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Catalytic conversion and DFT analysis of post DDBD-catalysis system for degradation of toluene,ethyl acetate and acetone with different metal-oxides catalysts

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Journal of Rare Earths 2023年第2期41卷 215-223页

作者： Xin liu jianqi liu Jiayao Chen Fangchuan Zhong College of Environmental Science and Engineering Donghua UniversityShanghai 201620China College of Science Donghua UniversityShanghai 201620China Member of Magnetic Confinement Fusion Research Centre Ministry of EducationShanghai 201620China

A series of multiphase metal-oxide catalysts(MnOx/γ-Al_(2)O_(3),CuOx/γ-Al_(2)O_(3),FeO_(x/γ)-Al_(2)O_(3),CeO_(x)/γ-Al_(2)O_(3)and LaOx/γ-Al_(2)O_(3))were prepared for plasma-catalyst degradation of multicomponent volatile organic compounds(VOCs,such as toluene,acetone and ethyl acetate).The results reveal that the degradation efficiency(DE)of acetone,toluene and ethyl acetate in the DDBD system can be arranged as follows:Mn_(2)O_(3)/γ-Al_(2)O_(3)>Fe2O3/γ-Al_(2)O_(3)>CuO_(/γ)-Al_(2)O_(3)>CeO_(2)/γ-Al_(2)O_(3)>La_(2)O_(3)/γ-Al_(2)O_(3)>γ-Al_(2)O_(3),and the highest DE(49.5%for acetone,93.3%for toluene and 79.8%for ethyl acetate)is obtained in Mn_(2)O_(3)/γ-Al_(2)O_(3)+double dielectric barrier discharge(DDBD)system at specific input energy(SIE)of 700 J/L.Compared with the other catalysts,Mn_(2)O_(3)/γ-Al_(2)O_(3)also exhibits the most significant inhibitory effect on the production of ozone(O3).On the other hand,CeO_(2)/γ-Al_(2)O_(3)and La_(2)O_(3)/γ-Al_(2)O_(3)catalysts display different catalytic selectivity.Both catalysts can slightly raise the DE of VOCs and remarkably facilitate VOCs’mineralization.The carbon balance(CB)is increased by 30.2%and 38.8%,and the CO_(2)selectivity(SCO_(2))is raised by 70.5%and 11.9%in the CeO_(2)/γ-Al_(2)O_(3)+DDBD system and La_(2)O_(3)/γ-Al_(2)O_(3)+DDBD system at SIE of 700 J/L,respectively.To further understand the catalytic effect of the catalysts,the adsorption of O3on different catalysts was simulated by a DFT model.According to the results of the DFT model,it is found that the adsorption energy of other metal oxides seems to be used as a reference for catalytic effect to a certain extent except CeO_(2).The higher the absolute values of adsorption energy,the higher the improvement of VOCs degradation efficiency by catalyst.

关键词： Multiphase metal-oxide catalysts Plasma-catalyst Multicomponent volatile organic compounds Rare earths

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超长隧道平面控制测量横向贯通误差预估研究

测绘通报 2024年第1期 155-160页

作者：司大刚熊文豪张世杰马倩苗培培刘建琪兰州资源环境职业技术大学甘肃兰州730022 内蒙古自治区测绘地理信息中心内蒙古呼和浩特010000 北京飞马航遥科技有限公司北京100192

相向开挖20 km以上的超长隧道,洞内施工环境复杂,相关的洞内外横向贯通误差影响因素的综合分析案例较少,也无超长隧道测量的相关标准规范,导致洞内测量横向摆动难以控制。为给超长隧道建设提供贯通前误差预估,本文分析了横向贯通误差来... 详细信息

相向开挖20 km以上的超长隧道,洞内施工环境复杂,相关的洞内外横向贯通误差影响因素的综合分析案例较少,也无超长隧道测量的相关标准规范,导致洞内测量横向摆动难以控制。为给超长隧道建设提供贯通前误差预估,本文分析了横向贯通误差来源,研究了洞外、洞内控制测量对横向贯通误差的影响规律,估算了洞外GNSS、测角误差、测距误差等对横向贯通的影响值,设计了洞内仿真计算试验,试验顾及了对中误差、观测误差等因素。在不同测角精度、不同导线边长条件下,推导并仿真计算了20~30 km范围内不同隧道长度的洞内横向贯通中误差值。结果表明,提高测角精度对横向贯通精度增益效果明显,仿真计算的结果准确可靠,且以2 km隧道长度为划分区间,获得了超长隧道洞外、洞内横向贯通中误差的推荐值。

关键词：超长隧道横向贯通控制测量观测误差误差估算仿真计算

E-Healthcare Supported by Big Data

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ZTE Communications 2014年第3期12卷 46-52页

作者： jianqi liu Jiafu Wan Shenghua He Yanlin Zhang School of Information Engineering Guangdong Mechanical and Electrical College School of Electrical Engineering and Automation Jiangxi University of Science and Technology

The era of open information in healthcare has arrived. E-healthcare supported by big data supports the move toward greater trans-parency in healthcare by making decades of stored health data searchable and usable. This paper gives an overview the e-health-care architecture. We discuss the four layers of the architecture-data collection, data transport, data storage, and data analysis-as well as the challenges of data security, data privacy, real-time delivery, and open standard interface. We discuss the necessity of establishing an impeccably secure access mechanism and of enacting strong laws to protect patient privacy.

关键词： healthcare wireless body network big data disease prediction remote monitoring medical data

Cosmological Constraints on Neutrino Masses in Light of JWST Red and Massive Candidate Galaxies

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Research in Astronomy and Astrophysics 2024年第4期24卷 7-12页

作者： Jian-Qi liu Zhi-Qi Huang Yan Su School of Physics and Astronomy Sun Yat-sen UniversityZhuhai 519082China CSST Science Center for the Guangdong-Hong Kong-Macao Greater Bay Area Zhuhai 519082China

The overabundance of the red and massive candidate galaxies observed by the James Webb Space Telescope(JWST)implies efficient structure formation or large star formation efficiency at high redshift z~10.In the scenario of a low or moderate star formation efficiency,because massive neutrinos tend to suppress the growth of structure of the universe,the JWST observation tightens the upper bound of the neutrino masses.Assuming A cold dark matter cosmology and a star formation efficiency∈[0.05,0.3](flat prior),we perform joint analyses of Planck+JWST and Planck+BAO+JWST,and obtain improved constraints∑m_(ν)<0.196 eV and ∑m_(ν)+<0.111 eV at 95% confidence level,respectively.Based on the above assumptions,the inverted mass ordering,which implies ∑m_(ν)≥0.1 eV,is excluded by Planck+BAO+JWST at 92.7% confidence level.

关键词： (cosmology:)cosmological parameters galaxies:abundances galaxies:formation neutrinos

Plasmon-enhanced self-powered GaN/ZnTe core/shell nanopillar array photodetector

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Nano Research 2024年第6期17卷 5569-5577页

作者： jianqi Dong Dongqi Zhang Yi Ma Daotong You Jinping Chen Bin liu Xingfu Wang Zengliang Shi Chunxiang Xu State Key Laboratory of Digital Medical Engineering School of Biological Science and Medical EngineeringSoutheast UniversityNanjing 210096China Jiangsu Provincial Key Laboratory of Advanced Photonic and Electronic Materials National Laboratory of Solid State MicrostructuresSchool of Electronic Science and EngineeringNanjing UniversityNanjing 210093China Institute of Photonics Technology Jinan UniversityGuangzhou 510632China Guangdong Engineering Research Center of Optoelectronic Functional Materials and Devices Institute of SemiconductorsSouth China Normal UniversityGuangzhou 510631China

Nanostructure photodetectors,as the core component of optoelectronic devices,are mainly focused on the precise preparation of mixed-component nano-heterostructures and the realization of zero power consumption devices.Herein,we successfully fabricated n-GaN/p-ZnTe core/shell nanopillar array and realized self-power ultraviolet/violet photodetection.The radial heterojunction nanodevice reveals high light-dark current ratio of 104 at 0 V bias,indicating effective carriers’separation.And more,by integrating plasmonic effect,the responsivity and detectivity of the Au nanoparticles decorated device are increased from 3.85 to 148.83 mA/W and 4.45×1011 to 2.33×1012 Jones under 325 nm UV light irradiation.While the rise and the fall time are decreased 1.3 times and 6.8 times under 520 nm visible light irradiation at 0 V bias.The high photocurrent gain is derived from that the oscillating high-energy hot electrons in Au nanoparticles spontaneously inject into the ZnTe conduction band to involve the photodetection process.This work presents an effective route to prepare high-performance self-power photodetector and provides a promising blueprint to realize different functional photoelectronic devices based on core/shell nanostructure.

关键词： GaN/ZnTe core/shell nanopillar array self-power ultraviolet/visible photodetector plasmonic effect

Automation in road distress detection,diagnosis and treatment

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Journal of Road Engineering 2024年第1期4卷 1-26页

作者： Xu Yang jianqi Zhang Wenbo liu Jiayu Jing Hao Zheng Wei Xu School of Future Transportation Chang'an UniversityXi'an 710064China School of Highway Chang'an UniversityXi'an 710064China School of Information Engineering Chang'an UniversityXi'an 710064China

Road transportation plays a crucial role in society and daily life,as the functioning and durability of roads can significantly impact a nation's economic development.In the whole life cycle of the road,the emergence of disease is unavoidable,so it is necessary to adopt relevant technical means to deal with the disease.This study comprehensively reviews the advancements in computer vision,artificial intelligence,and mobile robotics in the road domain and examines their progress and applications in road detection,diagnosis,and treatment,especially asphalt roads.Specifically,it analyzes the research progress in detecting and diagnosing surface and internal road distress and related techniques and algorithms are compared.In addition,also introduces various road gover-nance technologies,including automated repairs,intelligent construction,and path planning for crack sealing.Despite their proven effectiveness in detecting road distress,analyzing diagnoses,and planning maintenance,these technologies still confront challenges in data collection,parameter optimization,model portability,system accuracy,robustness,and real-time performance.Consequently,the integration of multidisciplinary technologies is imperative to enable the development of an integrated approach that includes road detection,diagnosis,and treatment.This paper addresses the challenges of precise defect detection,condition assessment,and unmanned construction.At the same time,the efficiency of labor liberation and road maintenance is achieved,and the automation level of the road engineering industry is improved.

关键词： Road detection Road diagnosis Road treatment Deep learning Intelligent maintenance

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基于全局特征点匹配的全局定位方法

计算机工程与应用 2023年第3期59卷 264-275页

作者：彭泽鑫曾碧刘建圻广东工业大学计算机学院广州510006

针对传统全局定位方法存在对传感器要求多、计算量大的问题,提出了一种基于全局特征点匹配的移动机器人定位方法。该方法采用普通2D雷达作为传感器,在机器人建立全局地图的过程中同步地提取全局特征点,在全局定位算法中,通过建立局部地... 详细信息

针对传统全局定位方法存在对传感器要求多、计算量大的问题,提出了一种基于全局特征点匹配的移动机器人定位方法。该方法采用普通2D雷达作为传感器,在机器人建立全局地图的过程中同步地提取全局特征点,在全局定位算法中,通过建立局部地图和提取局部地图特征点,实时将局部地图特征点和全局地图特征点进行匹配后求解全局位姿。在两个数据集上的测试,结果优于蒙特卡罗自适应定位(adaptive Monte Carlo localization,AMCL)和Cartographer的全局定位效果,运算速度更快。结果表明,与已有的方法相比,该全局定位方法能够更快地完成全局定位和有效减少计算资源的消耗。

关键词：全局定位全局特征点匹配移动机器人

催化剂协同介质阻挡放电等离子体对不同VOCs的催化选择性

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环境工程学报 2022年第6期16卷 1862-1871页

作者：刘鑫刘建奇陈佳尧钟方川东华大学环境科学与工程学院上海201620 东华大学理学院上海201620 教育部磁约束核聚变研究中心东华大学上海201620

为考察混合气体中各组分对VOCs降解的影响,以及催化剂在协同低温等离子体降解多组分VOCs气体中的表现,选取甲苯、丙酮及乙酸乙酯组成混合VOCs进行低温等离子体降解,进而研究混合降解方式对混合VOCs气体各组分降解效果的影响。先制备了Mn... 详细信息

为考察混合气体中各组分对VOCs降解的影响,以及催化剂在协同低温等离子体降解多组分VOCs气体中的表现,选取甲苯、丙酮及乙酸乙酯组成混合VOCs进行低温等离子体降解,进而研究混合降解方式对混合VOCs气体各组分降解效果的影响。先制备了Mn_(2)O_(3)/γ-Al_(2)O_(3)催化剂,采用催化剂后置方式研究催化剂在协同低温等离子体降解多组分混合VOCs气体过程中的表现。结果表明:多组分混合VOCs降解时,甲苯和乙酸乙酯的降解率相较单独降解时都有所提升,当特定输入能量(SIE)为700 J·L^(-1)时,提升率分别为69.1%和12.64%,而丙酮的降解率相较单独降解时却发生了明显下降,下降了40.74%;多组分混合VOCs降解时的臭氧产量相较3种VOCs单独降解时均有微弱下降;多组分混合VOCs相较单种VOCs降解时的碳平衡均略有下降;在协同低温等离子体降解多组分VOCs气体过程中,Mn_(2)O_(3)/γ-Al_(2)O_(3)催化剂对混合VOCs中甲苯、乙酸乙酯及丙酮降解率有明显提升,且随VOCs降解难度的上升而更加明显,并使得各条件下VOCs降解的碳平衡均得到了提升。本研究结果可为低温等离子体降解VOCs的实际应用提供参考。

关键词：混合VOCs降解催化选择性介质阻挡放电

一种边缘梯度插值的双分支deeplabv3+语义分割模型

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智能系统学报 2023年第3期18卷 604-612页

作者：王潇棠闫河刘建骐张烨重庆理工大学两江人工智能学院重庆401135

针对deeplabv3+解码器采用双线性插值的单一分支结构易导致图像的高频分量损失、语义分割精度不高的问题,采用索伯(Sobel)算子计算各像素点沿不同方向的边缘梯度值并结合双三次插值算法,提出一种边缘梯度插值方法;在此基础上,对1/8输入... 详细信息

针对deeplabv3+解码器采用双线性插值的单一分支结构易导致图像的高频分量损失、语义分割精度不高的问题,采用索伯(Sobel)算子计算各像素点沿不同方向的边缘梯度值并结合双三次插值算法,提出一种边缘梯度插值方法;在此基础上,对1/8输入图像与编码器输出采用边缘梯度2倍上插值再经特征融合和边缘梯度2倍上插值操作,并与1/4输入图像经特征融合后再进行边缘梯度4倍上插值操作,从而提出一种边缘梯度插值的双分支deeplabv3+意义分割模型。对比实验结果表明,本文方法在VOC2012数据集上较原分割模型平均交并比指标有2.2%的提升,且对图像边缘细节分割有较好的视觉效果。

关键词：边缘梯度图像插值双三次插值双线性插值 deeplabv3+ 双分支结构解码器语义分割