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Sulfur atom occupying surface oxygen vacancy to boost the charge transfer and stability for aqueous Bi2O3 electrode

Journal of Energy Chemistry 2025年第2期101卷 751-759页

作者： Guangmin Yang Jianyan lin Guanwu li Tian li Dong Wang Weitao Zheng College of Physics Changchun Normal University School of Materials Science and Engineering Northwestern Polytechnical University Key Laboratory of Automobile Materials of MOE School of Materials Science and Engineering and Jilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy Materials Jilin University

Oxygen vacancies（Ov） within metal oxide electrodes can enhance mass/charge transfer dynamics in energy storage ***,construction of surface Ovoften leads to instability in electrode structure and irreversible electrochemical reactions,posing a significant *** overcome these challenges,atomic heterostructures are employed to address the structural instability and enhance the mass/charge transfer dynamics associated with phase conversion mechanism in aqueous electrodes,Herein,we introduce an atomic S-Bi2O3heterostructure(sulfur（S） anchoring on the surface Ovof Bi2O3).The integration of S within Bi2O3lattice matrix triggers a charge imbala nce at the heterointerfaces,ultimately resulting in the creation of a built-in electric field（BEF）.Thus,the BEF attracts OH-ions to be adsorbed onto Bi within the regions of high electron cloud overlap in S-Bi2O3,facilitating highly efficient charge ***,the anchored S plays a pivotal role in preserving structural integrity,thus effectively stabilizing the phase conversion reaction of *** a result,the S-Bi2O3electrode achieves72.3 mA h g-1at 10 A g-1as well as high-capacity retention of 81.9% after 1600 *** innovative SBi2O3design presents a groundbreaking approach for fabricating electrodes that exhibit efficient and stable mass and charge transfer ***,it enhances our understanding of the underlying reaction mechanism within energy storage electrodes.

关键词： Anchoring effect Atomic heterostructure Charge/mass transfer Oxygen vavancy Structural integrity

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Rationally constructing metallic Sn-ZnO heterostructure via in-situ Mn doping for high-rate Na-ion batteries

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Chinese Chemical Letters 2025年第2期36卷 518-525页

作者： Bin Fenga Tao Long Ruotong li Yuan-li Ding College of Materials Science and Engineering Hunan University College of Materials and Chemical Engineering Key laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials China Three Gorges University

Developing a heterostructure for alloying-based anode for sodium-ion batteries（SIBs） is an efficient solution to accommodate volume change upon sodiation/desodiation and boost sodium storage since it combines the merits of each component. Herein, we report a metallic and microphone-like Sn-Zn0.9Mn0.1O heterostructure via an in-situ Mn doping strategy. Based on theoretical calculations and experimental results, the introduction of Mn into Zn O（a small amount of Mn also diffuses into the Sn lattice） can not only enhance intrinsic electronic conductivity but also reduce the Na+diffusion barrier inside the Sn phase. When evaluated as anode for SIBs, the obtained heterostructures show a high reversible capacity of 395.1 mAh/g at 0.1 A/g, rate capability of 332 mAh/g at 5 A/g, and capacity retention of almost 100%after 850 cycles at 5 A/g, indicating its great potential for high-power application of SIBs.

关键词： Heterostructures Mn-doping Sn anode Sn-Zn0.9Mn0.1O Sodium-ion battery

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Influence of heat treatment on microstructure of a newβ-solidifyingγ-TiAl alloy

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Journal of Iron and Steel Research International 2025年第1期32卷 239-248页

作者： li Quan Xiao-bing li Peng Xue Jun-jie Hao Kun Qian Bo Chen Jian-zhong li Kui liu School of Metallurgy Northeastern UniversityShenyang110819LiaoningChina Department of Materials Science and Technology Ji Hua LaboratoryFoshan528200GuangdongChina

The high strength and stability of the full-lamellar structure guarantee the industrial application of theβ-solidifyingγ-TiAl ***,it is a huge challenge to design an alloy with good hot-deformability as well as the full-lamellar *** low-cost Ti-42.5Al-2Mn-0.4Mo-0.1B-0.1C(at.%)alloy was designed,which undergoes bothβandαsingle-phase region during the *** is found that the full-lamellar structure can be obtained by the solution heat treatment at 1230℃ for 20 min and then aging treatment at 800℃ for 3 ***,a new microstructure,namely,the pearlitic-like microstructure(PM)induced by theα_(2)/γ→βo+γcellular reaction was observed when the aging temperature is increased to above 800℃.The volume fraction of the PM is gradually increased from 0%to 25.5%,65%,and 94%according to elevated aging temperature from 800 to 900,1000,and 1050℃,*** mechanism of the reducedα_(2)/γlamellae and PM formation was discussed regarding the heterogeneous distribution ofβstabilizing elements and the interface energy stored inα_(2)/γlamellae.

关键词： β-γ-TiAl Alloy design Two-step heat treatment Full-lamellar structure Cellular reaction

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An efficient quantum proactive incremental learning algorithm

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Science China(Physics,Mechanics & Astronomy) 2025年第1期68卷 45-53页

作者： lingxiao li Jing li Yanqi Song Sujuan Qin Qiaoyan Wen Fei Gao State Key Laboratory of Networking and Switching Technology Beijing University of Posts and TelecommunicationsBeijing 100876China School of Cyberspace Security Beijing University of Posts and TelecommunicationsBeijing 100876China

In scenarios where a large amount of data needs to be learned,incremental learning can make full use of old knowledge,signif-icantly reduce the computational cost of the overall learning process,and maintain high *** this paper,taking the MaxCut problem as our example,we introduce the idea of incremental learning into quantum computing,and propose a Quantum Proactive Incremental Learning algorithm(QPIL).Instead of a one-off training of quantum circuit,QPIL contains a multi-phase training on gradually-increased subgraphs of all vertices,proactively reducing large-scale problems to smaller ones to solve in steps,providing an efficient solution for ***,some vertices and corresponding edges are randomly selected for training to obtain optimized parameters of the quantum circuit at ***,in each incremental phase,the remaining vertices and corresponding edges are gradually added and the parameters obtained from the previous phase are reused in the parameter initialization of the current *** perform experiments on 120 different small-scale graphs,and it shows that QPIL performs superior to prevalent quantum and classical baselines in terms of approximation ratio(AR),time cost,anti-forgetting,and solv-ing *** particular,QPIL’s AR surpasses 20%of mainstream quantum baselines,and the time cost is less than 1/5 of *** idea of QPIL is expected to inspire efficient and high-quality solutions in large-scale MaxCut and other combinatorial optimization problems.

关键词： variational quantum algorithm incremental learning multi-phase training MaxCut quantum computing

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Deciphering environmental factors influencing phytoplankton community structure in a polluted urban river

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Journal of Environmental Sciences 2025年第2期148卷 375-386页

作者： Xiaxia li Kai Chen Chao Wang Tianyu Zhuo Hongtao li Yong Wu Xiaohui Lei Ming li Bin Chen Beibei Chai School of Water Conservancy and Hydroelectric Power Hebei University of EngineeringHandan 056038China Collaborative Innovation Center for Intelligent Regulation and Comprehensive Management of Water Resources School of Water Conservancy and HydroelectricHebei University of EngineeringHandan 056038China Hebei Key Laboratory of Intelligent Water Conservancy Hebei University of EngineeringHandan 056038China Tianjin Water Group Binhai Water Co. Ltd.Tianjin 300308China State Key Laboratory of Simulation and Regulation of Water Cycle in River Basin China Institute of Water Resources and Hydropower ResearchBeijing 100038China School of Architecture and Civil Engineering Xi’an University of Science and TechnologyXi’an 710054China Chengdu University of Technology Chengdu 610059China College of Natural Resources and Environment Northwest A&F UniversityYangling 712100China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentBeijing Normal UniversityBeijing 100875China

Tuojiang River Basin is a first-class tributary of the upper reaches of the Yangtze River—which is the longest river in *** phytoplankton are sensitive indicators of trophic changes inwater bodies,characterizing phytoplankton communities and their growth influencing factors in polluted urban rivers can provide new ideas for pollution ***,we used direct microscopic count and environmental DNA(eDNA)metabarcoding methods to investigate phytoplankton community structure in Tuojiang River Basin(Chengdu,Sichuan Province,China).The association between phytoplankton community structure and water environmental factors was evaluated by Mantel *** environmental monitoring data were used to pinpoint major factors that influenced phytoplankton growth based on structural equation *** the phylum level,the dominant phytoplankton taxa identified by the conventional microscopic method mainly belonged to Bacillariophyta,Chlorophyta,and Cyanophyta,in contrast with Chlorophyta,Dinophyceae,and Bacillariophyta identified by eDNA ***α-diversity analysis,eDNA metabarcoding detected greater species diversity and achieved higher precision than the microscopic *** growth was largely limited by phosphorus based on the nitrogen-to-phosphorus ratios>16:1 in all water *** analysis and structural equation modeling also confirmed that the nitrogen-to-phosphorus ratio was the principal factor influencing phytoplankton *** results could be useful for implementing comprehensive management of the river basin *** is recommended to control the discharge of point-and surface-source pollutants and the concentration of dissolved oxygen in areas with excessive nutrients(e.g.,Jianyang-Ziyang).Algae monitoring techniques and removal strategies should be improved in 201 Hospital,Hongrihe Bridge and Colmar Town areas.

关键词： Environmental DNA Microscopic count Phytoplankton growth Structural equation modeling Tuojiang River Basin

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乡村振兴背景下陕南羌族刺绣艺术创新设计研究

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鞋类工艺与设计 2022年第19期2卷 74-76页

作者：李婧溪张欣悦周川渝陕西国际商贸学院陕西西安712046

随着国家对非遗文化重视程度的加深以及乡村振兴战略的提出,本文通过分析羌族刺绣纹样,挖掘其背后的文化内涵,从而对羌族刺绣进行艺术创新,打造出让大众喜闻乐见且具有民族特色的文化产品,形成推进和实现乡村振兴的新途径。

关键词：羌族刺绣乡村振兴创新文化产品

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Research on the hazards of gas leakage and explosion in a full-scale residential building

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Defence Technology(防务技术) 2025年第1期43卷 168-181页

作者： Chengjun Yue li Chen Zhan li Bin Feng Ruizhi Xu Engineering Research Center of Safety and Protection of Explosion&Impact of Ministry of Education Southeast UniversityNanjing 211189China

The gas explosion in residential building has always been a highly concerned *** in homogeneous mixtures have been extensively ***,mixtures are often inhomogeneous in the practical scenarios due to the differences in the densities of methane and *** order to investigate the effects of gas explosions in inhomogeneous mixtures,experimental studies involving gas leakage and explosion are conducted in a full-scale residential building to reproduce the process of gas *** fitting the dimensionless buoyancy as a function of dimensionless height and dimensionless time,a distribution model of gas in large-scale spaces is established,and the mechanism of inhomogeneous distribution of methane is also be ***,the stratified reconstruction method(SRM)is introduced for efficiently setting up inhomogeneous concentration fields in *** simulation results highlight that for the internal overpressure,the distribution of methane has no effect on the first overpressure peak(ΔP1),while it significantly influences the subsequent overpressure peak(ΔP2),and the maximum difference between the overpressure of homogeneous and inhomogeneous distribution is174.3%.Moreover,the initial concentration distribution also has a certain impact on the external overpressure.

关键词： Methane distribution Inhomogeneous mixture Gradient layer Gas explosion Explosive simulation

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蝇蛆粉对蛋鸡免疫力和生产性能的影响

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中国农学通报 2012年第8期28卷 38-41页

作者：郝贵增付亮李敬玺安阳工学院河南安阳455000 河南科技学院河南新乡453003

为研究蝇蛆粉对蛋鸡免疫力和生产性能的影响。选择3000只星杂288蛋仔鸡,进行为期6周饲养实验(试验Ⅰ);选择3000只生产期星杂288蛋鸡,进行为期3个月饲养实验(试验Ⅱ),根据蛋白饲料的不同又分为试验组(蝇蛆粉型日粮)和对照组(鱼粉型日粮)... 详细信息

为研究蝇蛆粉对蛋鸡免疫力和生产性能的影响。选择3000只星杂288蛋仔鸡,进行为期6周饲养实验(试验Ⅰ);选择3000只生产期星杂288蛋鸡,进行为期3个月饲养实验(试验Ⅱ),根据蛋白饲料的不同又分为试验组(蝇蛆粉型日粮)和对照组(鱼粉型日粮)。结果显示:试验Ⅰ中,试验组与对照组相比,每吨食粮降低原料成本约60元,成活率提高3.2%(P<0.05),均匀度提高8%(P<0.05);试验Ⅱ中,在试验期内产蛋数提高9.2%(P<0.05),蛋重提高9.616%(P<0.05)。与对照组相比试验组T-淋巴细胞、B-淋巴细胞的数量均有不同程度的增加。生产蛋鸡免疫球蛋白IgG提高9.5%、IgM提高7.1%。因此蝇蛆粉代替鱼粉饲喂蛋鸡是合理利用饲料资源、降低生产成本、提高经济效益的有效途径。

关键词：蝇蛆粉蛋鸡免疫力生产性能

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17α-methyltestosterone induced hepatocyte apoptosis through endoplasmic reticulum stress in Takifugu fasciatus

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Journal of Oceanology and limnology 2025年第1期43卷 219-231页

作者： Xuanyin CHEN Sheng LUO Yanfang li Rui li Xiaojun li Zhengyang HU Shaowu YIN Tao WANG College of Marine Science and Engineering Jiangsu Province Engineering Research Center for Aquatic Animals Breeding and Green Efficient Aquacultural TechnologyNanjing Normal UniversityNanjing 210023China Co-Innovation Center for Marine Bio-Industry Technology of Jiangsu Province Lianyungang 222005China

17α-methyltestosterone(17α-MT)is an emerging pollutant,which is harmful to the endocrine system and reproduction of *** investigated the effects of different concentrations of 17α-MT(0,5,30,60,and 100 mg/kg)on endoplasmic reticulum stress(ERS)and apoptosis in the liver of Takifugu *** show that:(1)with the increase of 17α-MT treatment concentration,liver transaminases(alanine aminotransferase;aspartate aminotransferase)and the mRNA expression of ERS marker genes(glucose-regulated protein 78;calreticulin)of *** were significantly increased compared with the control group(Pliver of *** increased with the increase of 17α-MT concentration compared with the control group(P<0.05);(3)by using 4-phenylbutyricacid(4-PBA)inhibitors to stimulate ERS through in vitro experiments,the expression of ERS and apoptosis-related genes significantly decreased(P<0.05),and the apoptosis rate of *** hepatocytes was significantly inhibited(P<0.05)under 17α-MT *** study confirmed that ERS played an important role in the induction of apoptosis in the hepatocytes of ***,which enriched the ecotoxicological information of environmental androgens.

关键词： 17α-methyltestosterone Takifugu fasciatus liver endoplasmic reticulum stress apoptosis

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Effect of lysozyme combined with hydrothermal pretreatment on excess sludge and anaerobic digestion

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Journal of Environmental Sciences 2025年第1期147卷 36-49页

作者： Xiuqin Cao Songyue li Chaolei liu School of Environment and Energy Engineering Beijing University of Civil Engineering and ArchitectureBeijing 100044China Key Laboratory of Urban Storm water System and Water Environment(Ministry of Education) Beijing University of Civil Engineering and ArchitectureBeijing 100044China

Anaerobic digestion(AD)is widely employed for sludge stabilization and waste ***,the slow hydrolysis process hinders methane production and leads to prolonged sludge *** this study,an efficient and eco-friendly lysozyme pre-treatment method was utilized to address these *** optimizing lysozyme dosage,hydrolysis and cell lysis were ***,lysozyme combined with hydrothermal pretreatment enhanced overall *** indicate that:(1)When lysozyme dosage reached 90 mg/g TS after 240 min of pretreatment,SCOD,soluble polysaccharides,and protein content reached their maxima at 855.00,44.09,and 204.86 mg/L,*** represented an increase of 85.87%,365.58%,and 259.21%compared to the untreated *** fluorescence spectroscopy revealed the highest fluorescence intensity in the IV region(soluble microbial product),promoting microbial metabolic activity.(2)Lysozyme combined with hydrothermal pretreatment significantly increased SCOD,soluble proteins,and polysaccharide release from sludge,reducing SCOD release *** experiments identified Group 3 as the most effective for SCOD and soluble polysaccharide release,while Group 9 released the most soluble *** significance order of factors influencing SCOD,soluble proteins,and polysaccharide release is hydrothermal temperature>hydrothermal time>enzymatic digestion time.(3)The lysozyme-assisted hydrothermal pretreatment group exhibited the fastest release and the highest SCOD concentration of 8,135.00 mg/L during anaerobic *** SCOD consumption and cumulative gas production increased by 95.89%and 130.58%,respectively,compared to the control group,allowing gas production to conclude 3 days earlier.

关键词： Excess sludge Lysozyme Hydrothermal pre-treatment Anaerobic digestion Gas production

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