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Rare Metals 2024年第2期43卷 511-521页

作者： jian-Peng Sun Yu zheng Zi-Sheng Zhang Xiang-Chao Meng Zi-Zhen Li Key Laboratory of Marine Chemistry Theory and Technology(Ministry of Education) College of Chemistry and Chemical EngineeringOcean University of ChinaQingdao266100China Shanxi Institute of Energy Taiyuan030600China Department of Chemical and Biological Engineering Faculty of EngineeringUniversity of OttawaOttawaONK1N6 N5Canada

Herein,a novel single-atomic Pt doping and interface-rich CoS/Co(OH)_(2)(Pt-CoS/Co(OH)_(2)/C)electrocatalyst has been successfully *** from precise regulation of d-orbital electronic structure modulation on Co site,Pt-CoS/Co(OH)_(2)/C exhibited remarkable HER activity and high stability for hydrogen evolution in splitting both water(73 mV@10 mA·cm^(−2)) and seawater(87 mV@10 mA·cm^(−2)).Notably,atomic Pt doping was introduced into CoS/Co(OH)_(2),which could produce local unbalanced Coulombic force and significantly increased the number of S vacancies,and then expose abundant Co ***,Co(OH)_(2) in Pt-CoS/Co(OH)_(2)/C could act as the adsorption sites for H_(2)O in hydrogen evolution reaction *** functional theory results also proved that atomic Pt doping,S vacancies and Co(OH)_(2) coupling could result in the formation of enriched electronic Co sites and optimize d_(z2) orbital electronic structure,and then realize the depth upward shift of d-band center and enhance the adsorption of H*on Co sites.

关键词： Electrocatalysts Hydrogen evolution reaction Pt-CoS/Co(OH)_(2) d-band center Electronic structure Water/seawater electrolysis

Industrial utilization of arsenic-containing gold dressing tailings as pellet prepared by straight grate process

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Journal of Central South University 2024年第6期31卷 1888-1899页

作者： LIU Wei guo zheng-qi ZHU De-qing PAN jian ZHANG Wu-ju WANG Jin ZHANG Ying-qun YIN Fu-xing School of Minerals Processing and Bioengineering Central South UniversityChangsha 410083China Low-carbon and Hydrogen Metallurgy Research Center Central South UniversityChangsha 410083China Heqing Beiya Mining Co. Ltd.Dali 671507China

The utilization of arsenic-containing gold dressing tailings is an urgent issue faced by gold production companies *** thermodynamic analysis results indicate that ferrous arsenate(FeAsO_(4)),pyrite(FeS_(2))and sodium cyanide(NaCN)in the arsenic-containing gold metallurgical tailings can be effectively removed using straight grate process,and the removal of pyrite and sodium cyanide is basically completed during the preheating stage,while the removal of ferrous arsenate requires the roasting *** pellets undergo a transformation from magnetite to hematite during the preheating process,and are solidified through micro-crystalline bonding and high-temperature recrystallization of hematite(Fe_(2)O_(3))during the roasting ***,pellets with removal rates of 80.77% for arsenic,88.78% for sulfur,and 99.88% for cyanide are obtained,as well as the iron content is 61.1% and the compressive strength is 3071 N,meeting the requirements for blast furnace *** study provides an industrially feasible method for treating arsenic-containing gold smelting tailings,benefiting gold production enterprises.

关键词： arsenic-containing gold dressing tailings pelletizing straight grate process recycling

基于混合策略自适应学习的并行粒子群优化算法

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控制与决策 2013年第7期28卷 1087-1093页

作者：伍大清郑建国东华大学旭日工商管理学院上海200051 南华大学计算机科学与技术学院湖南衡阳421001 人工智能四川省重点实验室四川自贡643000

针对当前各种粒子群优化算法解决问题时存在的局限性,提出一种基于混合策略自适应学习的粒子群优化算法(HLPSO).该算法从收敛速度、跳出局部极值、探索、开发几个不同角度融合了4种具有不同优势的变异策略,当面对不同形态的复杂问题时... 详细信息

针对当前各种粒子群优化算法解决问题时存在的局限性,提出一种基于混合策略自适应学习的粒子群优化算法(HLPSO).该算法从收敛速度、跳出局部极值、探索、开发几个不同角度融合了4种具有不同优势的变异策略,当面对不同形态的复杂问题时通过自适应学习机制选择出合适的策略来完成全局寻优.通过对7个标准测试函数的仿真实验并与其他算法相比较,所得结果表明了所提出的算法具有较快的收敛速度、较高的精度以及很强的跳出局部极值的能力.

关键词：粒子群优化自适应学习变异策略函数优化

NIR-Ⅱ responsive Janus nanoparticles amplify immunogenic cell death for enhanced cancer immunotherapy

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Science China(Technological Sciences) 2024年第1期67卷 321-329页

作者： CHEN BeiBei guo KangLi WANG HaoRan XU Fu-jian WANG JuLin ZHAO NaNa State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical TechnologyBeijing 100029China Key Laboratory of Biomedical Materials of Natural Macromolecules(Beijing University of Chemical Technology) Beijing Laboratory of Biomedical MaterialsBeijing University of Chemical TechnologyBeijing 100029China College of Materials Sciences and Engineering Beijing University of Chemical TechnologyBeijing 100029China Beijing Key Laboratory of Electrochemical Process and Technology for Materials Beijing University of Chemical TechnologyBeijing 100029China

Immunotherapy brings new hope for tumor treatment by inducing immunogenic cell death(ICD)of tumor ***,insufficient immunogenicity and low immune response rate greatly limit antitumor ***,by optimizing the composition and morphology,the rational design of Janus nanoparticles composed of Fe_(3)O_(4) nanospheres and SiO_(2)nanorods was realized for enhanced cancer immunotherapy through amplified *** glucose oxidase(GOx)was loaded by the Janus nanoparticles,the resultant M-FS-GOx consumes glucose at tumor sites to generate gluconic acid and hydrogen peroxide(H_(2)O_(2))for starvation therapy while the H_(2)O_(2)supply promotes the production of highly toxic·OH to achieve effective chemodynamic therapy(CDT).Under a 1064 nm light irradiation,the photothermal effect of M-FS-GOx enhances the enzyme activity of GOx for improved starvation ***,both tumor-associated antigens released during the process of ICD and the intrinsic immunoadjuvant property of M-FS-GOx stimulate dendritic cell maturation to activate antitumor immune *** work provides a promising strategy for the construction of Janus nanoparticles to achieve enhanced cancer immunotherapy through combination therapy-amplified ICD.

关键词： Janus nanoparticles immunogenic cell death cancer immunotherapy

BIO-inspired intelligent navigation: from methodology, system theory, to behavioural science

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Science China(Information Sciences) 2024年第9期67卷 333-335页

作者： Wenshuo LI Xin LIU Pengwei HU jian YANG Xiang YU Lei guo Hangzhou Innovation Institute of Beihang University School of Automation Science and Electrical Engineering Beihang University School of Instrumentation and Optoelectronic Engineering Beihang University

It is crucial for unmanned systems to determine their motion information accurately, reliably, and in real time. This function is accomplished by the autonomous navigation module of the unmanned systems. By analogy to the animals,the autonomous navigation module can be regarded as the“sensory nerve center” of an unmanned system.

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Difference in microstructural characteristics of stamp-charged coke and gravity-charged coke with approximate macroscopic performance

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Journal of Iron and Steel Research International 2024年第5期31卷 1050-1062页

作者： Chong Zou zheng-yan Huang jian-yun Li Bin Li Shi-wei Liu Yuan She School of Metallurgical Engineering Xi’an University of Architecture and TechnologyXi’an710311ShaanxiChina Technical Center of Shandong Iron and Steel Co. Ltd.(Laiwu Branch)Jinan271104ShandongChina

The microstructural characteristics including optical texture,porosity and pore structure and chemical structure of stamp-charged coke(SCC)and gravity-charged coke(GCC)with similar conventional macro-indicators were investigated,and the properties including micro-strength,reactivity of coke matrix and that after alkali enrichment were comparatively studied by various characterization *** anisotropic structure of SCC is composed of high content of fine mosaic texture,while the content of medium mosaic texture,coarse texture and fibrous texture is *** statistical average shows that the fine mosaic average of SCC(24.89%)is 3.78 times the GCC average(6.58%),and the coarse mosaic average(1.24%)is only about 1/3 of the GCC average(3.43%).The porosity of SCC is lower than that of GCC,but tamping process does not lead to the fact that the number of closed pores of SCC is significantly lower than that of *** the structure of SCC is compact,its pore number is large and the pore wall is *** of coke with diameter less than 150 nm seem unaffected by tamping *** aromatic structure of SCC was less ordered than that of GCC,which was speculated to be related to the addition of more low metamorphic coal in *** microscopic strength and structural strength of SCC are lower than those of *** reactivity of coke matrix is affected by the specific surface area,but it is not the determining factor of its *** improvement in dissolution reactivity of coke after potassium enrichment is independent of coke type.

关键词： Stamp-charged coke Optical texture Porosity Microstructure Reactivity

Environmental benefits and farmers' adoption of winter cover crops in the North China Plain

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Pedosphere 2024年第1期34卷 159-169页

作者： Shufang guo Yitao ZHANG Limei ZHAI jian LIU Hongyuan WANG Hongbin LIU State Key Laboratory of Efficient Utilization of Arid and Semi-arid Arable Land in Northern China Key Laboratory of Nonpoint Source Pollution ControlMinistry of Agriculture and Rural AffairsInstitute of Agricultural Resources and Regional PlanningChinese Academy of Agricultural SciencesBeijing 100081China Institute of Agricultural Environment and Resources Yunnan Academy of Agricultural SciencesKunming 650205China Shandong Yucheng Agro-ecosystem National Observation Research Station Key Laboratory of Ecosystem Network Observation and ModelingInstitute of Geographic Sciences and Natural Resources ResearchChinese Academy of SciencesBeijing 100101China The Norwegian Institute of Bioeconomy Research(NIBIO) Akershus 1431Norway

The introduction of cover crops into monoculture systems to improve soil health has been widely adopted worldwide. However, little is known about the environmental risks and application prospects of different cover crops in spring maize(Zea mays L.) monocultures proposed in the North China Plain. A pot experiment was conducted to evaluate the effects of different winter cover crops on subsequent maize yield, soil fertility, and environmental risks of nitrogen(N) loss, and a questionnaire survey was conducted to examine factors influencing farmers' willingness to adopt cover crops in the North China Plain. Based on the same fertilization regime during the maize growing period, four winter cover crop treatments were set up, including bare fallow, hairy vetch(Vicia villosa Roth.), February orchid(Orychophragmus violaceus), and winter oilseed rape(Brassica campestris L.). The results indicated that winter cover crops significantly increased subsequent maize yield and soil organic carbon, total N, and microbial biomass carbon and N compared with the bare fallow *** incorporation of cover crops led to a negligible increase in nitrous oxide(N_(2)O) emissions and had a very limited effect on ammonia(NH_(3)) *** incorporation of February orchid and winter oilseed rape decreased nitrate leaching compared with the hairy vetch treatment in the maize growing *** N losses via N_(2)O and NH_(3) emissions and N leaching accounted for 71%–84% of the N surplus. However, yield increase and environmental benefits were not the main positive factors for farmers to accept cover crops. Financial incentive was rated by 83.9% of farmers as an “extremely important” factor, followed by other costs, when considering winter cover cropping. These results indicate that the environmental benefits depend on the type of cover crop. Maintaining high levels of soil fertility and maize yield, providing sufficient subsidies, and encouraging large-area cultivation of cover crops

关键词： cover crop N leaching NH_(3)emission N_(2)O emission spring maize willingness to accept

How do high-voltage cathode and PEO electrolyte get along well?EIS analysis mechanism&potentiometric control strategy

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Journal of Energy Chemistry 2024年第9期96卷 424-436页

作者： Xiaodong Bai Chaoliang zheng Heng Zhang jian Liu Panpan Wang Baojia Xia jianling Li State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China Shanghai Institute of Microsystem and Information Technology Chinese Academy of SciencesShanghai 201800China

PEO-based all-solid-state electrolytes are extensively utilized and researched owing to their exceptional safety,low-mass-density,and ***,the low oxidation potential of PEO makes the interface problem with the high-voltage cathode extremely *** this work,the impedance of PEO-based all-solid-state batteries with high-voltage cathode(NCM811)was studied at different *** Nyquist plots displayed a gyrate arc at low-frequencies for NCM811/PEO *** on the kinetic modeling,it was deduced that there is a decomposition reaction of PEO-matrix in addition to de-embedded reaction of NCM811,and the PEO intermediate product(dehydra-PEO)adsorbed on the electrode surface leading to low-frequency inductive ***,the distribution of relaxation time shows the dehydra-PEO results in the kinetic tardiness of the charge transfer process in the temporal ***,an artificial interface layer(CEI_(x))was modified on the surface of NCM811 to regulate the potential of cathode/electrolyte interface to prevent the high-voltage deterioration of ***/CEI_(x)/PEO batteries exhibit capacity retentions of 96.0%,84.6%,and 76.8%after undergoing 100 cycles at cut-off voltages of 4.1,4.2,and 4.3 V,***,here the failure mechanism of high-voltage PEO electrolyte is investigated by EIS and a proposed solving strategy is presented.

关键词： PEo-based electrolyte High-voltage cathode Electrochemical impedance spectroscopy Mechanism research Electrochemical characteristic

Double-confined nanoheterostructure Sb/Sb_(2)S_(3)@Ti_(3)C_(2)T_(x)@C toward ultra-stable Li-/Na-ion batteries

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Rare Metals 2024年第5期43卷 2067-2079页

作者： Dan Wang Qun Ma Huan He Zhi-Yuan Wang Run-guo zheng Hong-Yu Sun Yan-guo Liu Chun-Li Liu School of Materials Science and Engineering Northeastern UniversityShenyang110819China School of Resources and Materials Northeastern University at QinhuangdaoQinhuangdao 066004China Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province Qinhuangdao 066004China Department of Physics and Oxide Research Center Hankuk University of Foreign StudiesYongin 17035Korea

Antimony-based materials with high capacities and moderate potentials are promising anodes for lithium-/-sodium-ion ***,their tremendous volume expansion and inferior conductivity lead to poor structural stability and sluggish reaction ***,a doubleconfined nanoheterostructure Sb/Sb_(2)S_(3)@Ti_(3)C_(2)T_(x)@C has been fabricated through a solvothermal method followed by low-temperature heat *** dual protection of“MXene”and“carbon”can better accommodate the volume expansion of Sb/Sb_(2)S_(3).The strong covalent bond(Ti-S,Ti-O-Sb,C-O-Sb)can firmly integrate Sb-based material with Ti_(3)C_(2)T_(x)and carbon,which significantly improves the structure *** addition,the carbon layer can restrain the oxidation of MXenes,and the nano-Sb/Sb_(2)S_(3)can facilitate electron/ion transport and suppress the restacking of *** heterogeneous interface between Sb and Sb_(2)S_(3)can further promote interfacial charge *** MXene-Sb/Sb_(2)S_(3)@C-1 with the optimal Sb content shows high specific capacities,comparable rate properties and ultra-stable cycling performances(250 m Ah·g^(-1)after 2500 cycles at 1 A·g^(-1)for sodium-ion batteries).Ex situ X-ray diffractometer(XRD)test reveals the storage mechanism including the conversion and alloying process of MXene-Sb/Sb_(2)S_(3)@*** voltammetry(CV)test results demonstrate that the pseudocapacitance behavior is dominant in MXene-Sb/Sb_(2)S_(3)@C-1,especially at large *** design paves the way for exploring high-performance alloy-based/conversion-type anode for energy storage devices.

关键词： Sb/Sb_(2)S_(3) MXene Carbon Anode Lithium-ion batteries Sodium-ion batteries

Dynamically updated digital twin for prognostics and health management:Application in permanent magnet synchronous motor

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Chinese Journal of Aeronautics 2024年第6期37卷 244-261页

作者： Haoyu guo Shaoping WANG jian SHI Tengfei MA Giorgio GUGLIERI Rujun JIA Fausto LIZZIO School of Automation Science and Electrical Engineering Beihang UniversityBeijing 100191China Tianmushan Laboratory Hangzhou 310023China Department of Mechanical and Aerospace Engineering Polytechnic University of TurinTurin 10129Italy Beihang Ningbo Research Institute Ningbo 315800China

Current research on Digital Twin(DT)based Prognostics and Health Management(PHM)focuses on establishment of DT through integration of real-time data from various sources to facilitate comprehensive product monitoring and health ***,there still exist gaps in the seamless integration of DT and PHM,as well as in the development of DT multi-field coupling modeling and its dynamic update *** the product experiences long-period degradation under load spectrum,it is challenging to describe the dynamic evolution of the health status and degradation progression *** addition,DT update algorithms are difficult to be integrated simultaneously by current *** paper proposes an innovative dual loop DT based PHM framework,in which the first loop establishes the basic dynamic DT with multi-filed coupling,and the second loop implements the PHM and the abnormal detection to provide the interaction between the dual loops through updating *** proposed method pays attention to the internal state changes with degradation and interactive mapping with dynamic parameter ***,the Independence Principle for the abnormal detection is proposed to refine the theory of *** at the first loop focus on accurate modeling of multi-field coupling,while the events at the second loop focus on real-time occurrence of anomalies and the product degradation *** interaction and collaboration between different loop models are also ***,the Permanent Magnet Synchronous Motor(PMSM)is used to verify the proposed *** results show that the modeling method proposed can accurately track the lifecycle performance changes of the entity and carry out remaining life prediction and health management effectively.

关键词： Digital Twin(DT) Dynamic Update Independence Principle Multi-field Coupling Permanent Magnet Synchronous Motor(PMSM) Prognostics and Health Management(PHM)