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Unlocking the stable interface in aqueous zinc-ion battery with multifunctional xylose-based electrolyte additives

Journal of Energy Chemistry 2025年第1期100卷 770-778页

作者： Xiaoqin Li jian Xiang Lu Qiu Xiaohan Chen Yinkun zhao Yujue Wang Qu Yue Taotao Gao Wenlong Liu Dan Xiao zhaoyu Jin Panpan Li Institute for Advanced Study Chengdu University School of Mechanical Engineering Chengdu University College of Food and Biological Engineering Chengdu University Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of China College of Materials Science and Engineering Sichuan University

The growth of dendrites and the side reactions occurring at the Zn anode pose significant challenges to the commercialization of aqueous Zn-ion batteries（AZIBs）. These challenges arise from the inherent conflict between mass transfer and electrochemical kinetics. In this study, we propose the use of a multifunctional electrolyte additive based on the xylose（Xylo） molecule to address these issues by modulating the solvation structure and electrode/electrolyte interface, thereby stabilizing the Zn anode. The introduction of the additive alters the solvation structure, creating steric hindrance that impedes charge transfer and then reduces electrochemical kinetics. Furthermore, in-situ analyses demonstrate that the reconstructed electrode/electrolyte interface facilitates stable and rapid Zn2+ion migration and suppresses corrosion and hydrogen evolution reactions. As a result, symmetric cells incorporating the Xylo additive exhibit significantly enhanced reversibility during the Zn plating/stripping process, with an impressively long lifespan of up to 1986 h, compared to cells using pure ZnSO4electrolyte. When combined with a polyaniline cathode, the full cells demonstrate improved capacity and long-term cyclic stability. This work offers an effective direction for improving the stability of Zn anode via electrolyte design, as well as highperformance AZIBs.

关键词： Solvation

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Intelligent interaction system based on multimodal conformal triboelectric nanogenerator patch for disabled sports and life

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Science China Technological Sciences 2025年

作者： Yuzhang WEN Mengqi ZHANG Zhenning XIE Zida AN Bing LIU Fengxin SUN Tianming zhao Zuojun YU fei WANG Yupeng MAO Physical Education Department Northeastern University(Shenyang) Faculty of Robot Science and Engineering Northeastern University Criminal Investigation Police University of China State Key Laboratory of Robotics Shenyang Institute of Automation Chinese Academy of Sciences China Ice Sports College Beijing Sport University

Intelligent interaction technology based on advanced sensing units has become a research hotspot. In this paper, an intelligent interaction system (IIS) based on a multimodal conformal triboelectric nanogenerator patch (MCTP) is reported for sports monitoring and life promotion of the disabled. This IIS consists of a cloud-based smart sports recognition program and a smart life application. The porous micro-reinforced structure of polyurethane (PU) Sponge&Ecoflex, and the surface modification of PTFE by coating it with MXene endows the MCTP with excellent electrical properties. It shows good angle and force sensitivities of 1.1 V/°and 1.61 V/N, respectively, and has an ultra-fast response time of 15 ms, meeting the needs of human motion monitoring. The MCTP can also capture the mechanical energy, producing a maximum output power of 139μ*** with the commercial inertial measuring unit (IMU), the MCTP shows better consistency in human joint angle sensing. A precise analysis of wheelchair curling sports monitoring points is achieved by combining the MCTP and the human anatomy model. The cloud-based smart sports recognition program utilizes machine learning to achieve visual feedback on the three throwing technologies of draw, takeout and clearing. In addition, the developed smart life application uses a highsensitivity MCTP-sensor array design to achieve a variety of smart home interactions through simple finger touches. Overall,the IIS integrates the three major functions of smart sports sensing, energy capture, and smart home control, providing important application prospects in the fields of smart sports and human-computer interaction for the disabled.

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Positive effect of Mo on mechanical properties of a Ni-42W-10Co-x Mo medium heavy alloy

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China Foundry 2025年

作者： Guo-xin Cao jian-xin Dong Yong-sheng He He jiang Fang Hao Zhi-hua Nie Teng-fei Ma Bao-quan Fu School of Materials Science and Engineering University of Science and Technology Beijing Xi'an Superalloy Technology Co. Ltd. School of Materials Science and Engineering Beijing Institute of Technology Key Laboratory of Air-driven Equipment Technology of Zhejiang Province Quzhou University

In this study,a novel Ni-W-Co-Mo medium heavy alloy (MHA) was designed to improve its mechanical strength via Mo *** the Ni-42W-10Co-xM o alloy series,where x represents the weight percent of Mo and varies between 0,1,2,5,and 10,the microstructure transitions from a dendritic structure to a hypoeutectic structure as the Mo content increases from 0 to 5wt.%.Moreover,as the Mo content increases from 0to 10wt.%,the distribution of theμ-phase shifts from being individually dispersed to forming aggregates,and its volume fraction rises from 0.5%to 7.9%.Notably,theμ-phase evolves into an eutectic microstructure,which helps in minimizing the segregation of *** change is accompanied by a substantial enhancement in mechanical properties;specifically,the compressive yield strength at room temperature increases from 350 MPa to 646 MPa,indicating a significant 85%***,the microhardness increases from 230 HV to 304 *** dynamics simulations further reveal that the strengthening mechanism of Ni-42W-10Co-xM o alloys is Mo-induced solid solution strengthening and precipitation strengthening.

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Efficient and Stable Photoassisted Lithium‑Ion Battery Enabled by Photocathode with Synergistically Boosted Carriers Dynamics

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Nano-Micro Letters 2025年第3期17卷 440-454页

作者： Zelin Ma Shiyao Wang Zhuangzhuang Ma Juan Li Luomeng zhao Zhihuan Li Shiyuan Wang Yazhou Shuang Jiulong Wang Fang Wang Weiwei Xia Jie jian Yibo He Junjie Wang Pengfei Guo Hongqiang Wang State Key Laboratory of Solidification Processing Center for Nano Energy MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical University and Shaanxi Joint Laboratory of Graphene(NPU)Xi’an 710072People’s Republic of China State Key Laboratory of Solidification Processing School of Materials Science and Engineering DepartmentNorthwestern Polytechnical UniversityXi’an 710072People’s Republic of China State Key Laboratory of Solidification Processing Center of Advanced Lubrication and Seal MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072People’s Republic of China Research and Development Institute of Northwestern Polytechnical University in Shenzhen Shenzhen 518063People’s Republic of China Key Laboratory of Applied Surface and Colloid Chemistry Shaanxi Key Laboratory for Advanced Energy DevicesShaanxi Engineering Lab for Advanced Energy TechnologySchool of Materials Science and EngineeringNational Ministry of EducationShaanxi Normal UniversityXi’an 710119People’s Republic of China

Efficient and stable photocathodes with versatility are of significance in photoassisted lithium-ion batteries(PLIBs),while there is always a request on fast carrier transport in electrochemical active *** work proposes a general approach of creating bulk heterojunction to boost the carrier mobility of photocathodes by simply laser assisted embedding of plasmonic *** employed in PLIBs,it was found effective for synchronously enhanced photocharge separation and transport in light charging ***,experimental photon spectroscopy,finite difference time domain method simulation and theoretical analyses demonstrate that the improved carrier dynamics are driven by the plasmonic-induced hot electron injection from metal to TiO_(2),as well as the enhanced conductivity in TiO2 matrix due to the formation of oxygen vacancies after Schottky *** from these merits,several benchmark values in performance of TiO2-based photocathode applied in PLIBs are set,including the capacity of 276 mAh g^(−1)at 0.2 A g^(−1)under illumination,photoconversion efficiency of 1.276%at 3 A g^(−1),less capacity and Columbic efficiency loss even through 200 *** results exemplify the potential of the bulk heterojunction strategy in developing highly efficient and stable photoassisted energy storage systems.

关键词： Photoassisted lithium-ion batteries Bulk heterojunction Carrier dynamics TiO2 nanofiber Plasmonic metal nanocrystals

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考虑场地效应的多点地震动作用下边坡永久位移分析

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岩土工程学报 2025年第1期47卷 65-75页

作者：宋健潘驭航陆朱汐姬建张飞高玉峰河海大学岩土力学与堤坝工程教育部重点实验室江苏南京210024 河海大学土木与交通学院江苏南京210024

地震动引起的边坡土层非线性动力响应可能导致坡体不同位置的地震动加速度时程不一致,从而对整个滑动体的极限平衡状态及之后的地震累积永久位移产生影响。为了研究场地效应对边坡地震永久位移的影响,基于极限平衡条分法,通过对不同土... 详细信息

地震动引起的边坡土层非线性动力响应可能导致坡体不同位置的地震动加速度时程不一致,从而对整个滑动体的极限平衡状态及之后的地震累积永久位移产生影响。为了研究场地效应对边坡地震永久位移的影响,基于极限平衡条分法,通过对不同土条赋予不同的水平和竖向地震动时程,推导出一种考虑场地效应的圆弧和任意形状滑面的多点地震作用下边坡永久位移分析方法。通过与有限差分软件FLAC的数值模拟结果进行对比,验证了该方法能够合理考虑地震动的场地效应。通过研究不同分布形式的多点地震动及竖向地震动对边坡永久位移的影响,结果表明:场地效应引起的水平地震动放大以及多点地震动不同分布模式会导致整个滑体平均地震惯性力作用位置发生改变,从而影响地震作用下滑动体沿滑面的永久变形量,竖向地震动对边坡地震位移影响较小。将方法应用于Lexington土石坝震后变形案例分析,计算得到的坝坡地震永久位移与实际震后观测值相吻合,证明了考虑场地效应的重要性及本文方法的合理性。

关键词：地震边坡稳定性场地效应永久位移极限平衡条分法多点地震动

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攻角对长杆弹高速斜侵彻性能的影响

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科学技术与工程 2016年第34期16卷 206-210页

作者：李建飞赵太勇昝守东史俊青张孝中中北大学地下目标毁伤技术国防重点学科实验室太原030051 国营803厂西安710043 山东特种工业集团淄博255201

为了提高穿甲弹的侵彻性能,研究了攻角对杆式弹侵彻性能的影响规律。利用非线性动力学有限元分析软件,对长径比为21的钨芯长杆弹高速斜侵彻匀质钢板进行了一系列数值模拟,得到了侵蚀杆式弹侵彻半无限靶板时弹靶系统的变化过程。理论计... 详细信息

为了提高穿甲弹的侵彻性能,研究了攻角对杆式弹侵彻性能的影响规律。利用非线性动力学有限元分析软件,对长径比为21的钨芯长杆弹高速斜侵彻匀质钢板进行了一系列数值模拟,得到了侵蚀杆式弹侵彻半无限靶板时弹靶系统的变化过程。理论计算及数值模拟均表明,带攻角侵彻时弹道轨迹向有利于穿透靶板的一侧偏转。通过对剩余动能、侵彻深度、剩余速度、穿透时间各因素的分析,得出了对长径比为21的钨合金杆式弹穿深有利的攻角范围为-0.2°<δ<0°,给弹丸设计及发射过程中的参数优化提供理论依据。

关键词：长杆弹斜侵彻数值模拟攻角

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Integrated Modeling of Process–Microstructure–Property Relations in Friction Stir Additive Manufacturing

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Acta Metallurgica Sinica(English Letters) 2020年第1期33卷 75-87页

作者： zhao Zhang Zhi-Jun Tan jian-Yu Li Yu-fei Zu jian-Jun Sha State Key Laboratory of Structural Analysis for Industrial Equipment Department of Engineering MechanicsFaculty of Vehicle Engineering and MechanicsDalian University of TechnologyDalian 116024China School of Aeronautics and Astronautics Dalian University of TechnologyDalian 116024China

Friction stir additive manufacturing is a newly developed solid-state additive manufacturing *** material in the stirring zone can be re-stirred and reheated,and mechanical properties can be changed along the building *** integrated model is developed to investigate the internal relations of process,microstructure and mechanical *** heat source model is used to simulate the friction stir additive manufacturing process to obtain the temperature histories,which are used in the following microstructural *** Carlo method is used for simulation of recrystallization and grain *** evolution model is used for calculation of precipitate size *** property is then *** are used for validation of the predicted grains and *** indicate that the average grain sizes on diff erent layers depend on the temperature in stirring and re-stirring *** the increase in building height,average grain size is decreased and hardness is *** increase in layer thickness can lead to temperature decrease in reheating and re-stirring processes and then lead to the decrease in average grain size and increase of hardness in stir zone.

关键词： Additive manufacturing Friction stir welding Integrated model Precipitate Re-stirring Reheating

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The construction and approximation of some neural networks operators

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Applied Mathematics(A Journal of Chinese Universities) 2012年第1期27卷 69-77页

作者： CHEN Zhi-xiang CAO fei-long zhao jian-wei Department of Mathematics Shaoxing UniversityShaoxing 312000China Department of Mathematics China Jiliang UniversityHangzhou 310018China

In this paper, the technique of approximate partition of unity is used to construct a class of neural networks operators with sigmoidal functions. Using the modulus of continuity of function as a metric, the errors of the operators approximating continuous functions defined on a compact interval are estimated. Furthmore, Bochner-Riesz means operators of double Fourier series are used to construct networks operators for approximating bivariate functions, and the errors of approximation by the operators are estimated.

关键词： approximation sigmoidal function neural network operator Bochner-Riesz mean.

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Enhancement of La2O3 to Li-Mn/WO3/TiO2 for oxidative coupling of methane

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Journal of Rare Earths 2020年第2期38卷 167-174页

作者： fei Cheng jian Yang Liang Yan Jun zhao Huahua zhao Huanling Song Ling Jun Chou State Key Laboratory for Oxo Synthesis and Selective Oxidation Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China University of Chinese Academy of Sciences Beijing 100049China Suzhou Research Institute of LICP Chinese Academy of SciencesSuzhou 215123China

A series of La2O3-promoted Li-Mn/WO3/TiO2 catalysts were prepared by varying the concentration of La2O3 *** effect of La2O3 promoter on its properties and catalytic performance for OCM was characterized with XRD,FT-IR,O2-TPD,Raman,CO2-TPD,H2-TPR,XPS and CH4-TPSR,The results show that all the La2O3-promoted Li-Mn/WO3/TiO2 catalysts possess a larger amount of strong basic sites and more abundant chemisorbed oxygen species in comparison with Li-Mn/WO3/TiO2,which is beneficial to OCM ***,La2O3 promoter can enhance the mobility of the oxygen species and the Mn species redox ability,which can also be favorable for the improvement of the catalytic performance for OCM,Due to the optimal synergistic interaction of these factors,5 wt%La2O3-Li-Mn/WO3/TiO2 exhibits the best performance among all the catalysts,on which the highest C2 yield of 19.2% is achieved at 750℃.

关键词： OCM La2O3 Oxygen species CH4-TPSR Rare earths

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Nano-Ferric Oxide Embedded in Graphene Oxide:High-performance Electrocatalyst for Nitrogen Reduction at Ambient Condition

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Energy & Environmental Materials 2021年第1期4卷 88-94页

作者： fei Wang Lixue Xia Xin Li Weixiang Yang Yan zhao jian Mao College of Materials Science and Engineering Sichuan UniversityChengdu 610065China State Key Laboratory of Silicate Materials for Architectures International School of Materials Science and EngineeringWuhan University of TechnologyWuhan 430070China School of Materials Science and Engineering Southwest Petroleum UniversityChengdu 610500China The Institute of Technological Sciences Wuhan UniversityWuhan 430070China

Nitrogen(N_(2))fixation at ambient condition by electrochemical N_(2)reduction reaction(NRR)is energy-efficient and eco-friendly as compared to the traditional Harber–Bosch process,but it is extremely *** and design of high-performance NRR electrocatalysts are indispensable to achieve the *** this work,a strongly coupled hybrid of nano-Fe3O4 with reduced graphene oxide(rGO)is synthesized via an in situ redox hydrothermal approach,and the synthesized Fe_(3)O_(4)@r GO hybrid has excellent activity,selectivity,and stability as an NRR *** NH_(3) yield rate of 28.01μg h^(-1)mg^(-1)at-0.3 V and the Faradaic efficiency(FE)of 19.12%at-0.1 V are obtained in 0.1 M Na_(2)SO_(4) solutions at ambient *** superior NRR performance is attributed to the chemical coupling effect between r GO and nano-Fe_(3)O_(4) particles,which leads to the enhancement of the binding affinity to N_(2) molecules,improvement of the conductivity,and lowering the free energy of reaction for the limiting reaction *** work provides a facile route in fabricating hybrid NRR catalysts with superior performance and shed lights on the reaction mechanism with theoretical mechanistic calculations.

关键词： density functional theory graphene nano-ferric oxide nitrogen reduction reaction

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