检索结果-南通市图书馆

Ti_(3)C_(2)T_(x) MXene/carbon composites for advanced supercapacitors:Synthesis,progress,and perspectives

Carbon Energy 2024年第2期6卷 113-142页

作者： Yanqing Cai Xinggang Chen Ying Xu Yalin zhang Huijun Liu Hongjuan zhang jing Tang College of Materials Science and Engineering North China University of Science and TechnologyTangshanChina Hebei Iron and Steel Laboratory North China University of Science and TechnologyTangshanChina Songshan Lake Materials Laboratory DongguanChina Shanghai Key Laboratory of Green Chemistry and Chemical Processes School of Chemistry and Molecular EngineeringEast China Normal UniversityShanghaiChina State Key Laboratory of Petroleum Molecular and Process Engineering(SKLPMPE) Sinopec Research Institute of Petroleum Processing Co.Ltd.BeijingChina Institute of Eco-Chongming ShanghaiChina

MXenes are a family of two-dimensional(2D)layered transition metal carbides/nitrides that show promising potential for energy storage applications due to their high-specific surface areas,excellent electron conductivity,good hydrophilicity,and tunable *** various types of MXenes,Ti_(3)C_(2)T_(x) is the most widely studied for use in capacitive energy storage applications,especially in supercapacitors(SCs).However,the stacking and oxidation of MXene sheets inevitably lead to a significant loss of electrochemically active *** overcome such challenges,carbon materials are frequently incorporated into MXenes to enhance their electrochemical *** review introduces the common strategies used for synthesizing Ti_(3)C_(2)T_(x),followed by a comprehensive overview of recent developments in Ti_(3)C_(2)T_(x)/carbon composites as electrode materials for ***_(3)C_(2)T_(x)/carbon composites are categorized based on the dimensions of carbons,including 0D carbon dots,1D carbon nanotubes and fibers,2D graphene,and 3D carbon materials(activated carbon,polymer-derived carbon,etc.).Finally,this review also provides a perspective on developing novel MXenes/carbon composites as electrodes for application in SCs.

关键词： electrochemical performance MXene/carbon composites supercapacitors

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Effects of thinning and understory removal on water use efficiency of Pinus massoniana:evidence from photosynthetic capacity and stable carbon isotope analyses

引用

Journal of Forestry Research 2024年第2期35卷 42-53页

作者： Ting Wang Qing Xu Beibei zhang Deqiang Gao Ying zhang jing Jiang Haijun Zuo Key Laboratory of Forest Ecology and Environment of National Forestry and Grassland Administration Ecology and Nature Conservation InstituteChinese Academy of ForestryBeijing 100091People’s Republic of China College of Agronomy and Agricultural Engineering Liaocheng UniversityLiaocheng 252000People’s Republic of China Department of Forest and Conservation Sciences Faculty of ForestryUniversity of British ColumbiaVancouverBC V6T 1Z4Canada

Understanding the relationship between forest management and water use efficiency(WUE)is important for evaluating forest adaptability to climate ***,the effects of thinning and understory removal on WUE and its key controlling processes are not well understood,which limits our comprehension of the physiological mechanisms of various management *** this study,four forest management measures(no thinning:NT;understory removal:UR;light thinning:LT;and heavy thinning:HT)were carried out in Pinus massoniana plantations in a subtropical region of *** capacity and needle stable carbon isotope composition(δ^(13)C)were measured to assess instantaneous water use efficiency(WUE_(inst))and long-term water use efficiency(WUE_(i)).Multiple regression models and structural equation modelling(SEM)identified the effects of soil properties and physiological performances on WUE_(inst)and WUE_(i).The results show that WUE_(inst)values among the four treatments were ***,compared with the NT stand(35.8μmol·mol^(-1)),WUE_(i)values significantly increased to 41.7μmol·mol^(-1)in the UR,50.1μmol·mol^(-1)in the LT and 46.6μmol·mol^(-1)in HT treatments,largely explained by photosynthetic capacity and soil water *** removal did not change physiological performance(needle water potential and photosynthetic capacity).Thinning increased the net photosynthetic rate(A_n)but not stomatal conductance(g_s)or predawn needle water potential(ψ_(pd)),implying that the improvement in water use efficiency for thinned stands was largely driven by radiation interception than by soil water *** general,thinning may be an appropriate management measure to promote *** WUE to cope with seasonal droughts under future extreme climates.

关键词： Stable carbon isotope Water use efficiency Thinning Understory removal Photosynthetic capacity Needle water potential

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Resilience-oriented Hardening and Expansion Planning of Transmission System Under Hurricane Impact

引用

CSEE Journal of Power and Energy Systems 2024年第4期10卷 1746-1760页

作者： jing Zhou Heng zhang Haozhong Cheng Shenxi zhang Lu Liu Zheng Wang Xiaohu zhang Key Laboratory of Control of Power Transmission and Conversion Ministry of EducationElectrical Engineering DepartmentShanghai Jiao Tong UniversityShanghai 200240China State Grid East China Branch Shanghai 200120China

In this paper,we propose a two-stage transmission hardening and planning(TH&P)model that can meet the load growth demand of normal scenarios and the resilience requirements of hurricane-induced damage *** better measure the resilience requirements,the proposed TH&P model includes two resilience assessment indexes,namely,the load shedding(LS)under the damage scenario and the average connectivity degree(ACD)at different *** first-stage model,which aims to meet the load growth demand while minimizing the LS,is formulated as a mixed-integer linear program(MILP)to minimize the total planning and hardening cost of transmission lines,the operating cost of generators,and the penalty cost of wind power and load shedding in both normal and damage *** second-stage model aims to further improve the ACD when the ACD of the scheme obtained from the first-stage model cannot reach the ***,the contribution of each transmission line to the ACD is calculated,and the next hardened line is determined to increase the *** process is repeated until the ACD meets the *** studies of the modified IEEE RTS-24 and two-area IEEE reliability test system-1996 indicate the proposed TH&P model can meet the requirements for both normal and damage scenarios.

关键词： Hardening hurricane disaster resilience transmission expansion planning

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Single Fe atom-anchored manganese dioxide for efficient removal of volatile organic compounds in refrigerator

引用

Nano Research 2024年第5期17卷 3927-3933页

作者： Yiwen Wang Jun zhang Yongfei zhang Yu zhang Zhe Wang jing Wang Yuen Wu Department of Endocrinology the First Affiliated Hospital of USTCDivision of Life Science and MedicineUniversity of Science and Technology of ChinaHefei 230001China School of Chemistry and Materials Science University of Science and Technology of ChinaHefei 230026China Hefei Hualing Co. LtdHefei 230088China Linkway Technology Co. LtdResearch Institute of Single Atom Catalysts Industry TechnologyNanning 530000China

The efficient and rapid removal of volatile organic compounds(VOCs)holds significant importance for ensuring food quality and human health,particularly within the low-temperature confined spaces in ***,achieving effective VOCs degradation under such conditions poses challenges in terms of activating inert bonds and facilitating mass *** this study,we propose a novel solution by designing a cleaner module that incorporates 1.07%single Fe atom-anchored manganese dioxide catalysts(FeSAs-MnO_(2)).The combination of single Fe atoms and defect-rich MnO_(2) substrate efficiently activates molecular oxygen,leading to enhanced generation of highly reactive oxygen species(ROS).Non-thermal plasma(NTP)and circulating fan are introduced to facilitate the regeneration of catalytic activity and improve mass *** FeSAs-MnO_(2) cleaner module demonstrates exceptional performance in trimethylamine(TMA)removal,achieving a conversion efficiency of 98.9%for 9 ppm within just 9 ***,accelerated aging tests predict an extended service life of up to 45 years for the FeSAs-MnO_(2) cleaner module,surpassing the expected lifespan of refrigerators significantly.

关键词： single atom catalysts volatile organic compounds(VOCs) trimethylamine(TMA) non-thermal plasma(NTP) refrigerator

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Feasible Synthesis of N,O-Bidentate Difluoroboron Chromophores through Direct Functionalization of Quinoxalin-2(1H)-ones with Ketones in One Shot

引用

Chinese Journal of Chemistry 2024年第13期42卷 1481-1486页

作者： Shuaichen zhang jing zhang Xiang Ling Yifan Zhao Yue Ma Peng Sun State Key Laboratory for Quality Ensurance and Sustainable Use of Dao-di Herbs Artemisinin Research Center and Institute of Chinese Materia MedicaChina Academy of Chinese Medical SciencesBeijing 100700China Department of Pharmaceutics School of PharmacyChina Pharmaceutical UniversityState Key Laboratory of Natural MedicinesNanjingJiangsu 210009China

Organic difluoroboron complexes are a kind of potential platforms for a wide range of applications owing to their excellent photophysical ***,we have explored a simple and direct synthesis methodology for a library of N,O-bidentate difluoroboron complexes from quinoxalin-2(1H)-ones and ketones in one *** photophysical properties of the generated complexes were evaluated and the application potential of these compounds on subcellular imaging was also explored.

关键词： N,O-Bidentate difluoroboron Chromophores Quinoxalin-2(1H)-ones Ketones/Green chemistry Synthetic method C-CcouplingI Boron

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Association of prealbumin with short-term and long-term outcomes in patients with acute ST-segment elevation myocardial infarction

引用

Journal of Geriatric Cardiology 2024年第4期21卷 421-430页

作者： jing TAN Jin SI Ke-Ling XIAO Ying-Hua zhang Qi HUA jing LI Department of Cardiology Xuanwu Hospital Capital Medical UniversityBeijingChina Department of Geriatric Medicine Xuanwu Hospital Capital Medical UniversityNational Clinical Research Center for Geriatric DiseasesBeijingChina

BACKGROUND Prealbumin is considered to be a useful indicator of nutritional status. Furthermore, it has been found to be associated with severities and prognosis of a range of diseases. However, limited data on the association of baseline prealbumin level with outcomes of patients with acute ST-segment elevation myocardial infarction(STEMI) are *** We analyzed 2313 patients admitted for acute STEMI between October 2013 and December 2020. In-hospital outcomes and mortality during the 49 months(interquartile range: 26–73 months) follow-up period were compared between patients with the low prealbumin level(170 mg/L) and those with the high prealbumin level(≥ 170 mg/L).RESULTS A total of 114 patients(4.9%) died during hospitalization. After propensity score matching, patients with the low prealbumin level than those with the high prealbumin level experienced higher incidences of heart failure with Killip class Ⅲ(9.9%vs. 4.4%, P = 0.034), cardiovascular death(8.4% vs. 3.4%, P = 0.035) and the composite of major adverse cardiovascular events(19.2%vs. 10.3%, P = 0.012). Multivariate logistic regression analysis identified that the low prealbumin level(170 mg/L) was an independent predictor of in-hospital major adverse cardiovascular events(odds ratio = 1.918, 95% CI: 1.250–2.942, P = 0.003). The cutoff value of prealbumin level for predicting in-hospital death was 170 mg/L(area under the curve = 0.703, 95% CI: 0.651–0.754, P1;sensitivity = 0.544, specificity = 0.794). However, after multivariate adjustment of possible confounders, baseline prealbumin level(170 mg/L) was no longer independently associated with 49-month cardiovascular death. After propensity score matching, Kaplan-Meier survival curves revealed consistent *** Decreased prealbumin level closely related to unfavorable short-term outcomes. However, after multivariate adjustment and controlling for baseline differences, baseline prealbumin level was not independently assoc

关键词： patients admitted infarction

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

The main strategies for soil pollution apportionment:A review of the numerical methods

引用

Journal of Environmental Sciences 2024年第2期136卷 95-109页

作者： Bin Shi jing Meng TieyuWang Qianqian Li Qifan zhang Guijin Su Research Center for Eco-Environmental Sciences Chinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China Guangdong Provincial Key Laboratory of Marine Disaster Prediction and Prevention Shantou UniversityShantou 515063China

Nowadays,a large number of compounds with different physical and chemical properties have been determined in *** behaviors and source identification of pollutants in soil are the foundation of soil pollution *** and quantitative analysis of potential pollution sources are the prerequisites for its prevention and *** efforts have made to develop methods for identifying the sources of soil *** efforts have involved the measurement of source and receptor parameters and the analysis of their relationships via numerical statistics *** have comprehensively reviewed the progress made in the development of source apportionment methodologies to date and present our *** numerical methods,such as spatial geostatistics analysis,receptor models,and machine learning methods are addressed in *** most cases,however,the effectiveness of any single approach for source apportionment remains *** multiple methods to address soil quality problems can reduce uncertainty about the sources of soil *** review also constructively highlights the key strategies of combining mathematical models with the assessment of chemical profiles to provide more accurate source *** review intends to provide a comprehensive summary of source apportionment methodologies to help promote further development.

关键词： Soil pollutants Source attribution Methodologies Chemical profiles Mathematical models

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Skin neuropathy and immunomodulation in diseases

引用

Fundamental Research 2024年第2期4卷 218-225页

作者： Manze zhang Tingting Liu jing Yang Department of Biology Stanford UniversityStanfordCA 94305USA Department of Biochemistry Weill Cornell Medical CollegeNew YorkNY 10065USA IDG/McGovern Institute for Brain Research Center for Life SciencesSchool of Life SciencesPeking UniversityBeijing 100871China Peking University Third Hospital Cancer Center Beijing 100191China

Skin is a vital barrier tissue of the *** responses in the skin must be precisely controlled,which would otherwise cause severe disease conditions such as psoriasis,atopic dermatitis,or pathogenic *** evidence has increasingly demonstrated the essential roles of neural innervations,i.e.,sensory and sympathetic signals,in modulating skin ***,neuropathic changes of such neural structures have been observed in skin disease conditions,implicating their direct involvement in various pathological *** in-depth understanding of the mechanism underlying skin neuropathy and its immunomodulatory effects could help reveal novel entry points for therapeutic ***,we summarize the neuroimmune interactions between neuropathic events and skin immunity,highlighting the current knowledge and future perspectives of this emerging research frontier.

关键词： Skin Neuropathy Neuroimmune Psoriasis Atopic dermatitis Pathogenic infection

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Selective photosynthesis of Z-olefins through crystalline metal-organic cage-initiated expeditious cascade reactions

引用

Carbon Energy 2024年第3期6卷 118-131页

作者： Jia-Ni Lu Yunze Huang Yuan-Sheng Xia Long-zhang Dong Lei zhang jing-jing Liu Lan-Gui Xie Jiang Liu Ya-Qian Lan Jiangsu Key Laboratory of New Power Batteries School of Chemistry and Materials ScienceJiangsu Collaborative Innovation Centre of Biomedical Functional MaterialsNanjing Normal UniversityNanjingChina School of Chemistry South China Normal UniversityGuangzhouChina

The semi-hydrogenation of alkyne to form Z-olefins with high conversion and high selectivity is still a huge challenge in the chemical ***,flammable and explosive hydrogen as the common hydrogen source of this reaction increases the cost and danger of industrial ***,we connect the photocatalytic hydrogen evolution reaction and the semihydrogenation reaction of alkynes in series and successfully realize the high selective production of Z-alkenes using low-cost,safe,and green water as the proton *** the cascade reaction,a series of isomorphic metal–organic cage catalysts(Co_(x)Zn_(8−x)L_(6),x=0,3,4,5,and 8)are designed and synthesized to improve the yield of the photocatalytic hydrogen *** them,Co_(5)Zn_(3)L_(6) shows the highest photocatalytic activity,with a H_(2) generation rate of 8.81 mmol g^(−1) h^(−1).Then,Co_(5)Zn_(3)L_(6) is further applied in the above tandem reaction to efficiently reduce alkynes to Z-alkenes under ambient conditions,which can reach high conversion of>98%and high selectivity of>99%,and maintain original catalytic activity after multiple ***“one-pot”tandem reaction can achieve a highly selective and safe stepwise conversion from water into hydrogen into Z-olefins under mild reaction conditions.

关键词： alkyne semi-hydrogenation hydrogen evolution reaction metal-organic cages photocatalysis Z-olefins

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Real-time,single-particle chemical composition,volatility and mixing state measurements of urban aerosol particles in southwest China

引用

Journal of Environmental Sciences 2024年第2期136卷 361-371页

作者： Luyao Chen Junke zhang Jiaqi Li Xiaojuan Huang Yuzheng Xiang jing Chen Tingru Pan Wei zhang Faculty of Geosciences and Environmental Engineering Southwest Jiaotong UniversityChengdu 611756China School of Atmospheric Sciences Chengdu University of Information TechnologyChengdu 610225China Sichuan Environmental Monitoring Center Chengdu 610074China

To investigate the volatility of atmospheric particulates and the evolution of other particulate properties(chemical composition,particle size distribution and mixing state)with temperature,a thermodenuder coupled with a single particle aerosol mass spectrometer was used to conduct continuous observations of atmospheric fine particles in Chengdu,southwest *** of their complex sources and secondary reaction processes,the average mass spectra of single particles contained a variety of chemical components(including organic,inorganic and metal species).When the temperature rose from room temperature to280℃,the relative areas of volatile and semi-volatile components decreased,while the relative areas of less or non-volatile components ***(>80%)nitrate and sulfate existed in the form of NH_(4)NO_(3)and(NH_(4))_(2)SO_(4),and their volatilization temperatures were50–100℃and 150–280℃,*** contribution of biomass burning(BB)and vehicle emission(VE)particles increased significantly at 280℃,which emphasized the important role of regional biomass burning and local motor vehicle emissions to the core of *** the increase in temperature,the particle size of the particles coated with volatile or semi-volatile components was reduced,and their mixing with secondary inorganic components was significantly *** formation of K-nitrate(KNO_(3))and K-sulfate(KSO_(4))particles was dominated by liquid-phase processes and photochemical reactions,*** KNO_(3)and BB particles is the key to improving *** new results are helpful towards better understanding the initial sources,pollution formation mechanisms and climatic effects of fine particulate matter in this megacity in southwest China.

关键词： Atmospheric fine particles TD-SPAMS Chemical composition Volatility Mixing state

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

欢迎您,

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案：

请选择收藏分类：

通借通还

欢迎您,

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：