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Nano-Micro Letters 2024年第12期16卷 201-216页

作者： Qinhua gu yiqi Cao Junnan chen Yujie Qi Zhaofeng Zhai Ming Lu Nan Huang Bingsen zhang shenyang National Laboratory for Materials science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016People’s Republic of China school of Materials science and Engineering University of Science and Technology of ChinaShenyang 110016People’s Republic of China The Joint Laboratory of MXene Materials Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of EducationKey Laboratory of Preparation and Application of Environmental Friendly Materials of the Ministry of EducationJilin Normal UniversityChangchun 130103People’s Republic of China

Fluorine owing to its inherently high electronegativity exhibits charge delocalization and ion dissociation capabilities;as a result,there has been an influx of research studies focused on the utilization of fluorides to optimize solid electrolyte interfaces and provide dynamic protection of electrodes to regulate the reaction and function performance of ***,the shuttle effect and the sluggish redox reaction kinetics emphasize the potential bottlenecks of lithium-sulfur *** fluorine modulation regulate the reaction process of Li-s chemistry?Here,the TiOF/Ti_(3)C_(2)MXene nanoribbons with a tailored F distribution were constructed via an NH4F fluorinated *** on in situ characterizations and electrochemical analysis,the F activates the catalysis function of Ti metal atoms in the consecutive redox *** positive charge of Ti metal sites is increased due to the formation of O-Ti-F bonds based on the Lewis acid-base mechanism,which contributes to the adsorption of polysulfides,provides more nucleation sites and promotes the cleavage of s-s *** facilitates the deposition of Li_(2)s at lower ***,fluorine has the capacity to capture electrons originating from Li_(2)s dissolution due to charge compensation *** fluorine modulation strategy holds the promise of guiding the construction of fluorine-based catalysts and facilitating the seamless integration of multiple consecutive heterogeneous catalytic processes.

关键词： Catalysis Fluorination MXene Lithium-sulfur battery shuttle effect

Detector development at the Back-n white neutron source

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辐射探测技术与方法(英文) 2023年第2期7卷 171-191页

作者： Fan Ruirui Li Qiang Bao Jie Li Yang Liu Rong Jiang wei Ren Jie zhang Qiwei Cao Ping gu Minhao Ren Zhizhou yi Han Tang Jingyu An Qi Bai Haofan Bai Jiangbo chen Qiping chen Yonghao chen Zhen Cui Zengqi Fan Anchuan Feng Changqing Feng Fanzhen Gao Keqing Han Changcai Han Zijie He guozhu He Yongcheng Hong Yang Hu yiwei Huang Hanxiong Jia weihua Jiang Haoyu Jiang Zhijie Jin Zhengyao Kang Ling Li Bo Li Chao Li Gong Li Jiawen Li Xiao Liu Jie Liu shubin Luan guangyuan Ning Changjun Qi Binbin Ruan Xichao song Zhaohui sun Kang Tan Zhixin Tang shengda wang Pengcheng wang Zhaohui Wen Zhongwei Wu Xiaoguang Wu Xuan Xie Likun Yang yiwei Yu Yongji zhang guohui zhang Linhao zhang Mohan zhang Xianpeng zhang Yuliang zhang Yue zhang Zhiyong Zhao Maoyuan Zhou Luping Zhou Zhihao Zhu Kejun The CsNs Back-n Collaboration institute of High Energy physics CASBeijing 100049People’s Republic of China spallation Neutron source science Center Dongguan 523803People’s Republic of China state Key Laboratory of Particle Detection and Electronics Beijing 100049People’s Republic of China Key Laboratory of Nuclear Data China Institute of Atomic EnergyBeijing 102413People’s Republic of China institute of Nuclear physics and Chemistry China Academy of Engineering PhysicsMianyang 621900People’s Republic of China Department of Modern physics University of Science and Technology of ChinaHefei 230026People’s Republic of China state Key Laboratory of Particle Detection and Electronics Hefei 230026People’s Republic of China state Key Laboratory of Nuclear physics and Technology School of PhysicsPeking UniversityBeijing 100871People’s Republic of China UsTC archaeometry lab University of Science and Technology of ChinaHefei 230026People’s Republic of China Northwest institute of Nuclear Technology Xi’an 710024People’s Republic of China University of chinese academy of sciences Beijing 100049People’s Republic of China 不详

Purpose Back-n is a white neutron beamline at china spallation neutron source,which was established in the year of *** is a powerful facility for nuclear data measurement,neutron detector calibration,and radiation effect *** A series of detectors were built for different experiments,including beam monitoring,beam profile measurement,neutron induced secondaries(fission fragments,light charged particles and gamma)cross section measurement,and neutron resonance radiography,etc.A common digitization electronics and a cluster-based DAQ were developed for these detector *** detectors have been employed at Back-n and serviced for experiments from the beginning of the beamline *** and conclusion As an overview of detectors of Back-n,the details of the detector design and the experiment performing are described in this *** developing systems,e.g.,MTPC and B-MCP,are also included.

关键词： White neutron source Beam diagnostics Fission fragment Charged particle Gamma Neutron resonance radiography

Electron-Deficient Zn-N_(6) Configuration Enabling Polymeric Carbon Nitride for Visible-Light Photocatalytic Overall Water splitting

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Nano-Micro Letters 2022年第12期14卷 602-616页

作者： Daming Zhao yiqing wang Chung-Li Dong Fanqi Meng Yu-cheng Huang Qinghua zhang Lin gu Lan Liu shaohua shen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049People’s Republic of China state Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022People’s Republic of China Department of physics Tamkang UniversityNew Taipei City 25137TaiwanPeople’s Republic of China Beijing National Laboratory for Condensed Matter physics Institute of PhysicsChinese Academy of SciencesBeijing 100190People’s Republic of China

Despite of suitable band structures for harvesting solar light and driving water redox reactions,polymeric carbon nitride(PCN)has suffered from poor charge transfer ability and sluggish surface reaction kinetics,which limit its photocatalytic activity for water ***,atomically dispersed Zn-coordinated three-dimensional(3D)sponge-like PCN(Zn-PCN)is synthesized through a novel intermediate coordination *** characterizations and theoretical calculations well evidence that Zn single atoms are coordinated and stabilized on PCN in the form of Zn-N_(6) configura-tion featured with an electron-deficient *** an electronic configuration has been demonstrated contributive to promoted electron excitation,accelerated charge separation and transfer as well as reduced water redox *** benefited from the abundant surface active sites derived from the 3D porous structure,Zn-PCN realizes visible-light photocatalysis for overall water splitting with H_(2) and O_(2) simultaneously evolved at a stoichiometric ratio of 2:*** work brings new insights into the design of novel single-atom photocatalysts by deepening the understanding of electronic configurations and reactive sites favorable to excellent photocatalysis for water splitting and related solar energy conversion reactions.

关键词： Zn single atoms Polymeric carbon nitride Overall water splitting Photocatalysis

“一带一路”共建国家应对气候变化合作战略及对策建议

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中国科学院院刊 2023年第9期38卷 1363-1370页

作者：王毅谭显春张井勇李仁强陈敏鹏顾佰和张建平中国科学院科技战略咨询研究院北京100190 中国科学院大学公共政策与管理学院北京100049 中国科学院科技战略咨询研究院碳中和战略研究中心北京100190 中国科学院大气物理研究所北京100029 中国科学院地理科学与资源研究所北京100101 中国人民大学农业与农村发展学院北京100872 对外经济贸易大学中国世界贸易组织研究院北京100029 商务部国际贸易经济合作研究院北京100710

开展“一带一路”应对气候变化合作将有利于处理好经济发展和应对气候变化的关系,对实现区域经济绿色转型具有重要意义。本研究从生物多样性的影响“一带一路”共建国家气候变化的事实和预估出发,分析气候变化对该地区水资源、农业及生... 详细信息

开展“一带一路”应对气候变化合作将有利于处理好经济发展和应对气候变化的关系,对实现区域经济绿色转型具有重要意义。本研究从生物多样性的影响“一带一路”共建国家气候变化的事实和预估出发,分析气候变化对该地区水资源、农业及生物多样性影响,并探讨了“一带一路”共建国家在应对气候变化技术、资金及能力建设等方面的需求缺口。研究发现,相比于减缓技术,多数“一带一路”共建国家对适应技术的需求更为迫切。但“一带一路”共建国家大部分为发展中国家,经济实力相对薄弱,推动其减缓和适应气候变化的各项行动将面临大量的资金缺口,并且多数“一带一路”共建国家在防灾减灾、生态系统治理、低碳产业、森林碳汇、生物多样性等减缓和适应领域均存在能力建设缺口。在此基础上,文章围绕构建人类命运共同体理念,从合作国家、合作领域、合作对策3个方面阐述了“一带一路”气候合作的总体战略,明确了东南亚和非洲作为“一带一路”气候合作的重点地区,以及在技术、资金、能力建设等方面的重点领域。进而提出了整合“顶层设计—资金保障—科技创新—能力建设—话语体系”多措并举的系统化合作方案。

关键词： “一带一路”倡议气候合作技术资金能力建设

search for hidden-charm tetraquark with strangeness in e^(+)e^(−)→K^(+)D_(s)^(∗−) D^(∗0 )+ c.c.

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chinese physics C 2023年第3期47卷 1-14页

作者：麦迪娜 M.N.Achasov P.Adlarson M.Albrecht R.Aliberti A.Amoroso 安美儒安琪白羽 O.Bakina R.Baldini Ferroli I.Balossino Y.Ban V.Batozskaya D.Becker K.Begzsuren N.Berger M.Bertani D.Bettoni F.Bianchi E.Bianco J.Bloms A.Bortone I.Boyko R.A.Briere A.Brueggemann 蔡浩蔡啸 A.Calcaterra 曹国富曹宁 s.A.Cetin 常劲帆常万玲车国荣 G.Chelkov 陈琛陈超陈刚陈和生陈玛丽陈申见陈少敏 T.chen 陈旭荣 X.T.chen 陈元柏陈卓俊成伟帅 s.K.Choi 初晓 G.Cibinetto F.Cossio 崔佳佳代洪亮代建平 A.Dbeyssi R.E.de Boer D.Dedovich 邓子艳 A.Denig I.Denysenko M.Destefanis F.De Mori 丁勇丁逸董静董燎原董明义董翔杜书先段宗欢 P.Egorov 范玉兰方建房双世方文兴方易 R.Farinelli L.Fava F.Feldbauer G.Felici 封常青冯俊华 K Fischer M.Fritsch C.Fritzsch 傅成栋高涵高原宁高扬 s.Garbolino I.Garzia 葛潘婷葛振武耿聪 E.M.Gersabeck A Gilman K.Goetzen 龚丽龚文煊 W.Gradl M.Greco 谷立民顾旻皓顾运厅关春懿郭爱强郭立波郭如盼郭玉萍 A.guskov 韩文颖郝喜庆 F.A.Harris 何凯凯何康林 F.H.Heinsius C.H.Heinz 衡月昆 C.Herold 侯国一侯颖锐侯治龙胡海明 J.F.Hu 胡涛胡誉黄光顺黄凯旋黄麟钦黄性涛黄燕萍黄震 T.Hussain N Hüsken W.Imoehl M.Irshad J.Jackson s.Jaeger s.Janchiv E.Jang J.H.Jeong 纪全姬清平季晓斌季筱璐吉钰瑶贾泽坤蒋沛成姜赛赛江晓山 Y.Jiang 焦健斌焦铮金山金毅荆茂强 T.Johansson s.Kabana N.Kalantar-Nayestanaki 康晓琳康晓珅 R.Kappert M.Kavatsyuk 柯百谦 I.K.Keshk A.Khoukaz R.Kiuchi R.Kliemt L.Koch O.B.Kolcu B.Kopf M.Kuemmel M.Kuessner A.Kupsc W.Kühn J.J.Lane J.s.Lange P.Larin A.Lavania L.Lavezzi 雷天天雷祚弘 H.Leithoff M.Lellmann T.Lenz 李聪李翠李春花李澄李德民李飞李刚李慧李贺李海波李惠静 H.N.Li J.Q.Li 李静舒李井文李科 L.J Li 李龙科李蕾李明浩李培荣李素娴栗帅迎李腾李卫东李卫国李旭红李晓玲李晓宇李彦谷李振轩李紫源梁畅梁浩梁昊梁勇飞梁羽铁廖广睿廖龙洲 J.Libby A.Limphirat 林创新林德旭 T.Lin 刘北江刘成刘春秀 D.Liu 刘福虎刘芳刘峰 G.M.Liu H.Liu 刘宏邦刘怀民刘欢欢刘汇慧刘建北刘佳俊刘晶译刘凯刘魁勇刘珂刘亮刘露刘美宏刘佩莲刘倩刘树彬刘桐刘维克刘卫民刘翔刘英刘玉斌刘振安刘智青娄辛丑卢飞翔吕海江吕军光陆小玲卢宇卢云鹏卢泽辉罗成林罗民兴罗涛罗小兰吕晓睿吕翌丰马凤才马海龙马连良马明明马秋梅马润秋马瑞廷马骁妍马尧 F.E.Maas M.Maggiora s.Maldaner s.Malde Q.A.Malik A.Mangoni 冒亚军毛泽普 s.Marcello 孟召霞 J.G.Messchendorp G.Mezzadri H.Miao 闵天觉 R.E.Mitchell 莫晓虎 N.Yu.Muchnoi Y.Nefedov F.Nerling I.B.Nikolaev 宁哲 s.Nisar 牛艳 s.L.Olsen 欧阳群 s.Pacetti 潘祥潘越 A.Pathak 裴宇鹏 M.Pelizaeus 彭海平 K.Peters 平加伦平荣刚 s.Plura s.Pogodin V.Prasad 齐法制齐航漆红荣祁鸣齐天钰钱森钱文斌钱圳乔从丰秦佳佳秦丽清覃潇平秦小帅秦中华邱进发屈三强 K institute of High Energy physics Beijing 100049China Beihang University Beijing 100191China Beijing institute of PetrochemicalTechnology Beijing 102617China Bochum Ruhr-University D-44780 BochumGermany Carnegie Mellon University PittsburghPennsylvania15213USA Central china Normal University Wuhan 430079China Central south University Changsha 410083China china Center of Advancedscience and Technology Beijing 100190China china University of Geosciences Wuhan 430074China COMsATs University Islamabad LahoreCampusDefence RoadOff Raiwind Road54000 LahorePakistan Fudan University Shanghai 200433China G.I.Budker institute of Nuclearphysics sB RAs(BINP) Novosibirsk 630090Russia GsI Helmholtzcentre for Heavy Ion Research GmbH D-64291 DarmstadtGermany guangxiNormal University Guilin 541004China guangxi University Nanning 530004China Hangzhou Normal University Hangzhou 310036China Hebei University Baoding 071002China Helmholtz institute Mainz Staudinger Weg 18D-55099 MainzGermany Henan NormalUniversity Xinxiang 453007China Henan University of science and Technology Luoyang 471003China Henan University of Technology Zhengzhou 450001China Huangshan College Huangshan 245000China Hunan Normal University Changsha 410081China Hunan University Changsha 410082China Indian institute of Technology Madras Chennai 600036India Indiana University BloomingtonIndiana 47405USA INFN Laboratori Nazionali di Frascati INFN Laboratori Nazionali di FrascatiI-00044FrascatiItaly INFN Laboratori Nazionali di Frascati INFN Sezione di PerugiaI-06100PerugiaItaly INFN Laboratori Nazionali di Frascati University of PerugiaI-06100PerugiaItaly INFN sezione di Ferrara INFN Sezione di FerraraI-44122FerraraItaly INFN sezione di Ferrara University of FerraraI-44122FerraraItaly institute of Modern physics Lanzhou 730000People's Republic of China institute of physics and Technology Peace Avenue 54BUlaanbaatar 13330Mongolia Instituto de Alta Investigación Universidad de TarapacáCasilla 7DAricaChile Jilin Univers

We report a search for a heavier partner of the recently observed Z_(cs)(3985)^(-) state,denoted as Z_(cs)^('-),in the process e^(+)e^(−)→K^(+)D_(s)^(∗−) D^(∗0 )+ c.c.,based on e^(*)e^(-)collision data collected at the center-of-mass energies of √s=4.661,4.682 and 4.699 GeV with the BEsIII *** Z_(cs)^('-) is of interest as it is expected to be a candidate for a hidden-charm and open-strange tetraquark.A partial-reconstruction technique is used to isolate K^(+)recoil-mass spectra,which are probed for a potential contribution from Z_(cs)^('-)→D_(s)^(∗−) D^(∗0 )+ *** find an excess of Z_(cs)^('-)→D_(s)^(*-)-D^(*0)(c.c.)candidates with a significance of 2.1o,after considering systematic uncertainties,at a mass of(4123.5±0.7_(sat)±4.7_(syst.))MeV/c^(2).As the data set is limited in size,the upper limits are evaluated at the 90%confidence level on the product of the Born cross sections(σ^(Borm))and the branching fraction(B)of Z_(cs)^('-)→D_(s)^(*-)-D^(*0),under different assumptions of the Z_(cs)^('-) mass from 4.120 to 4.140 MeV and of the width from 10 to 50 MeV at the three center-of-mass *** upper limits of σ^(Born).B are found to be at the level of O(1)pb at each *** data samples are needed to confirm the Z_(cs)^('-) state and clarify its nature in the coming years.

关键词： electron-positron collision BEsIl hadron spectroscopy tetraquark