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Nanocavity enriched CuPd alloy with high selectivity for CO_(2) electroreduction toward C_(2)h_(4)

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Rare Metals 2024年第4期43卷 1513-1523页

作者： Ze-Yu Zhang hai-Bin Wang Fei-Fei Zhang jing-Wei Li Xin-Zhuo hu Si-Wei Yan Yi-Ming Bai Xun Zhang Gu-Rong Shen Peng-Fei Yin jing yang Cun-Ku Dong jing Mao hui Liu Xi-Wen Du Institute of New-Energy Materials School of Materials Science and EngineeringTianjin UniversityTianjin300350China

Electrocatalysis of CO_(2)reduction reaction is an effective way to convert CO_(2)into high value-added products,but the selectivity of Cu-based catalysts for C2+products needs to be improved due to the high energy barrier of C-C ***,a viable catalyst design strategy to decrease energy barrier of C-C coupling should be put ***,a nanocavity-enriched CuPd single atom alloy(CuPd SAA)catalyst is designed to promote CC coupling *** faradaic efficiency of CuPd SAA for ethylene and C_(2+)reaches 75.6%and 85.7%at-0.7 V versus reversible hydrogen electrode(RhE),*** on the results given by in situ characterization,the porous hollow structure dramatically increases the ratio of the linear-bond*CO,thus enhancing the faradaic efficiency for *** functional theory(DFT)calculation reveals that the Pd doping can regulate the electronic structure of neighboring Cu atoms to decrease the energy barrier of C-C coupling,further improving the faradaic *** work provides a new idea for designing catalyst with high selectivity for ethylene.

关键词： Adsorption configuration C-C coupling CO_(2) electrocatalysis Ethylene Single atom alloy

The MADS-box gene RhAGL6 plays a master role in regulating the receptacle malformation in rose at low temperature

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horticultural Plant Journal 2024年第5期10卷 1214-1229页

作者： Weikun jing Shuai Zhang Qingcui Zhao yang Liu Liangjun Zhao Junping Gao Nan Ma Xiaofeng Zhou Yonghong Li School of Food and Drug Shenzhen PolytechnicShenzhen 518055China Department of Ornamental horticulture College of HorticultureChina Agricultural UniversityBeijing 100193China Postdoctoral Innovation Practice Base Shenzhen PolytechnicShenzhen 518055China Flower Research Institute of Yunnan Academy of Agricultural Sciences KunmingYunnan 650205China

Low temperature usually results in the developmental deformity of flower organs,immensely affecting the quality of rose ***,it's largely unknown about the regulatory mechanisms activated by low ***,we used a low temperature-sensitive Rosa hybrida cv.‘Peach Avalanche’to screen a MADS-box gene RhAGL6 via conjoint analysis between RNA sequencing(RNA-seq)and whole-genome bisulfite sequencing(WGBS).Furthermore,we found that low temperature induced the hypermethylation and elevated histone 3 lys-27 trimethylation(h3K27me3)level on the RhAGL6 promoter,leading to decreased RhAGL6 *** addition,RhAGL6 silencing resulted in the formation of abnormal *** also found that the levels of gibberellins(GA3)and abscisic acid(ABA)in the receptacle under low temperature were lower and higher,respectively,than under normal *** activity analysis revealed that GA3 significantly activated RhAGL6 promoter activity,whereas ABA inhibited ***,we propose that RhAGL6 regulates rose receptacle development by integrating epigenetic regulation and phytohormones signaling at low temperature.

关键词： Rosa hybrida Low temperature RhAGL6 Receptacle development DNA methylation h3K27me3 Phytohormone

Estimating Critical Clearing Time of Grid Faults Using DA of State-Reduction Model of Power Systems

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CSEE Journal of Power and Energy Systems 2024年第2期10卷 807-820页

作者： yang Liu Zhongyang Chen huanjin Yao Lin Yi Q.h.Wu School of Electric Power Engineering South China University of TechnologyGuangzhou 510640China China Southern Power Grid Research Institute Guangzhou 510663China

This paper proposes a critical clearing time (CCT) estimation method by the domain of attraction (DA) of a state-reduction model of power systems using sum of squares (SOS) programming. By exploiting the property of the Jacobian matrix and the structure of the boundary of the DA, it is found the DA of the state-reduction model and that of the full model of a power system are topological isomorphism. There are one-to-one correspondence relationships between the number of equilibrium points, the type of equilibrium points, and solutions of the two system models. Based on these findings, an expanding interior algorithm is proposed with SOS programming to estimate the DA of the state-reduction model. State trajectories of the full model can be transformed to those of the state-reduction model by orthogonal or equiradius projection. In this way, CCT of a grid fault is estimated with the DA of the state-reduction model. The calculational burden of SOS programming in the DA estimation using the state-reduction model is rather small compared with using the full model. Simulation results show the proposed expanding interior algorithm is able to provide a tight estimation of DA of power systems with higher accuracy and lower time costs.

关键词： Critical clearing time domain of attraction expanding interior algorithm state-reduction model SOS programming

Boosting electrocatalytic nitrate reduction to ammonia via Cu_(2)O/Cu(Oh)_(2)heterostructures promoting electron transfer

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Nano Research 2024年第6期17卷 4898-4907页

作者： jing Geng Sihan Ji Anhui Province International Research Center on Advanced Building Materials School of Materials Science and Chemical EngineeringAnhui Jianzhu UniversityHefei 230601China Anhui Province Key Laboratory of Advanced Building Materials Anhui Jianzhu UniversityHefei 230601China School of Energy Materials and Chemical Engineering Hefei UniversityHefei 230601China

Electrocatalytic nitrate(NO_(3)^(−))reduction to ammonia(Nh_(3))offers a viable approach for sustainable Nh_(3)production and environmental ***(Cu)possesses a distinctive electronic structure,which can augment the reaction kinetics of NO_(3)^(−)and impede hydrogen evolution reaction(hER),rendering it a promising contender for the electrosynthesis of Nh_(3)from NO_(3)^(−).Nevertheless,the role of Cu_(2)O in copper-based catalysts still requires further investigation for a more comprehensive ***,the Cu_(2)O/Cu(Oh)_(2)heterostructures are successfully fabricated through liquid laser irradiation using CuO nanoparticles as a *** and theoretical researches reveal that Cu_(2)O/Cu(Oh)_(2)heterostructure exhibits enhanced electrocatalytic performance for NO_(3)^(−)to Nh_(3)because Cu(Oh)_(2)promotes electron transfer and reduces the valence state of Cu active site in Cu_(2)***−0.6 V(*** hydrogen electrode(RhE)),the Nh_(3)yield reaches its maximum at 1630.66±29.72μg·h^(−1)·mgcat^(−1),while the maximum of Faraday efficiency(FE)is 76.95%±5.51%.This study expands the technical scope of copper-based catalyst preparation and enhances the understanding of the electrocatalytic mechanism of NO_(3)^(−)to Nh_(3).

关键词： Cu_(2)O/Cu(Oh)_(2)heterostructures electron transfer ammonia synthesis electrocatalysts nitrate

Implicit Function Based Open-loop Analysis Method for Detecting the SSR Using Identified System Parameters

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CSEE Journal of Power and Energy Systems 2024年第5期10卷 2016-2026页

作者： Luonan Qiu Tianhao Wen yang Liu Q.h.Wu School of Electric Power Engineering South China University of TechnologyGuangzhou 510640China

This paper proposes an implicit function based open-loop analysis method to detect the subsynchronous resonance(SSR),including asymmetric subsynchronous modal attraction(ASSMA)and asymmetric subsynchronous modal repulsion(ASSMR),of doubly-fed induction generator based wind farms(DFIG-WFs)penetrated power *** some important parameters of DFIG-WF are difficult to obtain,reinforcement learning and least squares method are applied to identify those important *** predicting the location of closed-loop subsynchronous oscillation(SSO)modes based on the calculation of partial differentials of characteristic equation,both ASSMA and ASSMR can be *** proposed method in this paper can select SSO modes which move to the right half complex planes as control parameters ***,the proposed open-loop analysis method is adaptive to parameter *** studies are carried out on the 4-machine 11-bus power system to verify properties of the proposed method.

关键词： Open-loop modal analysis reinforcement learning based parameter identification subsynchronous resonance

Manipulating d-d orbital hybridization induced by Mo-doped Co_(9)S_(8) nanorod arrays for high-efficiency water electrolysis

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Journal of Energy Chemistry 2024年第6期93卷 592-600,I0015页

作者： Xue Zhou jing Li Guangyao Zhou Weiran huang Yucan Zhang Jun yang huan Pang Mingyi Zhang Dongmei Sun Yawen Tang Lin Xu Jiangsu Key Laboratory of New Power Batteries Jiangsu Collaborative Innovation Centre of Biomedical Functional MaterialsSchool of Chemistry and Materials ScienceNanjing Normal UniversityNanjing 210023JiangsuChina 'College of Science Jinling Institute of TechnologyNanjing 211169JiangsuChina State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China Nanjing IPE Institute of Green Manufacturing Industry Nanjing 211100JiangsuChina School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhou 225009JiangsuChina Key Laboratory for Photonic and Electronic Bandgap Materials Ministry of EducationSchool of Physics and Electronic EngineeringHarbin Normal UniversityHarbin 150025HeilongjiangChina

Precisely refining the electronic structure of electrocatalysts represents a powerful approach to further optimize the electrocatalytic ***,we demonstrate an ingenious d-d orbital hybridization concept to construct Mo-doped Co_(9)S_(8) nanorod arrays aligned on carbon cloth(CC)substrate(abbreviated as Mo-Co_(9)S_(8)@CC hereafter)as a high-efficiency bifunctional electrocatalyst toward water *** has experimentally and theoretically validated that the 4d-3d orbital coupling between Mo dopant and Co site can effectively optimize the h_(2)O activation energy and lower h^(*)adsorption energy barrier,thereby leading to enhanced hydrogen evolution reaction(hER)and oxygen evolution reaction(OER)*** to the unique electronic and geometrical advantages,the optimized Mo-Co_(9)S_(8)@CC with appropriate Mo content exhibits outstanding bifunctional performance in alkaline solution,with the overpotentials of 75 and 234 mV for the delivery of a current density of 10 mA cm^(-2),small Tafel slopes of 53.8 and 39.9 mV dec~(-1)and long-term stabilities for at least 32 and 30 h for hER and OER,*** impressively,a water splitting electrolylzer assembled by the self-supported Mo-Co_(9)S_(8)@CC electrode requires a low cell voltage of 1.53 V at 10 mA cm^(-2)and shows excellent stability and splendid reversibility,demonstrating a huge potential for affordable and scalable electrochemical h_(2) *** innovational orbital hybridization strategy for electronic regulation herein provides an inspirable avenue for developing progressive electrocatalysts toward new energy systems.

关键词： d-d orbital hybridization Transition metal sulfides Nanorods arrays Water electrolysis

Connections Between Induction Generator Effect and Open-loop Modal Proximity to Cause Sub-synchronous Oscillations in Series-compensated Power System

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CSEE Journal of Power and Energy Systems 2024年第3期10卷 963-973页

作者： Wenjuan Du yang Wang h.F.Wang Tao Zhao Tim Littler College of Electrical Engineering Sichuan UniversityChengduChina School of Electrical Engineering the Queen’s University of BelfastBelfastUK IEEE

The induction generator effect(IGE)and the openloop modal proximity(OLMP)are two different reasons why subsynchronous oscillations(SSOs)in a series-compensated power system(SCPS)may *** IGE attributes the growing SSOs to negative resistance,while the OLMP explains the SSO mechanism from the standpoint of modal *** this paper,we investigate the connections between the IGE and the OLMP through equivalent RLC circuit and open-loop modal *** investigation is conducted for two types of seriescompensated power systems where either a synchronous generator or a DFIG is connected at the sending *** investigation reveals the conditions,in which the IGE and the OLMP may jointly cause the growing SSOs,i.e.,both the IGE and the OLMP can explain why the growing SSOs ***,the investigation indicates that the IGE and the OLMP may be totally irrelevant and lead to growing SSOs *** implies that it is possible that in a SCPS,the growing SSOs are only due to the IGE,and the OLMP is non-existent,and vice ***,when the growing SSOs occurs in a SCPS,examination based on both the IGE and the OLMP should be carefully conducted in order to find if the oscillatory instability is due to the IGE,or the OLMP,or both of them.

关键词： Induction generator effect open-loop modal proximity series compensation sub-synchronous oscillations

Expanding Annular Domain Algorithm to Estimate Domains of Attraction for Power System Stability Analysis

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CSEE Journal of Power and Energy Systems 2024年第5期10卷 1925-1934页

作者： Yuqing Lin Tianhao Wen yang Liu Q.h.Wu School of Electric Power Engineering South China University of TechnologyGuangzhou 510640China

This paper presents an Expanding Annular Domain(EAD)algorithm combined with Sum of Squares(SOS)programming to estimate and maximize the domain of attraction(DA)of power *** proposed algorithm can systematically construct polynomial Lyapunov functions for power systems with transfer conductance and reliably determine a less conservative approximated DA,which are quite difficult to achieve with traditional *** linear SOS programming,we begin from an initial estimated DA,then enlarge it by iteratively determining a series of so-called annular domains of attraction,each of which is characterized by level sets of two successively obtained Lyapunov ***,the EAD algorithm is theoretically analyzed in detail and its validity and convergence are shown under certain *** the end,our method is tested on two classical power system cases and is demonstrated to be superior to existing methods in terms of computational speed and conservativeness of results.

关键词： Domain of attraction Lyapunov functions power system transient stability sum of squares programming

Management of locally advanced non-small cell lung cancer: State of the art and future directions

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Cancer Communications 2024年第1期44卷 23-46页

作者： Da Miao jing Zhao Ying han Jiaqi Zhou Xiuzhen Li Ting Zhang Wen Li yang Xia Key Laboratory of Respiratory Disease of Zhejiang Province Department of Respiratory and Critical Care MedicineSecond Affiliated Hospital of Zhejiang University School of MedicineHangzhouZhejiangP.R.China Department of Oncology Shaoxing Second HospitalShaoxingZhejiangP.R.China Department of Medical Oncology Second Affiliated Hospital of Zhejiang University School of MedicineHangzhouZhejiangP.R.China Department of Chemoradiotherapy The Affiliated People’s Hospital of Ningbo UniversityNingboZhejiangP.R.China Key Discipline of Jiaxing Respiratory Medicine Construction Project Jiaxing Key Laboratory of Precision Treatment for Lung CancerAffiliated Hospital of Jiaxing UniversityJiaxingZhejiangP.R.China Department of Pathology Second Affiliated Hospital of Zhejiang University School of MedicineHangzhouZhejiangP.R.China Department of Radiation Oncology Second Affiliated Hospital of Zhejiang University School of MedicineHangzhouZhejiangP.R.China Cancer Center Zhejiang UniversityHangzhouZhejiangP.R.China

Lung cancer is the second most common and the deadliest type of cancer ***,non-small cell lung cancer(NSCLC)is the most com-mon pathological type of lung cancer;approximately one-third of affected patients have locally advanced NSCLC(LA-NSCLC,stage III NSCLC)at *** of its heterogeneity,LA-NSCLC often requires multidisciplinary ***,the prognosis of affected patients is much below satisfac-tion,and the efficacy of traditional therapeutic strategies has reached a *** the emergence of targeted therapies and immunotherapies,as well as the continuous development of novel radiotherapies,we have entered an era of novel treatment paradigm for ***,we reviewed the landscape of relevant therapeutic modalities,including adjuvant,neoadjuvant,and periop-erative targeted and immune strategies in patients with resectable LA-NSCLC with/without oncogenic alterations;as well as novel combinations of chemora-diation and immunotherapy/targeted therapy in unresectable *** addressed the unresolved challenges that remain in the field,and examined future directions to optimize clinical management and increase the cure rate of LA-NSCLC.

关键词： locally advanced non-small cell lung cancer neoadjuvant therapy adjuvant therapy immunotherapy targeted therapy