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A Generative Adversarial Network with an Attention Spatiotemporal Mechanism for Tropical Cyclone Forecasts

Advances in Atmospheric Sciences 2025年第1期42卷 67-78页

作者： Xiaohui LI Xinhai han jingsong YANG Jiuke WANG Guoqi han Jun DING Hui SHEN Jun YAN Satellite Ocean Environment Dynamics Second Institute of OceanographyMinistry of Natural ResourcesHangzhou 310012China School of Oceanography Shanghai Jiao Tong UniversityShanghai 200240China Southern Marine Science and Engineering Guangdong Laboratory(Zhuhai) Zhuhai 519082China School of Artificial Intelligence Sun Yat-sen UniversityZhuhai 519082China Fisheries and Oceans Canada Institute of Ocean SciencesSidney V8L 4B2Canada Zhejiang Marine Monitoring and Forecasting Center Hangzhou 310007China

Tropical cyclones(TCs)are complex and powerful weather systems,and accurately forecasting their path,structure,and intensity remains a critical focus and challenge in meteorological *** this paper,we propose an Attention Spatio-Temporal predictive Generative Adversarial Network(AST-GAN)model for predicting the temporal and spatial distribution of *** model forecasts the spatial distribution of TC wind speeds for the next 15 hours at 3-hour intervals,emphasizing the cyclone's center,high wind-speed areas,and its asymmetric *** effectively capture spatiotemporal feature transfer at different time steps,we employ a channel attention mechanism for feature selection,enhancing model performance and reducing parameter *** utilized High-Resolution Weather Research and Forecasting(HWRF)data to train our model,allowing it to assimilate a wide range of TC motion *** model is versatile and can be applied to various complex scenarios,such as multiple TCs moving simultaneously or TCs approaching *** proposed model demonstrates superior forecasting performance,achieving a root-mean-square error(RMSE)of 0.71 m s^(-1)for overall wind speed and 2.74 m s^(-1)for maximum wind speed when benchmarked against ground truth data from ***,the model underwent optimization and independent testing using ERA5reanalysis data,showcasing its stability and *** fine-tuning on the ERA5 dataset,the model achieved an RMSE of 1.33 m s^(-1)for wind speed and 1.75 m s^(-1)for maximum wind *** AST-GAN model outperforms other state-of-the-art models in RMSE on both the HWRF and ERA5 datasets,maintaining its superior performance and demonstrating its effectiveness for spatiotemporal prediction of TCs.

关键词： tropical cyclones spatiotemporal prediction generative adversarial network attention spatiotemporal mechanism deep learning

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Total synthesis of(+)-taberdicatine B and(+)-tabernabovine B

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Chinese Chemical Letters 2025年第02期36卷 349-353页

作者： Tengfei Xuan Xinyu Zhang Wei han Yidong Huang Weiwu Ren Molecular Synthesis Center&Key Laboratory of Marine Drugs Chinese Ministry of EducationSchool of Medicine and PharmacyOcean University of China Laboratory for Marine Drugs and Bioproducts Laoshan Laboratory

The first total synthesis of(+)-taberdicatine B and(+)-tabernabovine B has been accomplished in 10steps with 26.9% overall yield and 15 steps with 7.3% overall yield, respectively. The prominent features of this efficient synthetic strategy include the following:(1)(+)-Taberdicatine B and(+)-tabernabovine B were accessed from common advanced intermediates by varying the substituents;(2) A one-pot asymmetric bromocyclization/hydrolysis was explored to assemble HPI skeleton;(3) Dieckmann condensation to form β-keto ester for the assembly of seven-membered ring;(4) An ester reduction/amide semireduction/cyclization sequence was applied to form the cage-like framework.

关键词： Asymmetric dearomatization Hexahydropyrrolo[2,3-b]indole Taberdicatine B Tabernabovine B Total synthesis

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Exposure of individuals aged 18-44 years to personal care products in Beijing,China:Exposure profiles,possible influencing factors,and risk assessment

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Journal of Environmental Sciences 2025年第2期148卷 691-701页

作者： Xu Zhang Linxue han Qi Sun Xiaochen Wang Xiaojian Hu Xiao Lin Ying Zhu China CDC Key Laboratory of Environment and Population Health National Institute of Environmental HealthChinese Center for Disease Control and PreventionBeijing 100021China The Bureau for Health Inspection and Supervision of Haidian District Beijing 100037China

Personal care products(PCPs)are a class of emerging pollutants that have attracted public concern owing to their harmful effects on humans and the *** data is valuable for insight the levels of PCPs in the human body and can be crucial for identifying potential health *** gain a better understanding of timely exposure profiles and health risk of reproductive-age population to PCPs,we determined six parabens,six benzophenone-type ultraviolet filters,and three disinfectants in 256 urine samples collected from young adults aged 18-44 years in Beijing,*** urinary levels of benzophenone-3(BP-3)and 4-hydroxybenzophenone(4-OHBP)were significantly higher in summer compared to winter,suggesting these compounds have different seasonal usage ***,the total concentration of 15 PCPs in female was 430 ng/mL,approximately two times higher than that in male.P-chloro-m-xylenol(PCMX),as a new type of antibacterial agent,has the greatest level among all target analytes,indicating the increasingly use of this antibacterial alternative *** potential influencing factors that lead to the elevated exposure level of PCPs were *** 19%of the target population had a high hazard index value(greater than 1)which was attributed to exposure to propyl paraben(PrP),benzophenone-1(BP-1),BP-3 and PCMX,indicating that PCPs may pose a relatively high exposure risk at environmental levels that should be a cause for concern.

关键词： Personal care products Hazard quotient Risk assessment Exposure patterns Urine

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Oxidation behavior of artificial magnetite pellets

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International Journal of Minerals,Metallurgy and Materials 2017年第6期24卷 603-610页

作者： han-quan Zhang jin-tao Fu School of Resource and Civil Engineering Wuhan Institute of Technology Wuhan 430205 China Western Mining Company Xi’ning 810001 China

The oxidation behavior of artificial magnetite pellets was investigated through measurements of the oxidation degree and mineralogical analysis. The results show that artificial magnetite pellets are much easier to oxidize than natural magnetite. The oxidation is controlled through two different reaction mechanisms. The oxidation of artificial magnetite is dominated by internal diffusion, with an activation energy of 8.40 kJ/mol, at temperatures less than 800°C, whereas it is controlled by chemical reaction, with a reaction activation energy of 67.79 kJ/mol, at temperatures greater than 800°C. In addition, factors such as the oxygen volume fraction and the pellet diameter strongly influence the oxidation of artificial magnetite: a larger oxygen volume fraction and a smaller pellet diameter result in a much faster oxidation process.

关键词： artificial magnetite pellets oxidation reaction mechanisms

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Potential role of tanycyte-derived neurogenesis in Alzheimer's disease

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Neural Regeneration Research 2025年第6期20卷 1599-1612页

作者： Guibo Qi han Tang Jianian Hu Siying Kang Song Qin Department of Anatomy Histologyand EmbryologySchool of Basic Medical SciencesFudan UniversityShanghaiChina State Key Laboratory of Medical Neurobiology and MOE Frontiers Center for Brain Science Fudan UniversityShanghaiChina

Tanycytes, specialized ependymal cells located in the hypothalamus, play a crucial role in the generation of new neurons that contribute to the neural circuits responsible for regulating the systemic energy balance. The precise coordination of the gene networks controlling neurogenesis in naive and mature tanycytes is essential for maintaining homeostasis in adulthood. However, our understanding of the molecular mechanisms and signaling pathways that govern the proliferation and differentiation of tanycytes into neurons remains limited. This article aims to review the recent advancements in research into the mechanisms and functions of tanycyte-derived neurogenesis. Studies employing lineage-tracing techniques have revealed that the neurogenesis specifically originating from tanycytes in the hypothalamus has a compensatory role in neuronal loss and helps maintain energy homeostasis during metabolic diseases. Intriguingly,metabolic disorders are considered early biomarkers of Alzheimer's disease. Furthermore,the neurogenic potential of tanycytes and the state of newborn neurons derived from tanycytes heavily depend on the maintenance of mild microenvironments, which may be disrupted in Alzheimer's disease due to the impaired blood–brain barrier ***, the specific alterations and regulatory mechanisms governing tanycyte-derived neurogenesis in Alzheimer's disease remain unclear. Accumulating evidence suggests that tanycyte-derived neurogenesis might be impaired in Alzheimer's disease, exacerbating neurodegeneration. Confirming this hypothesis, however, poses a challenge because of the lack of long-term tracing and nucleus-specific analyses of newborn neurons in the hypothalamus of patients with Alzheimer's disease. Further research into the molecular mechanisms underlying tanycyte-derived neurogenesis holds promise for identifying small molecules capable of restoring tanycyte proliferation in neurodegenerative diseases. This line of investigation could pro

关键词： Alzheimer's disease blood–brain barrier ependymoglial cells hypothalamus metabolic diseases neural stem cells neurogenesis neuroinflammatory diseases neurons tanycyte

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Deep eutectic solvents for separation and purification applications in critical metal metallurgy:Recent advances and perspectives

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 1-19页

作者： Shuo Chen Shengpeng Su Yanfang Huang Bingbing Liu Hu Sun Shuzhen Yang Guihong han School of Chemical Engineering Zhengzhou UniversityZhengzhou 450001China Zhongyuan Critical Metals Laboratory Henan ProvinceZhengzhou 450001China

Solvent extraction,a separation and purification technology,is crucial in critical metal *** solvents commonly used in solvent extraction exhibit disadvantages,such as high volatility,high toxicity,and flammability,causing a spectrum of hazards to human health and environmental *** solvents have been recognized as potential alternatives to these harmful organic *** the past two decades,several neoteric solvents have been proposed,including ionic liquids(ILs)and deep eutectic solvents(DESs).DESs have gradually become the focus of green solvents owing to several advantages,namely,low toxicity,degradability,and low *** this critical review,their classification,formation mechanisms,preparation methods,characterization technologies,and special physicochemical properties based on the most recent advancements in research have been systematically ***,the major separation and purification applications of DESs in critical metal metallurgy were comprehensively ***,future opportunities and challenges of DESs were explored in the current research *** conclusion,this review provides valuable insights for improving our overall understanding of DESs,and it holds important potential for expanding separation and purification applications in critical metal metallurgy.

关键词： deep eutectic solvents preparations properties separation and purification critical metal metallurgy

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白酒中香味物质的顶空—气相色谱/质谱联用分析

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酿酒 2008年第5期35卷 50-51页

作者：任红波黑龙江省农业科学院农产品质量检验中心哈尔滨150086

研究建立了一种快速简单的检测白酒中的香气成份的检测方法,即顶空-气相色谱/质谱联用分析方法,该方法采用静态顶空进样,GC-MS分离鉴定,总离子流色谱的峰面积归一化定量分析白酒中酯类和醇类等香气成份,方法操作简单,定性可靠准确。

关键词：白酒香气顶空气相色谱质谱

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Charge polarity inversion and zincophilicity improvement for chitosan separator towards durable aqueous zinc-ion batteries

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Journal of Energy Chemistry 2025年第2期101卷 110-119页

作者： Jiaqi Yu Bo Liu Hong Ma Zehua Fan Xiang han Qinghua Tian Jizhang Chen Co-Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and Engineering Nanjing Forestry University College of Mathematics and Physics Jinggangshan University Key Laboratory of Surface & Interface Science of Polymer Materials of Zhejiang Province School of Chemistry and Chemical Engineering Zhejiang Sci-Tech University

Aqueous zinc-ion batteries encounter enormous challenges such as Zn dendrites and parasitic *** modification is a highly effective strategy to address these *** the advantages of low cost,nontoxicity,biodegradability,good film-forming ability,superior hydro phi licity,and rich functional groups,chitosan is an ideal matrix for constructing ***,the presence of positive charges within chitosan in weakly acidic electrolytes is unfavorable for dendrite ***,Schiff base reaction is introduced to modify chitosan matrix,transforming its charge polarity from positive to ***,NbN with excellent zincophilicity is coated onto chitosan matrix,forming a Janus separator with low thickness of 19 μm and considerably improved mechanical *** resultant separator can promote the transport of Zn2+ions while triggering a repulsive shielding effect against anions,therefore dramatically enhancing Zn2+ion transfer number from 0.28 to *** separator can also facilitate desolvation process,improve exchange current density,restrict two-dimensional Zn2+ion diffusion,and enhance electrochemical kinetics,contributing to significantly inhibited dendrite growth,by-product formation,and hydrogen ***,stable and reversible Zn stripping/plating process is enabled for over 2500 h at 2 mA cm-2and 2 mAh *** great rate capability and excellent cyclability can be achieved for full batteries even under harsh *** work provides new insights into separator design for Zn-based batteries.

关键词： Aqueous zinc-ion batteries Charge polarity regulation Chitosan utilization Dendrite inhibition Separator modification

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Coordinated Control Strategy of New Energy Power Generation System with Hybrid Energy Storage Unit

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Energy Engineering 2025年第1期122卷 167-184页

作者： Yun Zhang Zifen han Biao Tian Ning Chen Yi Fan School of Mechano-Electronic Engineering Xidian UniversityXi’an710071China Electric Power Control Center State Grid Gansu Electric Power CompanyLanzhou730030China Electric Power Control Center State Grid Gansu Electric Power Company Zhangye Power Supply BranchZhangye734000China

The new energy power generation is becoming increasingly important in the power *** as photovoltaic power generation has become a research hotspot,however,due to the characteristics of light radiation changes,photovoltaic power generation is unstable and random,resulting in a low utilization rate and directly affecting the stability of the power *** solve this problem,this paper proposes a coordinated control strategy for a newenergy power generation system with a hybrid energy storage unit based on the lithium iron phosphate-supercapacitor hybrid energy storage ***,the variational mode decomposition algorithm is used to separate the high and low frequencies of the power signal,which is conducive to the rapid and accurate suppression of the power fluctuation of the energy storage ***,the fuzzy control algorithm is introduced to balance the power between energy *** this paper,the actual data is used for simulation,and the simulation results show that the strategy realizes the effective suppression of the bus voltage fluctuation and the accurate control of the internal state of the energy storage unit,effectively avoiding problems such as overshoot and over-discharge,and can significantly improve the stability of the photovoltaic power generation systemand the stability of the Direct Current *** is of great significance to promote the development of collaborative control technology for photovoltaic hybrid energy storage units.

关键词： Photovoltaic power suppression hybrid energy storage unit variationalmodal decomposition fuzzy control power distribution control

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Experimental Study on Energy Storage Characteristics of Sintered Ore Particle Packed Beds

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Journal of Thermal Science 2025年第1期34卷 242-253页

作者： LAI Zhenya DING Liwei LYU Hongkun HOU Chenglong CHEN Jiaying GUOXutao han Gaoyan ZhanG Kang State Grid Zhejiang Electric Power Research Institute Hangzhou 310014China State Key Laboratory of Clean Energy Utilization Zhejiang UniversityHangzhou 310027China

The particle packed bed energy storage system has advantages such as low costs and wide temperature ranges,which can be combined with solar thermal power generation systems to solve the inherent volatility and discontinuity of renewable *** new materials with low costs and excellent storage performances is one of the eternal research hotspots in the field of energy *** paper innovatively uses sintered ore particles as energy storage material and studies the effect of particle size on the airflow resistance characteristics,energy storage characteristics,and thermocline evolution characteristics of the packed bed through thermal energy storage *** results indicate that for the particles in the macro scale,the smaller the particle,the lower the absolute permeability of the bed and the greater the airflow *** packed bed with smaller particles has a larger specific surface area,larger bulk mass,and smaller bed ***,the packed beds with smaller particles have better thermocline characteristics,less irreversible loss,and can achieve higher thermal efficiency and higher exergy efficiency in the heat storage *** cycle thermal efficiency in packed beds with 25-40 mm,16-25 mm,and 10-16 mm particles is 53.58%,56.27%,and 57.60%,respectively,and the cycle exergy efficiency is 61.81%,69.25%,and 74.13%,***,this paper also studies the effect of discharging airflow rates on thermal storage *** experimental results indicate that suitable discharging strategies should be selected based on different heat demands.

关键词： particle packed bed airflow resistance thermal energy storage thermocline evolution

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