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Tungsten 2022年第2期4卷 121-129页

作者： Meng Zhao Xi-Yu Zhu Yan-Zhen Li jiang-nan chang Ming-Xue Li Li-Hua Ma Xiao-Yuan Guo Henan Key Laboratory of Polyoxometalate Chemistry Institute of Molecular and Crystal EngineeringSchool of Chemistry and Chemical EngineeringHenan UniversityKaifeng475004China Agricultural Products’Quality and Safety Testing Center of Kaifeng Kaifeng Agriculture and Rural BureauHenan475004China

In this paper,a new organic–inorganic hybrid compound[Co(L)_(2)]2[W_(6)O_(19)](1)(HL=2-acetylpyridine thiosemicarbazone)was prepared and characterized.The compound 1 exhibits remarkable antibacterial activity by determination of minimum inhibitory concentration(MIC)against Staphylococcus aureus(S.aureus,0.06μg·mL^(−1))and Escherichia coli(E.coli,0.24μg·mL^(−1)),respectively.Furthermore,the potential mechanism of compound 1 was studied in detail.The potential causes of bacteria death were cell wall/membrane disruption,inhibition of intracellular respiratory chain dehydrogenases(RCD)activity,destruction of reactive oxygen species(ROS)and depletion of glutathione(GSH).

关键词： Isopolytungstate Thiosemicarbazone Bioactivity Mechanism of action

Pollutant emissions from biomass burning:A review on emission characteristics,environmental impacts,and research perspectives

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Particuology 2024年第2期85卷 296-309页

作者： Ke jiang Ran Xing Zhihan Luo Wenxuan Huang Fan Yi Yatai Men nan Zhao Zhaofeng chang jinfeng Zhao Bo Pan Guofeng shen College of Urban and Environmental Sciences Peking UniversityBeijing100871China Beijing Key Lab Plant Resources Research and Development Beijing Technology and Business UniversityBeijing100048China College of Ecology and Environment Zhengzhou UniversityZhengzhou450001China Facultyof Environmental Sciences and Engineering Kunming University of Science and TechnologyYunnan Provincial Key Laboratoryof Soil Carbon Sequestration and Pollution ControlKunming650500China Institute of Carbon Neutrality Peking UniversityBeijing100871China

Biomass is one most abundant resource on the earth providing important energies in support of so-cioeconomic development in many areas.Burning of biomass fuels comprises to nearly 10%of the total energy from anthropogenic combustion processes:however,as the burning is usually incomplete,this process yields products of incomplete combustion posing consequently significant impacts on air quality,human health,and climate change.Here,we analyzed spatiotemporal characteristics in intentional and unintentional biomass burning from different sectors,discussed impacts of biomass burning emissions on indoor and outdoor air quality,and consequent influences on human health.The global total con-sumption amount of biomass including both natural and anthropogenic sources was approximately 7900 Tg in 2019,with significantly large regional and sectorial discrepancies among regions.Globally,anthropogenic biomass burning amounts increased gradually,but notably in some developing countries like China residential consumption of biomass fuels,as one large sector of biomass use,decreased over time.Uncommercial biomass consumption needs to be accurately quantified.There are relatively rich datasets of pollutant emission factors from biomass burning,including laboratory and field tests,but still large variations exit and contribute substantially to the uncertainty in emission inventory.Global pri-mary PM2.5,black carbon and organic carbon emissions from biomass burning were about 51,4.6,and 29 Tg,respectively,contributing to nearly 70%,55%,and 90%of the total emission from all sources,and emissions from the residential sector and open fires are major sources.Brown carbon emissions from biomass burning attracts growing interests but available studies adopted different methodologies challenging the comparability of those results.Biomass burning emissions polluted not only ambient air but more severely indoor air quality,adversely affecting human health.Future studies that should be emphasized and promoted are suggested.

关键词： Biomass burning Carbonaceous aerosol Emission Air quality Human health

Ionic Liquid-Enhanced Assembly of nanomaterials for Highly Stable Flexible Transparent Electrodes

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nano-Micro Letters 2024年第7期16卷 441-455页

作者： Jianmin Yang Li chang Xiqi Zhang Ziquan Cao Lei jiang Key Laboratory of Bio-Inspired Materials and Interfacial Science Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190People’s Republic of China University of Chinese Academy of Sciences Beijing 100049People’s Republic of China College of Chemistry and Chemical Engineering Chongqing University of TechnologyChongqing 400054People’s Republic of China Binzhou Institute of Technology Binzhou 256600People’s Republic of China nanomics Biotechnology Co. Ltd.HangzhouPeople’s Republic of China

The controlled assembly of nanomaterials has demon-strated significant potential in advancing technological devices.However,achieving highly efficient and low-loss assembly technique for nanomate-rials,enabling the creation of hierarchical structures with distinctive func-tionalities,remains a formidable challenge.Here,we present a method for nanomaterial assembly enhanced by ionic liquids,which enables the fabrication of highly stable,flexible,and transparent electrodes featuring an organized layered structure.The utilization of hydrophobic and non-volatile ionic liquids facilitates the production of stable interfaces with water,effectively preventing the sedimentation of 1D/2D nanomaterials assembled at the interface.Furthermore,the interfacially assembled nanomaterial monolayer exhibits an alternate self-climbing behavior,enabling layer-by-layer transfer and the formation of a well-ordered MXene-wrapped silver nanowire network film.The resulting composite film not only demonstrates exceptional photoelectric performance with a sheet resistance of 9.4Ωsq^(-1) and 93%transmittance,but also showcases remarkable environmental stability and mechanical flexibility.Particularly noteworthy is its application in transparent electromagnetic interference shielding materials and triboelectric nanogenerator devices.This research introduces an innovative approach to manufacture and tailor functional devices based on ordered nanomaterials.

关键词： Ionic liquids Assembly Silver nanowires MXene nanosheets Flexible transparent electrodes

Unraveling the complex roles of macrophages in obese adipose tissue:an overview

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Frontiers of Medicine 2024年第2期18卷 205-236页

作者： chang Peng Jun Chen Rui Wu Haowen jiang Jia Li Hangzhou Institute for Advanced Study University of Chinese Academy of SciencesHangzhou310000China State Key Laboratory of Drug Research Shanghai Institute of Materia MedicaChinese Academy of SciencesShanghai201203China University of Chinese Academy of Sciences Beijing100049China Department of Prosthodontics Shanghai Engineering Research Center of Advanced Dental Technology and MaterialsShanghai Key Laboratory of Stomatology&Shanghai Research Institute of StomatologyNational Clinical Research Center for Oral DiseasesShanghai Ninth People’s HospitalCollege of StomatologyShanghai Jiao Tong University School of MedicineShanghai200011China

Macrophages,a heterogeneous population of innate immune cells,exhibit remarkable plasticity and play pivotal roles in coordinating immune responses and maintaining tissue homeostasis within the context of metabolic diseases.The activation of inflammatory macrophages in obese adipose tissue leads to detrimental effects,inducing insulin resistance through increased inflammation,impaired thermogenesis,and adipose tissue fibrosis.Meanwhile,adipose tissue macrophages also play a beneficial role in maintaining adipose tissue homeostasis by regulating angiogenesis,facilitating the clearance of dead adipocytes,and promoting mitochondrial transfer.Exploring the heterogeneity of macrophages in obese adipose tissue is crucial for unraveling the pathogenesis of obesity and holds significant potential for targeted therapeutic interventions.Recently,the dual effects and some potential regulatory mechanisms of macrophages in adipose tissue have been elucidated using single-cell technology.In this review,we present a comprehensive overview of the intricate activation mechanisms and diverse functions of macrophages in adipose tissue during obesity,as well as explore the potential of drug delivery systems targeting macrophages,aiming to enhance the understanding of current regulatory mechanisms that may be potentially targeted for treating obesity or metabolic diseases.

关键词： obesity inflammation adipose tissue macrophages adipose tissue homeostasis

Research on Optimal Preload Method of Controllable Rolling Bearing Based on Multisensor Fusion

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Computer Modeling in Engineering & Sciences 2024年第6期139卷 3329-3352页

作者： Kuosheng jiang Chengrui Han Yasheng chang School of Mechanical and Electrical Engineering Anhui University of Science and TechnologyHuainan232001China School of Optical and Electronic Information Suzhou City University&Suzhou Key Laboratory of BiophotonicsSuzhou215104China State Key Laboratory for Manufacturing Systems Engineering Xi’an Jiaotong UniversityXi’an710054China

Angular contact ball bearings have been widely used in machine tool spindles,and the bearing preload plays an important role in the performance of the spindle.In order to solve the problems of the traditional optimal preload prediction method limited by actual conditions and uncertainties,a roller bearing preload test method based on the improved D-S evidence theorymulti-sensor fusion method was proposed.First,a novel controllable preload system is proposed and evaluated.Subsequently,multiple sensors are employed to collect data on the bearing parameters during preload application.Finally,a multisensor fusion algorithm is used to make predictions,and a neural network is used to optimize the fitting of the preload data.The limitations of conventional preload testing methods are identified,and the integration of complementary information frommultiple sensors is used to achieve accurate predictions,offering valuable insights into the optimal preload force.Experimental results demonstrate that the multi-sensor fusion approach outperforms traditional methods in accurately measuring the optimal preload for rolling bearings.

关键词： Multi-sensor information fusion neural network preload force

Atomically Dispersed Ruthenium Catalysts with Open Hollow Structure for Lithium-Oxygen Batteries

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nano-Micro Letters 2024年第2期16卷 154-164页

作者： Xin Chen Yu Zhang chang Chen Huinan Li Yuran Lin Ke Yu Caiyun nan Chen Chen Beijing Advanced Innovation Center for Materials Genome Engineering Institute of Solid State ChemistryUniversity of Science and Technology BeijingBeijing 100083People’s Republic of China Engineering Research Center of Advanced Rare Earth Materials Department of ChemistryTsinghua UniversityBeijing 100084People’s Republic of China Beijing Key Laboratory of Energy Conversion and Storage Materials Institution College of ChemistryBeijing Normal UniversityBeijing 100875People’s Republic of China

Lithium–oxygen battery with ultrahigh theoretical energy density is considered a highly competitive next-generation energy storage device,but its practical application is severely hindered by issues such as difficult decomposition of discharge products at present.Here,we have developed N-doped carbon anchored atomically dispersed Ru sites cathode catalyst with open hollow structure(h-RuNC)for Lithium–oxygen battery.On one hand,the abundance of atomically dispersed Ru sites can effectively catalyze the formation and decomposition of discharge products,thereby greatly enhancing the redox kinetics.On the other hand,the open hollow structure not only enhances the mass activity of atomically dispersed Ru sites but also improves the diffusion efficiency of catalytic molecules.Therefore,the excellent activity from atomically dispersed Ru sites and the enhanced diffusion from open hollow structure respectively improve the redox kinetics and cycling stability,ultimately achieving a high-performance lithium–oxygen battery.

关键词： Atomically dispersed Open hollow structure Discharge product Lithium Oxygen battery

Cell Consistency Evaluation Method Based on Multiple Unsupervised Learning Algorithms

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Big Data Mining and Analytics 2024年第1期7卷 42-54页

作者： jiang chang Xianglong Gu Jieyun Wu Debu Zhang Stellantis China Technology Center Shanghai 200233China

Unsupervised learning algorithms can effectively solve sample imbalance.To address battery consistency anomalies in new energy vehicles,we adopt a variety of unsupervised learning algorithms to evaluate and predict the battery consistency of three vehicles using charging fragment data from actual operating conditions.We extract battery-related features,such as the mean of maximum difference,standard deviation,and entropy of batteries and then apply principal component analysis to reduce the dimensionality and record the amount of preserved information.We then build models through a collection of unsupervised learning algorithms for the anomaly detection of cell consistency faults.We also determine whether unsupervised and supervised learning algorithms can address the battery consistency problem and document the parameter tuning process.In addition,we compare the prediction effectiveness of charging and discharging features modeled individually and in combination,determine the choice of charging and discharging features to be modeled in combination,and visualize the multidimensional data for fault detection.Experimental results show that the unsupervised learning algorithm is effective in visualizing and predicting vehicle core conformance faults,and can accurately predict faults in real time.The“distance+boxplot”algorithm shows the best performance with a prediction accuracy of 80%,a recall rate of 100%,and an F1 of 0.89.The proposed approach can be applied to monitor battery consistency faults in real time and reduce the possibility of disasters arising from consistency faults.

关键词： battery consistency charging segment data unsupervised learning

Spin-orbit interaction induced Casimir-Lifshitz torque between two-dimensional electron gases

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Science China(Physics,Mechanics & Astronomy) 2024年第8期Mechanics & Astronomy) .卷 138-146页

作者： Jia-nan Rong Liang Chen Kai chang State Key Laboratory of Superlattices and Microstructures Institute of SemiconductorsChinese Academy of Sciences College of Materials Science and Opto-electronic Technology University of Chinese Academy of Sciences School of Mathematics and Physics North China Electric Power University School of Physics Zhejiang University

We investigate theoretically the Casimir interaction between two parallel two-dimensional electron gases(2DEGs) with Rashba and Dresselhaus spin-orbit interactions(SOIs), based on the quantum field theory. We derive an analytical expression for the polarization tensor and obtain the solution to the motion equation of the electromagnetic(EM) field. We calculate the CasimirLifshitz torque(CLT) between two parallel 2DEGs with Rashba and Dresselhaus SOIs, which can be tuned by changing the relative strength between two SOIs. The anisotropic Casimir energy between 2DEGs caused by the interplay between the SOIs of 2DEGs offers a new origin of CLT and a new type of optoelectronic device.

关键词： Casimir torque two-dimensional electron gas spin-orbit interaction

Cobalt-based heterogeneous catalysts for photocatalytic carbon dioxide reduction

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Tungsten 2024年第2期6卷 410-421页

作者： Hong Yuan Jian-Hua Mei Yun-nan Gong Di-chang Zhong Tong-Bu Lu MOE International Joint Laboratory of Materials Microstructure Institute for New Energy Materials and Low Carbon TechnologiesSchool of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China

Solar light-driven CO_(2)reduction to high value-added chemicals has considered as an outstanding way to solve energy crisis and climate warming.Recently,various photocatalysts have been developed to achieve this reaction.Among them,cobaltbased heterogeneous catalysts have attracted great interest because of their promising performance,product selectivity and stability.Herein,we systematically summarize the research progress of various cobalt-based heterogeneous catalysts for the photoreduction of CO_(2),such as single-atom cobalt,and cobalt-based oxides,nitrides,sulfi des,phosphides,metal-organic frameworks and covalent-organic frameworks.Meanwhile,the advantages and structure-activity relationship of these catalysts in photocatalytic CO_(2)reduction reaction are discussed.Finally,the challenges and prospects for constructing cobaltbased heterogeneous catalysts with high effi ciency are highlighted.

关键词： Cobalt Heterogeneous catalysts CO_(2)reduction Photocatalysis

Molecular phylogenetic relationships based on mitochondrial genomes of novel deep-sea corals(Octocorallia:Alcyonacea):Insights into slow evolution and adaptation to extreme deep-sea environments

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Zoological Research 2024年第1期45卷 215-225页

作者： Zhan-Fei Wei Kai-Wen Ta nan-nan Zhang Shan-Shan Liu Liang Meng Kai-Qiang Liu Chong-Yang Cai Xiao-Tong Peng chang-Wei Shao National Key Laboratory of Mariculture Biobreeding and Sustainable Goods Yellow Sea Fisheries Research InstituteChinese Academy of Fishery SciencesQingdaoShandong 266071China BGI-Qingdao BGI-ShenzhenQingdaoShandong 266555China Institute of Deep-Sea Science and Engineering Chinese Academy of SciencesSanyaHainan 572000China

A total of 10 specimens of Alcyonacea corals were collected at depths ranging from 905 m to 1633 m by the manned submersible Shenhai Yongshi during two cruises in the South China Sea(SCS).Based on mitochondrial genomic characteristics,morphological examination,and sclerite scanning electron microscopy,the samples were categorized into four suborders(Calcaxonia,Holaxonia,Scleraxonia,and Stolonifera),and identified as 9 possible new cold-water coral species.Assessments of GC-skew dissimilarity,phylogenetic distance,and average nucleotide identity(ANI)revealed a slow evolutionary rate for the octocoral mitochondrial sequences.The nonsynonymous(Ka)to synonymous(Ks)substitution ratio(Ka/Ks)suggested that the 14 protein-coding genes(PCGs)were under purifying selection,likely due to specific deep-sea environmental pressures.Correlation analysis of the median Ka/Ks values of five gene families and environmental factors indicated that the genes encoding cytochrome b(cyt b)and DNA mismatch repair protein(mutS)may be influenced by environmental factors in the context of deep-sea species formation.This study highlights the slow evolutionary pace and adaptive mechanisms of deep-sea corals.

关键词： Mitochondrial genome Alcyonacea Ka/Ks evolution Environmental factors