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Ultrastable and High-Performance Silk Energy Harvesting Textiles

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Nano-Micro Letters 2020年第1期12卷 143-157页

作者： Chao Ye Shaojun Dong Jing Ren Shengjie Ling School of Physical Science and Technology ShanghaiTech University

Energy harvesting textiles(EHTs)have attracted much attention in wearable electronics and the internet-of-things for real-time mechanical energy harvesting associated with human activities.However,to satisfy practical application requirements,especially the demand for long-term use,it is challenging to construct an energy harvesting textile with elegant trade-off between mechanical and triboelectric performance.In this study,an energy harvesting textile was constructed using natural silk inspired hierarchical structural designs combined with rational material screening;this design strategy provides multiscale opportunities to optimize the mechanical and triboelectric performance of the final textile system.The resulting EHTs with traditional advantages of textiles showed good mechanical properties(tensile strength of 237±13 MPa and toughness of 4.5±0.4 MJ m−3 for single yarns),high power output(3.5 mW m−2),and excellent structural stability(99%conductivity maintained after 2.3 million multi-type cyclic deformations without severe change in appearance),exhibiting broad application prospects in integrated intelligent clothing,energy harvesting,and human-interactive interfaces.

关键词： Silk Energy harvesting textile Co-wrapped yarn Triboelectric nanogenerator

Study on the mechanism and reaction characteristics of metal-supported phosphogypsum as oxygen carrier in a chemical looping gasification application

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Journal of Environmental Sciences 2024年第4期138卷 428-438页

作者： jing Yang Yujie ren Shuoyu Chen Jinsuo Lu School of Environmental and Municipal Engineering Xi’an University of Architecture and TechnologyXi’an 710055China

This study aimed to explore the chemical looping gasification(CLG)reaction characteristics of the metal-supported composite phosphogypsum(PG)oxygen carriers(OCs)and the thermodynamic mechanism.The FactSage 7.1 thermodynamic simulation was used to explore the oxygen release and H_(2)S removal mechanisms.The experimental results showed that the syngas yield of CLG with PG-CuFe_(2)O_(4)was more than that with PG-Fe_(2)O_(3)20/CuO40 or PG-Fe_(2)O_(3)30/CuO30 OC at 1023 K when the water vapor content was 0.3.Furthermore,the maximum syngas yield of the CO selectivity was 70.3% and of the CO_(2)selectivity was 23.8%.The H_(2)/CO value was 0.78,and the highest carbon conversion efficiency was 91.9% in PG-CuFe_(2)O_(4)at the gasification temperature of 1073 K.The metal-supported PG composite oxygen carrier was proved not only as an oxygen carrier to participate in the preparation of syngas but also as a catalyst to catalyze coal gasification reactions.Furthermore,both the experimental results and FactSage 7.1 thermodynamic analysis revealed that the trapping mechanism of H_(2)S by composite OCs was as follows:CuO first lost lattice oxygen as an oxygen carrier to generate Cu_(2)O,which,in turn,reacted with H_(2)S to generate Cu_(2)S.This study provided efficient guidance and reference for OC design in CLG.

关键词： Metal-supported composite phosphogypsum Reaction characteristics Thermodynamic mechanism Chemical looping gasification

Femtosecond laser-engineered 3D microfluidic chips: Synthesis system sprouting highly efficient multiphase organic reactions

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Chinese Chemical Letters 2023年第4期34卷 338-344页

作者： Jing Ren Kexin Niu Miao Wu Ya Cheng Guoyue Shi School of Chemistry and Molecular Engineering Shanghai Key Laboratory for Urban Ecological Processes and Eco-RestorationEast China Normal UniversityShanghai 200241China School of Physics and Electronic Science East China Normal UniversityShanghai 200241China

Recent developments in the utilization of microfluidic chips(MFCs) have shown their potential utility in multiphase organic synthesis by enabling efficient organic reactions in flow chemistry. However, MFCs technology has been wandering in the laboratory of small dose synthetic routes, which is limited to the level of "tiny" fluid flux. To address this issue, we herein report the first case of the chips with highthroughput 3D channels produced by femtosecond laser being used to create a time-saving, cost-effective and risk-free approach suitable for large-scale flow synthesis. Several multiphase reactions have been successfully prepared on demand in our designed flow synthesis system containing 3D MFCs: 1) benzyl alcohol was converted to benzaldehyde in 3 min with a yield of 97.50% by liquid-liquid two-phase transfer catalytic oxidation;2) organozinc reagents and α-cyano carbonyl carbon compounds were synthesized by solid-liquid two-phase metal insertion reaction in 7 min, and the yield was up to 100%;3) benzoic acid was synthesized by gas-liquid two-phase carboxylation reaction in 2.8 s with a yield of 96%. Significant gains in production rate result from the effective scaling of flow reactors from microliters per hour in MFCs to intermediate milliliters per minute without affecting mass transport performance. Meanwhile,our 3D MFCs show excellent mass and heat transfer efficiency in large-scale industrial units, breaking through the bottleneck in this field. As a result, it is possible to imagine the creation of a new, streamlined flow synthetic technique via MFCs for green multiphase organic synthesis.

关键词： 3D microfluidic chips Femtosecond laser micromachining Flow synthesis Multiphase reaction Organometrical reagents

A general method for one-step synthesis of monofluoroiodane(Ⅲ)reagents using silver difluoride

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Chinese Chemical Letters 2022年第11期33卷 4834-4837页

作者： Jing Ren Meng-Cheng Jia Feng-Huan Du Chi Zhang State Key Laboratory of Elemento-Organic Chemistry The Research Institute of Elemento-Organic ChemistryCollege of ChemistryNankai UniversityTianjin 300071China

Herein we report a new general method for one-step synthesis of four kinds of fluoroiodane(Ⅲ)reagents by treating the corresponding aryl iodides with silver difluoride(AgF_(2)).This is the first method applicable for the synthesis of all four fluoroiodane(Ⅲ)reagents including p-iodotoluene difluoride(1),fluoro-benziodoxole(2),fluoro-benziodoxolone(3),and fluoro-N-acetylbenziodazole(4).AgF_(2)was firstly employed in the direct oxidative fluorination of iodobenzene and thus has shown its outstanding oxidation and fluorine-transfer ability.The use of AgF_(2)has improved the synthesis of fluoroiodane(Ⅲ)reagents by shortening the reaction steps,avoiding the use of hazardous reagents,and simplifying the experimental operations.It was worth noting that we have developed the first one-step direct synthetic method for 3,while 3 can only be synthesized through Cl→F ligand exchange reaction previously.

关键词： Monofluoroiodane(Ⅲ)reagents Silver difluoride Iodobenzene derivatives One-step synthesis DFT calculations

Thermochromic Silks for Temperature Management and Dynamic Textile Displays

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Nano-Micro Letters 2021年第5期13卷 17-33页

作者： Yang Wang Jing Ren Chao Ye Ying Pei Shengjie Ling School of Physical Science and Technology ShanghaiTech University393 Middle Huaxia RoadShanghai 201210People’s Republic of China School of Materials Science and Engineering Zhengzhou UniversityZhengzhouPeople’s Republic of China

Silks have various advantages compared with synthetic polymer fibers,such as sustainability,mechanical properties,luster,as well as air and humidity permeability.However,the functionalization of silks has not yet been fully developed.Functionalization techniques that retain or even improve the sustainability of silk production are required.To this end,a low-cost,effective,and scalable strategy to produce TCSs by integrating yarn-spinning and continuous dip coating technique is developed herein.TCSs with extremely long length(>10 km),high mechanical performance(strength of 443.1 MPa,toughness of 56.0 MJ m−3,comparable with natural cocoon silk),and good interfacial bonding were developed.TCSs can be automatically woven into arbitrary fabrics,which feature super-hydrophobicity as well as rapid and programmable thermochromic responses with good cyclic performance:the response speed reached to one second and remained stable after hundreds of tests.Finally,applications of TCS fabrics in temperature management and dynamic textile displays are demonstrated,confirming their application potential in smart textiles,wearable devices,flexible displays,and human–machine interfaces.Moreover,combination of the fabrication and the demonstrated applications is expected to bridge the gap between lab research and industry and accelerate the commercialization of TCSs.

关键词： Silk Thermochromic Smart textile Dynamic display

Set pair three-way overlapping community discovery algorithm for weighted social internet of things

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Digital Communications and Networks 2023年第1期9卷 3-13页

作者： Chunying Zhang Jing Ren Lu Liu Shouyue Liu Xiaoqi Li Liya Wang College of Science North China University of Science and TechnologyTangshanHebeiChina Hebei Engineering Research Center for the Intelligentization of Iron Ore Optimization and Ironmaking Raw Materials Preparation Processes North China University of Science and TechnologyTangshanHebeiChina Hebei Key Laboratory of Data Science and Application North China University of Science and TechnologyTangshanHebeiChina The Key Laboratory of Engineering Computing in Tangshan City North China University of Science and TechnologyTangshanHebeiChina Tangshan Intelligent Industry and Image Processing Technology Innovation Center North China University of Science and TechnologyTangshanHebeiChina

There are many problems in Social Internet of Things(IoTs),such as complex topology information,different degree of association between nodes and overlapping communities.The idea of set pair information grain computing and clustering is introduced to solve the above problems so as to accurately describe the similarity between nodes and fully explore the multi-community structure.A Set Pair Three-Way Overlapping Community Discovery Algorithm for Weighted Social Internet of Things(WSIoT-SPTOCD)is proposed.In the local network structure,which fully considers the topological information between nodes,the set pair connection degree is used to analyze the identity,difference and reverse of neighbor nodes.The similarity degree of different neighbor nodes is defined from network edge weight and node degree,and the similarity measurement method of set pair between nodes based on the local information structure is proposed.According to the number of nodes'neighbors and the connection degree of adjacent edges,the clustering intensity of nodes is defined,and an improved algorithm for initial value selection of k-means is proposed.The nodes are allocated according to the set pair similarity between nodes and different communities.Three-way community structures composed of a positive domain,boundary domain and negative domain are generated iteratively.Next,the overlapping node set is generated according to the calculation results of community node membership.Finally,experiments are carried out on artificial networks and real networks.The results show that WSIoT-SPTOCD performs well in terms of standardized mutual information,overlapping community modularity and F1.

关键词： Social internet of things Set pair analysis K-means Local information structure Overlapping community

Seasonal variations in wave-induced stress over global ocean based on China France Oceanography Satellite

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Science China Earth Sciences 2023年第12期66卷 2930-2940页

作者： Jing Ren Sheng CHEN Xunqiang YIN Jianqiang LIU Ying XU Fangli QiAO College of Oceanic and Atmospheric Sciences Ocean University of ChinaQingdao 266100China First Institute of Oceanography Ministry of Natural ResourcesQingdao 266061China Key Laboratory of Marine Sciences and Numerical Modeling Ministry of Natural ResourcesQingdao 26661China Key Laboratory of Marine Sciences and Numerical Modeling Shandong ProvinceQingdao 266061China National Satellite Ocean Application Service Beijing 100081China

Due to the scarcity of simultaneous observations on global-scale wind and wave spectra,there has been limited research on the characteristics of global wave-induced stress and wind stress with wave effects using observed wave spectra,particularly their seasonal variations.The China France Oceanography Satellite(CFOSAT)for the first time can simultaneously observe global sea surface wind and wave spectra,providing a solid data basis for investigating this difficult issue.In this study,the seasonal characteristics of global sea surface wave-induced stress and wind stress were analyzed by combining one-year simultaneous wind and wave observations from CFOSAT with a wave boundary layer model.Waveinduced stress was divided into wind-wave-induced stress and swell-induced stress based on different wave forms.The results showed that the wave-induced stress presented a significant inverse correlation with swell index.A higher swell index corresponded to a larger proportion of swell-induced stress,resulting in a decrease in wind stress,and vice versa,wind-wave-induced stress was dominant,resulting in an increase in wind stress.From spring to winter in the Northern Hemisphere(NH),wind-wave-induced stress predominated in the westerly belt of the Southern Hemisphere(SH),while swell-induced stress predominated near the equator.Further analysis revealed that the seasonal variation in wind-waveinduced stress in the SH was not significant,however,wind-wave-induced stress during the boreal summer was significantly lower than that in other seasons.The absolute value of swell-induced stress in the SH showed a trend of decrease and then increase from spring to winter.The percentage of increase or decrease in wind stress after considering the waveinduced stress showed a roughly symmetrical pattern between the NH and SH during the spring and autumn seasons,while the summer and winter seasons showed an asymmetrical feature.Wave-induced stress significantly modulated wind stress,resulting in zonal mean variations by up to±30%.This findin

关键词： China France Oceanography Satellite(CFOSAT) Wave-induced stress Wind stress Seasonal characteristics

Quantitative Evaluation of Pseudo Strain Signals Caused by Yarn Structural Deformation

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Advanced Fiber Materials 2022年第2期4卷 214-225页

作者： Shihui Lin Leitao Cao Zhuochen Lv Jing Ren Shengjie Ling School of Physical Science and Technology ShanghaiTech University393 Middle Huaxia RoadShanghai 201210China

Yarn-based strain sensors(YSSs)have shown great promising in the fabrication of wearable devices for their good comfortability and fexible designability.However,the false signals generated by the changes in the yarn structure of the YSSs are usually ignored.In this study,the generation,the characteristic,and the prediction of these signals were investigated.We recognized that these signals are composed of two negative pseudo peaks and a spurious resistance response plateau.These responses are found to have nothing in common with a true tensile strain,but be attributed to plastic deformation of the fbers.This is due to the fact that the deformation of YSSs exceeds the linear elastic range of the fbers.Although the use of pure elastic fbers can eliminate the spurious resistance response plateau,it will lead to an increase in the pseudo peak to the value compared with a true strain signal peak.Hence,a theoretical model was established to decouple the real signals from the false responses,ensuring the high sensing accuracy of YSSs for applications in wearable devices and artifcial intelligence interfaces.This work provides an in-depth understanding of the response of the YSSs,which might provide inspiration and guidance in the design of high-accuracy fber-based strain sensors.

关键词： Textile strain sensor Pseudo-signal Structure-property relationship Contact resistance

Corneal Endothelial Cell Loss in Femtosecond Laser-assisted Descemet＇s Stripping Automated Endothelial Keratoplasty： A 12-month Follow-up Study

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Chinese Medical Journal 2017年第24期130卷 2927-2932页

作者： Yun Feng Hong-Qiang Qu Jing Ren Philipp Prahs jing Hong Department of Ophthalmology Peking University Third Hospital Peking University Eye Center Beijing 100191 China Department of Ophthalmology University of Regensburg Regensburg 93053 Germany

Background：Descemet＇s stripping automated endothelial keratoplasty （DSAEK） surgery offers a more standardized approach and reliable method to create corneal grafts with an instrument such as a microkeratome.With the development of Descemet＇s membrane endothelial keratoplasty,an excellent clinical outcome is seen in the treatment of corneal endothelial dysfunctions,which indicates that thinner corneal graft results in better clinical outcome.With the recent development of the femtosecond laser,ultrathin corneal graft preparation has become possible.This study aimed to report corneal graft endothelial cell loss （ECL） in a large series of cases undergoing DSAEK with femtosecond laser-assisted corneal graft preparation within a 12-month period.Methods：This study was designed as a prospective,noncomparative,interventional case series.Totally 126 consecutive eyes with endothelial failure of 120 patients,who had corneal endothelial decompensation and underwent femtosecond-assisted DSAEK using the VisuMax femtosecond laser system,were included in the study.Central endothelial cell density （ECD） was recorded postoperatively at 2 weeks （n =126）,1 month （n =126）,3 months （n =110）,6 months （n =101）,and 12 months （n =71） and then compared with the preoperative eye bank measurements.Pre-and postoperative central ECDs were evaluated using Heidelberg retina tomography-Ⅲ confocal microscopy.ECL was calculated for each postoperative time point.Graft thickness was examined using anterior segment-optical coherence tomography.Results：Mean preoperative cell count was 3383 ± 350 cells/mm^2.Mean postoperative cell counts were 2382 ± 707 cells/mm^2,2179 ± 685 cells/mm^2,2074 ± 688 cells/mm^2,1884 ± 662 cells/mm^2,and 1723 ± 624 cells/mm^2 at 2 weeks,1,3,6,and 12 months,respectively;these represented the ECL of 29.7 ± 19.7%,35.4 ± 19.5%,38.6 ± 19.8%,44.3 ± 18.9%,and 48.9 ± 18.4% at the each corresponding time point.The mean corneal graft thickness after surgery was 142 ± 48 μm,118 ± 41 μm,108 ± 37 μm,100 ± 32 μm,and 99 ± 32 μm at each cor

关键词： Corneal Transplantation Descemet＇s Stripping Endothelial Keratoplasty Femtoseconds