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Renewable non-edible oils derived long chain (C24.1) bio-based zwitterionic surfactant with ultralow interfacial tension between crude oil and formation brine

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Green Chemical Engineering 2023年第3期4卷 346-355页

作者： Homely Isaya Mtui Fang-Hui Liu Wei Wang jian-qiao lang Shi-Zhong Yang Bo-Zhong Mu State Key Laboratory of Bioreactor Engineering and School of Chemistry and Molecular Engineering East China University of Science and TechnologyShanghai200237China Engineering Research Center of Microbial Enhanced Oil Recovery Ministry of EducationEast China University of Science and TechnologyShanghai200237China Shanghai Collaborative Innovation Center for Biomanufacturing Technology Shanghai200237China

A new ultra-long chain monounsaturated 4-(N-nervonicamidopropyl-N,N-dimethylammonium)butane sulfonate(NDAS)zwitterionic surfactant with ultralow interfacial tensions was developed through the modification of nervonic acid derived from renewable non-edible seed oils by a simple and effective *** structure was characterized by ESI-HRMS,1 H NMR,and 13 C *** surfactant exhibited a strong interfacial activity(~10^(-4) mN/m)between the crude oil and the formation brine at a very low surfactant dosage(0.05 g/L)and at high salinity conditions,which is equivalent to 2%(w/w)of dosage of the most traditional surfactants used in the enhanced oil recovery ***,at a very low concentration(0.05 g/L),NDAS demonstrated strong NaCl compatibility up to 100 g/L,Ca^(2+)ions compatibility up to 200 mg/L,and temperature stability up to 90℃.The surface tension,emulsification,and biodegradability parameters were also *** work consolidates our hypothesis that increasing the hydrophobic chain length of a surfactant certainly contributes to the high interfacial activity and good compatibility of salts and ***,it will facilitate the design of a sustainable alternative to petroleum-based chemicals to develop bio-based surfactants and extend the domain of bio-based surfactants to new applications such as in enhanced oil recovery(EOR).

关键词： Bio-based surfactant Interfacial tension Salt tolerance Enhanced oil recovery Biodegradability

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NFXL1 functions as a transcriptional activator required for thermotolerance at reproductive stage in Arabidopsis

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Journal of Integrative Plant Biology 2024年第1期66卷 54-65页

作者： qiao‐Yun Zhu Lin‐Lin Zhang jian‐Xiang Liu State Key Laboratory of Plant Environmental Resilience College of Life SciencesZhejiang UniversityHangzhou 310027China

Plants are highly susceptible to abiotic stresses,particularly heat stress during the reproductive ***,the specific molecular mechanisms underlying this sensitivity remain largely *** the current study,we demonstrate that the Nuclear Transcription Factor,X-box Binding Protein 1-Like 1(NFXL1),directly regulates the expression of DEHYDRATION-RESPONSIVE ELEMENT-BINDING PROTEIN 2A(DREB2A),which is crucial for reproductive thermotolerance in ***1 is upregulated by heat stress,and its mutation leads to a reduction in silique length(seed number)under heat stress ***-Seq analysis reveals that NFXL1 has a global impact on the expression of heat stress responsive genes,including DREB2A,Heat Shock Factor A3(HSFA3)and Heat Shock Protein 17.6(HSP17.6)in flower ***,NFXL1 is enriched in the promoter region of DREB2A,but not of either HSFA3 or *** experiments using electrophoretic mobility shift assay have confirmed that NFXL1 directly binds to the DNA fragment derived from the DREB2A ***,effector-reporter assays have shown that NFXL1 activates the DREB2A *** DREB2A mutants are also heat stress sensitive at the reproductive stage,and DEREB2A is epistatic to NFXL1 in regulating thermotolerance in flower *** is known that HSFA3,a direct target of DREB2A,regulates the expression of heat shock proteins genes under heat stress ***,our findings establish NFXL1 as a critical upstream regulator of DREB2A in the transcriptional cassette responsible for heat stress responses required for reproductive thermotolerance in Arabidopsis.

关键词： Arabidopsis DREB2A heat stress NFXL1 reproductive thermotolerance

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An efficient schedulability analysis based on worst-case interference time for real-time systems

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Science China(Information Sciences) 2024年第09期67卷 88-104页

作者： Hongbiao LIU Mengfei YANG Lei qiao Xi CHEN jian GONG School of Computer Science and Technology Xidian University China Academy of Space Technology Beijing Institute of Control Engineering

Real-time systems are widely implemented in the Internet of Things(IoT) and safety-critical systems, both of which have generated enormous social value. Aiming at the classic schedulability analysis problem in real-time systems, we proposed an exact Boolean analysis based on interference(EBAI) for schedulability analysis in real-time systems. EBAI is based on worst-case interference time(WCIT), which considers both the release jitter and blocking time of the task. We improved the efficiency of the three existing tests and provided a comprehensive summary of related research results in the field. Abundant experiments were conducted to compare EBAI with other related results. Our evaluation showed that in certain cases, the runtime gain achieved using our analysis method may exceed 73% compared to the stateof-the-art schedulability test. Furthermore, the benefits obtained from our tests grew with the number of tasks, reaching a level suitable for practical application. EBAI is oriented to the five-tuple real-time task model with stronger expression ability and possesses a low runtime overhead. These characteristics make it applicable in various real-time systems such as spacecraft, autonomous vehicles, industrial robots, and traffic command systems.

关键词： five-tuple real-time task model real-time system spacecraft Internet of Things exact schedulability analysis worst-case interference time

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Influences of mechanized tillage and sowing modes on soil physical properties,soybean yield and economic benefits in mollisols region of Northeast China

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International Journal of Agricultural and Biological Engineering 2024年第3期17卷 130-139页

作者： Haitao Chen jian Sun Yiming Zhang Jinyou qiao College of Engineering Northeast Agricultural UniversityHarbin 150030China Heilongjiang Province Technology Innovation Center of Mechanization and Materialization of Major Crops Production Harbin 150030China College of Mechanical and Electrical Engineering East University of HeilongjiangHarbin 150066China

Appropriate mechanized straw returning and tillage sowing techniques were effective means to optimize soil physical properties and enhance agricultural productivity,as well as important measures for the conservation and restoration of mollisols region in Northeast *** the condition of full-scale maize straw returning,four mechanized tillage and sowing modes were set,including plough tillage and sowing(PTS),combined tillage and sowing(CTS),no-tillage and sowing(NTS),and no-tillage and sowing with straw mulching(NTSM).In 2020 and 2021,the study investigated the effects of different mechanized tillage and sowing modes on soil physical properties,soybean yield and economic *** results showed that during the pod-setting and pod-filling period of soybean,the NTS and NTSM treatments exhibited better effects on deep soil insulation and shallow soil moisture retention,the soil physical structure of PTS and CTS treatments were relatively *** with PTS and CTS treatments,NTS and NTSM treatments significantly increased soil gravimetric water content(SWC)by 2.35%to 7.98%in the 5-15 cm soil layer and increased soil temperature(ST)by 3.94%to 10.42%in the 25-35 cm soil layer(p0.05),the soybean yield of NTSM treatment in 2021 significantly increased by 7.30%and 5.84%over PTS and CTS treatments,*** the average annual profit per unit area of NTSM treatment increased by 12.84%,12.41%and 8.57%compared with PTS,CTS and NTS treatments,***,it was recommended to combine NTS

关键词： mechanized tillage and sowing modes full-scale straw returning soil physical properties soybean yield economic benefits mollisols conservation

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Pancreatic panniculitis as the first presentation of pancreatic ductaladenocarcinoma

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Hepatobiliary & Pancreatic Diseases International 2024年第1期23卷 106-108页

作者： Wei-Fang Zhu Shan Fang jian-Jun qiao Department of Dermatology the First Affiliated HospitalZhejiang University School of MedicineHangzhou 310003China

To the Editor:Pancreatic panniculitis,also known as pancreatic fat necrosis or enzymatic panniculitis,is a rare type of panniculitis that occurs in 0.3%−3%of patients with pancreatic disease such as acute or chronic pancreatitis and pancreatic carcinoma,especially acinar cell carcinoma[1,2].The clinical manifestations are nonspecific erythema tender nodules.

关键词： Pancreatic acute adenocarcinoma

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A highly sensitive LITES sensor based on a multi-pass cell with dense spot pattern and a novel quartz tuning fork with low frequency

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Opto-Electronic Advances 2024年第3期7卷 26-34页

作者： Yahui Liu Shunda qiao Chao Fang Ying He Haiyue Sun jian Liu Yufei Ma National Key Laboratory of Science and Technology on Tunable Laser Harbin Institute of TechnologyHarbin 150000China Zhengzhou Research Institute Harbin Institute of TechnologyZhengzhou 450000China Advanced Microscopy and Instrumentation Research Center School of Instrumentation Science and EngineeringHarbin Institute of TechnologyHarbin 150080China.

A highly sensitive light-induced thermoelectric spectroscopy(LITES)sensor based on a multi-pass cell(MPC)with dense spot pattern and a novel quartz tuning fork(QTF)with low resonance frequency is reported in this *** erbi-um-doped fiber amplifier(EDFA)was employed to amplify the output optical power so that the signal level was further *** optical path length(OPL)and the ratio of optical path length to volume(RLV)of the MPC is 37.7 m and 13.8 cm^(-2),respectively.A commercial QTF and a self-designed trapezoidal-tip QTF with low frequency of 9461.83 Hz were used as the detectors of the sensor,*** target gas selected to test the performance of the system was acetylene(C2H2).When the optical power was constant at 1000 mW,the minimum detection limit(MDL)of the C2H2-LITES sensor can be achieved 48.3 ppb when using the commercial QTF and 24.6 ppb when using the trapezoid-al-tip *** improvement of the detection performance by a factor of 1.96 was achieved after replacing the commer-cial QTF with the trapezoidal-tip QTF.

关键词： light-induced thermoelectric spectroscopy quartz tuning fork multi-pass cell gas sensing

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O_(2) adsorption on Fe_(3)O_(4) (110) surface and effect of gangue element Al doping: combined study of binding experiment and ab initio molecular dynamics

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Journal of Iron and Steel Research International 2024年第4期31卷 810-827页

作者： Zheng-jian Liu Hui-qing jiang Yao-zu Wang jian-liang Zhang Hong-mei qiao An-yang Zheng Fang-yu Guo School of Metallurgical and Ecological Engineering University of Science and Technology BeijingBeijing 100083China School of Intelligence Science and Technology University of Science and Technology BeijingBeijing 100083China Beijing Shougang Co. Ltd.Qian'an 064404HebeiChina Department of Physics National University of Defense TechnologyChangsha 410128HunanChina

At high temperature,the chemical reaction mechanism at the interface of magnetite and the influence mechanism of gangue element Al on the oxidation performance of magnetite are not *** addition,due to the limitation of existing experimental equipment,it is difficult to clarify the interface reaction mechanism in the oxidation process and the influence mechanism of Al on the surface oxidation reaction of Fe_(3)O_(4) at an atomic scale at high *** surface oxidation reaction mechanism of magnetite and the influence mechanism of Al on the oxidation of magnetite were studied by experiments and AIMD(ab initio molecular dynamics).The experimental results show that the existence of Al_(2)O_(3) will reduce the initial oxidation temperature and comprehensive oxidation performance of *** AIMD results show that aluminum can accelerate the interface reaction rate of Fe_(3)O_(4) in the high-temperature oxidation atmosphere,but the strong Al-O binding ability is not conducive to the transfer of O atoms in the oxidation process.

关键词： Ironmaking Magnetite oxidation Interface reaction Adsorption-Gangue aluminum AIMD

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A polymyxin B loaded hypoxia-responsive liposome with improved biosafety for efficient eradication of bacterial biofilms

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Nano Research 2024年第9期17卷 8325-8336页

作者： Fang Liu Lingyun Zou Yongcheng Chen Zuolong Liu Yue Huang qiao Jin jian Ji MOE Key Laboratory of Macromolecule Synthesis and Functionalization of Ministry of Education Department of Polymer Science and EngineeringZhejiang UniversityHangzhou 310027China State Key Laboratory of Transvascular Implantation Devices The Second Affiliated Hospital Zhejiang University School of MedicineHangzhou 310009China

Biofilm-associated bacterial infection brings serious threats to global public health owing to serious antibiotic *** is urgently needed to develop innovative strategies to combat biofilm-associated bacterial *** stand out as the last line of defense against Gram-negative ***,serious nephrotoxicity of polymyxins severely limits their clinical ***,a hypoxia-responsive liposome is designed as the nanocarrier of polymyxin B(PMB)to combat biofilms developed by Gram-negative bacteria.A metronidazole modified lipid(hypoxia-responsive lipid(HRLipid))is synthesized to fabricate hypoxia-responsive liposomes(HRLip).PMB loaded hypoxia-responsive liposomes(HRL-PMB)is then prepared to mitigate the nephrotoxicity of PMB while preserving its excellent bactericidal ***-PMB shows very low hemolysis and cytotoxicity due to liposomal encapsulation of *** can be readily released from HRL-PMB in response to hypoxic biofilm microenvironment,exerting its bactericidal activity to realize biofilm *** excellent in vivo antibiofilm ability of HRL-PMB is confirmed by a Pseudomonas aeruginosa infected zebrafish model and a *** pneumonia infection ***,HRL-PMB can greatly reduce the nephrotoxicity of PMB after intravenous *** hypoxia-sensitive liposomes held great promise to improve the biosafety of highly toxic antibiotics while preserving their intrinsic bactericidal ability,which may provide an innovative strategy for combating biofilm-associated infections.

关键词： bacterial biofilm hypoxia liposome polymyxin B nephrotoxicity

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Asymmetric reversible structural switching of a diene coordination polymer promoted by UV-visible light

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Science China Chemistry 2024年第2期67卷 536-541页

作者： Yong Wang qiaoqiao Zhang Yong-Yong Cao Qi Liu Brendan F.Abrahams jian-Ping lang College of Chemistry Chemical Engineering and MaterialsSoochow UniversitySuzhou215123China State Key Laboratory of Organometallic Chemistry Shanghai Institute of Organic ChemistryChinese Academy of SciencesShanghai200032China College of Biological Chemical Science and EngineeringJiaxing UniversityJiaxing314001China School of Chemistry University of MelbourneVictoria3010Australia

In natural and artificial systems,reversible reactions are commonly asymmetric with respect to the time scale and nature of the stimuli which drive the forward and backward *** applications for which switching behavior is required,it is desirable that the reversible reaction goes as close to symmetric as possible;however,such systems are ***,we report an example of ultraviolet(UV)-visible light-regulated asymmetric reversible structural switching involving a diene-based coordination polymer,CP1 and its monocyclobutane product,*** is possible to cycle at least ten times through a forward [2+2] photocycloaddition reaction and the reverse,photocleavage reaction.A single cycle can be completed within a few *** transformation is accompanied by fast and distinct fluorescence changes,arising from optimisation of the reaction *** functional theory calculations allow rationalisation of the asymmetric reversible transformation between CP1 and CP1a rather than between CP1 and its dicyclobutane product *** work provides a clear illustration of reversible structural switching which approaches symmetric behaviour with respect to reaction rate and *** insights gained from this work also assist in the design of fast,reversible switching materials.

关键词： asymmetrical reversible structural switching coordination polymer photocycloaddition UV-visible light-controlled fluorescence switching

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Safety and efficacy of omalizumab for antihistamine-resistant chronic urticaria in children:a case series and literature review

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World Journal of Pediatrics 2024年第3期20卷 294-298页

作者： Wei-Fang Zhu Chen Wang jian-Jun qiao Lan-Juan Li Department of Dermatology First Affiliated HospitalZhejiang University School of MedicineHangzhou 310003China State Key Laboratory for Diagnosis and Treatment of Infectious Diseases National Clinical Research Center for Infectious DiseasesCollaborative Innovation Center for Diagnosis and Treatment of Infectious DiseasesThe First Affiliated HospitalZhejiang University School of MedicineHangzhou 310003China

Chronic urticaria(CU)is a common skin disease characterized by the occurrence of wheals,with or without angioedema,lasting more than 6 *** prevalence of CU is about 0.7%[1],but higher in children,with an incidence of 1.38%[1].The occurrence of severe pruritus and unpredictable wheals may severely impact patients'quality of life,cause psychological problems,including sleep disorders and depression,and lead to economic burden due to limitation on daily life and work[2,3].

关键词： edema prevalence children

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