with pg level sensitivity,revealing a lower elimination rate constant(K_(e))of S-DIN(0.730 h^(-1))than R-DIN(0.746 h^(-1)).Secondly,the interaction mechanism between DIN metabolism and important endogenous bioactive molecules,such as aldehyde oxidase(AOX)and neurotransmitters,was revealed.The DIN nitro-group was converted into a guanidine group by the reducing site of nearby flavin adenine dinucleotide(FAD)in AOX with the preferred higher affinity of S-configuration.Meanwhile,the endogenous tryptophan(Trp)aldehyde metabolic intermediate,5-hydroxyindoleacetaldehyde(5-HIAL),provides a persistent electron donor for DIN reduction via the oxidation-catalyzed site in AOX,resulting in remarkable up-regulation of monoamine neurotransmitters such as serotonin and dopamine.Thirdly,the higher level of neurotransmitters further mediated dysregulation of oxylipin homeostasis via the serotonergic pathway,where S-DIN exhibited more pronounced liver lipid damage and environmental health risk with the accumulated lipid biomarkers,oxidized triglyceride(OxTG)and oxidized sphingomyelin(OxSM).This study elucidates the AOX-mediated enantioselectivity metabolic pathway of DIN,providing a new analytical method for chiral pollutants and paves the way for their health risk assessments.

关键词： neonicotinoid dinotefuran enantiomer aldehyde oxidase metabolomics health risk

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Mapping super-resolution image quality

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Light(Science & Applications) 2024年第2期13卷 178-180页

作者： Megan A.Steves Ke xu Department of Chemistry University of CaliforniaBerkeleyCA94720USA

The local quality of super-resolution microscopy images can be assessed and mapped by rolling Fourier ring correlation,even when image quality varies within a single image.

关键词： image resolution Mapping

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