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Dynamic recrystallization and silicide precipitation behavior of titanium matrix composites under different strains

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Transactions of Nonferrous Metals Society of China 2021年第11期31卷 3416-3427页

作者： Er-tuan ZHAO Shi-chen SUN jin-rui yu yu-kun AN Wen-zhen CHEN rui-run CHEN School of Mechanical Engineering Shandong University of TechnologyZibo 255022China School of Materials Science and Engineering Harbin Institute of TechnologyWeihai 264209China National Key Laboratory for Precision Hot Processing of Metals Harbin Institute of TechnologyHarbin 150001China

In order to elucidate the microstructure evolution and silicide precipitation behavior during high-temperature deformation,TiB reinforced titanium matrix composites were subjected to isothermal hot compression at 950℃,strain rate of 0.05 s^(−1) and employing different strains of 0.04,0.40,0.70 and *** results show that with the increase of strain,a decrease in the content,dynamic recrystallization of theαphase and the vertical distribution of TiB along the compression axis lead to stress ***,continuous dynamic recrystallization reduces the orientation difference of the primaryαphase,which weakens the texture strength of the *** recrystallization mechanisms are strain-induced grain boundary migration and particle stimulated nucleation by *** silicide of Ti_(6)Si_(3) is mainly distributed at the interface of TiB andα*** precipitation of silicide is affected by element diffusion,and TiB whisker accelerates the precipitation behavior of silicide by hindering the movement of dislocations and providing nucleation particles.

关键词： titanium matrix composites dynamic recrystallization silicide precipitation hot compression

Sulfur doping and oxygen vacancy in In2O3 nanotube co-regulate intermediates of CO2 electroreduction for efficient HCOOH production and rechargeable Zn-CO2 battery

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Journal of Energy Chemistry 2025年第2期101卷 474-484页

作者： yu Li Zhengrong Xu Quanxin Guo Qin Li rui Liu Key Laboratory of Advanced Civil Engineering Materials of Ministry of Education School of Materials Science and Engineering Tongji University

By manipulating the distribution of surface electrons,defect engineering enables effective control over the adsorption energy between adsorbates and active sites in the CO2reduction reaction（CO2RR）.Herein,we report a hollow indium oxide nanotube containing both oxygen vacancy and sulfur doping（V_o-Sx-In2O3） for improved CO2-to-HCOOH electroreduction and *** componential synergy significantly reduces the*OCHO formation barrier to expedite protonation process and creates a favorable electronic micro-environment for*HCOOH *** a result,the CO2RR performance of Vo-Sx-In2O3outperforms Pure-In2O3and V_o-In2O3,where V_o-S53-In2O3exhibits a maximal HCOOH Faradaic efficiency of 92.4% at-1,2 V *** hydrogen electrode（RHE） in H-cell and above 92%over a wide window potential with high current density(119.1 mA cm-2at-1.1 V ***) in flow ***,the rechargeable Zn-CO2battery utilizing V_o-S53-In2O3as cathode shows a high power density of 2.29 mW cm-2and a long-term stability during charge-discharge *** work provides a valuable perspective to elucidate co-defective catalysts in regulating the intermediates for efficient CO2RR.

关键词： CO2 electroreduction In2O3 Intermediate Oxygen vacancy Sulfur doping Zn-CO2 battery

Evaluating complementaries among urban water,energy,infrastructure,and social Sustainable Development Goals in China

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Journal of Environmental Sciences 2025年第3期149卷 585-597页

作者： Ke yu Yifan Song jin Lin Shen Qu School of Management and Economics Beijing Institute of TechnologyBeijing 100081China Center for Energy&Environmental Policy Research Beijing Institute of TechnologyBeijing 100081China

Urban areas’performance in water,energy,infrastructure,and socio-economic sectors is intertwined and measurable through Sustainable Development Goals(SDGs)6–*** synergy among these is critical for *** study constructs an indicator framework that reflects progress towards these urban SDGs in *** indicate underperformance in SDGs 8–11,suggesting the need for transformative *** network analysis,the research reveals complementarities among these ***,the SDG space divides into socio-economic and ecological clusters,with SDG 6(Clean Water and Sanitation)central to ***,SDG 8(Decent Work and Economic Growth)and SDG 9(Industry,Innovation,and Infrastructure)act as bridges,while greater synergies exist between SDG 12(Responsible Consumption and Production)and SDG 13(Climate Action).An in-depth view at the indicator-level shows a core-periphery structure,emphasizing indicators like SDG 6.2(Wastewater Treatment Rate)and SDG 6.6(Recycled Water Production Capacity per capita)as *** study confirms the urban SDG space’s stability and predictiveness,underscoring its value in steering well-aligned policy decisions for sustainable growth.

关键词： Sustainable development goals Synergy Urban development Policy decisions

Sporadic E responds to the 2022 Tonga volcano eruptions recorded by the Meridian Project

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Earth and Planetary Physics 2025年第1期9卷 20-28页

作者： YangYi Sun Tao yu jin Wang Chi Long School of Geophysics and Geomatics China University of Geosciences(Wuhan)Wuhan 430047China School of Physics and Electronic Science Guizhou Normal UniversityGuizhou 550001China

In this study,ionosonde observations over Fuke(19.5°N,109.1°E),Wuhan(30.5°N,114.4°E),and Mohe(53.5°N,122.3°E)were analyzed to demonstrate the responses of the sporadic E()to the severe atmospheric disturbances caused by the Tonga volcanic eruptions on January 15,*** most prominent signature was the disappearance of the layer after~10:00 UT over Wuhan and Fuke,which was attributed to the vertical drift caused by the *** occurred intermittently after 13:00 UT following the arrival of the tropospheric Lamb *** examine the causal mechanism for the intermittence,we also included data of horizontal winds in the mesosphere and lower thermosphere region recorded by the meteor radars at Wuhan and Mohe in this *** wind disturbances with periods of~20 hours contributed to the formation of the layer in the nighttime on January 15.

关键词： sporadic E Tonga eruptions neutral wind disturbances

Precision storage lifetime measurements of highly charged heavy ions in the CSRe storage ring using a Schottky resonator

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Nuclear Science and Techniques 2025年第1期36卷 150-160页

作者： Qian Wang Xin-Liang Yan Guang-yu Zhu Shahab Sanjari Li-Jun Mao He Zhao yuri ALitvinov rui-Jiu Chen Meng Wang yu-Hu Zhang You-jin yuan Jun-Xia Wu Hong-Yang Jiao yue yu Zu-Yi Chen Yin-Fang Luo Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China University of Chinese Academy of Sciences Beijing 100049China GSI Helmholtzzentrum für Schwerionenforschung Planckstrasse 164291 DarmstadtGermany FH Aachen University of Applied Sciences Heinrich-Mussmann-Str.152428 JülichGermany

Schottky mass spectrometry utilizing heavy-ion storage rings is a powerful technique for the precise mass and decay half-life measurements of highly charged *** to the nondestructive ion detection features of Schottky noise detectors,the number of stored ions in the ring is determined by the peak area in the measured revolution frequency *** of their intrinsic amplitude-frequency characteristic(AFC),Schottky detector systems exhibit varying sensitivities at different *** low-energy electron-cooled stored ions,a new method is developed to calibrate the AFC curve of the Schottky detector system of the Experimental Cooler Storage Ring(CSRe)storage ring located in Lanzhou,*** the amplitude-calibrated frequency spectrum,a notable refinement was observed in the precision of both the peak position and peak *** a result,the storage lifetimes of the electron-cooled fully ionized^(56)Fe^(26+)ions were determined with high precision at beam energies of 13.7 and 116.4 MeV/u,despite of frequency drifts during the *** electron cooling was turned off,the effective vacuum condition experienced by the 116.4 MeV/u^(56)Fe^(26+)ions was determined using amplitude-calibrated spectra,revealing a value of 2×10^(−10)mbar,which is consistent with vacuum gauge readings along the CSRe *** method reported herein will be adapted for the next-generation storage ring of the HIAF facility under construction in Huizhou,*** can also be adapted to other storage ring facilities worldwide to improve precision and enhance lifetime measurements using many ions in the ring.

关键词： Lifetime measurement Schottky mass spectrometry Sensitivity response Highly charged heavy ion Resonator UH vacuum Nondestructive diagnostics

Impact of temperature and salinity on fines detachment: AFM measurements and XDLVO theory

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Petroleum Science 2025年第1期22卷 338-347页

作者： Wei-Feng yuan yu-Long Yang Lu yuan Ji-rui Hou State Key Laboratory of Petroleum Resources and Engineering China University of Petroleum Unconventional Petroleum Research Institute China University of Petroleum

Fine particle detachment and subsequent migration can lead to severe pore plugging and consequent permeability decline. Therefore, it is crucial to quantify the critical condition when fine particle detachment occurs. The frequently observed deviations or even contradictions between experimental results and theoretical predictions of fines detachment arise from an insufficient understanding of adhesion force that can be highly influenced by salinity and temperature. To clarify the intrinsic influence of salinity and temperature on fines detachment, adhesion forces between carboxyl microspheres and hydrophilic silica substrates in an aqueous medium were measured at various salinities and temperatures using atomic force microscopy(AFM). The AFM-measured adhesion force decreases with increasing salinity or temperature. Trends of mean measured adhesion forces with temperature and salinity were compared with the DLVO and XDLVO theories. DLVO theory captured the trend with temperature via the impact of temperature on electric double layer interactions, whereas XDLVO theory captured the observed trend with salinity via the impact of salinity on the repulsive hydration force. Our results highlight the significance of hydration force in accurately predicting the fate of fines in porous media.

关键词： Adhesion force AFM Temperature Salinity XDLVO Hydration force

Mechanism of AsperosaponinⅥRelated to EGFR/MMP9/AKT/PI3K Pathway in Treatment of Rheumtoid Arthritis

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Chinese Journal of Integrative Medicine 2025年第2期31卷 131-141页

作者： LUO jin-fang yu Yang LIU Jian-xin School of Basic Medicine Guizhou University of Traditional Chinese MedicineGuiyang(550025)China Sino-Pakistan Center on Traditional Chinese Medicine China-Pakistan International Science and Technology Innovation Cooperation Base for Ethnic Medicine Development in Hunan ProvinceSchool of Pharmaceutical SciencesHunan University of MedicineHuaihua CityHunan Province(418000)China

Objective:To explore the mechanism of action of asperosaponinⅥ(AⅥ)in the treatment of rheumatoid arthritis(RA)and validate it in ex vivo experiments using network pharmacology and molecular docking ***:The predicted targets of AⅥwere obtained from PharmMaper,UniProt and Swiss Target Prediction platforms,the disease targets were collected from Online Mendelian Inheritance in Man,Therapeutic Target Database and Gene Cards databases,the intersection targets of AⅥand RA were obtained from Venny 2.1.0,and the protein-protein interaction(PPI)network was obtained from STRING database,which was analyzed by Cytoscape software and screened to obtain the core *** software was used to analyze PPI network and screen the core *** on the Database for Annotation,Visualization and Integrated Discovery database,Gene Ontology functional and Kyoto Encyclopedia of Genes and Genomes pathway enrichment analysis were performed,and Cytoscape software was used to construct the"DiseasePathway-Target-Drug"network,which was finally verified by molecular docking and animal ***:Network pharmacological studies showed that AⅥwas able to modulate 289 targets,with 102 targets for the potential treatment of RA,with the core pathway being the AKT/PI3K signaling pathway,and the core targets being the epidermal growth factor receptor(EGFR)and matrix metalloproteinase 9(MMP9).Molecular docking results showed that AⅥcould produce strong binding with both of the 2 core *** vitro cellular experiments showed that AⅥreduced nitric oxide,prostaglandin E_2,tumor necrosis factor-alpha(TNF-α),interleukin-6(IL-6),and IL-1βlevels(P<0.05)and inhibited cyclooxygenase-2,nitric oxide synthase,EGFR,MMP9,phosphorylated phosphoinositide 3-kinase(p-PI3K),and phosphorylated serine-threonine kinase(p-AKT)proteins(P<0.05).The results of in vivo studies showed that AⅥimproved RA score and foot swelling thickness and decreased TNF-α,IL-6,p-PI3K and p-AKT levels in RA rat

关键词： inflammation rheumatoid arthritis network pharmacology asperosaponinⅥ EGFR/MMP9/AKT/PI3K pathway

Pyrimidine derivative as eco-friendly corrosion inhibitor for nickel−aluminum bronze in seawater

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中国有色金属学报 2025年第1期35卷 207-224页

作者： jin-yu PI Qi WANG Chao-yang FU Key Laboratory of Material Chemistry for Energy Conversion and Storage Ministry of EducationHubei Key Laboratory of Materials Chemistry and Service FailureSchool of Chemistry and Chemical EngineeringHuazhong University of Science and TechnologyWuhan 430074China

A pyrimidine derivative,6-phenyl-2-thiouracil(PT),was synthesized for developing a corrosion inhibitor(CI)applied in the protection of the nickel−aluminum bronze(NAB)in *** anti-corrosion effect of PT was evaluated by the mass loss experiment,electrochemical tests and surface *** results show that PT exhibits excellent inhibition performance and the maximum inhibition efficiency of PT reaches 99.6%.The interaction mechanism was investigated through X-ray photoelectron spectroscopy(XPS)and molecule dynamics simulation based on the density functional theory(DFT).The S-Cu,Al-N and Cu-N bonds are formed by the chemical interactions,leading to the adsorption of PT on the NAB *** diffusion of corrosive species is hindered considerably by the protective PT film with composition of(PT-Cu)_(ads)and(PT-Al)_(ads)on the PT/NAB *** degree of suppression is increased with the addition of more PT molecules.

关键词： nickel−aluminum bronze corrosion inhibitor diffusion coefficient adsorption seawater

Unveiling solid-solid contact states in all-solid-state lithium batteries:An electrochemical impedance spectroscopy viewpoint

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Journal of Energy Chemistry 2025年第2期101卷 16-22页

作者： jin-Liang Li Liang Shen Zi-Ning Cheng Jun-Dong Zhang Ling-Xuan Li yu-Tong Zhang Yan-Bin Gao Chunli Guo Xiang Chen Chen-Zi Zhao rui Zhang Qiang Zhang Tsinghua Center for Green Chemical Engineering Electrification Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical Engineering Tsinghua University College of Materials Science and Engineering Taiyuan University of Technology Advanced Research Institute of Multidisciplinary Science School of Materials Science and Engineering Beijing Institute of Technology Beijing Huairou Laboratory Institute for Carbon Neutrality Tsinghua University Shanxi Research Institute for Clean Energy Tsinghua University

All-solid-state lithium batteries（ASSLBs） are strongly considered as the next-generation energy storage devices for their high energy density and intrinsic *** solid-solid contact between lithium metal and solid electrolyte plays a vital role in the performance of working ASSLBs,which is challenging to investigate quantitatively by experimental *** work proposed a quantitative model based on the finite element method for electrochemical impedance spectroscopy simulation of different solid-solid contact states in *** the assistance of an equivalent circuit model and distribution of relaxation times,it is discovered that as the number of voids and the sharpness of cracks increase,the contact resistance Rcgrows and ultimately dominates the battery *** accurate fitting,inverse proportional relations between contact resistance Rcand（1-porosity） as well as crack angle was *** contribution affords a fresh insight into clarifying solid-solid contact states in ASSLBs.

关键词： All-solid-state lithium batteries Distribution of relaxation times Electrochemical impedance spectroscopy Equivalent circuit model Finite element method Solid-solid contacts